Local magnetic susceptibility of the positive muon in the quasi-one-dimensional S=1/2 antiferromagnet dichlorobis (pyridine) copper (II)

We report muon spin rotation measurements of the local magnetic susceptibility around a positive muon in the paramagnetic state of the quasi-one-dimensional spin 1/2 antiferromagnet dichlorobis (pyridine) copper (II). Signals from three distinct sites are resolved and have a temperature dependent frequency shift which is significantly different than the magnetic susceptibility. This difference is attributed to a muon induced perturbation of the spin 1/2 chain. The obtained frequency shifts are compared with transfer matrix density-matrix renormalization-group numerical simulations.     

Contribution of spin-orbit interaction to the magnetic susceptibility of interacting electrons in metals

The effect of spin-orbit interaction on the magnetic susceptibility of metals has been investigated using a pseudopotential formalism. The orbital spin and spin-orbit contributions to the magnetic susceptibility of Zn and Cd have been calculated. An important feature is that the spin-orbit contribution is diamagnetic and is of the same order of magnitude as orbital contribution in the case of Zn and Cd.     

Effect of spin-orbit scattering on the magnetic and superconducting properties of nearly ferromagnetic metals: application to granular Pt

We calculate the effect of scattering on the static, exchange enhanced, spin susceptibility and show that, in particular, spin-orbit scattering leads to a reduction of the giant moments and spin glass freezing temperature due to dilute magnetic impurities. The harmful spin fluctuation contribution to the intragrain pairing interaction is strongly reduced opening the way for BCS superconductivity. We are thus able to explain the superconducting and magnetic properties recently observed in granular Pt as being due to scattering effects in single small grains.     

Effect of spin diffusion on the spin resonance in local moment systems

The effect of conduction electron spin diffusion on linewidth, lineshift and residue of the spin resonance in local moment systems is investigated. For the calculation of the transverse susceptibility a previously established kinetic equation approach is used. Low temperature Kondo-type anomalies of spin relaxation and diffusion are taken into account in the framework of Suhl's theory. The susceptibility exhibits considerable structure as a function of wavevector. In particular it is shown that the magnetic resonance bottleneck is broken for sufficiently large wavevectors. The effect of relaxation proceeding to local instead of total equilibrium is investigated and shown to introduce only minor modifications with one possible exception. Application of the theory to transmission electron spin resonance (TESR) is also discussed.     

Magnetic properties of neutron matter

The energy of interacting neutron matter with spin polarization is calculated in Hartree-Fock approximation by the method of unitary transformations for a hard core and a soft core potential. In addition the magnetic spin susceptibility is given and the possibility of a ferromagnetic transition investigated. It is shown that the effect of the nuclear forces for all densities considered depresses the magnetic spin susceptibility relative to that of the corresponding ideal Fermi gas.     

Magnetic susceptibility of the spin polaron states in the s-f exchange model above curie temperature

The static spin susceptibility tensor of magnetic semiconductor in a framework of the s-f exchange model above the Curie temperature is calculated. The Feynman path integral variational method is used to take into account the spin polaron formation. Free energy estimations of the phenomenological theory of Krivoglaz are justified microscopically. The spin polaron effect on ESR frequencies is considered.     

Generation of an external magnetic field with the spin orientation effect in a single layer Ising nanographene

In this work, the magnetic properties of the single layer Ising nanogaphene (SLING) are investigated by using Kaneyoshi approach (KA) within the effective field theory for different spin orientations of its magnetic atoms. We find that the magnetizations of the SLING has no phase transition, certain Curie temperature and distinct peak of susceptibility at T_c for the some spin orientations at the zero external magnetic field (H=0.0). Because these behaviors occur at H≠0.0, we suggest that the SLING generates an external magnetic field and behaves as an external magnetic field generator for these spin orientations. However, the SLING exhibits ferromagnetic behaviors for only one spin orientations. But, it exhibits antiferromagnetic behaviors for the others. For the AFM cases, diamagnetic susceptibility behaviors and type II superconductivity hysteresis behaviors are obtained. We hope that these results can open a door to obtain new class of single layer graphene and graphene-based magnetic field generator devices with the spin orientation effect.     

High Magnetic Field Consequences on the NMR Hyperfine Shifts in Solution

Pseudocontact shifts arise from the isotropic reorientational average of the dipolar coupling between unpaired electron and nuclei, in the presence of magnetic susceptibility anisotropy. The effect of residual orientation due to high magnetic fields on pseudocontact shifts is evaluated here. The effect is found to be smaller and of opposite sign with respect to another novel effect of high magnetic fields on hyperfine shifts due to saturation of the electron spin magnetic moment as described by the Brillouin equation.     

The temperature dependence of the magnetic susceptibility of spin glasses

The temperature dependence of the magnetic susceptibility of spin glasses is calculated exactly on the basis of a magnetic cluster model, following Néel. The susceptibility of a single cluster below its blocking temperature is taken to be negligibly small compared to its value above. A distribution of blocking temperatures may be obtained from observations on spin glasses. Conditions for the sharpness of the susceptibility peak are discussed and the low-temperature variation of the susceptibility is also obtained.     

Nonlinear 2D spin susceptibility in a finite magnetic field: spin-polarization dependence

By theoretically calculating the interacting spin susceptibility of a two-dimensional electron system in the presence of finite spin polarization, we show that the extensively employed technique of measuring the 2D spin susceptibility by linear extrapolation to a zero field from the finite-field experimental data is theoretically unjustified due to the strong nonlinear magnetic field dependence of the interacting susceptibility. Our work compellingly establishes that much of the prevailing interpretation of the 2D susceptibility measurements is incorrect, and, in general, the 2D interacting susceptibility cannot be extracted from the critical magnetic field for full spin polarization, as is routinely done experimentally.     

The observation of inherent spin Seebeck effect in Rh/YIG hybrid structure

Rhodium (Rh) is a 4d metal possessing a large spin orbit coupling strength and spin-Hall conductivity with a very small magnetic susceptibility, implying an insignificant magnetic proximity effect (MPE). We report here the observation of longitudinal spin Seebeck effect (LSSE) using Rh as a normal metal. A Rh film was sputtered on nanometer thick YIG films of highly crystalline nature and extremely low magnetic damping to obtain Rh/YIG hybrid structure. A clear thermal voltage V_th (SSE voltage) was obtained when a temperature gradient was applied on the Rh/YIG hybrid. The Rh film showed a very weak anomalous Hall resistance and the magneto-resistive testing clearly ruled out the magnetization of the Rh films via MPE. The anisotropic magnetoresistance (AMR) revealed a clear spin hall magnetoresistance (SMR) signal in Rh film implying a purely intrinsic spin current generation, free from any parasitic magnetic effects. The work can open a new window in the study of pure and uncontaminated spin current, generated in ferromagnetic insulators, using Rh as spin current detector.     

自旋相关的电子隧穿和自旋极化

研究了电子的自旋相关的隧穿和极化。在外加磁场的作用下，自旋向上的电子与自旋向下的电子具有不同的隧穿系数。当电子的自旋方向与磁场方向相反时，其隧穿概率受到磁场的抑制而变小；反之，当两平行时，电子的了隧穿系数增大。这种差异可以用本中定义的自旋极化率来表示。本对不同磁场下的自旋极化率进行了计算，结果也表明当电子的动能较小，这种自旋极化的效应越显。     

Spin fluctuations in metals: Application to the actinides

We present here a review of the spin fluctuation theory and of its applications to transition and actinide systems, with a particular emphasis to the latter where some very anomalous properties find an explanation in terms of spin fluctuation effects. Firstly, we summarize the development of the spin fluctuation model which had been initially applied to transition metals and alloys such as palladium or Pd–Ni alloys. Then, we present the extension of the paramagnon model to nearly magnetic actinide systems by taking into account explicitly the temperature dependence of the Stoner susceptibility, because the 5f-band of actinides is much narrower than the d-band of transition metals. As a result the paramagnon contribution to the resistivity departs from the usual T ² and T power laws at temperatures higher than the spin fluctuation one and saturates at high temperatures, with eventually the presence of a maximum at intermediate temperatures. We present also the calculation of the other properties of actinide systems, namely the thermal resistivity, the thermoelectric power, the magnetic susceptibility, the specific heat capacity and the NMR relaxation rate, which are generally enhanced by the presence of paramagnons. Finally, we have introduced the concept of ‘antiferromagnetic-like’ spin fluctuations which have a maximum of the q-dependent susceptibility _χ(q) at a q value different from q =0, in contrast to the regular ferromagnetic spin fluctuations; both types of spin fluctuation give the same resistivity behaviour, while they yield a markedly different behaviour of the magnetic susceptibility, in agreement with experiment. The spin fluctuation theory is applied successfully to the different properties of neptunium and plutonium metals and of many nearly magnetic compounds such as UAl₂.     

Theory of itinerant electron antiferromagnetism

Itinerant electron antiferromagnetism is studied by taking into account the realistic electronic structure and the effect of spin fluctuations within static Gaussian statistics. Expression for the magnetic susceptibility above and below the Néel temperature are obtained. It is shown that spin fluctuations can stabilize antiferromagnetism in a certain case. The character of magnetic transitions and the comparison with experiment are discussed.     

Direct observation of chiral susceptibility in the canonical spin glass AuFe

The extraordinary Hall resistivity rho(xy) and the magnetization M of a canonical spin glass AuFe (8 at.% Fe) were measured simultaneously as functions of temperature with the best care to the thermal and the magnetic field hysteresis. The data of rho(xy) show an anomaly at the spin glass transition temperature T(g) and have different zero field cooling (ZFC) and field cooling (FC) measurements below T(g). Moreover, the value of rho(xy)/M, which represents the chiral susceptibility of the system in the present case, also shows the difference between ZFC and FC measurements. The results are consistent with the predictions of the chirality scenario of canonical spin glasses by Kawamura.     

Magnetic susceptibility of dilute magnetic alloys

The magnetic susceptibility of dilute magnetic alloys is calculated using the Nagoaka approximation to the Kondo problem. We use the exact solutions of the Nagaoka equations, or equivalently Suhl's dispersion relations, as obtained recently. Our result is represented by a universal function of a certain temperature parameter. In the case of ferromagnetic coupling no appreciable change of the free spin susceptibility is found over the whole temperature range. In the case of antiferromagnetic coupling we find that the free spin susceptibility is greatly reduced. In fact, for spin 1/2, the result indicates the breakdown of the expansion in terms of the impurity concentration and suggests the onset of impurity ferromagnetism.     

Exact solution on the magnetism and ferroelectricity in the Ising spin chain

In this paper, we explore the magnetoelectric coupling in Ca₃CoMnO₆-type compound with the consideration of interaction between spins. Under the linear approximation of nearest-neighbor spin interaction with respect to the ion displacement, both the Hamiltonian and the partition function of the system can be simplified as the summation of two independent items, one is linear harmonic oscillator relevant to the lattice vibration, and the other is only relevant to the spin. We obtain the magnetic and ferroelectric quantities of Ca₃CoMnO₆-type rigorously on the basis of the transfer-matrix method, qualitatively exhibiting the corresponding curves taken in the presence of temperature for zero magnetic field and various magnetic fields, respectively, and our calculation results are basically consistent with the behaviors in the experiment. We find that the magnetic susceptibility in the absence of magnetic field takes on the features of ferromagnetic Ising-like behavior. Moreover, the influence of different next-nearest-neighbor exchange interaction on the magnetic susceptibility and relative dielectric constant is given as well, exhibiting the corresponding complex response of the magnetic susceptibility based on the up-up-down-down spin structure.     

Charge and spin dynamics in antiferromagnetic metallic phase of iron-based superconductors

The electronic states, charge dynamics, and spin dynamics in the antiferromagnetic metallic phase of iron-arsenide superconductors are investigated by mean-field calculations for a five-band Hubbard model. Taking into account the difference of observed magnetic moments between LaFeAsO (1111 system) and BaFe₂As₂ (122 system), we investigate the effect of the magnitude of the moments on band dispersion, optical conductivity, and dynamical spin susceptibility. We clarify how the magnitude affects on these quantities and predict different behaviors between the 1111 and 122 systems in the antiferromagnetic metallic phase.     

Rashba coupling induced spin susceptibility and magnetic phase transition of conduction electrons in monolayer graphene

Isolated graphene cannot be obtained by the known synthesis processes and it should be placed on a substrate. This substrate introduces a new type of spin–orbit interaction known as Rashba coupling. Using the Kubo formalism, the magnetic properties of the system in the linear regime have been investigated. Mainly the effect of non-magnetic substrate on the spin susceptibility is calculated. Results show that the Rashba coupling has a central role in the magnetic response function of the system and it is really remarkable since this type of spin orbit coupling can be effectively controlled by an external gate voltage. Most importantly, it was shown that, in the presence of the Rashba interaction a magnetic phase transition could be observed. This magnetic phase corresponds to a magnetic order of conduction electrons that takes place at some special frequencies of external magnetic field.     

On second-harmonic generation in nonuniformly magnetized media

This paper presents a theoretical study of new effects of double-frequency optical signal generation in magnetic media with a nonuniform magnetization distribution. The study is based on the hydrodynamic approximation of the motion of conduction electrons in the field of an electromagnetic wave and equations for the mean electron spin. Within this approach, the mechanisms of the toroidal moment effect, which was experimentally discovered earlier in a system of magnetic particles with a vertical magnetization distribution as well as in a multilayered magnetic system (which is a collinear nonuniform magnetic system), are demonstrated. A new effect that appears due to the presence of equilibrium spin currents in a nonuniform magnetic system is studied in detail. This effect was predicted from the symmetry and can occur only in noncollinearly magnetized media. It is shown that this effect has a resonance nature with a resonance at a pump frequency equal to the plasma frequency of conduction electrons. Estimates of the susceptibility at the double frequency for the parameters of nickel and the typical scale of variation in the magnetization, which is equal to 10 nm, show that the susceptibility near the frequency of the plasma resonance at the chosen parameters is on the order of 10^–9 esu, which holds up a hope of the experimental detection of this effect.