Beyond the N = 50 shell closure: High-spin excitations of 87Kr and ground-state spin of 87Br

The ⁸⁷Kr nucleus has been produced as fission fragment in the fusion reaction ¹⁸O + ²⁰⁸Pb at 85MeV bombarding energy and studied with the Euroball IV array. High-spin states of this neutron-rich isotope have been identified for the first time. Its level scheme has been obtained up to 6.3MeV excitation energy and spin I ∼ 23/2ℏ. Its structure is interpreted by analogy with those of the heavier isotones. The proposed configurations involve both proton and neutron excitations from several sub-shells located close to the Fermi levels, particularly νd_5/2, πp_3/2f_5/2 and πg_9/2. Moreover, a revised spin value of 5/2^- for the ⁸⁷Br ground state is proposed.     

Rotational bands and signature inversion phenomena in πh9/2⊗νi13/2 and πi13/2⊗νi13/2 structures in odd-odd 176Ir

The ^109,111,113Rh nuclei have been produced as fission fragments in the fusion reaction ¹⁸O + ²⁰⁸Pb at 85 MeV. Their level schemes have been built from gamma-rays detected using the Euroball IV array. High-spin states of the neutron-rich ^111,113Rh nuclei have been identified for the first time. Several rotational bands with the odd proton occupying the πg _9/2, πp _1/2 and π(g _7/2/d _5/2) sub-shells have been observed. A band of low-energy transitions has been identified at excitation energy around 2 MeV in ^109,111Rh, which can be interpreted in terms of three-quasiparticle excitation, πg _9/2νh _11/2νg _7/2/d _5/2. In addition another structure built on states located at low excitation energy (608 keV in ¹¹¹Rh, 570 keV in ¹¹³Rh) points out that, as already observed in the lighter isotopes ^107,109Rh, triaxial deformation plays a role in the neutron-rich Rh isotopes well beyond the mid-shell. Received: 15 July 2002 / Accepted: 9 October 2002 / Published online: 3 December 2002 RID="a" ID="a"e-mail: porquet@csnsm.in2p3.fr RID="b" ID="b"Present address: CSNSM IN2P3-CNRS and Université Paris-Sud 91405 Orsay, France. RID="c" ID="c"Present address: CEA/Saclay, DSM/DAPNIA/SPhN, 91191 Gif-sur-Yvette Cedex, France. Communicated by D. Schwalm     

Observation of a πh9/2 ⊗ νi13/2 oblate band in 188Tl

Excited states in ¹⁸⁸Tl have been studied experimentally using the ¹⁵⁷Gd (³⁵Cl, 4n) reaction at a beam energy of 170MeV. A rotational band built on the πh _9/2 ⊗ νi _13/2 configuration with oblate deformation has been established for ¹⁸⁸Tl. Based on the structure systematics of the oblate πh _9/2 ⊗ νi _13/2 bands in the heavier odd-odd Tl nuclei, we have tentatively proposed spin values for the new band in ¹⁸⁸Tl. The πh _9/2 ⊗ νi _13/2 oblate band in ¹⁸⁸Tl shows low-spin signature inversion, and it can be interpreted qualitatively by the two-quasiparticle plus rotor model including a J-dependent p-n residual interaction.     

The structure of 99Ru from (α,3n) reaction

The results of in-beam investigations of excited states of ⁹⁹Ru using the ⁹⁸Mo(α,3n) reaction are presented. Angular distributions of γ–rays and γ–γ coincidences have been measured. Excited states have been identified up to an energy of E = 5603 keV and spin of I^π= 31/2⁻. Mean lifetimes τ have been determined using the DSA method for eleven levels. Aligned angular momenta are discussed and the probable (νh _11/2) origin of a backbending at frequency about 0.5 MeV was confirmed. The possible role of (νd _5/2) alignment at frequencies above 0.5 MeV was pointed out. Received: 13 January 1999 / Revised version: 26 March 1999     

Level structure of 99Rh at high spins

High spins states in ⁹⁹Rh were populated via the ⁶⁶Zn(³⁷Cl, 2p2n)⁹⁹Rh reaction at an incident beam energy of 130 MeV. Seventeen new transitions have been observed in the present study and the level scheme has now been extended up to a spin of J∼ 25ħ and an excitation energy of about E _x∼ 10 MeV. The observation of a positive parity E2 cascade based on the 9/2⁺ isomeric level is suggestive of collective behaviour in this nucleus up to high spins. Spherical shell model (within restricted model space) and Cranked shell model calculations were performed to obtain an insight into the observed level structure. The new collective band observed up to a spin of J∼ 25ħ is suggested to be based on (πg _9/2 ³) ⊗ (νg _7/2 ²) quasi-particle excitations. Received: 12 July 1999 / Revised version: 14 September 1999     

Spectroscopy of the neutron-deficient nuclide 171Pt

The decay out of the πh _11/2νh _11/2 band to the known low-energy levels in ¹³²La was studied using the reaction ¹⁰⁰Mo + ³⁶S at 160 MeV beam energy. The low-energy level scheme has been further developed and unambiguous spin and parity values have been assigned to the levels connecting the band to the 6^- isomeric state. According to the new level scheme the spins in the πh _11/2νh _11/2 band are shifted up by one unit compared to the earlier tentative experimental values. The obtained new spins prove the existence of signature inversion in ¹³²La and give further support to the spin assignments made for the πh _11/2νh _11/2 bands in the neighbouring odd-odd La isotopes from level energy systematics. Received: 7 May 2002 / Accepted: 31 October 2002 / Published online: 17 January 2003 RID="a" ID="a"e-mail: timar@atomki.hu RID="b" ID="b"Present address: Dipartimento di Matematica e Fisica, Università di Camerino, via Madonna delle Carceri, I-62032 Camerino, Italy. Communicated by J. ?yst?     

Shape-driving effect of the proton 1/2[541] band in 171Ta

High-spin states in ¹⁷¹Ta were populated through the heavy-ion fusion-evaporation reaction ¹⁵⁷Gd (¹⁹F, 5n)¹⁷¹Ta at 105MeV beam energy. Lifetimes of the levels of the πh_9/21/2[541] band have been measured by using the Doppler shift attenuation method. The transition quadrupole moments ( Q_t) and the quadrupole deformation (β₂) have been extracted. Both β₂ and Q_t values decrease slightly with increasing rotational frequency. The average β₂ value of 0.26 is 18% larger than that of the πh_11/2 9/2[514] band. Total Routhian Surface calculations have been performed with the non-axial deformed Woods-Saxon potential and the predicted values of the quadrupole deformation β₂ are in good agreement with that deduced from our lifetime measurement. The shape-driving effect is discussed.     

Investigations of low- and high-spin states of <Superscript>132</Superscript>La

The fusion evaporation reaction ¹²²Sn(¹⁴N, 4n)¹³²La was used to populate the high-spin states of ¹³²La at the beam energy of 60 MeV. A new band consisting of mostly E2 transitions has been discovered. This band has the interesting links to the ground state 2^- and the isomeric state 6^-. A new transition of energy 351 keV connecting the low-spin states of the positive-parity band based on the πh _11/2 ⊗ νh _11/2 particle configuration, has been found. This has played a very important role in resolving the existing ambiguities and inconsistencies in the spin assignment of the band head. Received: 12 August 2002 / Accepted: 18 March 2003 / Published online: 7 May 2003     

Shape changes at high spin in 78Kr

High-spin states in ⁷⁸Kr have been studied via the ⁶³Cu (¹⁹F, 2p2n)⁷⁸Kr reaction at a beam energy of 60 MeV using the Indian National Gamma Array (INGA). In this nucleus, lifetimes have been measured upto the I^π=22⁺ level in the yrast positive-parity band and upto the I^π=15^- level in the negative-parity band using the Doppler Shift Attenuation Method (DSAM). The deduced transition quadrupole moments Q_t's are found to decrease with rotational frequency for both the bands.     

Rotational structures in 123Cs

High-spin states in ¹²³Cs, populated via the ¹⁰⁰Mo ( ²⁸Si, p4n) fusion-evaporation reaction at E _lab = 130 MeV, have been investigated employing in-beam γ-ray spectroscopic techniques. Rotational bands, built on πg _7/2, πg _9/2 and the unique-parity πh _11/2 orbitals, have been extended and evolve into bands involving rotationally aligned ν(h _11/2)² and π(h _11/2)² quasiparticles. A three-quasiparticle band based on the high-K πh _11/2 ⊗ νg _7/2 ⊗ νh _11/2 configuration has also been observed. Total Routhian Surface (TRS) calculations have been used to predict the nuclear shape parameters ( β₂, β₄, γ) for the various assigned configurations. The assigned configurations have been discussed in the framework of a microscopic theory based on the deformed Hartree-Fock (HF) and angular-momentum projection techniques.     

Beta-decay of the N = Z nucleus 72Kr

The beta-decay of the N = Z, even-even nucleus ⁷²Kr has been studied at the ISOLDE PSB facility at CERN. Measurements of βγ and βγγ coincidences have enriched the decay scheme of the daughter nucleus ⁷²Br with 27 new low spin levels. A more precise half-life of T _1/2 = 17.1(2) s has been determined. Strong feeding to the ⁷²Br ground state is established yielding an unambiguous J ^π = 1⁺ assignment for this state. Candidates for the ⁷²Br g.s. wave function are discussed in the framework of a self-consistent deformed mean-field calculation with SG2 Skyrme force and pairing correlations. A search for beta-delayed particle emission was made and an upper limit of 10^-6 for this decay branch obtained. The cumulated experimental level density of 1⁺ states has been fitted with the constant temperature formula. The comparison indicates that most likely all 1⁺ levels up to 1.2 MeV have been observed in this investigation. The corresponding nearest-neighbour level spacing does not follow a Poisson distribution. The Gamow-Teller strength distribution is compared, in terms of nuclear deformation, with different calculations made in the framework of the quasiparticle random phase approximation. Received: 7 February 2002 / Accepted: 31 October 2002 / Published online: 6 March 2003 RID="a" ID="a"e-mail: borge@pinar2.csic.es RID="b" ID="b"Present address: Centre d' Etudes Nucléaires de Bordeaux-Gradignan, Le Haut Vigneau, F-33175 Gradignan Cedex, France. RID="c" ID="c"Present address: University Mentouri, 25000 Constantine, Algeria. Communicated by J. ?yst?     

High-spin levels based on the 11/2- isomer in 135Ba

High-spin states in the ¹³⁵Ba nucleus have been studied with the reaction ¹³⁰Te(⁹Be, 4n) at a beam energy of 45 MeV. The level scheme based on the h _11/2 isomer has been expanded with spins up to 35/2 ℏ. At low spins, the yrast collective structure built on the ν h _11/2 ^-1 multiplet may show a transitional shape with γ > 30^° according to the systematical behavior observed in neighboring nuclei as well as the calculations of the triaxial rotor-plus-particle model. The configurations for several high-spin states have been discussed from a systematical comparison with neighboring isotones.     

High-spin study of odd- A 49In isotopes beyond the neutron mid-shell

The ^{115, 117, 119, 121}In nuclei have been produced as fission fragments in three reactions induced by heavy ions: ¹²C + ²³⁸U at 90MeV bombarding energy, ¹⁸O + ²⁰⁸Pb reaction at 85MeV, and ³¹P + ¹⁷⁶Yb at 152MeV. Their level schemes have been built from gamma-rays detected using the EUROBALL III and IV arrays. High-spin states of ^{117, 119, 121}In nuclei have been identified for the first time. Moreover, isomeric states lying around 2.5MeV have been established in ^{119, 121}In from the delayed coincidences between the fission fragment detector SAPhIR and the gamma array. Most of the observed states can be described by coupling a proton g _9/2 hole to a Sn core, while the intruder band based on an orbital from the π[g _7/2/d _5/2] sub-shells behaves as the ground-state band of neighbouring Cd isotopes. Received: 24 May 2002 / Accepted: 11 June 2002 / Published online: 19 November 2002 RID="a" ID="a"e-mail: porquet@csnsm.in2p3.fr RID="b" ID="b"Present address: CEA-DIF, DAM/DCRE/SDE/LDN, 91680 Bruyères-le-Chatel, France. RID="c" ID="c"Present address: CSNSM IN2P3-CNRS and Université Paris-Sud 91405 Orsay, France. RID="d" ID="d"Present address: CEA/Saclay, DSM/DAPNIA/SPhN, 91191 Gif-sur-Yvette Cedex, France. Communicated by D. Schwalm     

Signature inversion in πi13/2⊗νi13/2 structure in 178Ir

High-spin states in ¹⁷⁸Ir were investigated by means of in-beam γ-ray spectroscopy techniques using the multidetector array GASP. Excited states of ¹⁷⁸Ir were populated through the ¹⁵⁹Tb(²⁴Mg, 5n) fusion-evaporation reaction at E(²⁴ Mg) = 131-141 MeV. Several rotational bands were observed. Among them, the πi _13/2⊗νi _13/2 structure has been identified up to spin 36 ?. This band exhibits an anomalous signature splitting and a signature inversion around spin 25 ?. Received: 13 December 2000 / Accepted: 11 April 2001     

Octupole-deformed molecular bands in 21Ne

Cluster states up to 12 MeV in the stable light nucleus ²¹Ne, based on the ¹⁶O + n + α molecular configurations, have been populated in the incomplete-fusion reaction ¹⁶ ₈O(⁷₃Li, np)²¹₁₀Ne at 29.4 MeV. The observation of both intra- and inter-band transitions leads to a re-interpretation of some levels in the K^π = ^- and K^π = ^- bands. The implications of this re-ordering on the octupole doublet bands are examined. The data allow a more accurate determination of some previously uncertain level energies. The “missing” I^π = ^- level is also discussed.     

Rotational structures in the 125Cs nucleus

The collective band structures of the ¹²⁵Cs nucleus have been investigated by in-beam γ-ray spectroscopic techniques following the ¹¹⁰Pd ( ¹⁹F, 4n) reaction at 75MeV. The previously known level scheme, with rotational bands built on πg_7/2, πg_9/2 and πh_11/2 orbitals, has been extended and evolves into bands involving rotationally aligned ν(h_11/2)² and π(h_11/2)² quasiparticles. A strongly coupled band has been reassigned a high-K πh_11/2 ⊗ νg_7/2 ⊗ νh_11/2 three-quasiparticle configuration and a new side band likely to be its chiral partner has been identified. Configurations assigned to various bands are discussed in the framework of Principal/Tilted Axis Cranking (PAC/TAC) model calculations.     

High-spin states in the <Superscript>97</Superscript>Tc nucleus

High-spin states in the ⁹⁷Tc nucleus have been studied by in-beam γ-ray spectroscopy with the reaction ⁸²Se(¹⁹F,4nγ) at 68 MeV incident energy. Excited states have been observed up to about 8 MeV excitation and spin 43/2. The observed level scheme is compared with results of shell model calculations. Received: 22 November 2002 / Accepted: 23 December 2002 / Published online: 18 March 2003 RID="a" ID="a"e-mail: bucurescu@tandem.nipne.ro RID="b" ID="b"Present address: INFN, Laboratori Nazionali di Legnaro, Legnaro, Italy. RID="b" ID="b"Present address: INFN, Laboratori Nazionali di Legnaro, Legnaro, Italy. RID="b" ID="b"Present address: INFN, Laboratori Nazionali di Legnaro, Legnaro, Italy. RID="c" ID="c"Present address: Università di Padova, Padova, Italy. Communicated by C. Signorini     

New high-spin states of 147Nd and 145Ce: Octupole correlation in the N = 87 isotones

High-spin states of the N = 87 nuclei, ¹⁴⁷Nd and ¹⁴⁵Ce, have been populated in the ¹²C + ²³⁸U and ¹⁸O + ²⁰⁸Pb fusion-fission reactions at 90 MeV and 85 MeV bombarding energy, respectively. The emitted γ-radiation was detected using the Euroball III and IV arrays. High-spin states of the ¹⁴⁷Nd isotope have been identified for the first time. The high-spin yrast and near-to-yrast structures of the ¹⁴⁵Ce nucleus have been considerably extended. The newly observed structures, discussed by analogy with the neighbouring isotones, show the coupling of an h_9/2 neutron to the quadrupole and octupole excitations of the core.     

Maximally aligned states in 99Ag

Excited states of ⁹⁹Ag were populated via the ⁵⁰Cr + ⁵⁸Ni (261 MeV) reaction using the NORDBALL detector array equipped with charged-particle and neutron detector systems for reaction channel separation. On the basis of the measured γγ-coincidence relations and angular distribution ratios a significantly extended level scheme has been constructed up to E _x ∼ 7.8 MeV and I = 35/2. The experimental results were described within the framework of the shell model. Candidates for states fully aligned in the πg _9/2 ^-3ν(d _5/2, g _7/2)² valence configuration space were found at 4109 and 6265 keV. Received: 18 June 2002 / Accepted: 11 October 2002 / Published online: 4 February 2003 RID="a" ID="a"e-mail: sohler@atomki.hu Communicated by J. ?yst?     

Nuclear quadrupole moments of 5/2<Superscript>-</Superscript> and 9/2<Superscript>-</Superscript> states in <Superscript>169</Superscript>Ta

The nuclear spectroscopic quadrupole moments for the πh_9/25/2^-, 1/2^-[541] and the πh_11/29/2^-, 9/2^-[514] isomeric states in ¹⁶⁹Ta have been measured employing the time differential perturbed angular-distribution technique following the nuclear reaction ¹⁵⁹Tb(¹⁶O, 6nγ)¹⁶⁹Ta at beam energy 104 MeV. The ratio of the intrinsic quadrupole moments has been derived as 1.87(13) from the measured quadrupole precession frequencies of the corresponding states. The model-independent analysis of the equilibrium deformation indicates strong prolate- and oblate-driving nature of the 1/2^-[541] and 9/2^-[514] orbitals in ^169,171Ta isotopes, respectively.