Supersolid magnetic phase in the two-dimensional Ising-like antiferromagnet with strong single-ion anisotropy

The Ising model with the frustrated exchange interaction for strongly anisotropic antiferromagnetic ultrathin film is investigated in the mean field approximation at low temperatures. It is shown that a spatially inhomogeneous state can be accomplished in the system at a certain relation of material constants values, along with homogeneous states: ferromagnetic, quadrupolar or supersolid magnetic phases. The phase diagram of the system is built on the basis of stability lines analysis.     

Unconventional dynamics in triangular Heisenberg antiferromagnet NaCrO2

We report magnetization, specific heat, muon spin rotation, and Na NMR measurements on the S=3/2 rhombohedrally stacked Heisenberg antiferromagnet NaCrO2. This compound appears to be a good candidate for the study of isotropic triangular Heisenberg antiferromagnets with very weak interlayer coupling. While specific heat and magnetization measurements indicate the onset of a transition in the range Tc approximately 40-50 K, both muon spin rotation and NMR reveal a fluctuating crossover regime extending well below Tc, with a peak of relaxation rate T1(-1) around T approximately 25 K. This novel finding is discussed within the context of excitations in the triangular Heisenberg antiferromagnets.     

Anisotropy modulated stepwise magnetization in triangular Heisenberg antiferromagnet

During the course of tuning anisotropy from Ising type to zero, the variation of magnetization (M) steps against magnetic field (h) is investigated in a triangular antiferromagnetic Heisenberg model using Monte Carlo techniques. It is revealed that the anisotropy is an essential key to induce the temperature-dependent stepwise M(h) curve observed in frustrated magnetic system, and it can be employed to modulate this steplike magnetic behavior effectively. When the anisotropy is strengthened, a ground state transition occurs from the homogeneous 120° triangular structure to the collinear partially disordered antiferromagnetic state. No M step is detected in the system without anisotropy. But if the anisotropy is nonzero, the M₀/3 step (where M₀ is the saturated M) will emerge on M(h) curve, which is due to an h-induced quasi-collinear ferrimagnetic state. This M₀/3 step can be extended by increasing the anisotropy. When the M₀/3 plateau dominates the h-range broad enough, the equidistant metastable substeps, which originates from the disorders frozen in the frustrated collinear spin structure, appear to be superposed on the M₀/3 plateau. Thus the system with a strong anisotropy presents the whole temperature evolution of stepwise M(h) curve in quantitative agreement with the experiments of Ca₃Co₂O₆.     

Quantum anisotropic Heisenberg triangular antiferromagnet: application to CsCuCl3

Triangular anisotropic Heisenberg antiferromagnet shares with the triangular planar antiferromagnet the rich phenomenology found in presence of an external magnetic field. The physical interest in the triangular Heisenberg model is obvious because the planar model has not the quantum analogous one and, more seriously, it does not allow out-of-plane fluctuations so that it provides a very rough representation of actual magnetic insulators. Indeed, we show that magnetic resonance data on CsCuCl₃ are satisfactorily understood on the basis of the properties of the quantum triangular Heisenberg antiferromagnet with easy-plane exchange anisotropy.     

Perturbation theory for a microemulsion with triangular well potential

The perturbation approach of Barker and Henderson (1967, 1968) has been applied to a microemulsion obeying triangular well potential as a perturbative attractive tail over the Percus-Yevick (PY) hard sphere model by calculating the Rayleigh ratio,R ₉₀, under the mean spherical approximations. The results are in better agreement with experimental values. Presented at the 70th Indian Science Congress, Tirupathi, January 3–8, 1983.     

Gauge theory of two-dimensional spin- Heisenberg antiferromagnet

A gauge theory of the spin- Heisenberg antiferromagnet (HA) on a two-dimensional square lattice is developed, which is based on the diagonal G_D of the group product SO(3)×SU(2). For classical gauge fields G_D is homeomorphic to SO(3). The structure of the theory is such that the quantum spin- field propagates on the background gauge field. For special gauges the excitations of the spin-field are computed and compared to the excitations of the O(3) σ model for the same gauge. The significance of negative excitational modes with respect to a semiclassical actionГ_sc of the spin- HA is discussed. Some properties ofГ_sc represented as a chiral SO(3) model in a continuum representation are worked out.     

Surface modes with biquadratic coupling and uniaxial anisotropy in semi-infinite Heisenberg antiferromagnet

We address the role and the influence of both biquadratic exchange and uniaxial anisotropy in the study of bulk and surface magnetic excitations for a two-sublattices semi-infinite Heisenberg antiferromagnet. The calculations apply to combined effect and are based on a matching technique within the framework of both non-interacting spin-wave theory and random phase approximation. Emphasis has been laid upon the advantage of handling bulk and surface spin precessional fields, characterized by their symmetry in particular. Analytic expressions for the bulk and surface equations of motion are also derived which enables us to analyze qualitatively the nature of the modes by observing the response of the energy branches to the variation of both biquadratic exchange and single-ion anisotropy field as well as exchange parameters occurring on the surface. Two numerical applications of the theoretical formalism developed in this work are described. First concerns the situation when the free surface model is assumed. The second application considers the existence of surface perturbations and treats the effects of the presence of biquadratic exchange term on the bulk and surface spin-wave spectra showing two kinds of surface propagating modes which depend on the presence or not of the uniaxial anisotropy contribution and also on the variations of the bulk-surface exchange parameters. A significant conclusion which this work reached relates to the checking of the results obtained in the literature by using our own theoretical formalism. We show that this formalism is very well adapted to calculations of localized bulk and surface spin-wave modes associated with the simultaneous presence of biquadratic exchange and uniaxial anisotropy. Also, the results obtained for the bulk spin fluctuations field as well as for the magnetic surface waves, are found to be in qualitative agreement with those obtained in the literature. The analytic formulation presented in this work provides an accurate and practical scheme for calculating the surface spin dynamics under the influence of surface exchange parameters, biquadratic coupling and uniaxial anisotropy terms.     

TheS=1/2 Heisenberg antiferromagnet on the triangular lattice: Exact results and spin-wave theory for finite cells

We study the ground state properties of theS=1/2 Heisenberg antiferromagnet (HAF) on the triangular lattice with nearest-neighbour (J) and next-nearest neighbour (J) couplings. Classically, this system is known to be ordered in a 120° Néel type state for values-<1/8 of the ratio of these couplings and in a collinear state for 1/8<<1. The order parameter and the helicity /gC of the 120° structure are obtained by numerical diagonalisation of finite periodic systems of up toN=30 sites and by applying the spin-wave (SW) approximation to the same finite systems. We find a surprisingly good agreement between the exact and the SW results in the entire region-<<1/8. It appears that the SW theory is still valid for the simple triangular HAF (=0) although the sublattice magnetisation is substantially reduced from its classical value by quantum fluctuations. Our numerical results for the order parameterM of the collinear order support the previous conjecture of a first order transition between the 120° and the collinear order at 1/8.     

Comparative study between a two-dimensional anisotropic Heisenberg antiferromagnet with easy-axis single-ion anisotropy and one with easy-axis exchange anisotropy

Generally, in literature, easy-axis single ion anisotropy and easy-axis exchange anisotropy was treated in indistinct way. In this work we propose to perform a comparative study of the effects of these two easy-axis anisotropies on the behavior of the magnetization and the critical temperature (_Tc)$(T_{\mathrm{c}})$ in the 2D classical Heisenberg antiferromagnetic model. In order to study the low-temperature thermodynamics of this model, we should consider the contribution of anisotropic spin waves, using a self-consistent harmonic approximation (SCHA) theory. We compare the predictions of SCHA with numerical simulations on L×L$L\times L$ square lattices using Monte Carlo (MC) simulations, which include effects due to all thermodynamically allowed excitations. Our SCHA results are in good agreement with our MC simulations results and have shown that the strong K$K$ limit gives two different Ising-like behavior. In the exchange anisotropic case, the dependence of _Tc$T_{\mathrm{c}}$ on anisotropic parameter K$K$ becomes linear and in the single-ion anisotropic case, _Tc$T_{\mathrm{c}}$ becomes independent of K$K$. Also, using MC simulations and finite size scaling, we show that the critical exponents in the two anisotropic case are compatible with the 2D Ising values α=0.125$\alpha =0.125$ and γ=1.75$\gamma =1.75$.     

Magnetic properties of Heisenberg triangular antiferromagnet V15 cluster studied by NMR

The magnetic properties of an s?=?1/2 Heisenberg triangular antiferromagnet V15 have been studied by proton nuclear magnetic resonance (NMR) at very low temperature down to 100 mK using a He³-He⁴ dilution refrigerator. In total spin S _T?=?3/2 ground state above 2.7 Tesla, proton spin-lattice relaxation rate (1/T₁) shows thermally activated behavior as a function of temperature. On the other hand, a temperature independent behavior of 1/T₁ at very low temperatures is observed in frustrated S _T?=?1/2 ground state below 2.7 Tesla. Possible origins for the peculiar behavior of 1/T₁ will be discussed in terms of magnetic fluctuations due to spin frustration.     

Bond operator theory for the frustrated anisotropic Heisenberg antiferromagnet on a square lattice

The quantum anisotropic antiferromagnetic Heisenberg model with single ion anisotropy, spin S=1 and up to the next-next-nearest neighbor coupling (the J₁–J₂–J₃ model) on a square lattice, is studied using the bond-operator formalism in a mean field approximation. The quantum phase transitions at zero temperature are obtained. The model features a complex T=0 phase diagram, whose ordering vector is subject to quantum corrections with respect to the classical limit. The phase diagram shows a quantum paramagnetic phase situated among Neél, spiral and collinear states.