A study of the 59Co(n,n′γ)59Co reaction

The ⁵⁹Co(n, n'γ)⁵⁹Co reaction has been studied for incident neutron energies ranging from 1.3 to 3.9 MeV. The pulsed-beam time-of-flight technique was employed to discriminate between the inelastically scattered neutrons and the de-excitation γ-rays, which were detected by means of a true-coaxial Ge(Li) detector. Thirty-five levels were identified in this way, and their excitation functions have been extensively compared with the predictions of the statistical theory of the compound nucleus. Possible spin assignements to the levels of ⁵⁹Co are discussed and compared with the results available from previous works.     

59Co nuclear magnetic resonance in antiferromagnetic CsCoCl3

The ⁵⁹Co NMR in a CsCoCl₃ single crystal has been observed by the spin echo method at 4.2 K. The obtained spectrum is composed of seven distinct lines split by the nuclear-quadrupole interaction. The frequency of the central (± $\text{1}\text{2}$ ? ± $\text{1}\text{2}$) transition 502.08±0.05 MHz corresponds to the hyperfine field of 499.38 ± 0.05 kOe, which agrees well with the calculated value. Due to the interaction of the nucleus with the electronic moment induced by the external field, a shift as large as 18% was observed for the nuclear g-factor.     

Neutron diffraction studies of the magnetic ordering in the rare earth compounds TbNi2Si2, HoCo2Si2 and TbCo2Si2

Neutron diffraction studies and magnetic measurements on the compounds TbNi₂Si₂ (1), HoCo₂Si₂ (2) and TbCo₂Si₂ (3) revealed a collinear antiferromagnetic order below T_N = 10 ± 1 K (1), T_N = 13 ± 1 K (2) and T_N = 30 ± 2 K (3) with the rare earths moments oriented along the c-axis [m₀ = 8.8 ± 0.2 μ_B (1), m₀ = 8.1 ± 0.2 μ_B (2), m₀ = 8.8 ± 0.2 μ_B (3)] and the corresponding wavevector are $\text{k}\text{= [}\text{1}\text{2}\text{1}\text{2}\text{0] (1)}\text{and}\text{k}\text{= [ 0 0 1] (2) (3)}$. The magnetic structure of the compounds HoCo₂Si₂ and TbCo₂Si₂ consists of ferromagnetic layers perpendicular to the c-axis coupled antiferromagnetically (+?+?) while for TbNi₂Si₂ the ordering within (0 0 1) plane is antiferromagnetic and the planes (0 0 1) are indeed decoupled.     

A study of the (α, t) reaction on 19F, 27Al, 51V and 59Co

The angular distributions of tritons from the (α, t) reaction on ¹⁹F, ²⁷Al, ⁵¹V and ⁵⁹Co nuclei corresponding to the (0⁺) ground states and (2⁺) excited states in the final nuclei have been measured in the angular range between 15° and 170° at α-particle energies of 25 MeV. For reactions on ²⁷Al and ⁵¹V nuclei, the differential excitation functions have also been obtained at different angles of outgoing tritons at E_α from 20 to 25 MeV. The experimental angular distributions are analysed by the DWBA approximation on the assumption of a nucleon stripping mechanism. The analyses of the present results and the data obtained earlier for the (α, t) reaction on the 1 p shell nuclei, A ? 30, reveal that the distinguishing feature of the reaction under study is the presence of backward angle peaks in the reaction cross section, which appear to be associated with exchange processes. For the (α, t) reaction on the heavier nuclei (A > 30), the dominant mechanism is nucleon stripping.     

Temperature-induced local magnetic moments in CoSe2-59Co NMR

From the temperature dependences of the ⁵⁹Co Knight shift and the nuclear spin-lattice relaxation rate in the exchange-enhanced paramagnetic metal CoSe₂, it is shown that the amplitudes of the temperature-dependent spin density fluctuations are saturated at $\text{T}{}^1\text{= 130 K}$. This fact indicates that there exist local moment type fluctuations above T¹. The results obtained from the present NMR investigation are in general accord with the predictions based on the general theory of spin fluctuations in itinerant electron systems developed recently by Moriya and Takahashi.     

Magnetization reorientation in HoCo2

In order to confirm the magnetization reorientation in HoCo₂, torque measurements have been performed at various temperatures on a spherical single crystal, in the (001) and (011) planes. The easy magnetization direction is the [110] axis at 4.2 K and the [100] axis above 16 K. Furthermore, between 11 K and 16 K, the easy magnetization direction rotates progressively within the (001) plane. These results agree with the magnetization measurements and can be interpreted by a crystal field model.     

Anisotropic chemical shifts of 59Co in Co(NH3)6Cl

The chemical shift tensors of ⁵⁹Co in a single crystal of Co(NH₃)₆Cl₃ at the five nonequivalent cobalt sites were measured at room temperature. The principal axes of these tensors almost coincide with the principal directions of the electric field gradient tensors. Assuming that these directions are parallel to the symmetry axes about which the different Co(NH₃)₆³⁺ octahedra reorientate, possible reorientation axes of the octahedra at the five nonequivalent sites are proposed.     

The magnetic structure of HoCo2Si2

We have carried out neutron diffraction on a HoCo₂Si₂ powder sample at 4.2 K. The magnetic structure of this compound is collinear antiferromagnetic with the holmium magnetic moments parallel to the c-axis of the crystal. The magnetic moment value of holmium is 9.85 μ_B. The magnetic space group is I4/mm'm' (Sh⁴¹⁰₁₂₈) k = 000 The ordering temperature is t_n = 12(1) K.     

Nuclear magnetic resonance of 59Co on A and B sites in Co3S4

A comment is made on a recent paper by Saji and Yamadaya, who erroneously attribute a single cobalt NMR line in Co₃S₄ to cobalt at the B sites of the spinel lattice. A summary is given of earlier published work which describes cobalt NMR at both A and B sites.     

Spectroscopic study of 55Co via the 54Fe(τ, d)55Co and 54Fe(τ, dp̃)54Fe reactions

The ⁵⁴Fe(τ, d)⁵⁵Co reaction has been studied at 25 MeV incident energy with a split-pole spectrometer. About one hundred levels have been observed in ⁵⁵Co up to 10 MeV excitation energy. Angular distributions have been measured and analyzed with DWBA and Gamow functions as form factors for unbound levels. The ⁵⁴Fe(τ,dp?)⁵⁴ reaction has been investigated at 24 MeV incident energy. The angular distributions of the emitted protons were measured in coincidence using method 2 of Litherland and Ferguson, with 0 detection of deuteron groups. Spins, population parameters, branching ratios and proton partial widths for the transitions to the ground and excited states of ⁵⁴Fe were determined from the analysis of the angular correlation data. The results of these two experiments provide a large number ofspectroscopic properties of unbound proton states and in particular of analog states of ⁵⁵Fe low-lying levels. The IAS of the $\text{3}\text{2}{}^{\mathrm{?}}$ ground state of ⁵⁵Fe is observed to be split between two individual levels. The amplitude of neutron coupling to the first 2⁺ excited state of ⁵⁴Fe is obtained for the $\text{lg}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}$ and $\text{2}\text{d}\text{5}\text{2}$ low-lying parent statfes in ⁵⁵Fe. summed spectroscopic factors and the centroid energies of the proton states in ⁵⁵Co are obtained. A comparison is made with previous (τ, d), (d, p) and (p, p) results.     

Momentum transfer in 30–200 MeV 4H induced reaction with 59Co

Thick-target recoil ranges of radioactive nuclei produced in 30–200 MeV alpha-particle bombardment of ⁵⁹Co have been used to deduce the longitudinal momentum transfer per projectile nucleon (p₆/A) as a function of residue mass and bombarding energy. The average value of p₆/A increases monotonically with bombarding energy and reaches a maximum value of ≈ 160 MeV/c at ≈ 23 MeV/u, and decreases thereafter. The maximum value of p₆/A is equal to the incident momentum up to ≈ 23 MeV/u and saturates at a value of ≈ 220 MeV/c beyond this energy.     

Magnetic properties of NdCo2Ge2, ErCo2Ge2 and PrFe2Ge2 compounds

Magnetometric and neutron diffraction studies of polycrystalline NdCo₂GE₂, ErCo₂Ge₂ and PrFe₂Ge₂ compounds were carried out in the temperature range between 4.2 and 300 K. All samples are antiferromagnetic with Néel temperature 26.5, ～ 4.2 and 13 K, respectively. The RECo₂Ge₂ compounds have collinear antiferromagnetic order of +?+? type. For PrFe₂Ge₂ a sinusoidal magnetic structure is observed. Magnetic moment is localized on RE atoms only and is equal to that of RE³⁺ free ion value. In ErCo₂Ge₂ the magnetic moment of Er atoms is perpendicular to the c-axis, whereas for remaining compounds it is parallel to the c-axis.     

The 59Co nuclear magnetic resonances in the intermetallic compounds

The anisotropic hyperfine fields of the intermetallic compounds have been studied by the spin echo method and were obtained from the NMR spectra of ⁵⁹Co nuclei in ThCo₅ and YCo₅ which have the high anisotropy fields resulting from the orbital moments. The intermetallic compounds, ThCo_5.3 and YCo_5.3, have been also investigated.     

The 59Co (d, 3He)58Fe reaction and 58Fe levels in the particle-vibration coupling model

The ⁵⁹Co(d, ³He)⁵⁸Fe reaction at a deuteron energy of 33.3 MeV was used to populate proton hole states in ⁵⁸Fe. Angular distributions were measured for the states up to 6 MeV excitation. From DWBA analysis, l-values and spectroscopic factors were extracted. The particle-vibration coupling model was used to interpret the positive-parity states observed in the present experiment as well as the related properties of ⁵⁸Fe established so far. The model calculation has reproduced rather well the level properties of ⁵⁸Fe.     

Spectroscopy of two coincident charged particles emitted following bound pion absorption in 12C, 59Co and 197Au

Energy spectra and angular distributions of two coincident charged particles emitted following stopped negative pion absorption in ¹²C, ⁵⁹Co and ¹⁹⁷Au were measured. Most of the data can be understood within the framework of a pair absorption model including final-state interactions. Ground-state transitions in the missing mass spectra of ⁴H and ⁴He deduced from the αα and tα spectra of ¹²C, respectively, show that reactions involving a large part of the nucleus also occur.     

Origin of magnetostriction in TbAl2 and TbCo2 compounds

Magnetostriction measurements are reported for TbAl₂ below the ordering temperature. Single crystal magnetostriction coefficients are estimated for TbAl₂. From the measured data together with the results obtained earlier for TbCo₂, it is found that the source of the magnetostriction is the strain-dependent anisotropy of the Tb sublattice.     

Magnetic structures of PrCO2Si2 and TbCo2Si2 compounds

Neutron diffraction studies of polycrystalline PrCo₂Si₂ and TbCo₂Si₂ compounds were carried out at 4.2 and 293 K. Both samples have collinear antiferromagnetic order below T_N(31(1) and 46(1) K for Pr and Tb compound respectively), with their magnetic moments parallel to the c axis. The ordered magnetic moment values of Pr and Tb at 4.2 K (3.19 and 9.12 μ_B respectively), are close to the saturation value of the free ions. The corresponding magnetic space group P_l4/mnc (Sh⁴¹⁰₁₂₈) is body-anticentered ($\text{k =}\text{111}\text{222}$ refering to P_l cell).     

The hyperfine specific heat of HoCo2

The specific heat of HoCo₂ has been measured between 1.3 and 5K, a temperature range in which the nuclear specific heat predominates. The magnetic moment of holmium determined from the data is (10 ± 0.2)μ_B. This value is compared with the values deduced from magnetization and elastic neutron scattering experiments.     

The influence of easy direction of magnetisation on 59Co NMR spectrum in R2(Co1−xMnx)17 compounds

The spin echo NMR spectra of ⁵⁹Co in R₂(Co_1-xMn_x)₁₇, (R = Y, Gd) measured at 4.2 K are reported. The large shift of resonance lines is observed, that is explained as caused by reorientation of easy axis of magnetisation from easy plane to easy direction (c axis). It is suggested to explain quantitatively the spectra, that only two of four Co sites (9d and 18f) in R₂Co₁₇ structure play a dominant role in determining of anisotropy energy and the Co atoms at the 6c sites (“dumb-bell” atoms) give no direct contribution to the anisotropy energy of the compound. The corresponding changes of local anisotropy energy and the orbital part of cobalt magnetic moment characteristic for each of cobalt structural sites are calculated and discussed.