Optical absorptions of an exciton in a disc-like quantum dot under an electric field

An exciton in a disc-like quantum dot (QD) with the parabolic confinement, under applied electric field, is studied within the framework of the effective-mass approximation. Both the electric field and the confinement effects on the transition energy and the oscillator strength were investigated. Based on the computed energies and wave functions, the linear, the third-order nonlinear and the total optical absorption coefficients were also calculated. We found that the optical absorption coefficients with considering excitonic effects are stronger than those without considering excitonic effects and the absorption peak will move to the right side induced by the electron-hole interaction, which shows an excitonic effect blue-shift of the resonance in QDs. The applied electric field may affect either the size or the position of absorption peaks of excitons. However, the applied electric field may only affect the size of absorption peaks of an electron-hole pair without considering excitonic effects. It is very important to take excitonic effects into account when we study the optical absorption for disc-like QDs. We may observe the excitonic effect induced by the external electric field.     

用Ξ形四能级模型研究非对称耦合量子阱非定域激子复合发光

基于Ξ形四能级模型运用密度矩阵方程研究了非对称量子阱中非定域激子复合发光特性.理论结果表明：非定域激子复合发光具有双峰特征，两峰相对于中心跃迁频率的红移和蓝移量与电子和空穴的振荡频率密切相关.与单量子阱相比，这种频率移动对外加电场相当敏感，即当外加反向电场作小的变化时，两峰有较大的移动，表现强量子限域斯塔克效应.这意味着利用非对称量子阱在新一代高速调制器和光开关中具有潜在的应用价值. 关键词： 非对称耦合量子阱 共振隧穿 非定域激子 量子限域斯塔克效应     

Polarised hot electron luminescence in p-GaAs: Electric field effects

Electrons photo-excited to high-energy conduction band states of GaAs exhibit complex energy and momentum distributions determined by the anisotropic valence band structure and the optical matrix elements. In p-type GaAs a fraction of these hot electrons combine with localised acceptor states, producing a hot electron luminescence (HEL) spectrum with a cascade of peaks corresponding to discrete energy losses resulting from LO-phonon emission. The highest peak involves unscattered electrons, and their energy distribution is due to warping of the initial heavy-hole (HH) bands. We report measurements of the line shape of this 0-HH peak, and its polarisation profile which identifies emission from electrons along particular directions. An applied electric field of 1 kV cm⁻¹ distorts the hot electron momentum distribution, and this is reflected in the polarisation profile. These line shapes and profiles, with and without field, are calculated using a computer model incorporating a band structure and optical matrix elements, the effect of electric field being included using a k-broadening model. The data and model are in good quantitative agreement assuming an electron lifetime of 100 fs, and confirm the expected differences in the profiles for different excitation polarisation states and applied field directions.     

Influence of the magnetic field strength and excitation intensity on the shape of microphotoluminescence spectra of quantum-well structures based on GaN/InGaN doped with Sm and Eu + Sm

This paper presents the results of complex measurements of the microphotoluminescence spectra of quantum-well structures based on InGaN/GaN〈Sm〉 and the determination of the concentration and charge state of the Sm dopant. It has been shown that an increase in the magnetic field strength and the excitation intensity of the microphotoluminescence spectra leads to an increase in the luminescence intensity and a shift in the position of the maximum of the emission wavelength toward the short-wavelength region of the spectrum. Measurements of the microphotoluminescence spectra with variations in the external magnetic field strength, as well as with the introduction of paramagnetic and magnetic impurities, provide additional information on the mechanisms of formation of luminescence spectra in the quantum-well structures InGaN/GaN〈Sm〉,〈Eu + Sm〉. In the long-wavelength region, the influence of the magnetic field on the shape of the microphotoluminescence spectra of the InGaN/GaN structures doped with Sm and Sm + Eu is less pronounced than that in the short-wavelength region.     

Exciton optical absorption coefficients and refractive index changes in a strained InAs/GaAs quantum wire: The effect of the magnetic field

Magnetic field induced exciton binding energy is investigated in a strained InAs/GaAs quantum wire within the framework of single band effective mass approximation. The strain contribution to the potential is determined through deformation potentials. The interband emission energy of strained InAs/GaAs wire is investigated in the influence of magnetic field with the various structural parameters. Magnetic field induced photoionization cross section of the exciton is studied. The total optical absorption and the refractive index changes as a function of normalized photon energy between the ground and the first excited state in the presence of magnetic field are analyzed. The optical absorption coefficients and the refractive index changes strongly depend on the incident optical intensity and the magnetic field. The occurred blueshift of the resonant peak due to the magnetic field will give the information about the variation of two energy levels in the quantum well wire. The optical absorption coefficients and the refractive index changes are strongly dependent on the incident optical intensity and the magnetic field.     

Luminescence due to metallic electron-hole liquid in GaAs

Emission spectra of high-purity GaAs have been studied at 4.2K under very intense optical excitation. The results give the first experimental evidence for an important contribution of the electron-hole liquid phase in the luminescence of a direct-allowed semiconductor. Theoretical fit of the luminescence band-shape is satisfactory. The effects of applied electric field on the emission spectra are explained well using a concept of the metallic electron—hole plasma state.     

二苯乙烯衍生物的制备及结构-光学性能关系的研究

有机共轭材料由于在电子、非线性光学和发光领域具有广泛应用,引起人们广泛兴趣。苯乙烯衍生物是一类重要的有机共轭化合物。文章采用相转移Wittig反应和钯催化Heck反应合成了三种不同取代基二苯乙烯衍生物。研究了分子结构与电子吸收光谱和材料发光性能关系。同没有取代基的化合物3a相比(电子最大吸收峰波长358 nm),化合物3c中CH₃取代导致电子吸收光谱轻微红移到356 nm,硝基取代的化合物3b呈现出更大的吸收光谱红移现象,电子吸收最大峰红移到388 nm。同时发现：CH₃取代的化合物3c产生荧光发射峰在414 nm,同没有取代基的化合物3a相比,荧光发射强度明显增强;相反具有吸电子NO₂取代基的化合物3b荧光发射峰位于525 nm, 荧光发射强度明显减弱。可见二苯乙烯分子中取代基结构对分子光学性能产生重要影响。这为发光材料的分子设计提供新的思路。     

Dependence of resonance condition on pressure in an RF resonancemethod

The plasma density is shown as functions of pressure and magnetic flux density in an RF resonance method using the XPDP1 simulation code. The RF resonance method has the unique feature that a strong electric field in bulk controls the plasma density. Owing to the balance between the electric field decrease and the collision rate increase, the plasma density in the RF resonance method has a peak with respect to pressure. The plasma density with respect to the magnetic flux density depends on the condition of the RF resonance method, and the dependence is strong at low pressure because of the strong resonance. Sheath thickness is the most important parameter that determines the strength of the resonance induced. It is shown that the sheath thickness s is related to the plasma density n as a function of ns, obtained from a dispersion relation at constant external parameters. The magnetic flux density which induces the strong resonance is determined from sheath thickness. The plasma density in the RF resonance method can be predicted from discharge parameters using the relation between plasma density and sheath thickness     

Enhancing magnetic dipole emission with magnetic metamaterials

Magnetic dipole(MD) transitions are important for a range of technologies from quantum light sources and displays to lasers and bio-probes. However, the typical MD transitions are much weaker than their electric counterparts and are usually neglected in practical applications. Herein, we experimentally demonstrate that the MD transitions can be significantly enhanced by the well-developed magnetic metamaterials in the visible optical range. The magnetic metamaterials consist of silver nanostrips and a thick silver film, which are separated with an Eu~(3+):polymethyl methacrylate(PMMA) film. By controlling the thickness of the Eu~(3+):PMMA film, the magnetic resonance has been tuned to match the emission wavelength of MDs. Consequently,the intensity of MD emission has been significantly increased by around 30 times at the magnetic resonance wavelength, whereas the intensity of electric dipole emission is well-preserved. The corresponding numerical calculations reveal that the enhancement is directly generated by the magnetic resonance, which strongly increases the magnetic local density of states around the MD emitter and can efficiently radiate the MD emission into the far field. This is the first demonstration, to the best of our knowledge, that MD transitions can be improved by an additional degree of magnetic freedom, and we believe this research shall pave a new route towards bright magnetic emitters and their potential applications.     

一维反铁磁光子晶体光学双稳态效应研究

基于传递矩阵方法和光局域化原理, 本文研究了一维反铁磁光子晶体共振频率附近光学双稳态效应随电磁波入射角、 外磁场强度及电介质层数的变化.研究发现, 当外磁场为1.0 kG(1 G=10^-4 T)、电磁波小角度入射时, 反铁磁材料高低共振频率附近均可探测到光学双稳态效应; 当电磁波大角度入射时, 仅在高共振频率附近探测到光学双稳态效应. 然而, 当外磁场强度增加到2.0 kG时, 由于反铁磁材料的高低共振频率向两侧移动, 低共振频率附近缺失的光学双稳态频率窗口又被有效激发. 此外, 电磁波小角度入射时, 电介质层数在低共振频率附近对双稳态效应影响较明显.     

Electroluminescence and internal screening of domains upon polarization switching of ferroelectric ceramics in a pulsed self-consistent field

This paper reports on the results of investigations into the electroluminescence induced by polarization switching of a ferroelectric ceramic material in an electric field with a rapidly increasing strength. A correlation between the polarization switching and luminescence kinetics is revealed. It is demonstrated that tunneling of electrons to the conduction band and impact ionization in field concentrators are the main mechanisms of generation of free charge carriers responsible for the electroluminescence and internal screening of switching domains.     

调制n型掺杂ZnSe/BeTe Ⅱ型量子阱结构的发光特性

报道了调制n型掺杂ZnSe/BeTe/ZnSe Ⅱ型量子阱(type-II QW)在极低温至室温(14—296K)条件下的各种光学性质. 反射光谱显示了对于非掺杂样品,激子(X)的跃迁起着支配作用,而只有在掺杂样品的光谱里展示了一个典型的负的带电激子(X^-)的跃迁特征. PL光谱及其直线偏振度P_l都显著地依赖于n型掺杂量和平行于QW生长方向的外加电场. 这个特征被认为是由n型掺杂导致了内秉电场(built 关键词： 光致发光 二维电子气 带电激子 Ⅱ型量子阱     

Effect of a change in the optical density of a magnetic emulsion in electric and magnetic fields

The change in the optical density of an emulsion of magnetic fluid drops suspended in a mineral oil under the action of electric and magnetic fields has been investigated. It is found that the sign of the change in transparency in an ac electric field depends on the field frequency. It is shown that, joint action of codirectional low-frequency electric and dc magnetic fields can compensate for the change in the optical density. Calculation of the change in the emulsion optical density within the anomalous diffraction approximation showed that this effect can be explained by small field-induced deformation of microdrops.     

Electric field effect on the second-order nonlinear optical properties in semiparabolic quantum wells

Electric field effect on the second-order nonlinear optical properties in semiparabolic quantum wells are studied theoretically. Both the second-harmonic generation susceptibility and nonlinear optical rectification depend dramatically on the direction and the strength of the electric field. Numerical results show that both the second-harmonic generation susceptibility and nonlinear optical rectification are always weakened as the electric field increases where the direction of the electric field is along the growth direction of the quantum wells, which is in contrast to the conventional case. However, the second-harmonic generation susceptibility is weakened, but the nonlinear optical rectification is strengthened as the electric field increases where the direction of the electric field is against the growth direction of the quantum wells. Also it is the blue (or red) shift of the resonance that is induced by increasing of the electric field when the direction of the electric field is along (or against) the growth direction of the quantum wells. Finally, the resonant peak and its corresponding to the resonant energy are also taken into account.     

Spectral tuning by selective enhancement of electric and magnetic dipole emission

We demonstrate that magnetic dipole transitions provide an additional degree of freedom for engineering emission spectra. Without the need for a high-quality optical cavity, we show how a simple gold mirror can strongly tune the emission of trivalent europium. We exploit the differing field symmetries of electric and magnetic dipoles to selectively direct the majority of emission through each of three major transitions (centered at 590, 620, and 700 nm), and present a model that accurately predicts this tuning from the local electric and magnetic density of optical states.     

Über den Einfluß der Temperatur auf die Feldverstärkung und Feldauslöschung der Kathodolumineszenz

The luminescence of manganese activated zinc sulfide has been investigated. It was found that the luminescence, excited by cathode rays, is profoundly influenced by alternating electric fields. At room temperature the emission due to the manganese is enhanced, and that due to selfactivation is quenched by the field. At lower temperatures, however, the direction of the energy transport controlled by the electric field changes the sign: the emission of mangenese is quenched by the field, whereas the luminescence due to selfactivation is enhanced. This behaviour may be explained with reference to our model according to which the electrons gain energy in the electric field and the number of occupied states changes.     

Effect of laser radiation on optical properties of disk shaped quantum dot in magnetic fields

The optical absorption coefficients and changes in the refractive index in GaAs/AlGaAs, disk shaped quantum dots (DSQD) with simultaneously applied laser and magnetic field are studied in detail. The use of the density matrix formalism is made to study the variations in linear and non-linear polarizability with the frequency of the electric field. It is found that the absorption coefficient and the refractive index changes depend not only on the optical wave but also on the strength of the static magnetic field.     

Orientational transitions in ferromagnetic liquid crystals with bistable coupling between colloidal particles and the matrix

We study the orientational response of a ferromagnetic liquid crystal that is induced by magnetic and electric fields. A modified form of the energy of the orientational interaction between magnetic impurity particles and the liquid crystal matrix that leads to bistable coupling is considered. It is shown that apart from magnetic impurity segregation, first-order orientational transitions can be due to the bistability of the potential of the orientational coupling between the director and the magnetization. The ranges of material parameters that lead to optical bistability are determined. The possibility of first-order orientational transitions is analyzed for the optical phase difference between the ordinary and extraordinary light rays transmitted through a ferronematic cell. It is shown that an electric field applied in the given geometry considerably enhances the magneto-orientational response of the ferronematic.     

Noise-driven optical absorption coefficients of impurity doped quantum dots

We make an extensive investigation of linear, third-order nonlinear, and total optical absorption coefficients (ACs) of impurity doped quantum dots (QDs) in presence and absence of noise. The noise invoked in the present study is a Gaussian white noise. The quantum dot is doped with repulsive Gaussian impurity. Noise has been introduced to the system additively and multiplicatively. A perpendicular magnetic field acts as a source of confinement and a static external electric field has been applied. The AC profiles have been studied as a function of incident photon energy when several important parameters such as optical intensity, electric field strength, magnetic field strength, confinement energy, dopant location, relaxation time, Al concentration, dopant potential, and noise strength take on different values. In addition, the role of mode of application of noise (additive/multiplicative) on the AC profiles has also been analyzed meticulously. The AC profiles often consist of a number of interesting observations such as one photon resonance enhancement, shift of AC peak position, variation of AC peak intensity, and bleaching of AC peak. However, presence of noise alters the features of AC profiles and leads to some interesting manifestations. Multiplicative noise brings about more complexity in the AC profiles than its additive counterpart. The observations indeed illuminate several useful aspects in the study of linear and nonlinear optical properties of doped QD systems, specially in presence of noise. The findings are expected to be quite relevant from a technological perspective.