HI－13串列加速器上的核结构研究

本文综述了中国原子能科学研究院ＨＩ－１３串列加速器上的核结构研究．在原于核高自旋态方面．简要地介绍了稀土区奇质子核带交叉反常现象研究,质量数为Ａ＝９０和Ａ＝１３０核区的高自旋态研究、原子核高自旋能级寿命研究和三轴形变研究．在原于核巨共振方面介绍了矮共振区的ＧＤＲ研究,形变核的ＧＤＲ以及高温转动核的ＧＤＲ研究． The nuclear structure studies carried out at the HI-13 tandem in China Institute of Atomic Energy are reviewed. Brief introductions in the field of high spin state physics are given, such as the anomolous band crossing for odd-proton rare earth nuclei, high spin state studies in the mass 90 and 130 regions, nuclear high spin state life time study and the investigation of the triaxial de formation. Brief introductions in the field of GDR studies of pygmy resonance and GDR studies in deformed...     

A=135核区N=79的同中异位素高自旋结构研究

摘要: 对清华大学在束γ谱实验组近年来在A=135缺中子核区N=79的同中异位素 135Ba, 137Ce和 139Nd的高自旋态实验研究进行了介绍。 实验是在中国原子能科学研究院HI 13串列加速器上用在束γ的实验技术、 分别通过重离子核反应 130Te(9Be, 4n), 124Sn(18O, 5n), 128Te(16O, 5n)进行的。 实验结果扩展了这3个核的高自旋态能级纲图。 研究表明, 这3个核的低自旋态结构均起源于 νh-111/2空穴与其偶偶核芯的耦合。 用粒子 转子模型对其结构进行了计算, 得到这3个核的形变参量γ值均稍大于30°, 为偏向于扁椭的三轴形变, 从而可看出Ba, Ce和Nd 3个同位素链在低自旋态下由长椭边到扁椭边的形状转变都发生在中子数N=77—79之间。 对于中等自旋态下一些能级的组态进行了指定与系统学比较。 在高自旋态下, 在 137Ce中发现一条γ≈－60°的扁椭形变带, 在 139Nd中则发现3条这样的扁椭形变带, 对这些扁椭形变带的起源及结构特性进行了讨论。 The progress of research on the high spin states at N=79 isotopes 135Ba, 137Ce and 139Nd in A=135 neutron deficient region by the research group of Tsinghua University has been reviewed. The experiments were carried out by using in beam γ ray spectroscopy technology and heavy ion nuclear reactions 130Te(9Be, 4n), 124Sn(18O, 5n) and 128Te(16O, 5n) at China Institute of Atomic Energy (CIAE). The high spin level schemes of these nuclei have been expanded. The results indicate that the lower spin states of these nuclei originated from νh-111/2 hole state coupling with the neighboring even even nucleus cores. All the deformation parameters γ values of these three isotones are larger than 30°, which indicates that they have triaxial deformation with oblate side. The prolate oblate transition in Ba, Ce and Nd isotopic chains indeed happens between N=77 and N=79. Through systematical comparison with the neighboring isotones, the configurations for some middle spin state levels have been assigned. At the high spin states, one oblate band in 137Ce and three ones in 139Nd with γ≈ -60° were discovered. The origination and structural character of these oblate bands have been discussed.     

爆发性核合成与核结构

讨论了天体物理环境中爆发性核合成及其与核结构的紧密关系.用反射不对称壳模型计算了远离稳定线丰中子核148Ba的低能八极转动带,结果与实验很好符合.展示了其应用于不稳定核低能态计算的有效性 ,以及在核天体物理研究中的应用前景.The explosive nucleosynthesis in the astrophysical environment and its close link to nuclear structure are discussed. The low lying octupole bands for neutron rich nucleus 148 Ba far from the stability line have been calculated by the reflection asymmetric shell model and the results are in good agreement with the experimental data, presenting the capability of the model for calculations of the low lying states of unstable nuclei as well as the foreground of application in nuclear astrophysics.     

实验核物理进展

本文回顾我所实验核物理科研人员在低能核反应机制、中子物理、核衰变性质及核结构研究中所做一系列工作,同时简单介绍了目前工作和设想． The paper reviews the research activities at SINR on experimental nuclear physics. The studies have been focused on mechanism of nuclear reactions, neutron physics,properties of nuclear decay and nuclear structure. Brief introductions are given to the ongoing research projects and future plans in the field of research.     

准幻核中的近似广义辛弱数守恒（英文）

对称性在了解诸如原子核的转动、自旋和宇称、及同位旋等核结构性质中都起着重要的作用,并且使复杂的原子核结构问题得以简化。辛弱数就是由于原子核的对相互作用中的对称性所导出的众所周知的好量子数。通过对丰中子和缺中子核素及核素的高自旋态的衰变数据分析来揭示辛弱数的近似守恒性质。研究结果表明,在准幻核的高自旋同质异能素链中,无论所涉及的价空间的核子轨道有何不同,广义辛弱数总是近似的好量子数。Symmetry plays an important role in understanding the nuclear structure properties from the rotation of a nucleus to the spin, parity and isospin of nuclear states. This simplifies the complexity of the nuclear problems in one way or the other. Seniority is also a well known quantum number which arises due to the symmetry in the pairing interaction of nuclei. We present empirical as well as theoretical evidences based on decay rates which support the goodness of seniority at higher spins as well as in nrich or, n-deficient nuclei. We find that the generalized seniority governs the identical trends of high-spin isomers in different semi-magic chains, where different set of nucleon orbitals from different valence spaces are involved.     

Delta-Davidson method for interior eigenproblem in many-spin systems

Many numerical methods,such as tensor network approaches including density matrix renormalization group calculations,have been developed to calculate the extreme/ground states of quantum many-body systems.However,little attention has been paid to the central states,which are exponentially close to each other in terms of system size.We propose a delta-Davidson(DELDAV)method to efficiently find such interior(including the central)states in many-spin systems.The DELDAV method utilizes a delta filter in Chebyshev polynomial expansion combined with subspace diagonalization to overcome the nearly degenerate problem.Numerical experiments on Ising spin chain and spin glass shards show the correctness,efficiency,and robustness of the proposed method in finding the interior states as well as the ground states.The sought interior states may be employed to identify many-body localization phase,quantum chaos,and extremely long-time dynamical structure.     

高自旋同质异能态束流及其在核谱学中的应用

介绍了在日本理化学研究所利用高自旋同质异能态束流装置上取得的核谱学研究结果。强调了可利用重离子核反应中逆运动学产生高自旋同质界能态束流,并用其进行二次核反应,描述了首次利用高自旋同质异能态束流完成的物理实验． The study of nuclear spectroscopy by using the High spin isomer Beam(HSIB)facility in RIKEN was introduced.The production of HSIB based on the inverse kinematics in heavy ion nuclear reaction,and its application for secondary nuclear reaction were stressed The first experimental result by using HSIB was also briefly discribed.     

核物理研究新进展

本文介绍了国际核物理研究的趋势,核物理研究的前沿已从传统核物理转向亚核自由度变得重要的领域,讨论了在核结构、核反应、相对论性重离子碰撞、亚核自由度、放射性核束和核天体物理学等领域所获得的最新成果. It is presented the trend of the nuclear physics research in the world,the fron- tier of nuclear physics research has been moved from the traditional nuclear physics to the field in which the subnuclear freedoms become very important.New research results obtained in the fields of nuclear structures,nuclear reactions,relativistic heavy ion collisions, subnuclear freedoms,radioactive nuclear beams and nuclear astrophysics are discussed.     

稀土区奇A核晕带存在从转动到振动形状演化的直接证据(英文)

原子核的形状演化效应是核结构研究的重要基础问题之一。通常认为,A=160质量区的奇A核位于大形变核区域,它们的激发态能谱将呈现出典型的转动激发特征。然而,基于E-GOS曲线方法,发现随着角动量的增加,该质量区奇A核的晕带具有显著地从转动激发演化成为振动激发的形状演化现象。此外,为深入理解原子核形状演化的微观机制,采用Total-Routhian-Surface（TRS）方法针对稀土区的奇A核进行了理论计算,结果表明,165Yb和157Dy同位素在低激发态时具有稳定的长椭形变,当角动量大于0.50 MeV后,核芯的四极形变显著减小并开始产生三轴形变。The phase transition of nuclei with increasing angular momentum (or spin) and excitation energy is one of the most fundamental topics of nuclear structure research. The odd-N nuclei with A ≈160 are widely considered belonging to the well-deformed region, and their excitation spectra are energetically favored to exhibit the rotational characteristics. In this work, however, the evidence suggesting that the nuclei changes from rotation to vibration along the yrast lines as a function of spin was found. The simple method, named as E-Gamma Over Spin (E-GOS) curves, would be used to discern the evolution from rotational to vibrational structure in nuclei for various spin ranges. Meanwhile, in order to understand the band structure properties of nuclei, theoretical calculations have been performed for the yrast bands of the odd-A rare-earth nuclei within the framework of the total routhian surface (TRS) model. The TRS plots predict that the 165Yb and 157Dy isotopes have large quadrupole shapes at low spin states. At higher rotational frequency (hω~ >0.50 MeV), a clear reduction of the quadrupole deformation is indicated by the present results, and the isotopes become rigid in the γ deformation.     

强子结构与核结构

本文列举了核内存在非核子自由度的证据;论证了核结构的研究必须突破传统的框架,进入到核子及介子的内部结构,才能对原子核内部运动有深入的了解.本文还扼要论述了核物理研究的现状与前景. This paper presents some important experimental evidences of non-nucleonic degrees of freedom in nuclei.From these evidences,the nuclear structure research must go be- yond the traditional framework of nuclear research.To get deeper understanding of the nucle- us,one has to go to the internal structure of hadrons.The present status and future prospects of this new development in nuclear physics are also dicussed briefly.     

清华大学物理系原子核物理研究的新进展

在清华大学物理系成立80周年之际,对近年来清华大学物理系原子核物理研究的主要进展情况作一介绍,包括原子核高自旋态的实验研究,原子核结构的理论研究,高能核物理的理论研究.在高自旋态研究方面,内容包括在A～100丰中子核区核的集体振动转动带结构、新的准粒子带特性、新手征二重带等特性研究;在A～140丰中子核区核的八极形变及八级关联等特性研究;在A～130缺中子核区核的形状驱动效应,包括扁椭形变带、形状共存等特性研究.在原子核结构理论研究方面,内容包括用相互作用玻色子模型、推转壳模型、投影壳模型以及相对论平均场对原子核特性的研究;对原子核结构或其他量子系统的各种对称性和代数方法的研究,如动力学对称性、超对称性、势代数方法等;与对称性紧密联系的普通李代数和非线性李代数的表示,如普通李代数、李超代数、平方根型非线性李代数、多项式型非线性李代数等.在高能核物理研究方面,内容主要包括量子色动力学（QCD）在高温高密条件下的相变以及在相对论重离子碰撞中相变信号的研究.     

Angular momentum dependence of giant dipole vibrations in hot dysprosium nuclei

The spin dependence of the giant dipole resonance built on excited states in ¹⁵⁶Dy has been studied with a new technique using Ge-BGO spectrometers. The observed structure of the GDR and the measured γ-ray anisotropies are consistent with a change in nuclear shape from prolate to oblate with increasing spin. No evidence is found for centroid shifts nor for superdeformed shapes at high temperature.     

用于指导仲氢诱导核极化状态保存的己烯分子中五自旋的单重态制备和寿命研究

仲氢诱导核极化（PHIP）技术能极大地增强核磁共振（NMR）信号的灵敏度,已被应用于磁共振成像、原位化学反应监测等领域．除了不断提高不同分子极化后的灵敏度外,延长和保存高极化度状态对PHIP技术的应用也至关重要,其中将极化后的状态制备成核自旋单重态是目前被研究较多的一种方法．本文以能被PHIP技术极化的己烯分子为研究对象,通过设计优化控制脉冲,对分子中的一个五自旋体系进行操控,制备了多种核自旋单重态,结果表明：己烯分子的碳-碳双键上存在三种不同的核自旋单重态,它们的寿命均长于仲氢极化后产生的初始态的寿命,可以作为延缓极化度衰减的一种中间态;通过对比单重态的寿命与相应自旋的纵向弛豫时间发现,将极化后己烯的状态转化为纵向磁化可能也是一种保存极化度的有效方法．     

ESR study of exchange coupled pairs in copper diethyldithiocarbamate—explanation of the low temperature hyperfine anomaly

A study of the hyperfine interaction in the ESR of Cu-Cu pairs in single crystals of copper diethyldithiocarbamate as a function of temperature has shown distinct differences in the hyperfine structure in the two fine structure transitions at 20 K, the spectrum not having the same hyperfine intensity pattern in the low field fine structure transition in contrast to that of the high field transition. The details of the structure of both the fine structure transitions in the 20 K spectrum have now been explained by recognizing the fact that the mixing of the nuclear spin states caused by the anisotropic hyperfine interaction affects the electron spin states | + 1 > and | −> differently. This has incidentally led to a determination of the sign ofD confirming the earlier model. The anomalous hyperfine structure is found to become symmetric at 77 K and 300 K. It is proposed that the reason for this lies in the dynamics of spin-lattice interaction which limits the lifetime of the spin states in each of the electronic levels | − 1 >, | 0 > and | + 1 > The estimate of spin-lattice relaxation time agrees with those indicated from other studies. The model proposed here for the hyperfine interaction of pairs in the electronic triplet state is of general validity.     

Hyperfine anomaly arising from the nuclear spin-forbidden transition,and absolute sign determination of the zero-field splitting constant

It has been found in the triplet E.S.R. spectra of radical pairs in irradiated potassium deuterium fumarate that the hyperfine structure of the two transitions, M _s = 1?0 and M _s = 0?+1, are entirely different. This anomaly has been interpreted in terms of the forbidden transition arising from the mixing of the nuclear spin states by the anisotropic hyperfine interaction. The theory has been developed for multiplet electron spin systems and includes the nuclear Zeeman interaction which is often neglected. The theoretical predictions are in good agreement with the observed separations and intensities of the anomalous hyperfine lines. In addition, it has been found that since the forbidden lines of the electron spin multiplet system with S ≥ 1 appear strongly only in transitions which include some specific electronic spin states, the anomalous features of the spectra make it possible to determine the absolute sign of the zero-field or hyperfine splitting constant, if the sign for one of them is known. Using this principle, attempts have been made to determine the absolute sign of the zero-field splitting constant for a number of triplet E.S.R. spectra which exhibit a hyperfine anomaly arising from the proposed mechanism.     

Fascinating electronic games in iron complexes

Summary Coordination compounds of transition metal ions with open-shell electron configurations may exhibit dynamic electronic-structure phenomena, depending on the nature of the coordinating ligand sphere. The change of spin state with temperature (?thermal spin-crossover?), light-induced electron transfer processes leading to long-lived metastable charge and spin states (e.g., ?LIESST? effect), are some of the fascinating electronic games encountered in transition metal compounds, which are presently under extensive study by chemists and physicists. M?ssbauer spectroscopy plays a dominant role in the investigation of such phenomena in iron compounds, as will be demonstrated in this paper. This work will focus on selected examples of ?thermal spin-crossover? in iron(II) complexes and switching between different spin states by irradiation with light of different wavelength (LIESST effect), demonstrating that M?ssbauer spectroscopy besides other physical techniques proves to be a highly elegant tool for following the spin state conversion and the concomitant changes of molecular and crystal structure properties. Finally, M?ssbauer emission spectroscopy, both time integral and time differential, has been employed to generate and identify long-lived excited spin states by making use of the nuclear disintegration of⁵⁷Co as an intrinsic molecular light source (NIESST=nuclear decay-induced excited-spin-state trapping). Lifetime measurements by optical techniques on LIESST states and by time-differential M?ssbauer coincidence spectroscopy on NIESST states prove that the relaxation pathways in the mechanisms for LIESST and NIESST are identical. Dedicated to Prof. Harry B. Gray on the occasion of his 60th birthday. Paper presented at ICAME-95, Rimini, 10–16 September 1995.     

Electrical detection of coherent nuclear spin oscillations in phosphorus-doped silicon using pulsed ENDOR

We demonstrate the electrical detection of pulsed X-band electron nuclear double resonance (ENDOR) in phosphorus-doped silicon at 5 K. A pulse sequence analogous to Davies ENDOR in conventional electron spin resonance is used to measure the nuclear spin transition frequencies of the (31)P nuclear spins, where the (31)P electron spins are detected electrically via spin-dependent transitions through Si/SiO(2) interface states, thus not relying on a polarization of the electron spin system. In addition, the electrical detection of coherent nuclear spin oscillations is shown, demonstrating the feasibility to electrically read out the spin states of possible nuclear spin qubits.     

Quantum readout and fast initialization of nuclear spin qubits with electric currents

Nuclear spin qubits have the longest coherence times in the solid state, but their quantum readout and initialization is a great challenge. We present a theory for the interaction of an electric current with the nuclear spins of donor impurities in semiconductors. The theory yields a sensitivity criterion for quantum detection of nuclear spin states using electrically detected magnetic resonance, as well as an all-electrical method for fast nuclear spin qubit initialization.