契形结构光纤表面等离子体共振传感器研究

提出了一种契形端面结构的光纤表面等离子体共振(SPR)传感器激励模型. 采用时域有限差分法对契形SPR波导的共振模型进行数值模拟, 通过在光纤出射端抛磨契形角度并进行敏感膜修饰, 制出具有契形端面结构的类Kretschmann微棱镜式光纤SPR传感器, 实现激发SPR的光波调制.结果表明, 在1.3330–1.4215折射率范围内, 制备的契形光纤SPR传感器相对于常规光纤SPR传感器, 其平均灵敏度提高了近1–6倍, 1倍和6倍分别出现在小角度结构(15° 契形) 传感器和大角度结构(60°契形) 传感器, 且仍保持 10^-5 等级的分辨率. 该类型结构的传感器具有契形端面激励模式, 设计灵活性高、制备工艺简单、可微量检测样本等优点, 能够很好地适应于不同环境和测量条件的实际生化检测、环境监测需求. 关键词： 光纤传感器 表面等离子体共振 契形端面结构 折射率灵敏度     

Absorption enhancement of ultrathin crystalline silicon solar cells with frequency upconversion nanosphere arrays

A design of ultrathin crystalline silicon solar cells patterned with α-NaEr_(0.2)Y_(0.8)F_4 upconversion nanosphere(NSs) arrays on the surface was proposed. The light trapping performance ofα-NaEr_(0.2)Y_(0.8)F_4 NSs with different ratios of sphere diameter to sphere pitch was systematically studied by COMSOL Multiphysics. The influence of different NS diameters and ratio to the average optical absorption of ultrathin crystalline silicon solar cell was calculated, as well as the short circuit current densities. The results show that the average optical absorption of solar cells with 2.33 μm silicon covered by α-NaEr_(0.2)Y_(0.8)F_4 NSs of 100 nm in diameter and 5.2 in ratio has improved by 8.5% compared to planar silicon solar cells with the same thickness of silicon. The light trapping performance of different thicknesses of silicon solar cells with the optimized configuration of NSs was also discussed. The results indicate that our structure enhances the light absorption. The presented model will be the basis for further simulations concerning frequency upconversion of α-NaEr_(0.2)Y_(0.8)F_4 materials.     

Work function changes and surface chemistry of oxygen, hydrogen, and carbon on indium tin oxide

The surface chemistry of indium tin oxide (ITO) has been investigated with Auger electron spectroscopy (AES) and high resolution electron energy loss spectroscopy (HREELS). A vibrating Kelvin probe (KP) with a graphite reference was used to monitor the absolute work function (Φ) of ITO as a function of chemical modification. The ITO was exposed in situ to molecular hydrogen (H₂), hot-filament-activated oxygen (O₂^*), and hot-filament-activated deuterium (D₂^*). The initial Φ of ITO was determined to be 5.2 eV, and surface chemical changes had strong effects on this value, as seen by KP. Exposure of clean ITO to O₂^* increased Φ to 5.6 eV, but the increase was short-lived. The changes in Φ over time were correlated with the uptake of carbon impurities in ultra high vacuum (UHV), as monitored by AES.

The HREELS of ITO revealed significant hydrocarbon impurities. Chemical reduction of ITO produced a metallic surface and dehydrogenated the adsorbed hydrocarbons. Both re-oxidation of metallic ITO and oxidation of clean ITO temporarily removed adventitious carbon from the surface, but oxidized ITO adsorbed an even larger quantity of carbon over time.     

Three-dimensional cytoplasmic calcium propagation with boundaries

Ca²⁺plays an important role in cell signal transduction.Its intracellular propagation is the most basic process of Ca²⁺signaling,such as calcium wave and double messenger system.In this work,with both numerical simulation and mean field ansatz,the three-dimensional probability distribution of Ca²⁺,which is read out by phosphorylation,is studied in two scenarios with boundaries.The coverage of distribution of Ca²⁺is found at an order of magnitude ofμm,which is consistent with experimental observed calcium spike and wave.Our results suggest that the double messenger system may occur in the ER-PM junction to acquire great efficiency.The buffer effect of kinase is also discussed by calculating the average position of phosphorylations and free Ca²⁺.The results are helpful to understand the mechanism of Ca²⁺signaling.     

Investigation of 3D Dirac semimetal supported terahertz dielectric-loaded plasmonic waveguides

The tunable propagation properties of 3D Dirac semimetal (DSM)-supported dielectric-loaded surface plasmons structures have been investigated in the THz regime, including the influences of the Fermi level of 3D DSM layer, the fiber shape and operation frequencies. The results indicate that the shape of dielectric fiber affects the hybrid mode significantly, on the condition that if a_x (the semi-minor axis length of the dielectric semi-ellipse) is relatively small, the fiber shows good mode confinement and low loss simultaneously, and the figure of merit reaches more than 200. The propagation property can be manipulated in a wide range by changing the Fermi level of 3D DSM, e.g. if the Fermi level varies in the range of 0.05 eV–0.15 eV, the propagation length changes in the range of 9.073×10³–2.715×10⁴ μm, and the corresponding modulation depth is 66.5%. These results are very helpful to understand the tunable mechanisms of the 3D DSM plasmonic devices, such as switchers, modulators, and sensors.     

准晶体结构光纤表面等离子体共振传感器特性研究

光纤表面等离子体共振传感器在高灵敏度传感和在线实时监测等领域具有重要意义. 设计了一种六重准晶体结构环形通道光纤表面等离子体共振传感器, 基于有限元法对该传感器的传感特性进行了数值模拟. 研究了光纤各结构参量对传感器特性的影响规律. 研究结果表明: 待测液折射率的有效监测范围为1.25–1.331, 最高灵敏度可达26400 nm·RIU^-1, 传感器具有损耗谱杂峰少、探测范围广、灵敏度高、设计灵活性高和光路可弯曲等特点, 在生化检测、公共安全、环境污染监测以及高灵敏度传感等领域具有广泛的应用前景.     

Surface plasmon resonance based fiber optic sensor utilizing indium oxide

A highly sensitive surface plasmon resonance (SPR) based fiber optic sensor with indium oxide (In₂O₃) layer coated on the core of the optical fiber is presented and theoretically analyzed. The sensitivity of the SPR based fiber optic sensor has been evaluated numerically. It is shown that the proposed SPR based fiber optic sensor with In₂O₃ layer possesses high sensitivity in the near infrared region of spectrum, which needs attention to many environmental and security applications and offers more accurate and highly reproducible measurements. In addition, the sensitivity of the SPR based fiber optic sensor decreases with the increase in the thickness of In₂O₃ layer. With sensitivity as high as 4600 nm/RIU, the 170 nm thick In₂O₃ layer based fiber optic SPR sensor demonstrates better performance.     

光纤SPR湿敏传感器及其共振光谱特性研究

提出并研制了基于光纤SPR传感探针的新型湿敏传感器。首先研究了光纤SPR传感探针对环境湿度变化的敏感特性,在此基础上提出在光纤SPR传感探针表面增覆不同厚度且具有水分子吸附功能的PVA薄膜来实现环境相对湿度的监测。研究结果表明,增覆双层PVA薄膜的光纤SPR传感探针在高湿区具有较好监测效果,其共振强度对应的相对湿度测量灵敏度达到1.59%/%RH,较光纤SPR探针呈现显著提高。而增覆单层PVA薄膜的光纤SPR传感探针在高湿区共振波长对应的相对湿度监测灵敏度达到2.411nm/%RH。此外所提出的新型光纤SPR湿敏探针在PVA薄膜失效后经过特殊工艺处理仍可重复镀膜使用。     

Numerical study of a highly sensitive surface plasmon resonance sensor based on circular-lattice holey fiber

A new design of surface plasmon resonance (SPR) sensor employing circular-lattice holey fiber to achieve high-sensitivity detection is proposed. The sensing performance of the proposed sensor is numerically investigated and the results indicate that our proposed SPR sensor can be applied to the near-mid infrared detection. Moreover, the maximum wavelength sensitivity of our proposed sensor can reach as high as 1.76×10⁴ nm/refractive index unit (RIU) and the maximum wavelength interrogation resolution can be up to 5.68×10^-6 RIU when the refractive index (RI) of analyte lies in (1.31, 1.36). Thanks to its excellent sensing performance, our proposed SPR sensor will have great potential applications for biological analytes detection, food safety control, bio-molecules detection and so on.     

Mono-top signature from stop decay at the HE-LHC

Searching for the top squark(stop)is a key task to test the naturalness of SUSY.Different from stop pair production,single stop production relies on its electroweak properties and can provide some unique signatures.Following the single production process pp→t^~1X(~)1→tX^~1⁰X^~1^-,the top quark has two decay channels:leptonic channel and hadronic channel.In this paper,we probe the observability of these two channels in a simplified minimal supersymmetric standard model scenario.We find that,at the 27 TeV LHC with the integrated luminosity of L=15 ab^-1,mt^-1<1900 GeV andμ<750 GeV can be excluded at 2σthrough the leptonic mono-top channel,while m_t^-1<1200 GeV andμ<350 GeV can be excluded at 2σthrough the hadronic channel.     

基于全相位滤波技术的光纤表面等离子体共振传感解调算法

基于生物样品检测对折射率传感的迫切需求,构建一种全光纤表面等离子体共振(surface plasmon resonance,SPR)系统,并针对其设计了基于全相位滤波技术的SPR特征波长传感解调算法.基于系统仿真,理论计算了光纤SPR传感器的折射率传感灵敏度.采用全相位滤波技术提取光纤SPR传感器透射光谱的特征波长,理论推导了全相位滤波器的解析表达式.实验结果表明,使用本算法的光纤SPR传感器折射率传感灵敏度为1640.4 nm/RIU,折射率检测的分辨率是7.36×10~(-4)RIU,与传统方法相比,有效提高了系统的检测精度和抗光源扰动性能,降低了实验成本.     

Surface plasmon resonance based tapered fiber optic sensor with different taper profiles

A theoretical model for surface plasmon resonance (SPR) based tapered fiber optic sensor is proposed with three different taper profiles, namely, linear, parabolic, and exponential-linear. The effect of taper ratio and taper profiles on the sensor’s performance is studied in detail and the design considerations for significantly enhanced sensitivity are reported. The study shows that the exponential-linear taper profile with high taper ratio provides the best performance. The physical reasons behind sensitivity enhancement due to taper ratio and taper profile are given, wherever required.     

Theoretical analysis of surface plasmon resonance based fiber optic sensor using indium nitride

An extremely sensitive surface plasmon resonance based fiber optic sensor with indium nitride (InN) layer coated on the core of the optical fiber is theoretically analyzed. The proposed sensor exhibits high sensitivity in the near infrared region of spectrum. The optimized value of thickness of InN layer is found to be 70 nm. Possessing high sensitivity of 4493 nm/RIU, the 70 nm thick InN layer based fiber optic SPR sensor illustrates good sensing behavior.     

Decay properties of the X(3872) through the Fierz rearrangement

We systematically construct all the tetraquark currents of J^PC = 1⁺⁺ with the quark configurations $[{cq}][\bar{c}\bar{q}]$, $[\bar{c}q][\bar{q}c]$, and $[\bar{c}c][\bar{q}q]$ (q = u/d). Their relations are derived using the Fierz rearrangement of the Dirac and color indices, through which we study decay properties of the X(3872) under both the compact tetraquark and hadronic molecule interpretations. We conduct a search for the X(3872) → χ_c0π, η_cππ, and χ_c1ππ decay processes in particle experiments.     

基于光纤SPR光谱分析的水质矿化度检测研究

从溶液离子影响表面等离子体共振(SPR)光谱特征的角度,分析讨论了光纤SPR光谱对水溶液离子成分检测的灵敏特征,基于此并应用于以矿化度为代表的水质检测中。研究通过对不同离子状态的电解质溶液(NaCl,KCl,CaCl₂,MgCl₂,Na₂CO₃,MgSO₄和ZnSO₄)和非电解质溶液(蔗糖、丙三醇、葡萄糖)下的光纤SPR光谱分析,得到水环境的杂质离子含量对SPR光谱的影响规律,进而实现了水质矿化度的检测。研究同时给出了光纤SPR光谱法与电导率分析法在八种不同水样的检测对比分析,光纤SPR光谱法拥有高灵敏度、快速响应、抗电磁干扰等优点,对光纤SPR技术在水质检测领域的应用打下良好的基础。     

Consistency of optimizing finite-time Carnot engines with the low-dissipation model in the two-level atomic heat engine

The efficiency at the maximum power (EMP) for finite-time Carnot engines established with the low-dissipation model, relies significantly on the assumption of the inverse proportion scaling of the irreversible entropy generation ΔS^(ir) on the operation time τ, i.e. ΔS^(ir) ∝ 1/τ. The optimal operation time of the finite-time isothermal process for EMP has to be within the valid regime of the inverse proportion scaling. Yet, such consistency was not tested due to the unknown coefficient of the 1/τ-scaling. In this paper, we reveal that the optimization of the finite-time two-level atomic Carnot engines with the low-dissipation model is consistent only in the regime of η_C < 2(1 − δ)/(1 + δ), where η_C is the Carnot efficiency, and δ is the compression ratio in energy level difference of the heat engine cycle. In the large-η_C regime, the operation time for EMP obtained with the low-dissipation model is not within the valid regime of the 1/τ-scaling, and the exact EMP of the engine is found to surpass the well-known bound η₊ = η_C/(2 − η_C).     

波长和强度同时响应的锥形多模光纤温度传感器

通过将一段长为17 mm的多模光纤两端分别与单模光纤对芯熔接,然后对多模光纤部分进行拉锥处理,得到一种波长和强度同时对温度响应的锥形多模光纤温度传感器。实验研究了30 ℃~80 ℃范围内传感器的温度传感特性。实验结果表明:当环境温度发生变化时,该传感器在1 542 nm附近干涉波谷的波长和强度对温度的响应灵敏度分别可达到0. 041 nm/℃和0. 106 dB/℃,并且传感器干涉条纹的波长响应和强度响应之间呈良好的线性关系。基于传感器波长响应与强度响应之间的该线性关系,通过传感信号强度的检测即可实现干涉型光纤传感器的相位解调,该方法为传感解调信号提供了新思路,具有重要的参考价值。     

Structural properties of diamond fine particles and clusters prepared by detonation and decomposition of TNT

The thermal parameter B for three different particle sizes of diamond samples (bulk powder 1–4 μm, fine particle 144–195 Å and cluster 55–61 Å) was determined by the grazing incidence X-ray diffraction method. The values of B were found to be in the range 0.50–0.70 Å² for particles in the size range 195–55 Å and 0.27 Å² for 1–4 μm. All of them are larger than that of diamond bulk. A clear size dependence of B, increasing with decreasing particle size, was found. By analysing X-ray diffraction data at several temperatures the magnitude of B was found to be due to B_S (static part) instead of B_T (dynamic part). The average B_S values obtained were 0.04 Å², 0.19 Å² and 0.27 Å² for bulk powder, fine particle and cluster samples respectively. Ultrahigh resolution transmission electron microscope (TEM) observation confirmed the presence of strain, distortion, roughness and dislocation lines in many particles. TEM images of particles indicate that the clusters were not spherical in shape; they were mostly cubiform and some were truncated prism-like polyhedral. The present study reveals that the B_S component is responsible for the large B value in diamond fine particles and clusters. No clear surface local atomic distortion was found in the particles.