一种在光抽运实验中检测射频共振的新方法

利用微波-射频多量子跃迁对单量子微波跃迁谱线强度的影响,我们在实验上找到了一种在光抽运实验中观察射频共振的灵敏的新方法。 关键词：     

光抽运实验中的微波-射频多量子跃迁

在⁸⁷Rb气泡光抽运实验中,我们同时用微波场和射频场作用在⁸⁷Rb原子上,观察到了⁸⁷Rb原子基态微波-射频多量子跃迁的光检测共振谱线。 关键词：     

光磁共振实验中双量子跃迁及射频场谐波干扰

由于射频场谐波的存在,致使其二次谐波的共振跃迁与双量子跃迁信号重叠。因此观察双量子跃迁,必须首先排除射频场二次谐波共振的影响,本文分析了光磁双共振实验中关于双量子跃迁产生的条件、判断和观测,并分析了多频率共振的原因。     

铷原子蒸气中超精细基态的双光子相干操控

二能级量子体系的相干操控对于精密测量和量子信息处理非常重要,如原子钟、原子干涉仪和量子计算等。在实验上观察到相干微波-射频(MW-RF)场驱动下的铷原子超精细基态的双光子Rabi振荡现象。基于塞曼子能级之间热弛豫过程的标定和微波跃迁的测量,清晰地分辨出叠加有热弛豫过程的原子态布居相干振荡。实验测得并详细讨论了广义Rabi频率与中间态失谐和微波/射频功率的关系。当中间态失谐较大时,实验结果与等效二能级理论模型非常吻合;但当中间态失谐较小时,少量原子占据中间态造成实测的Rabi频率偏离理论值。这些结果为二能级量子系统的相干操控提供了有力的理论支持。     

啁啾微波场中里德伯锂原子的相干激发与控制

运用含时多态展开方法和B-样条函数研究了微波场中里德伯锂原子高激发态的性质,得到锂原子量子态n=70-75,l=0-5的能量,并分析了里德伯锂原子高激发态n=70-75,l=0-5在微波场中的跃迁几率.结果表明:通过优化微波场参数可以实现量子系统从初始态到目标态的完全跃迁,且在跃迁过程中,每个l态都起至关重要的作用.     

光泵磁共振信号幅度与射频场振幅的关系

在光泵磁共振实验中观测到单量子跃迁共振信号幅度随射频场振幅增加而迅速增加,并很快达到饱和,然后单调缓慢下降的关系.当射频场振幅更大时(约大于3.5V),观测到双量子跃迁共振信号,信号幅度与射频场振幅成二次函数关系.本文对实验结果进行了分析和解释.     

高阶多量子跃迁的一维直接检测——Raman磁共振方法

研究了异核AX₃自旋体系的初始态为最高阶量子相干态时的Raman磁共振谱.研究表明,唯有制备高阶多量子相干的初始态时才有可能对高阶多量子跃迁进行有效检测.积算符理论的精确性使得理论上准确地预言了Raman磁共振谱中各阶多量子跃迁频率、谱线强度,使得各阶多量子跃迁频率相互交错时仍有可能解析谱图.在Raman磁共振实验中采用了正负频偏交替变化采样的方法,对单量子信号进行压制,使其更有效地观察高阶多量子跃迁.     

应用积算符理论研究弱耦合双自旋体系的Raman磁共振谱

从积算符理论和实验上详细地研究了弱耦合双自旋体系（CHCl₃的C-H双自旋体系）的Raman磁共振谱．对不同射频场强度及频偏的Raman谱进行了细致的理论和实验研究，表明积算符理论的计算与实验不仅在弱射频场而且在强射频场时都符合得相当好，克服了微扰论的局限，这为进一步研究复杂自旋体系的Raman谱提供了强有力的理论方法．研究还表明，小的射频频偏将有利于多量子跃迁信号的观测，而适当的射频场强则会提高多量子峰的强度 关键词：     

微波场驱动下V型三能级原子的吸收和色散特性

当用微波场作用到V型三能级原子的两个激发态能级时,系统跃迁路径之间发生交叉耦合导致了量子相干效应.通过调节微波场的强度,可实现对原子吸收和色散性质的改变,并呈现零吸收高折射率现象.此外,微波场诱导的量子相干也可实现相对相位对探测光增益的控制.     

微波场驱动下V型三能级原子的吸收和色散特性

当用微波场作用到V型三能级原子的两个激发态能级时,系统跃迁路径之间发生交叉耦合导致了量子相干效应.通过调节微波场的强度,可实现对原子吸收和色散性质的改变,并呈现零吸收高折射率现象.此外,微波场诱导的量子相干也可实现相对相位对探测光增益的控制.     

Synchronized double rotation 2D NMR

Analytical expressions for multi-quantum signal generation of quadrupole nuclei have been derived. Combined with numerical simulation of the double rotor motion, a strategy is suggested for partial sideband suppression in multi-quantum NMR spectra. Synchronization of multi-quantum excitation and selective flip pulses with outer rotor motion increase outer rotor speed effectively two times. This is also demonstrated experimentally by triple–single quantum correlation spectra of ²³Na and ⁶⁷Rb.     

A new multi-quantum version of the HBHA(CBCACO)NH experiment with enhanced sensitivity for partially deuterated samples

A new multi-quantum version of the HBHA(CBCACO)NH experiment for partially deuterated protein samples is presented. The method is based on the significant reduction of the proton and carbon relaxation rates due to multi-quantum delays in highly deuterated proteins recently published by our group. The introduction of a multi-quantum period in the coherence transfer pathway of the HBHA(CBCACO)NH experiment yields a dramatic increase of sensitivity-on average 46% with a 75% deuterated sample of the homodimeric 31 kDa E. coli IIAMan domain. Additional resolution in the proton dimension can be achieved by a double time shared approach keeping the 1H single-quantum period at a minimum.     

Application of band theory to experimental eigen-state energies of In0.53Ga0.47As quantum wells lattice-matched to InP

Nonparabolic band structure of InGaAs/InAlAs multi-quantum wells was studied theoretically and experimentally. The electron effective mass was derived even from eigen-states and this nonparabolicity was explicitly determined as a function of energy. Electron eigen-state energies applying Kane’s bulk band theory fitted very well with our experiments in the multi-quantum wells.     

电子全息方法测定GaN/AlGaN多量子阱结构的极性

介绍一种通过用电子全息方法测定GaN/AlGaN多量子阱结构生长极性的方法. 该方法可以分别测量多量子阱结构中各层内建电场方向. 由于多量子阱结构中的内建电场是由各层膜中的极化共同作用产生的，电场的方向和生长极性有确定的对应关系，所以通过测定内建电场的方向就可以确定结构的生长极性. 还用会聚束电子衍射方法对电子全息方法的测定结果进行了验证. 关键词： 电子全息 生长极性 极化     

Effect of annealing on photoluminescence and microstructures of InGaN／GaN multi-quantum well with Mg-doped p-type GaN

InGaN/GaN multi-quantum well structure with Mg-doped p-type GaN was grown by low-pressure metalorganic vapour phase epitaxy. After rapid-thermal-annealing at 700 and 900${^\circ}$C, both the red-shift and the blue-shift of the photoluminescence (PL) peak, the decreased and the enhancement of the PL intensity were observed. The transmission electron microscopic images showed that InGaN multi-quantum-dots-like (MQD-like) structures with dimensions less than 5$\tm$10nm were formed in InGaN wells. The changes of PL spectra could be tentatively attributed to the competition between the red-shift mechanism of the quantum-confined Stark effect and the blue-shift mechanism of the quantum size effect due to MQD-like structures.     

Multi-quantum photoconductivity in Cdln2S4

A study has been made of photoconductivity in Cdln₂S₄ induced by 1.17 eV photons from a Q-switched neodymium laser. Both three-photon absorption, and two-photon absorption involving the emission of a phonon, have been investigated. The experimental data are in satisfactory agreement with the theory of multi-quantum transitions which takes into account the peculiarities of crystal zone structure.The investigation of competing multi-quantum transitions is a new method which permits one to obtain information on the fundamental optical constants of solids.     

Electronic Green's functions in a T-shaped multi-quantum dot system

We developed a set of equations to calculate the electronic Green's functions in a T-shaped multi-quantum dot system using the equation of motion method. We model the system using a generalized Anderson Hamiltonian which accounts for finite intradot on-site Coulomb interaction in all component dots as well as for the interdot electron tunneling between adjacent quantum dots. Our results are obtained within and beyond the Hartree–Fock approximation and provide a path to evaluate all the electronic correlations in the multi-quantum dot system in the Coulomb blockade regime. Both approximations provide information on the physical effects related to the finite intradot on-site Coulomb interaction. As a particular example for our generalized results, we considered the simplest T-shaped system consisting of two dots and proved that our approximation introduces important corrections in the detector and side dots Green's functions, and implicitly in the evaluation of the system's transport properties. The multi-quantum dot T-shaped setup may be of interest for the practical realization of qubit states in quantum dot systems.     

2H T2rho relaxation dynamics and double-quantum filtered NMR studies

In this study 2H T2rho DQF NMR spectra of water in MCM-41 were measured. The T2rho double-quantum filtered (DQF) NMR signal is generated by applying a radio frequency (RF) field for various durations and then observed after a monitor RF pulse. It was found that the transfer between different quantum coherences by the couplings during long-duration RF fields (i.e., soft pulses) and that residual quadrupolar interaction dominates the signal decay. Knowledge of coherence transfer during long-RF pulses has special significance for the development of sophisticated multi-quantum NMR experiments especially multi-quantum MRI applications.     

Characterisation of the influence of multi-quantum barrier reflectors within GaInP/AlGaInP quantum well lasers using near-field imaging techniques

Using a near-field scanning optical microscope, near-field photocurrent and topographic imaging has measured the effect on intrinsic electric fields and photocurrent propagation resulting from inserting multi-quantum barrier (MQB) super-lattices into quantum well lasers. Measurements on devices at two different excitation wavelengths have highlighted the sensitivity of the near-field optical technique. Strong correlations were seen in the photocurrent response of the multi-quantum barrier regions when compared with simulations made on the electric field generated within the structure. As a result, photocurrent attenuation was attributed to carrier confinement in these barrier regions when compared to a control sample. The measurements illustrate the effectiveness of the MQB, in addition to the sensitivity and power of the near-field photocurrent technique.