Polarization properties of stochastic spatially and spectrally partially coherent electromagnetic flat-topped pulses

The propagation behavior of the spectral degree of polarization of stochastic spatially and spectrally partially coherent electromagnetic flat-topped pulses in free space is studied. Numerical calculation results are given to illustrate the dependence of spectral degree of polarization on the beam order, pulse frequency, temporal coherence length, pulse duration and spatial correlation length. It is shown that with increasing beam order M the position z of the on-axis spectral degree of polarization P = 0 decreases, and the distribution of spectral degree of polarization is different for different values of M.     

Processing of metals by double pulses with short laser pulses

Experimental results related to the influence of time delayed pulses for ablation efficiency with short multi pulses (pulse duration of 5 ps) are reported. A significant improvement of the micro structuring quality at relatively high fluence regime in metals is obtained. Less removed or recast matter is observed and the processed surface appears to be smoother with better roughness. Ablation depths and burr heights are compared for single pulses and double pulses in steel, Al and Cu as a function of scans number. Best results are obtained for weak time delays, typically less than 1 ps. PACS 79.20.Ds; 42.62.Cf; 81.65.Cf     

Molecular alignment by trains of short laser pulses

We show that a dramatic field-free molecular alignment can be achieved after exciting molecules with proper trains of strong ultrashort laser pulses. Optimal two- and three-pulse excitation schemes are defined, providing an efficient and robust molecular alignment. This opens new prospects for various applications requiring macroscopic ensembles of highly aligned molecules.     

Numerical modeling of transient progression of plasma formation in biological tissues induced by short laser pulses

A theoretical model based on the rate equation for free electron density is proposed to investigate transient progression of plasma formation in soft biological tissues during laser shock processing. The laser focusing region around the focus point is considered to be one-dimensional along the direction of the incident beam, and is discretized into numerous thin control volumes. In simulation of the transient plasma progression, the laser intensity distribution and the temporal evolution of the free electron density are calculated sequentially for each control volume using a fourth-order Runge–Kutta method with adaptive time step control. The rate-equation formalism is first validated with previously published theoretical and experimental results. Simulation of the dynamics of plasma formation is then performed. The results include temporal evolution and spatial distribution of the free electron density as well as the growth of the plasma. It is shown that the threshold laser intensity for optical breakdown in water and the maximum length of the resulting plasma obtained from the present model are in good agreement with existing experimental data. PACS 42.65.-k; 52.38.-r; 87.80.-y     

Vacuum heating of solid target irradiated by femtosecond laser pulses

The interaction of femtosecond laser pulses with solid targets was studied through experiments and particle-in-cell (PIC) simulations. It is proved that the vacuum heating and the inverse bremsstralung process are the main mechanisms of the laser pulse absorption under such conditions. The distribution of hot electrons and that of X-ray are found to have double-temperature structure, which is confirmed by PIC simulations. While the lower temperature is attributed to the resonant absorption, the higher one, however, is caused by the laser-induced electric field in the target normal direction. The time-integrated spectra ofthe reflected laser pulse shows that the mechanism of electron acceleration is determined by the plasma density profile.     

Independent electron theory of multiple ionization of xenon by intense laser pulses

The intensity dependence of the multiphoton ionization spectra of Xe atoms has been investigated with an improved accuracy and well-controlled laser parameters. In particular, we have examined the ionization rates for X³⁺, X²⁻, X⁺ as functions of the laser intensity and the pressure in the target chamber. The apparatus used for these measurements is characterized by a high-energy resolution (better than 200 meV) and a completely digital acquisition system. The time-of-flight spectra clearly show the contributions of the different isotopes present in Xe gas. The laser pulses have been characterized with great accuracy by monitoring the energy, pulse width and divergence shot by shot. The ionization rates of the different ions have been used for testing the basic assumption of the Geltman theory of multiple ionization based on the single electron ionization model. We have found that for the small intensity range investigated the quantity (dXe ⁺/dI)·(dXe ³⁺/dI)/(dXe ²⁺/dI)² appears to be quite close to the value 0.5 predicted by this model.     

Self-focusing and the initial stages of plasma generation by short laser pulses

When a short high power laser pulse interacts with a transparent solid target in vacuum, radiation in the rising edge of the pulse can self-focus in the solid and cause “damage tracks”. The self-focusing stage of the laser/solid interaction has been studied, a method has been found to suppress the “damage tracks”, and information about the penetration of laser radiation through the critical layer of plasma, in the early stages of the interaction, has been obtained.     

Investigation of ultrafast nuclear spin polarization induced by short laser pulses

We theoretically investigate the dynamics of nuclear spin induced by short laser pulses and show that ultrafast nuclear spin polarization can take place. Combined use of the hyperfine interaction together with the static electric field is the key for that. Specifically we apply the idea to unstable isotopes, (27)Mg and (37)Ca, with nuclear spin of 1/2 and 3/2, respectively, and show that 88% and 62% of nuclear spin polarization can be achieved within a few to tens of ns, which is 2-3 orders of magnitude shorter than the time needed for any known optical methods. Because of its ultrafast nature, our scheme would be very effective not only for stable nuclei but also unstable nuclei with a lifetime as short as mus.     

Excitation of multiple wakefields by short laser pulses in quantum plasmas

We present a theoretical investigation of the excitation of multiple electrostatic wakefields by the ponderomotive force of a short electromagnetic pulse propagating through a dense plasma. It is found that the inclusion of the quantum statistical pressure and quantum electron tunneling effects can qualitatively change the classical behavior of the wakefield. In addition to the well-known plasma oscillation wakefield, with a wavelength of the order of the electron skin depth (λe=c/ωpe, which in a dense plasma is of the order of several nanometers, where c is the speed of light in vacuum and ωpe is the electron plasma frequency), wakefields in dense plasmas with a shorter wavelength (in comparison with λe) are also excited. The wakefields can trap electrons and accelerate them to extremely high energies over nanoscales.     

Amplification of short laser pulses by Raman backscattering in capillary plasmas

Short laser pulses can be significantly amplified in the process of Raman backscattering in plasma inside an oversized dielectric capillary. A dielectric capillary allows obtaining high intensities of the output radiation by sustaining efficient amplification at large distances compared to the diffraction length. The efficiency of the interaction between the pump wave and the amplified pulse is shown not to be critically sensitive to the transverse structure of the wave fields. For a quasi-single-mode initial seed pulse and a low pump intensity, the amplified pulse tends to preserve its transverse structure due to nonlinear competition of the capillary eigen-modes. At a high power of the pump wave, multimode amplification always takes place but the growth of the front peak of the pulse still follows the one-dimensional model. The Raman backscattering instability of the pump wave resulting in the noise amplification can be suppressed in detuned interaction by chirping the pump wave or arranging an inhomogeneous plasma density profile along the trace of amplification. The efficiency of the desired pulse amplification does not significantly depend on detuning in the case of a smooth detuning profile. Density inhomogeneities are shown to exert less influence on the amplification within a capillary than in the one-dimensional problem. Parameters of a future experiment on the Raman amplification of a short laser pulse inside a capillary are proposed.     

Spectroscopic investigation of sparks produced by short laser pulses in He

The spatial and temporal development of the temperature and the electron density of a spark produced in He at 10 atm in the focus of a lens by a mode-locked laser pulse having only 1.5 mJ energy have been investigated. Measuring the absolute intensity of the continuum radiation emitted by the spark and the broadening of a Heii-line it can be concluded that local thermodynamic equilibrium has established 15 ns after the initiation of the plasma. At this time a temperature of 65000 K and a maximum electron density of 1.4·10¹⁹ cm⁻³ was found with a pressure of 20 times the initial gas pressure. These values are in agreement with the values required for an expansion model given in an earlier work basing on a radiation mechanism which explains the stepwise growth of a laser spark under the influence of a train of mode-locked pulses.     

Nanostructuring of thin Au films by means of short UV laser pulses

The particle size distribution, morphology and optical properties of the Au nanoparticle (NP) structures for surface enhanced Raman signal (SERS) application are investigated in dependence on their preparation conditions. The structures are produced from relatively thin Au films (10–20 nm) sputtered on fused silica glass substrate and irradiated with several pulses (6 ns) of laser radiation at 266 nm and at fluencies in the range of 160–412 mJ/cm². The SEM inspection reveals nearly homogeneously distributed, spherical gold particles. Their initial size distribution of the range of 20–60 nm broadens towards larger particle diameters with prolonged irradiation. This is accompanied by an increase in the uncovered surface of the glass substrate and no particle removal is observed. In the absorption profiles of the nanostructures, the broad peak centred at 546 nm is ascribed to resonant absorption of surface plasmons (SPR). The peak position, halfwidth and intensity depend on the shape, size and size distribution of the nanostructured particles in agreement with literature. From peak intensities of the Raman spectra recorded for Rhodamine 6G in the range of 300–1800 cm⁻¹, the relative signal enhancement by factor between 20 and 603 for individual peaks is estimated. The results confirm that the obtained structures can be applied for SERS measurements and sensing.     

Effect of low-threshold air breakdown on material ablation by short laser pulses

Ablative formation of channels in steel by picosecond and nanosecond pulses of Nd lasers was studied. It was found that significant screening of the incident energy (up to 80–90%) in this pulse duration range is caused by breakdown of air contaminated with ablated microparticles. The breakdown threshold, size of particles, and time of their settling down were estimated. It was shown that this kind of plasma screening results in a decrease in the ablation rate and significant channel widening. Practical approaches to eliminate the low-threshold breakdown induced by microparticles were proposed and implemented. These approaches are based on experimental results of the study of the dependences of laser ablation on the pressure and repetition rate. It was shown that a moderate decrease in the pressure below 300–400 mbar makes it possible to avoid screening. In high-repetition-rate ablation, it was found that values above several kilohertz correspond to quasi-vacuum conditions in the ablation spot.     

On the role of prepulses during solid target heating by picosecond laser pulses

X-ray emission spectra of the plasma created at the surface of magnesium, aluminum, copper, and zinc targets heated by 1-ps laser pulses with a peak power density of up to 10¹⁶ W/cm² were measured. The effect of a picosecond prepulse on the spectra was studied for various power densities and intensity contrasts of the main laser pulse. It is established that the emission spectra of laser plasmas are weakly affected by a change from 10⁵ to 10⁷ in the main pulse contrast relative to the first prepulse. Variations in the parameters of emission from aluminum and magnesium plasmas were calculated using relative intensities and widths of the resonance lines of H-and He-like ions and their two-electron satellite peaks.     

Extension of a DNA molecule by local heating with a laser

Thermal convection and thermophoresis induced by mum-scale local heating are shown to elongate a single DNA molecule. An infrared laser used as a point heat source is converged into a dispersion solution of DNA molecules, which is observed under a fluorescent microscope. The thermal convection around the laser focus manifests as extensional flow for the long DNA chain. A simulation of thermal convection that reproduces the experimental condition provides numerical support for the stretching caused by thermal convection. This DNA elongation technique is a novel method for manipulating the intact single DNA molecules, and it can be applied to a "lab on a chip".     

Selective ablation of thin films with short and ultrashort laser pulses

Micromachining of CuInSe₂ (CIS)-based photovoltaic devices with short and ultrashort laser pulses has been investigated. Therefore, ablation thresholds and ablation rates of ZnO, Mo and CuInSe₂ thin films have been measured for irradiation with nanosecond laser pulses of ultraviolet and visible light and subpicosecond laser pulses of a Ti:sapphire laser. The experimental results were compared to the theoretical evaluation of the samples heat regime. In addition, the cells photo-electrical properties were measured before and after laser machining. Scanning electron microscopy (SEM) and energy dispersive X-ray (EDX) analyses were employed to characterise the laser-induced ablation channels. Using nanosecond laser pulses, two phenomena were found to limit the laser-machining process. Residues of Mo that were projected onto the walls of the ablation channel and the metallization of the CuInSe₂ semiconductor close to the channel lead to a shunt. The latter causes the decrease of the photovoltaic efficiency. As a consequence of these limiting effects, only subpicosecond laser pulses allowed the selective or complete ablation of the thin layers without a relevant change of the photo-electrical properties.