超短超强激光脉冲辐照超薄碳膜电离状态研究

为了进一步理解极端条件下物质的电离特性, 特别是超短超强激光脉冲辐照超薄靶时等离子体的形成与分布, 本文以超薄碳膜为例, 细致研究了超短超强激光脉冲辐照下原子的离化过程. 分析和比较了强激光场直接作用电离和靶内静电场电离等两种场致电离形式, 在碰撞电离可以忽略的情况下, 发现更多的电离份额是来自靶内静电场的电离方式. 研究了激光脉冲强度对电离的影响, 发现激光脉冲强度越强, 电离速度越快, 产生的高价态离子所占比例也越高.当激光强度为1×10²⁰ W/cm²时, 尽管该强度高于电离生成C⁺⁶所需要的激光强度阈值, 但该激光脉冲并不能将整个靶电离成C⁺⁶离子, 对此本文进行了详细的分析. 在研究激光脉冲宽度的影响时, 发现激光脉宽越小, 电离速度越快, 但越小的激光脉冲电离获得的高价态离子越少.     

Remarks on stochastic non-linear birth and death models

The first part of this paper is an attempt to formulate and motivate additional work on the important problem of obtaining global bounds applicable to the controlled truncation of the paper relates specifically to the linear birth, quadratic death model. Asymptotic results are given for the first finite difference ΔT_m where T_m is the exactly known mean time to extinction starting from state m (m= 0,1,…). These results are in terms of the environmental carrying capacity n^* taken to be large. For m near zero ΔT_me^n*/(n^*)²; whereas, for m near n^*ΔT_m ≈ (π/2)^1/2/(n^*)^3/2. This indicates the vastly different time scales in those two regions of state space - with considerably slower action near extinction than near n^*.     

Observation of Raman forward scattering and electron accelerationin the relativistic regime

Raman forward scattering (RFS) is observed in the interaction of a high intensity (>10¹⁸ W/cm²) short pulse (<1 ps) laser with an underdense plasma (n_e~10¹⁹ cm ^-3). Electrons are trapped and accelerated up to 44 MeV by the high-amplitude plasma wave produced by RFS. The laser spectrum is strongly modulated by the interaction, showing sidebands at the plasma frequency. Furthermore, as the quiver velocity of the electrons in the high electric field of the laser beam becomes relativistic, various effects are observed which can be attributed to the variation of electron mass with laser intensity     

锶原子光晶格钟自旋极化谱线的探测

87Sr原子存在核自旋,在磁场作用下原子能级会分裂成不同塞曼子能级.通过光抽运对原子进行自旋极化,其自旋极化谱线的探测为锶光钟系统的闭环锁定提供精确的频率参考.本文对~(87)Sr原子钟跃迁能级5s~2~1S_0→5s5p~3P_0中的m_F=+9/2和m_F=-9/2的塞曼磁子能级自旋极化谱线进行了探测.经过一级宽带冷却和二级窄线宽冷却与俘获后,锶冷原子温度为3.9μK,原子数目为3.5×10~6.利用邻近"魔术波长"的813.426 nm半导体激光光源实现水平方向的一维光晶格装载.采用归一化探测方法用线宽为Hz量级的698 nm钟激光对~1S_0→~3P_0偶极禁戒跃迁进行探测,在150 ms的探测时间下获得线宽为6.7 Hz的钟跃迁简并谱.在磁光阱竖直方向施加一个300 mGs的偏置磁场获得塞曼分裂谱,并通过689 nm的圆偏振自旋极化光进行光抽运,最终在探测时间为150 ms时,获得左右旋极化谱线线宽分别为6.2 Hz和6.8 Hz.     

Parameter analysis for a nuclear magnetic resonance gyroscope based on bf133Cs-129Xe/131Xe

We theoretically investigate several parameters for the nuclear magnetic resonance gyroscope based on ¹³³Cs-¹²⁹Xe/¹³¹Xe. For a cell containing a mixture of ¹³³Cs at saturated pressure, we investigate the optimal quenching gas (N₂) pressure and the corresponding pump laser intensity to achieve 30% ¹³³Cs polarization at the center of the cell when the static magnetic field B₀ is 5 μT with different ¹²⁹Xe/¹³¹Xe pressure. The effective field produced by spin-exchange polarized ¹²⁹Xe or ¹³¹Xe sensed by ¹³³Cs can also be discussed in different ¹²⁹Xe/¹³¹Xe pressure conditions. Furthermore, the relationship between the detected signal and the probe laser frequency is researched. We obtain the optimum probe laser detuning from the D2 (6²S_1/2→6²P_3/2) resonance with different ¹²⁹Xe/¹³¹Xe pressure owing to the pressure broadening.     

Frequency stabilization of laser diodes using 1.51-1.55 μm absorption lines of 12C2H2 and 13C2H2

Frequency stabilization of an 1.5 μm distributed feedback laser diode (DFB-LB) is demonstrated using a vibrational-rotational absorption of acetylene ¹²C₂H₂ and ¹³C₂H₂ molecules (VRAM). Frequency stability within 2 MHz peak-to-peak fluctuation can be achieved in the wavelength region of 1.51-1.55 μm. Frequency-stabilized distributed feedback (DFB) laser compact modules have been constructed. When the fiber-pigtail-type acoustic optical modulator was used for small laser frequency scanning, frequency stability within 3 MHz peak-to-peak fluctuation was achieved without any broadening of laser spectral linewidth. In addition, temperature and pressure dependencies of the acetylene absorption lines are characterized.     

Analytical solutions for a doubly driven two-level atom

We have deduced analytical solutions of an energy level diagram of the doubly driven/dressed atom for a two-level atom exposed to a strong near-resonant bichromatic laser field in a special case, i.e., the bichromatic field with frequencies ω1 and ω2, and Rabi frequencies ?1 and ?2, in which the first coupling field of ?1 acts on the bare atomic levels, and then the resulting singly dressed states are driven by the second coupling field of ?2, thus resulting in the doubly dressed atom.We have measured the probe absorption spectra of a doubly driven two-level atom. The system consists of 52S1/2, F= 2 and 5~2P_(3/2), F'= 3 states of ~(87)Rb atoms in a magneto-optical trap(MOT) as well as the cooling/trapping beams and an additional coupling field. As for the spectroscopic properties of the doubly driven two-level atom, theoretical analytical solutions are in general agreement with the experimental spectrum as a whole.     

锶原子互组跃迁谱的实验研究

观测了热原子束中锶原子(5s²)¹S₀—(5s5p)³P₁ 互组跃迁的荧光谱和饱和荧光谱, 实验测定了不同的参量下 ⁸⁸Sr(5s²)¹S₀—(5s5p)³P₁ 互组跃迁荧光谱. 研究结果表明: 不同的实验参数(温度、激光光强、激光扫描频率)对谱线有较大的影响, (5s5p)³P₁态的长寿命特点导致谱线强度随激光扫描频率呈倒数关系变化; 由于Doppler增宽, 渡越增宽等因素的影响, 谱线线宽远大于其自然线宽且随激光扫描频率呈正比关系变化.     

Resonant enhancement of field-induced annihilation rate for (π–π) atom: a possibility to measure np–ns energy splitting

Some possibilities are discussed for measuring the np–ns energy splitting in (π⁺–π⁻) atoms in experiments with relativistic particle beams, using the electromagnetic field control of annihilation process. Significant resonant enhancement of annihilation probability may be observed in an oscillating field. The resonance provides much more spectacular changes in the decay rate than corresponding decay rate changes in a steady field. The position of resonance on the frequency axis gives an additional and more accurate information on the np–ns transition energy, than the data on the ratio between the field-free and dc-field-induced annihilation rates. Numerical results are presented for the states n=2 and n=3.     

Electron localization of linear symmetric molecular ion H_3~(2+)

Electron localization in the dissociation of the symmetric linear molecular ion H_3~(2+) is investigated. The numerical simulation shows that the electron localization distribution is dependent on the central frequency and peak electric field amplitude of the external ultrashort ultraviolet laser pulse. When the electrons of the ground state are excited onto the 2pσ~2Σ_u~+ by a one-photon process, most electrons of the dissociation states are localized at the protons on both sides symmetrically. Almost no electron is stabilized at the middle proton due to the odd symmetry of the wave function. With the increase of the frequency of the external ultraviolet laser pulse, the electron localization ratio of the middle proton increases, for more electrons of the ground state are excited onto the higher 3pσ~2Σ_u~+ ustate. 50.9% electrons of all the dissociation events can be captured by the middle Coulomb potential well through optimizing the central frequency and peak electric field amplitude of the ultraviolet laser pulse. Besides, a direct current(DC) electric field can be utilized to control the electron motions of the dissociation states after the excitation of an ultraviolet laser pulse, and 68.8% electrons of the dissociation states can be controlled into the middle proton.     

高准确度的钙离子光频标

近年来,冷原子技术和激光技术促进了高精度光频标的发展,有望在建立时间基准、推动基础研究和满足国家需求等方面发挥重要的作用.本文介绍了中国科学院武汉物理与数学研究所近年来在高准确度钙离子(~(40)Ca~+)光频标研究方面的进展:采用新的ULE腔系统,实现了729 nm钟跃迁激光器1—100 s的频率稳定度均优于2×10~(-15),通过对外场和环境效应的控制及克服,特别是囚禁离子运动效应的抑制,获得单个钙离子光频标的不确定度优于5.5×10~(-17);通过两台光频标的比对,测得20000 s的稳定度也进入10~(-17)量级;基于高精度钙离子光频标平台,进行了相关精密测量的工作,包括:基于全球定位系统的超高精度远程光频绝对值测量方案,第二次测量了钙离子的光频跃迁绝对值,该测量结果再次被国际时间频率咨询委员会采纳,更新了钙离子的频率推荐值;精确测量了钙离子的钟跃迁魔幻波长,由此提出新型的全光囚禁离子光频标的方法;精密测量了钙离子的亚稳态寿命等参数.以上工作推动了基于冷原子的精密测量工作.     

A study of T1-weighted 31phosphorus MR-spectroscopy from patients with focal and diffuse liver disease.

³¹P-MR-Spectroscopy was performed in 28 patients with focal (n = 23) and diffuse (n = 5) liver disease and in 18 healthy volunteers. The spectra were obtained with a whole body scanner operating at 1.5 T by using a surface coil. To get T₁-weighted ³¹P-spectra a short TR of 600 msec was taken, because T₁-weighted spectra of focal liver disease were more significantly different from spectra from healthy volunteers than density weighted ones. The VOI from patients with focal superficial alterations showed a mean volume of 172 ml, with diffuse liver disease 196 ml, and from volunteers 158 ml. Focal tumors filled up the VOI on an average of 70%. This investigation demonstrated that PME/β-ATP- and PDE/β-ATP-ratios were sensitive indicators for focal liver disease. As a result of this study we could establish a significant increase of PME/β-ATP- (0.75 ± 0.30) and PDE/β-ATP-ratios (1.68 ± 0.62) in patients with superficial focal liver metastases (n = 19) compared to the control group (PME/β-ATP: 0.49 ± 0.17, PDE/β-ATP: 1.24 ± 0.24; t-test: p < 0.02). Patients with a hemangioma (n = 1), liver infarction (n = 1), empyema of gallbladder (n = 1) and a hepatic involvement by a malignant lymphoma (n = 1) showed a similar increase of PME/β-ATP and/or PDE/β-ATP. Up to now spectral changes seemed to be non-specific. The ratios of ³¹P metabolites of the cirrhoses (n = 4) and the fatty liver (n = 1) did not show any characteristic changes versus the volunteers.     

LD泵浦全固态608.1nm和频激光器

本文报道了一种全固态腔内和频608.1 nm激光器。在激光谐振腔两个分臂中,两支激光二极管分别泵浦Nd: YVO₄和Nd: YAG晶体,分别选择1 342 nm波长(Nd: YVO₄晶体的⁴F_3/2-⁴I_13/2谱线)与1 112 nm波长(Nd: YAG晶体的⁴F_3/2-⁴I_11/2谱线)振荡并进行腔内和频。通过优化谐振腔设计,腔内两个波长获得了较好的模式匹配。在两个分臂的交叠部分,利用LBO I类相位匹配进行和频,获得和频608.1 nm激光输出。实验表明,当Nd: YVO₄与Nd: YAG晶体泵浦功率分别为600和740 mW时,获得了功率为23.8 mW、波长为608.1 nm激光输出,激光输出稳定、噪声低。利用本文提出的和频结构是获得608.1 nm激光输出较为有效的方法。     

Doppler-free spectroscopy of Mg using uv-visible saturated absorption

Cascade double resonance saturation spectroscopy was performed on the Mg 3s ¹S₀-3p ¹P₁-5s ¹S₀ transitions. A strong dye laser at 571 nm induced an inverted dip on the 285 nm resonance line transmission spectrum probed by a second, frequency doubled, dye laser. New values for the isotopic shifts of the visible transition were obtained.     

A microsecond-pulse-length, frequency-stabilized virtual-cathodeoscillator using a resonant cavity

Experiments at the microsecond pulse length have demonstrated that the virtual-cathode oscillator generates narrowband (0.3% bandwidth) microwave pulses when the virtual cathode is surrounded by a resonant cavity and is driven by an appropriate electron beam. This result is a significant departure from the behavior of a free-running virtual-cathode oscillator where the frequency depends on the (current density)^1/2. The long-pulse experimental results are described     

Minimal renormalization without ε-expansion: Three-loop amplitude functions of the 0(n) symmetric Φ theory in three dimensions below Tc

We present an analytic three-loop calculation for thermodynamic quantities of the O(n) symmetric Φ⁴ theory below T_c within the minimal subtraction scheme at fixed dimension d = 3. Goldstone singularities arising at an intermediate stage in the calculation of O(n) symmetric quantities cancel among themselves leaving a finite result in the limit of zero external field. From the free energy we calculate the three-loop terms of the amplitude functions ƒ_Φ, F₊ and F₋ of the order parameter and the specific heat above and below Tc, respectively, without using the e = 4-d expansion. A Borel resummation for the case n = 2 yields resummed amplitude functions f_Φ and F₋ that are slightly larger than the one-loop results. Accurate knowledge of these functions is needed for testing the renormalization-group prediction of critical-point universality along the λ₋line of superfluid ⁴He. Combining the three-loop result for F₋ with a recent five-loop calculation of the additive renormalization constant of the specific heat yields excellent agreement between the calculated and measured universal amplitude ratio A⁺/A^- of the specific heat of ⁴He. In addition we use our result for f_Φ to calculate the universal combination Rc of the amplitudes of the order parameter, the susceptibility and the specific heat for n = 2 and n = 3. Our Borel-resummed three-loop result for R_c is significantly more accurate than the previous result obtained from the ε-expansion up to O(ε².     

非Maxwell电子速度分布对受激散射的影响

从考虑动理学效应的受激散射不稳定性的线性理论出发,对于n=2的Maxwell分布函数直到n=5的饱和情况的超高斯分布函数,计算了电子等离子体波和离子声波的频率和阻尼率。对受激喇曼散射和受激布里渊散射进行分析,结果表明,在激光高Z等离子体中,或者在具有激光热斑的中等Z等离子体中,电子等离子体波的阻尼率降低很多,离子声波的频率比Maxwell分布情况升高约15%。这些结果可和实验进行比较。     

Optical generation of a precise microwave frequency comb by harmonic frequency locking

A semiconductor laser under negative optoelectronic feedback is applied to the generation of a microwave frequency comb through the nonlinear dynamics. The laser system is operated in a harmonic frequency-locked pulsing state, where its power spectrum is a microwave frequency comb that consists of multiples of a locking frequency. Every frequency component of the comb can be simultaneously stabilized by simply injecting an external microwave modulation at any component of the comb. This phenomenon can be viewed as a kind of microwave injection locking of the laser dynamics.     

LaF3∶Er,Yb纳米颗粒掺杂有机/无机杂化材料制备光波导放大器及特性研究

采用LaF₃∶Er,Yb纳米颗粒掺杂有机/无机杂化材料作为有源材料,制备了掩埋条形结构光波导放大器,研究了放大器在室温下的增益特性和波导中的频率上转换现象. 当抽运功率60 mW时,波导中明显可见绿色上转换发光,观测到Er³⁺从²H_9/2,²H_11/2,⁴S_3/2,⁴F_9/2到基态⁴I_15/2跃迁分别对应的4个波长分别为405?nm, 520?nm, 544?nm和650?nm的发射峰,分析了其产生机理. 当输入信号光06?mW,抽运功率160 mW时,在1535?nm波长处获得15 dB/cm的相对增益. 关键词： 光波导放大器 增益 上转换     

Development of laser photoelectron spectroscopy based on resonantly enhanced multiphoton ionization

This review article is mainly concerned with laser photoelectron spectroscopy based on REMPI (resonantly enhanced multiphoton ionization), consisting of two parts. One is associated with the measurement of photoelectron kinetic-energy distribution and the other is associated with the measurement of zero-kinetic-energy (ZEKE) photoelectrons in very high resolution. These two techniques are complementary to each other. During the last three decades, the author and co-workers have carried out photoelectron spectroscopic studies of molecules in the gas phase, using the HeI 584 Å resonance line and a nanosecond tunable UV–visible laser. In this article, firstly the author’s background in the field of molecular photoelectron spectroscopy is described briefly, by mentioning three topics of HeI photoelectron spectroscopy. Secondly, the principle and characteristics of laser photoelectron kinetic-energy spectroscopy and its application to several typical topics, namely, one-photon forbidden states (O₂), autoionization from a super-excited state (NO), and small van der Waals molecules (NO–Ar and the NO₂ dimer), and some others. Thirdly, the principle and characteristics of ZEKE photoelectron spectroscopy are described, together with its application to the following several topics: (1) rotational spectra of NO⁺, (2) vibrational coupling of (naphthalene)⁺, (3) large-amplitude torsional motion of (tolane)⁺, (4) rotational isomers of (cis and trans n-propylbenzene)⁺ and structural isomers of (2-hydroxypyridine)⁺, (5) proton tunneling of (tropolone)⁺ and (9-hydroxyphenalenone)⁺, (6) intramolecular vibrational redistribution of trans stilbene, and (7) cation van der Waals molecules of aniline–Ar_n (n=1,2) and azulene–Ar. All the results mentioned as examples are those obtained in the author’s laboratory.