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1.
Soil samples were collected from different localities of districts Jhelum, Chakwal, Rawalpindi and Attock, Punjab Province, Pakistan with an aim to measure naturally occurring radionuclides, namely 226Ra, 232Th, 40K and fallout 137Cs radionuclide using a P-type coaxial high purity germanium (HPGe) γ-ray spectrometer. Measured specific activities of 226Ra, 232Th and 40K in these soil samples ranged from 26.02 ± 7.11 to 93.54 ± 8.13 Bq kg−1, 29.34 ± 2.58 to 114.41 ± 2.80 Bq kg−1 and 348.15 ± 3.20 to 752.98 ± 4.20 Bq kg−1, respectively. Activity due to 137Cs was observed in some locations which ranged from 0.4 ± 0.2 to 7.8 ± 0.3 Bq kg−1. From the measured activity concentrations, radium equivalent activity concentrations were determined followed by calculations of mean absorbed dose rate and mean annual effective dose for the inhabitants of the studied area. The mean radium equivalent activity, internal and external hazard indices values came out to be 179.26 ± 11.93 Bq kg−1, 0.64 ± 0.05 and 0.48 ± 0.03, respectively. Indoors and outdoor average annual effective dose values were found to be 0.42 ± 0.03 and 0.10 ± 0.01 mSv, respectively. Present data have been compared with the published data for other parts of the world and found to be safe for public and environment.  相似文献   

2.
The naturally occurring radioisotopes such as 238U, 232Th and 40K in the silt samples collected from Moticher lake, Gujarat were evaluated. The activity of 238U, 232Th and 40K was found to be 4.4-9.7 Bq kg−1 with a mean 6.4 ± 1.3 Bq kg−1, 10.5–21.2 Bq kg−1 with a mean 15.6 ± 2.5 Bq kg−1 and 102–231 Bq kg−1 with a mean 160 ± 40 Bq kg−1, respectively. The depth profile study could not reveal any significant vertical correlation on radioactivity levels of 238U, 232Th and 40K. Radium equivalent activity (Raeq), external hazard index (H ex) and internal hazard index (H int) were calculated by using the activity of 238U or 226Ra, 232Th and 40K in silt samples. Annual Effective Dose Equivalent (AEDE) level in Moticher silt was found to be 24.8 ± 5.0 μSv year−1, which is much lower than the worldwide average value. The relative contribution to dose due to 238U and 232Th series were found to be 14% and 53%, followed by the contribution of 33% due to 40K.  相似文献   

3.
This paper presents the results of measurement of natural and fallout radioactivity in soil samples of Chamba and Dharamshala areas in Himachal Pradesh, India. Spatial distribution of 238U, 226Ra, 232Th, 40K, 137Cs was determined using High resolution gamma-ray spectrometry. The mean activity concentration in Chamba region due to 238U, 232Th, 40K and 137Cs was 32.3, 58.4, 588.3, and 10.9 Bq kg−1, respectively, whereas in Dharamshala it was 35.7, 61.3, 594.9, 10.0 Bq kg−1, respectively. Absorbed gamma dose rate (D) in air was calculated using appropriate dose conversion factors, which was varying from 45 to 103 nGy h−1. To control the radiation exposure due to natural radioactivity in soil, if it is used as building materials, radium equivalent activity (Raeq) and activity index were also evaluated. Radium equivalent activity calculated for the soil ranged from 95.5 to 234.2 Bq kg−1 with average of 171.0 Bq kg−1.The calculated Activity concentration index was ranged from 0.34 to 0.85 with an average value of 0.64. The natural and fallout radioactivity in soil of this region is comparable with Indian average and other parts of the world. The percentage contribution of 238U, 232Th and 40K and 137Cs to the average external gamma dose rate was 22, 46, 32, 2%, respectively. This shows that the dose contribution due to fallout radioactivity is negligible as compared to the natural radioactivity.  相似文献   

4.
The present work investigated the activity concentrations of natural radionuclides 226Ra, 232Th and 40K in beach sand samples along coastal Kerala including high background radiation area. The activity of 232Th ranges from below detectable level to 23029.9 Bq kg−1 with a mean value of 2660.2 Bq kg−1 for 0–10 cm depth interval. For 10–20 cm depth, the 232Th activity ranged from below detectable to 4452.2 Bq kg−1 with a mean value of 815.5 Bq kg−1. The variation of 226Ra activity with depth is parallel with the 232Th activity distribution in beach sand. Its activity varied from below detectable to 5169.5 Bq kg−1 with a mean value 487.6 Bq kg−1 at 0–10 cm depth. For 10–20 cm depth interval, the 226Ra activity ranges from below detectable to 1823.6 Bq kg−1 with a mean value 296.0 Bq kg−1. Similarly the activity varies from below detectable to 1826.6 Bq kg−1 with a mean value of 211.0 Bq kg−1 for a depth interval of 20–30 cm. The activity of 40K at different depth is also discussed. Statistical analysis of radioactivity was also carried out. The results of these investigations are presented in this paper.  相似文献   

5.
In this study the concentration of natural radionuclides has been investigated in soil and water of Karun river by using a high resolution (HPGe detector, n-type) γ-spectrometry. The concentrations range in water sample was 47.6 ± 5.6–130.8 ± 6.3, 0.0–23.4 ± 0.5 and 0–6.4 ± 2.0 Bq L−1 for 40K, 232Th and 226Ra respectively. For soil samples the concentration range of 275.7 ± 8.6–458.6 ± 6.8, 19.2 ± 5.35–41.1 ± 3.95 and 29.9 ± 1.53–50 ± 1.54 Bq kg−1 was obtained respectively for 40K, 232Th and 238U. 137Cs was also detected in some part of the region in soil samples. The mean concentration of 137Cs was 5.5 ± 0.6 Bq kg−1. The origin of this activity is unknown. The average absorbed dose rate in outdoor air at a height of 1 m above the ground was found to be 54.3 ± 3.7 nGy h−1. The results of this study indicate that the area has standard background radiation level.  相似文献   

6.
This study presents the high purity germanium (HPGe) gamma spectrometric measurement of natural radioactivity mainly due to 226Ra, 232Th and 40K in soil samples collected in Ferozepur and Faridkot district of Punjab, India. 226Ra activity varied from 28.6 to 51.1 Bq kg−1 with the mean of 39.7 Bq kg−1. The range and mean activity of 232Th were 42.9–73.2 and 58.2 Bq kg−1, respectively. 40K activity was in the range of 470.9–754.9 Bq kg−1 with the mean of 595.2 Bq kg−1. The air kerma rate (AKR) at 1 m height from the ground was also measured using gamma survey meter in all the sampling locations, which was ranging from 92.1 to 122.8 nGy h−1 with the mean of 110.6 nGy h−1. The radiological parameters such as Raeq and activity index of the soil samples were also evaluated, which are the tools to assess the external radiation hazard due to building materials. The mean and range of the Raeq values were 168.7 and 132.9–210.4 Bq kg−1, respectively, whereas the activity index varied from 0.5 to 0.8 with the mean value of 0.62. These indices show that the indoor external dose due to natural radioactivity in the soil used for the construction will not exceed the dose criteria. The AKR was also evaluated from soil activity concentration and altitude correction of cosmic radiation contribution. The statistical tests such as Pearson correlation, spearman rank correlation, box and whisker plot, the Wilcoxon/Mann–Whitney test and chi-square test, were used to compare the measured AKR with evaluated AKR, which indicates good correlation.  相似文献   

7.
In this work, the radionuclide activity concentrations of 226Ra, 232Th and 40K in surface soils and radon levels in dwellings of Karabük, Turkey were determined in order to evaluate the environmental radioactivity. Concentrations of 226Ra, 232Th and 40K radionuclides were determined using gamma spectrometry with using HPGe detector. The etch track detectors (CR-39) were used to determine the distribution of radon concentrations. The average activity concentrations for 226Ra, 232Th and 40K were found as 21.0, 23.5 and 363.5 Bq kg−1, respectively. The calculated average annual effective dose equivalent from the outdoor terrestrial gamma radiation from 226Ra, 232Th and 40K is 53.5 μSv y−1. The average radon concentration and annual effective dose equivalent of 222Rn in Karabük dwellings were obtained 131.6 Bqm−3 and 3.32 mSv y−1, respectively. The evaluated data were compared with the data obtained from different countries.  相似文献   

8.
226Ra activity concentration in the mullet (Mugilidae) species Mugil cephalus whole individuals, and some organs (gills, gastrointestinal system, fins, muscle and bones), was measured by the γ-coincidence spectrometer PRIPYAT-2M. 226Ra transfer parameters [concentration factors (CFs)] from seawater, sediment and mud with detritus to fish tissues, and annual intake by humans consuming this fish species, have been estimated. Minimum detected radium activity concentration in whole M. cephalus individuals was found to be 0.89 ± 0.42 to 3.09 ± 0.41 Bq kg−1, with arithmetic mean of 1.65 ± 0.39 Bq kg−1. An average concentration in muscles is found to be 2.28 ± 0.84 Bq kg−1, in gills—5.02 ± 1.85 Bq kg−1, in gastrointestinal system—12.88 ± 1.71 Bq kg−1, and in bones—14.72 ± 3.75 Bq kg−1. No one fins showed radium activity above minimum detectable one. Annual intake of 226Ra by human consumers of this fish species is estimated to provide an effective dose of 0.006 mSv year−1. CFs for 226Ra indicating transfer from seawater to whole individuals ranged from 8.9 to 30.9, and those indicating transfer from the sediment and mud with detritus—from 0.11 to 0.39 and from 0.08 to 0.3, respectively. The seawater to bones CFs varied from 97.9 to 197.3, to gastrointestinal system—from 59 to 178.8, to gills—from 22.5 to 68.3, to muscles—from 17 to 30.8.  相似文献   

9.
In the present study, mussel (Mytilus galloprovincialis, Lamarck, 1819) and sediment samples were collected from the Bosphorus strait and the Golden Horn estuary in 2008 and 2009. Activity concentrations of 137Cs, 40K, 232Th and 238U were measured using a gamma spectrometer equipped with HPGe detector. Sediment samples were separated into <63 μm and >63 μm particle fractions. Analysis of radionuclides was carried out on these two fractions of sediment as well as the soft and shell tissues of mussels. Ranges of radioactivity concentrations in the soft parts of mussels were as follows: 137Cs, 0.86–2.43; 40K: 261.1–496.7; 232Th: 0.49–3.58; and 238U: BDL (below detection limit)-1.38 Bq kg−1 in dry weight. Ranges of radioactivity concentrations in the <63 and >63 sediment fractions were as follows: 137Cs, 8.58–67.92 and 1.12–26.40, 40K, 341.4–683.0 and 281.9–662.2; 232Th, 10.97–20.16 and 7.18–19.18 and 238U, 13.97–27.25 and 6.41–18 Bq kg−1 in dry weight, respectively. The effect of some physical–chemical parameters on the radionuclide accumulation was also examined in the sediment samples. All data in the current study were compared with data in the literature.  相似文献   

10.

The radioactivity concentrations of 226Ra, 232Th and 40K in 42 samples from different types of cements produced in Turkey were measured using gamma-ray spectrometer. The determined values were 18–143 Bq kg−1 (226Ra), 5–66 Bq kg−1 (232Th) and 142–540 Bq kg−1 (40K). Additionally, the calculated radiological hazard parameters such as absorbed dose rate, annual effective dose, radium equivalent activity, the external hazard, activity and alpha indices were found to be in the range of 38–158 nGy h−1, 188–776 µSv year−1, 41–182 Bq kg−1, 0.11–0.49, 0.15–0.65 and 0.09–0.71, respectively. Finally, the results were statistically evaluated and compared with the reported data in other countries and the international standard values given by European Commission and UNSCEAR.

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11.
137Cs activity concentrations were determined in samples of macrophytes Polysiphonia fucoides (red algae) and Zostera marina (vascular plant) collected during the entire vegetation season in the Gulf of Gdańsk in the southern Baltic Sea. The measurements showed considerable seasonality of 137Cs activity in both species; an increase of cesium concentrations was observed from spring to autumn with maximal levels 49.1 ± 1.4 Bq kgd.w.−1 (P. fucoides) and 14.5 ± 1.0 Bq kgd.w.−1 (Z. marina) in late autumn. 137Cs concentrations observed in a given season are the result of a number of processes, the intensity of which can differ depending on external environmental conditions. The effects of these processes can differ and their directions can frequently be opposite to one another. The examined macrophytobenthic plant species could serve as bioindicators of radionuclide pollution for monitoring purposes on condition that the samples of plants are taken within a strictly defined period of the year to give comparable results and to supply realistic information about pollution levels.  相似文献   

12.
This work presents the results of 137Cs, 40K, 232Th and 238U concentration (Bq kg−1) values in coastal marine sediments collected from 38 sites along the coastline of the island of Margarita, Venezuela. The purpose was to determine baseline values for these radionuclides in surface marine sediments and to detect if there were any anomalously high concentration values. Only three of the 38 sediments analyzed had measurable values above the detection limit of 0.9 Bq kg−1 for 137Cs and the highest only being 1.4 Bq kg−1. While, the concentration (Bq kg−1) ranges for the primordial radionuclides, 40K, 232Th and 238U were as follows: 12.2–211.7, <1.5–9.8 and <4.4–20.7, respectively. These concentration ranges for the primordial radionuclides can be considered as baseline values for surface marine sediments for areas that are considered not polluted by man or contaminated by nature. Finally, the concentration range of 137Cs can also be employed as baseline values, which only seem to have been the result of the atmospheric testing of nuclear weapons in the past.  相似文献   

13.

The mineral extraction activities may disturb the natural radioactivity, therefore current study aims to generate baseline data of natural radionuclides and anthropogenic 137Cs before the start of industrial activities. Gamma spectrometry and gross alpha and beta counting systems were used for activity measurement in environmental samples. In soil, the mean activity of 232Th, 226Ra, 40K and 137Cs were determined as 79 (66–117), 47 (34–80), 823 (602–1159) and 1.3 (1.1–4.5) Bq kg?1, respectively. The average annual effective dose rate (128.7 µSv h?1) in the study area was twice higher than world’s average value. Indoor hazard index was greater than unity at two places; therefore, proper ventilation is proposed during construction.

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14.
The aim of the present work was to determine the concentration of radionuclides in all kinds of tea available at the local Egyptian market. Radioactivity of the nuclides 238U, 226Ra, 210Pb, 228Th, 232Th, 226Ra, 137Cs and 40K were measured in tea by direct γ-ray spectrometry using HPGe detector and their mean values were 16.0±5.3, 3.1±0.7, 34.3±3.4, 3.4±1.2, 3.0±0.6, 3.1±0.8, 0.9±0.2 and 623±25 Bq·kg−1, respectively.  相似文献   

15.

The uptake of natural radioactivity by pasture-grass collected from seven different grasslands of Digor was calculated. The activities of 226Ra, 232Th and 40K in pasture-grass were in the range of 21.8 ± 6.3–49.6 ± 13.4, 51.9 ± 13.2–127.7 ± 23.8 and 309.5 ± 33.5–807.3 ± 64.4 Bq kg−1, respectively. The soil to pasture-grass transfer factors were evaluated and determined to be in the range from 0.26 ± 0.13 to 0.69 ± 0.34, 0.64 ± 0.27 to 1.99 ± 0.40 and 0.64 ± 0.014 to 1.40 ± 0.032 for 226Ra, 232Th and 40K, respectively. The distribution of 226Ra and 232Th in different parts of pasture-grass indicated a decreasing tendency in order of root > stem > leaf. 40K mainly accumulated in stem of pasture-grass and is followed by declining trend stem > leaf > root.

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16.
Determining radioactivity levels in foodstuffs is of great importance for the protection of human health. In addition, the literature includes few studies related to this subject in Turkey. In this study, gamma spectroscopic system was used in order to measure 226Ra, 232Th, 40K and 137Cs activity concentrations in vegetables and fruits produced in Elaz?? Region. The average activity concentrations in vegetables was calculated as 0.64 ± 0.26 Bq kg?1 for 226Ra, 0.65 ± 0.14 Bq kg?1 for 232Th, 13.98 ± 1.22 Bq kg?1 for 40K, and 0.54 ± 0.04 Bq kg?1 for 137Cs. The average activity concentrations in fruits were 1.52 ± 0.34, 0.98 ± 0.23, 18.66 ± 1.13 and 0.59 ± 0.16 Bq kg?1, respectively for 226Ra, 232Th, 40K and 137Cs. Total committed effective dose value was determined as 20 and 30.55 μSv y?1, respectively for vegetables and fruits. The findings were compared with previous data reported for Turkey and other regions of the world.  相似文献   

17.
In this article, we present results obtained from a radiometric survey that was conducted in the Leepa Valley of Azad Jammu & Kashmir, Pakistan. The purpose of current study is to appraise the radioactivity levels and the associated health hazards due to the terrestrial radionuclide in soil and rock samples. In this regard, 16 soil and 17 rock samples were collected from different locations of the Leepa Valley. After processing the samples, activity concentrations of primordial (232Th, 226Ra and 40K) and anthropogenic (137Cs) radionuclides were determined using a P-type coaxial high purity germanium detector. From the results obtained the mean activity concentrations of radionuclides 226Ra, 232Th and 40K in the soil samples were found to be 31.25 ± 0.46, 44.1 ± 1.07 and 575 ± 8.89 Bq kg?1 respectively. Whilst, in rock samples 226Ra, 232Th and 40K mean activities were found as 28.46 ± 0.45, 48.63 ± 1.12 and 666.7 ± 9.39 Bq kg?1, respectively. The 137Cs concentration level in soil and rock samples is found to be 15.04 ± 0.29 and 5.7 ± 0.16 Bq kg?1, respectively. The average radium equivalent activity (R aeq) was found as 143.16 and 142.93 Bq kg?1 in soil and rock samples, respectively. These findings are less than the recommended safe value of 370 Bq kg?1 as given in OECD report (1979). The values of external (H ex) and internal hazard index (H in) are also less than unity. Mean value of absorbed dose rate was found as 69.78 nGy h?1 for the soil samples, which is in good agreement with the world wide average value (70 nGy h?1). Mean value of absorbed dose rate from rock samples was found as 70.01 nGy h?1. Mean values of the annual effective dose is also lower than the values reported for different other countries of the world.  相似文献   

18.
《印度化学会志》2023,100(1):100856
The present work aims to measure and estimate radioactivity and hazardous radiation indices of the soil. Soil samples were collected from various locations in the Visakhapatnam district in Andhra Pradesh, India. The measurement of specific activity of 226Ra, 232Th, and 40K radionuclides is carried out with the help of HP-Ge based gamma spectrometer system. Activity concentration of radionuclides in the samples 226Ra, 232Th and 40K ranged from 20 ± 2 to 91 ± 2 Bq.kg-1, 45 ± 3 to 365 ± 3 Bq.kg-1, and 400 ± 9 to 607 ± 8 Bq.kg-1, and the respective mean values are 53.36 Bq.kg-1, 203.74 Bq.kg-1 and 479.19 Bq.kg-1. The measured mean value of the absorbed dose rate is 171.41 nGy.h-1, which was beyond the worldwide mean outdoor value of 60 nGy.h-1. Thus, the annual effective dose estimated from the above value is 1.04 mSv.y-1. The correlation was done among the measured 226Ra, 232Th, and 40K activity concentrations. The estimated radium equivalent dose is 381.60Bq.kg-1. The estimated health hazard index and annual effective dose rates of dwellers of Visakhapatnam were studied and compared to Indian average values. The study will help to generate the baseline data for assessing hazard indices to the public and geological mapping of natural radiation in India.  相似文献   

19.
We determined 137Cs concentrations in deep water samples of the subtropical gyre in the South Pacific collected during the BEAGLE2003 cruise. This was done at an underground facility to achieve extremely low background γ-spectrometry, and we, therefore, obtained reliable values of 137Cs activity in the deeper layers. 137Cs activity in the layers between 2000 and 4500 m ranged from 7 ± 4 mBq m−3 to 25 ± 11 mBq m−3. The inventory of 137Cs in the water column from 2000 m to the sea bottom was estimated to be 20 ± 8 Bq m−2 to 94 ± 41 Bq m−2 in this region.  相似文献   

20.
The present work investigated the radioactivity level of the rocks samples collected from different sites in Egypt. Twenty one rocks samples were analyzed by gamma-ray spectrometry using NaI(Tl) detector with specially designed shield. The concentration of three natural radionuclides namely 226Ra, 232Th and 40K has been determined and compared with chemical data obtained by XRF analysis. The results showed that these radionuclides were present in concentration ranges (3.4-99, 7.5-134 and 93-3382 Bq kg−1), (54.9-211.6, 20.71-170.5 and 2068-2344 Bq kg−1) and (13-106, 29.25-106.1 and 682-755 Bq kg−1) for gneiss, granite and basalt rocks, respectively, while the values were (7.5, 12.5 and 263.9 Bq kg−1) and (113, 148.5 and 1672 Bq kg−1) for 226Ra, 232Th and 40K in sandstone and siltstone rocks, respectively. Also radium equivalent activity, total dose rates and external hazard index of the rocks samples under consideration were calculated. The results showed that granite rocks contain a high proportion of natural radioactive elements, while sandstone rocks have lesser radioactivity concentration compared with other types of rocks.  相似文献   

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