Short Terahertz Pulse Generation from a Dispersion Compensated Modelocked Semiconductor Laser

Dispersion compensation is vital for the generation of ultrashort and single cycle pulses from modelocked lasers across the electromagnetic spectrum. It is typically based on addition of an extra dispersive element to the laser cavity that introduces a chromatic dispersion opposite to that of the gain medium. To date, however, no dispersion compensation schemes have been successfully applied to terahertz (THz) quantum cascade lasers for short and stable pulse generation in the THz range. In this work, a monolithic on‐chip compensation scheme is realized for a modelocked QCL, permitting THz pulses to be considerably shortened from 16ps to 4ps. This is based on the realization of a small coupled cavity resonator that acts as an ‘off resonance’ Gires‐Tournois interferometer (GTI), permitting large THz spectral bandwidths to be compensated. This novel application of a GTI opens up a direct and simple route to sub‐picosecond and single cycle pulses in the THz range from a compact semiconductor source.     

DAST/SiO2 multilayer structure for efficient generation of 6 THz quasi-single-cycle electromagnetic pulses

We propose a DAST/SiO(2) multilayer structure for efficient generation of near-single-cycle THz transients with average frequency around 6 THz via collinear optical rectification of 800 nm femtosecond laser pulses. The use of such a composite material allows compensation for the phase mismatch that accompanies THz generation in bulk DAST crystals. The presented calculations indicate a strong increase in the THz generation efficiency in the DAST/SiO(2) structure in comparison to the case of bulk DAST crystal.     

THz Radiation Generation via the Interaction of Ultra‐short Laser Pulses with the Molecular Hydrogen Plasma

In this paper, a two dimensional Particle In Cell‐Monte Carlo Collision simulation scheme is used to examine the THz generation via the interaction of high intensity ultra‐short laser pulses with an underdense molecular hydrogen plasma slab. The influences of plasma density, laser pulse duration and its intensity on the induced plasma current density and the subsequent effects on the generated THz signal characteristics are studied. It is observed that the induced current density in the plasma medium and THz spectral intensity are increased at the higher laser pulse intensities, laser pulse durations and plasma densities. Moreover, the generated THz electric field amplitude is reduced at the higher laser pulse durations. A wider frequency range for the generated THz signal is shown at the lower laser pulse durations and higher plasma densities. Additionally, it is found that the induced current density in hydrogen plasma medium is the dominant factor influencing the generation of THz pulse radiation. (© 2016 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)     

The dependence on optical energy of terahertz emission from air plasma induced by two-color femtosecond laser-pulses

The generation of terahertz （THz） emission from air plasma induced by two-color femtosecond laser pulses is studied on the basis of a transient photocurrent model. While the gas is ionized by the two-color femtosecond laser-pulses com- posed of the fundamental and its second harmonic, a non-vanishing directional photoelectron current emerges, radiating a THz electromagnetic pulse. The gas ionization processes at three different laser-pulse energies are simulated, and the corresponding THz waveforms and spectra are plotted. The results demonstrate that, by keeping the laser-pulse width and the relative phase between two pulses invariant when the laser energy is at a moderate value, the emitted THz fields are significantly enhanced with a near-linear dependence on the optical energy.     

Effects of the evolution of two cross‐focused Gaussian laser beams on the terahertz generation in thermal collisional plasma

Generation of the terahertz (THz) radiation based on the beating of two cross‐focused high intensity Gaussian laser beams in a warm rippled density plasma is numerically investigated, taking into account the ponderomotive force, Ohmic heating, and collisional nonlinearities. The beat ponderomotive force as a result of cross‐focusing of beams induces a vertical velocity component that by coupling with the rippled density gives rise to a nonlinear current deriving THz radiation. The effect of laser beams spot size evolution and plasma parameters on the THz generation is studied. It was found that there exist special electron temperature and laser intensity ranges with “turning points” where the generation of THz radiation reaches its maximum value and outside of these ranges, it disappears. The results also indicated that increasing the background electron density as well as taking into account the collision frequency help THz generation. Moreover, the maximum yield of THz radiation occurs when the beat wave frequency approaches the plasma frequency.     

Terahertz-wave generation with periodically inverted gallium arsenide

We overview methods of THz-wave generation using frequency down-conversion in GaAs with periodically-inverted crystalline orientation. First, we compare different nonlinear-optical materials suitable for THz generation, analyze THz generation process in quasi-phase-matched crystals and consider theoretical limits of optical-to-THz conversion. Then, we review single-pass optical rectification experiments with femtosecond pump pulses, performed in periodically-inverted GaAs, where monochromatic THz output tunable in the range 0.9–3.0 THz was produced. Finally, we describe a novel approach to create a compact highly efficient tunable (0.5–3.5 THz) room temperature monochromatic THz source, based on the concept of intracavity THz generation via resonantly-enhanced difference frequency mixing. This approach allowed generating of 1 mW of average THz power, potentially scalable to 10–100 mW.     

Few‐optical‐cycle light pulses with passive carrier‐envelope phase stabilization

One of the most advanced frontiers of ultrafast optics is the control of carrier‐envelope phase (CEP) ϕ of light pulses, which enables the generation of optical waveforms with reproducible electric field profile. Such control is important for pulses with few‐optical‐cycle duration, for which a CEP variation produces a strong change in the waveform, so that strongly nonlinear optical phenomena, such as multiphoton absorption, above‐threshold ionization and high‐harmonic generation become CEP‐dependent. In particular, CEP control is the prerequisite for the production of isolated attosecond pulses. Standard laser systems generate pulses that are CEP unstable; the CEP can be stabilized using either active or passive methods. Passive, all‐optical schemes rely on difference‐frequency generation (DFG) between two pulses sharing the same CEP: in this process the phases of the two pulses add up with opposite signs, leading to cancellation of the shot‐to‐shot CEP fluctuations. This paper presents an overview of passive CEP stabilization schemes, starting from the basic concepts and progressing to the details of the practical implementations of the idea. The passive approach allows the generation of CEP‐controlled few‐optical‐cycle pulses covering a very broad range of parameters in terms of carrier frequency (from visible to mid‐IR), energy (up to several mJs) and repetition rate (up to hundreds of kHz)     

Propagation of ultrawideband short pulses of terahertz radiation through submillimeter-diameter circular waveguides

We report experimental investigations in which quasi-optical methods were used to efficiently couple freely propagating, optoelectronically generated, subpicosecond pulses of terahertz (THz) radiation into submillimeter circular metal tubes (waveguides) and, consequently, to measure the transmitted pulses from these waveguides. We observe very dispersive low-loss propagation over the frequency band from 0.65 to 3.5 THz, with frequency-dependent group velocities nu(g) ranging from c/4 to c and phase velocities nu(p) from 4c to c , where nu(g)nu(p)=c(2) . The linearly polarized incoming THz pulses couple significantly only into the TE(11) , TM(11) , and TE(12) modes of the utilized 24- and 4-mm-long stainless-steel tubes, with inside diameters of 240 and 280microm , respectively.     

Nonlinear optical terahertz wave sources

We developed a Cherenkov phase-matching method for monochromatic THz-wave generation using the DFG, process with a lithium niobate crystal, which resulted in both high conversion efficiency and wide tunability. Although THz-wave generation by Cherenkov phase matching has been demonstrated using femtosecond pumping pulses, producing very high peak power, these THz-wave sources are not monochromatic. Our method generates monochromatic and tunable THz, waves using a nanosecond pulsed laser source. We also show that Cherenkov radiation with waveguide structure is an effective strategy for achieving extremely wide tunable THz-wave source. We fabricated MgO-doped lithium niobate slab waveguide and demonstrated difference frequency generation of THz-wave generation with Cherenkov phase matching. Extremely frequency-widened THz-wave generation, from 0.1 to 7 THz was observed.     

Experimental study on terahertz radiation

In this letter, we describe a coherent subpicosecond terahertz (THz) spectroscopy system based on nonresonant optical rectification for the generation of THz radiation. We studied the two-photon absorption (TPA) of ZnTe induced by femtosecond laser pulses via THz generation, and its influence on the generation of THz radiation. Experimental results demonstrated that the intensity of pump beam against TPA must be traded off to get an optimum generation of THz radiation. As an example, we measured absorption spectrum of water vapor by time-domain spectroscopy (TDS) in the frequency range from 0.5 to 2.5 THzwith a high overall accuracy.     

Temperature dependent narrow-band terahertz pulse generation in periodically poled crystals via difference frequency generation

Femtosecond optical pulse is used to generate narrow-band terahertz pulses depending on a quasi-phase-matched condition in periodically poled lithium niobate (PPLN) and stoichiometric lithium tantalate (PPSLT) crystals by difference frequency generation. The origin of narrow-band THz generation proved that the two frequency components of the fs pulse contribute to the frequency mixing. By cryogenic cooling, the absorption of THz waves in the crystal is significantly reduced which results in efficient THz generation. Simultaneously generated forward and backward THz pulses were 1.38 and 0.65 THz with as narrow as the bandwidth of 32 GHz in the PPSLT sample. Temperature dependence of the generated THz waveforms had good agreement with the simulation result using one dimensional plane-wave propagation model.     

Studies on the mechanisms of powerful terahertz radiations from laser plasmas

A survey on the mechanisms of powerful terahertz (THz) radiation from laser plasmas is presented.Firstly,an analytical model is described,showing that a transverse net current formed in a plasma can be converted into THz radiations at the plasma oscillation frequency.This theory is applied to explain THz generation in a gas driven by two-color laser pulses.It is also applied to THz generation in a tenuous plasma driven by a chirped laser pulse,a few-cycle laser pulse,a DC/AC bias electric field.These are well verified by particle-in-cell simulations,demonstrating that THz radiations produced in these approaches are nearly single-cycles and linear polarized.In the chirped laser scheme and the few-cycle laser scheme,THz radiations with the peak field strength of tens of MV/cm and the peak power of gigawatt can be achieved with the incident laser intensity less than 10 17 W/cm 2.     

Tunable few-cycle and multicycle coherent terahertz radiation from relativistic electrons

We report the generation of tunable, narrow-band, few-cycle and multicycle coherent terahertz (THz) pulses from a temporally modulated relativistic electron beam. We demonstrate that the frequency of the THz radiation and the number of the oscillation cycles of the THz electric field can be tuned by changing the modulation period of the electron beam through a temporally shaped photocathode drive laser. The central frequency of the THz spectrum is tunable from ～0.26 to 2.6 THz with a bandwidth of ～0.16 THz.     

Broadband Terahertz Wave Generation from Monolayer Graphene Driven by Few-Cycle Laser Pulse

We theoretically investigate the characteristics of terahertz(THz) radiation from monolayer graphene exposed to normal incident few-cycle laser pulses, by numerically solving the extended semiconductor Bloch equations. Our simulations show that the THz spectra in low frequency regions are highly dependent on the carrier envelope phase(CEP) of driving laser pulses. Using an optimal CEP of few-cycle laser pulses, we can obtain broadband strong THz waves, due to the symmetry breaking of the laser-graphene system. Our results also show that the strength of the THz spectra depend on both the intensity and central wavelength of the laser pulses. The intensity dependence of the THz wave can be described by the excitation rate of graphene, while wavelength dependence can be traced back to the band velocity and the population of graphene. We find that a near single-cycle THz pulse can be obtained from graphene driven by a mid-infrared laser pulse.     

Energy Scaling of Terahertz Pulses Produced through Difference Frequency Generation

We study the energy scaling of terahertz(THz) emission through difference frequency generation of near-infrared pulses, and demonstrate that Gigawatt few-cycle THz transients at the central frequency of 30 THz are produced from GaSe crystal pumped by two pulses at 1.65 and 1.95 micrometers, with the high quantum yield of 28%.Our analysis indicates that the high yield of DFG originates from the largely reduced group velocity mismatch as the long-wavelength pumping pulses are employed.     

少周期激光脉冲与气体作用产生的离化电流和THz波辐射

本文通过理论和数值模拟,研究少周期激光脉冲电离气体原子产生的离化电流 以及相应的THz波辐射.研究表明,少周期激光脉冲离化气体后能产生较大的离化电流, 因而可以产生较强的THz辐射.不同的少周期激光脉冲相位导致电离出的 电子初始速度和电离起始时刻不同,从而产生的离化电流有所不同, 辐射的THz波随激光脉冲的相位成周期性变化.该理论得到一维PIC数值模拟的验证. 对于给定的激光脉冲相位,离化电流和THz辐射振幅并没有随入射激光振幅的增加而单调增加, 而是存在一些极值点.与均匀分布气体相比,当气体分布具有一定梯度时, 辐射表现相似的规律,但频谱会发生一定的变化.     

Single-frequency terahertz source pumped by Q-switched fiber lasers based on difference-frequency generation in GaSe crystal

We demonstrate a unique terahertz (THz) source that is compact, utilizes recently developed all-fiber Q-switched lasers, and is based on difference-frequency generation in a GaSe crystal. A single piezo simultaneously Q switched the two fiber lasers by using stress-induced birefringence, to achieve the temporal overlap of pulses from the two fiber lasers. These correlated pulses then combine in the GaSe crystal to produce coherent and highly monochromatic THz pulses. The peak power for this THz source can reach 0.53 mW, corresponding to an average power of 0.43 microW and a conversion efficiency of 4.75 x 10(-7). The estimated linewidth of this THz source can be as narrow as approximately 35 MHz or 1.17 x 10(-3) cm(-1).     

Undistorted guided-wave propagation of subpicosecond terahertz pulses

We report efficient quasi-optic coupling of a freely propagating beam of terahertz (THz) pulses into a parallel-plate copper waveguide (with a plate separation of 108mum) and subsequent low-loss, single-TEM-mode propagation with virtually no group-velocity dispersion. Undistorted, low-loss propagation of the incoming 0.3-ps FWHM THz pulses was observed within the bandwidth from 0.1 to 4 THz for a length of 24.4 mm. We compare experimentally derived values for the absorption and phase velocity with theory to show consistency. This demonstration is direct proof of the excellent performance of the parallel-plate waveguide as a wideband THz interconnect.     

THz generation via optical rectification with ultrashort laser pulse focused to a line

We report on efficient THz pulse generation via optical rectification with femtosecond laser pulses focused to a line by a cylindrical lens. This configuration provides phase-matched conditions in the superluminal regime. 35 pJ THz pulses have been generated with this technique in a stoichiometric LiNbO₃ crystal pumped by 2 μJ femtosecond laser pulses at room temperature. An unusual superquadratic rise of the THz pulse energy with the laser pulse energy has been observed at high laser energies. This extraordinary energy dependence of the THz generation efficiency is explained by self-focusing of the laser beam in the crystal. Z-scan measurements and comparison of the THz pulse spectra created with laser pulses having different energies confirm this interpretation.     

THz radiation generation via the interaction of two‐colour ultra‐short laser pulses with SO2 and NH3 gases

In this work, using a two‐dimensional particle‐in‐cell Monte Carlo collision computation method, terahertz (THz) radiation generation via the interaction of two‐colour, ultra‐short, high‐power laser pulses with the polyatomic molecular gases sulphur dioxide (SO₂) and ammonia (NH₃) is examined. The influence of SO₂ and NH₃ pressures and two‐colour laser pulse parameters, i.e., pulse shape, pulse duration, and beam waist, on the THz radiation generation is studied. It is shown that the THz signal generation from SO₂ and NH₃ increases with the background gas pressure. It is seen that the THz emission intensity for both gases at higher laser pulse durations is higher. Moreover, for these polyatomic gases, the plasma current density increases with increase in the laser pulse beam waist. A more powerful THz radiation intensity with a larger time to peak of the plasma current density is observed for SO₂ compared to NH₃. In addition, many THz signals with small intensities are observed for both polyatomic gases. It is seen that for both SO₂ and NH₃ the generated THz spectral intensity is higher at higher gas pressures.