Localization of negatively charged excitons in GaAs/AlGaAs quantum wells

The localization of negatively charged excitons on isolated charged donors, located in a barrier at various fixed distances L from the heteroboundary, is investigated in isolated GaAs/AlGaAs quantum wells. The energy shift of the cyclotron replica in the emission spectra of a localized excitonic complex is studied as a function of L. It is shown that in undoped samples charged excitons localize on residual donors at distances L>350 Å on account of the formation of D ^? complexes at shorter distances. It is established that a cyclotron replica arises with the recombination of an excited state and not the ground state, as previously thought, of an excitonic complex.     

Condensation of interwell excitons in GaAs/AlGaAs double quantum wells

Experimental observations of the collective behavior of interwell excitons in the binary quantum wells with inclined bands under bias are discussed.     

Collective behavior of interwell excitons in GaAs/AlGaAs double quantum wells

Photoluminescence spectra of interwell excitons in double GaAs/AlGaAs quantum wells (n-i-n structures) have been investigated (an interwell exciton in these systems is an electron-hole pair spatially separated by a narrow AlAs barrier). Under resonance excitation by circularly polarized light, the luminescence line of interwell excitons exhibits a significant narrowing and a drastic increase in the degree of circular polarization of photoluminescence with increasing exciton concentration. It is found that the radiative recombination rate significantly increases under these conditions. This phenomenon is observed at temperatures lower than the critical point and can be interpreted in terms of the collective behavior of interwell excitons.     

Field-induced lifetime enhancement and ionization of excitons in GaAs/AlGaAs quantum wells

Picosecond and nanosecond luminescence studies of GaAs/AlGaAs quantum wells exposed to electric fields perpendicular to the layers are reported. The drastic red-shift of the photoluminescence with the electric field strength is accompanied by a strong increase of the electron-hole recombination lifetime. These features are most dominant for the wider wells due to the stronger polarization of the confined electron-hole pairs. Our observations are consistent with the model of the Quantum-Confined Stark Effect. In contrast, for high fields in the regime of ∼100 kV/cm field ionization limits the confinement of electrons and holes and leads to a strong decrease of the photoluminescence yield and lifetime with increasing field strength.     

Interwell excitons in GaAs/AlGaAs double quantum wells and their collective properties

Luminescence spectra of interwell excitons in GaAs/AlGaAs double quantum wells with electric-field-tilted bands (n-i-n) structures were studied. In these structures the electron and the hole in the interwell exciton are spatially separated between neighboring quantum wells by a narrow AlAs barrier. Under resonant excitation by circularly polarized light the luminescence line of the interwell excitons exhibited appreciable narrowing as their concentration increased and the degree of circular polarization of the photoluminescence increased substantially. Under resonant excitation by linearly polarized light the alignment of the interwell excitons increased as a threshold process with increasing optical pumping. By analyzing time-resolved spectra and the kinetics of the photoluminescence intensity under pulsed excitation it was established that under these conditions the rate of radiative recombination increases substantially. The observed effect occurs at below-critical temperatures and is interpreted in terms of the collective behavior of the interwell excitons. Studies of the luminescence spectra in a magnetic field showed that the collective exciton phase is dielectric and in this phase the interwell excitons retain their individual properties.     

Giant burst of the emission line intensity of spatially indirect excitons in GaAs/AlGaAs double quantum wells

A study is reported on the low-temperature (T≤30 K) photoluminescence in the spatially indirect exciton line in GaAs/Al_0.33Ga_0.67As double quantum wells as a function of optical pump power and applied electric field. We have revealed a giant (threefold) burst of luminescence intensity in a part of the spectral profile of the indirect-exciton line occurring at certain values of the external electric field, temperature, and optical pumping. We have also observed that this part of the indirect-exciton line profile varies in intensity (fluctuates) with time with a characteristic period of tens of seconds. The results obtained are discussed within a model of the Bose-Einstein condensation of a system of two-dimensional bosons that have, besides the free, a discrete energy spectrum lying below the bottom of the free-state band.     

Cretion and annihilation of negatively charged excitons in GaAs quantum wells

Il Nuovo Cimento D - The electroluminescence of p-i-n GaAs double-barrier resonant tunnelling diodes has been investigated for various concentrations of free carriers (either holes or electrons) in...     

Stark effect of negatively and positively charged excitons in semiconductor quantum wells

We study the effect of an electric field applied normal to the layers on the binding energy of charged excitons (or trions) in GaAs quantum wells. We find that, in contrast to the neutral exciton, their binding energy is sharply reduced by modest electric fields. The effect is stronger for the positively charged exciton than the negatively charged one. The ionisation of the excess carrier is explained by the field-induced polarisation of the electron and hole subband wave functions.     

A diffusion anomaly in dipole-oriented two-dimensional excitons in GaAs/AlGaAs coupled quantum wells

Il Nuovo Cimento D - We have observed an anomaly in the low-temperature photoluminescence of dipole-oriented long-lived excitons in a coupled quantum well under an electrical bias. A discrepancy...     

Absorption and emission of terahertz radiation in doped GaAs/AlGaAs quantum wells

Spontaneous emission of terahertz radiation from structures with GaAs/AlGaAs quantum wells in a longitudinal magnetic field has been studied. It is shown that some bands in the emission spectrum can be related to radiative electron transitions between resonant and localized impurity states, as well as to the transitions with participation of subband states. The temperature dependence of the equilibrium intraband absorption of terahertz radiation and its modulation in a longitudinal electric field in GaAs/AlGaAs quantum wells has been investigated.     

Phase diagram of the Bose condensation of interwell excitons in GaAs/AlGaAs double quantum wells

The luminescence of interwell excitons in GaAs/AlGaAs double quantum wells (n-i-n heterostructures) with large-scale fluctuations of random potential in the heteroboundary planes was studied at low temperatures down to 0.5 K. The properties of excitons whose photoexcited electron and hole are spatially separated in the neighboring quantum wells by a tunneling barrier were studied as functions of density and temperature. The studies were performed within domains about one micron in size, which played the role of macroscopic traps for interwell excitons. For this purpose, the sample surface was coated with a metal mask containing special openings (windows) of a micron size or smaller. Both photoexcitation and observation of luminescence were performed through these windows by the fiber optic technique. At low pumping powers, the interwell excitons were strongly localized because of the residual charged impurities, and the corresponding photoluminescence line was nonuniformly broadened. As the laser excitation power increased, a narrow line due to delocalized excitons arose in a threshold-like manner, after which its intensity rapidly increased with growing pumping and the line itself narrowed (to a linewidth less than 1 meV) and shifted toward lower energies (by about 0.5 meV) in accordance with the filling of the lowest exciton state in the domain. An increase in temperature was accompanied by the disappearance of the line from the spectrum in a nonactivation manner. The phenomenon observed in the experiment was attributed to Bose-Einstein condensation in a quasi-two-dimensional system of interwell excitons. In the temperature interval studied (0.5–3.6) K, the critical exciton density and temperature were determined and a phase diagram outlining the exciton condensate region was constructed.     

High-frequency magneto-oscillations in GaAs/AlGaAs quantum wells

We have observed very high-frequency, highly reproducible magneto-oscillations in modulation doped GaAs/AlGaAs quantum well structures. The oscillations are periodic in an inverse magnetic field (1/B) and their amplitude increases with temperature up to T approximately 700 mK. Being initially most pronounced around the filling factor nu=1/2, they move towards lower nu with increasing T. Front and back-gating data imply that these oscillations require a coupling to a parallel conducting layer. A comparison with existing oscillation models renders no explanation.     

Charged excitons in GaAs quantum wells

Il Nuovo Cimento D - We implement optical spectroscopy to study charged excitons (trions) in modulation-doped GaAs/AlGaAs quantum wells. We observe for the first time several new trions: the...     

Neutral and positively charged excitons in quantum ring

We study theoretically quantized states of the neutral and positively charged exciton complexes confined within a circular narrow ring in the presence of the magnetic field applied along the symmetry axis. We show that in the structural adiabatic limit, when the width of the pattern of the particles pathways within the ring is much smaller than its radius, the wave equations for both complexes are separable and their exact solutions can be found in a form of the Fourier series of one and two variables, respectively. We present results of calculation of the lower energies of complexes as functions of the ring's radius and the magnetic field strength for different values of the electron-to-hole mass ratio. We found that in the molecular adiabatic limit, when this ratio tends to zero and the model describes the corresponding donor complexes, the physical interpretation of the quantum-size effect and the oscillations of energy levels in threading magnetic field revealed for the excitons spectra becomes more transparent.     

Manifestation of collective properties of spatially indirect excitons in GaAs/AlGaAs asymmetric double quantum wells

Low-temperature (T=1.8, 4.2 K) luminescence of GaAs/Al_0.3Ga_0.7As double-coupled asymmetric quantum wells (DQW) is observed under variation of an electric field V _dc applied along the normal to the DQW plane. The FWHM of the indirect exciton (IX) emission line was found to undergo, within a certain interval of V _dc, a strong (up to a factor 3.5) narrowing, accompanied by anomalously large IX intensity fluctuations in time within the V _dc region where a strong decrease (or increase) of the FWHM is observed to occur. The dependence of the FWHM on the pumping level I _p also exhibits a substantial decrease of the FWHM within a certain I _p interval. The results obtained are discussed in the frame of an assumption which relates the observed phenomena to the onset of a condensed state in the interacting ensemble of spatially indirect excitons in DQWs. Fiz. Tverd. Tela (St. Petersburg) 41, 325–329 (February 1999)     

Collective state of interwell excitons in GaAs/AlGaAs double quantum wells under pulse resonance excitation

The time evolution and kinetics of photoluminescence (PL) spectra of interwell excitons in double GaAs/AlGaAs quantum wells (n-i-n structures) have been investigated under the pulse resonance excitation of intrawell 1sHH excitons using a pulsed tunable laser. It is found that the collective exciton phase arises with a time delay relative to the exciting pulse (several nanoseconds), which is due to density and temperature relaxation to the equilibrium values. The origination of the collective phase of interwell excitons is accompanied by a strong narrowing of the corresponding photoluminescence line (the line width is about 1.1 meV), a superlinear rise in its intensity, a long time in the change of the degree of circular polarization, a displacement of the PL spectrum toward lower energies (about 1.5 meV) in accordance with the filling of the lowest state with the exciton Bose condensate, and a significant increase in the radiative decay rate of the condensed phase. The collective exciton phase arises at temperatures T<6 K and interwell exciton densities n=3×10¹⁰ cm^?2. Coherent properties of the collective phase of interwell excitons and experimental manifestations of this coherence are discussed.