The modular group and super-KMS functionals

Every normal, faithful, self-adjoint functional on a von Neumann algebraA canonically determines a one-parameter-weakly continuous *-automorphism group (the analog of the modular group) and a canonical ₂ grading onA, commuting with . We show that the functional satisfies the weak super-KMS property with respect to and Furthermore, we prove that and are the unique pair of a-weakly continuous one-parameter *-automorphism group and a grading of the algebra, commuting with each other, with respect to which is weakly super-KMS. The above results thus provide a complete extension of the theory of Tomita and Takesaki to the nonpositive case.Supported in part by the National Science Foundation under Grant DMS-8922002.     

Cubic nonlinear tensor of a ferromagnet

The nonlinear properties of a ferromagnet are studied. Many-time retarded Green's functions are used to obtain an expression for the cubic nonlinearity tensor with allowance for spatial dispersion of a uniaxial ferromagnet. The components due to the dipole-dipole interaction of the spins and also due to the anisotropy energy are found. A comparative analysis is made of the different components of the cubic nonlinearity tensor in both the nonresonance case and for various resonances, in particular when ₀, 3 2w₀, 2 ₀, 3 ₀ for the case in tripling of the frequency. Here, is the frequency of the incident wave and ₀ is the frequency of uniform precession. It is shown that in the non-resonance case the largest components are those that are nonvanishing when no allowance is made for spatial dispersion; in the resonance cases the largest components are those due to the dipole-dipole interaction of the ferromagnetism spins.Translated from Izvestiya VUZ. Fizika, No. 12, pp. 53–58, December, 1973.     

Extensible Embeddings of Black-Hole Geometries

Removing a black hole conic singularity by means of Kruskal representation is equivalent to imposing extensibility on the Kasner–Fronsdal local isometric embedding of the corresponding black hole geometry. Allowing for globally non-trivial embeddings, living in Kaluza–Klein-like M ₅ × S ₁ (rather than in standard Minkowski M ₆ ) and parametrized by some wave number k, extensibility can be achieved for apparently forbidden frequencies in the range ₁ (k) ₂ (k). As k 0, _{1, 2} (0) _H (e.g., _H = 1/4M in the Schwarzschild case) such that the Hawking–Gibbons limit is fully recovered. The various Kruskal sheets are then viewed as slices of the Kaluza–Klein background. Euclidean k discreteness, dictated by imaginary time periodicity, is correlated with flux quantization of the underlying embedding gauge field.     

The Schrödinger equation and canonical perturbation theory

LetT ₀(, )+V be the Schrödinger operator corresponding to the classical HamiltonianH ₀()+V, whereH ₀() is thed-dimensional harmonic oscillator with non-resonant frequencies =(₁, ... , _d ) and the potentialV(q ₁, ... ,q _d) is an entire function of order (d+1)^–1. We prove that the algorithm of classical, canonical perturbation theory can be applied to the Schrödinger equation in the Bargmann representation. As a consequence, each term of the Rayleigh-Schrödinger series near any eigenvalue ofT ₀(, ) admits a convergent expansion in powers of of initial point the corresponding term of the classical Birkhoff expansion. Moreover ifV is an even polynomial, the above result and the KAM theorem show that all eigenvalues _n (, ) ofT ₀+V such thatn coincides with a KAM torus are given, up to order , by a quantization formula which reduces to the Bohr-Sommerfeld one up to first order terms in .     

Theoretical investigation of noncollinear phase-matched parametric four-photon amplification of ultrashort light pulses in isotropic media

The amplification of light signals (angular frequency _S in some isotropic media (D₂O, fused silica, and Schott type SF10 glasses) by noncollinear phase-matched parametric four-photon interaction ₁+_2S+₁ is studied theoretically. Computer simulations are carried out for fundamental and second-harmonic pump pulses of a mode-locked Nd: glass laser. Degenerate interaction (wavelength ₁=₂=1054nm or 527 nm) and nondegenerate interaction (₁=1054nm, ₂=527 nm are considered. Characteristic phase-matching parameters and gain parameters versus wavelength are determined. Limitations by spectral bandwidth, optical absorption, optical damage, self-phase modulation, self-focusing and stimulated Raman scattering are analysed.     

Spectral superbroadening of self-focused picosecond laser pulses in D2O

Intense picosecond light pulses of a mode-locked Nd: glass laser at _L =1054 nm (fundamental wavelength) and _SH =527 nm (second harmonic wavelength) are passed through a sample of D₂O under self-focusing conditions. Spectrally structured superbroadened, spatially bell-shaped emission in the forward direction is obtained. Primary generation processes are pump-pulse-degenerate stimulated parametric four-photon interaction (₁ + _{1 3} + ₄) and stimulated Raman scattering (_{1 R} + ), which occur concurrently (₁= _L or _SH angular pump frequency, #x03C9; _R first Stokes frequency, #x03C9; signal frequency, #x03C9;₃ signal frequency, #x03C9;₄ idler frequency). The parametric four-photon interaction occurs under collinear non-phase-matched conditions and under longitudinally phase-matched, transversally non-phase-matched (erenkov-like) conditions. Subsequent interaction processes are pump-pulse-nondegenerate four-photon interaction of the type ₁ + _{R 3} + ₄, coherent antiStokes Raman scattering (CARS, ₁ + ₁ – _{4 3}), inverse Raman scattering ( _A + ₁ + ), and cascading light up-conversion of the type ₁ + _(i) – _{R (i+1)}.     

A spectral characterization of KMS states

Let be a state on aC*-dynamical system . For each of the following properties of : (1) is -K MS with respect to for some given , 0<+, (2) is either a KMS state or a ground state, necessary and sufficient conditions are given involving only the spectral subspaces of associated with . The results provide a new insight in the concept of passivity, introduced by W. Pusz and S. L. Woronowicz.Aangesteld navorser N.F.W.O., Belgium, on leave from Katholieke Universiteit Leuven. Research partially supported by N.A.T.O.     

Normal mode configuration in an inorganic medium containing defects

The vibrational structure in an inorganic medium containing defects is analyzed as a function of the frequency of the applied field. Since the dispersion relations for the medium are nonlinear, the configuration of the normal modes depends differently upon and . It is shown that exponential damping of the optic branches is observed for <₀, and that the structure of these modes changes significantly over the range 0<<₀, so that only in the neighborhood of ₀ does it correspond to long wavelength vibrations with configurations of stress deviator waves.Institute for the Physics of Strength and Materials Science, Russian Academy of Sciences, Siberian Division. Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 10, pp. 87–90, October, 1994.     

Four-wave mixing in alkali halide crystals and aqueous solutions

Noncollinear phase-matched nonresonant four-photon frequency mixing _p+ _p– _{L s} in crystals and aqueous solutions of LiCl, CsCl, KF, and KI is studied. The concentration of the aqueous solutions is varied between 0.5 mol/l and saturation. Picosecond laser pulses of a mode-locked Nd-glass laser are applied as pump pulses. The energy conversion of laser light at frequency _L to frequency _S is measured and the nonlinear susceptibilities ⁽³⁾ are calculated. The dependence of the hyperpolarizabilities on concentration is analysed and gives information on the solute-solvent interaction.     

Two-photon resonance degenerate four-wave mixing in a three-level polar molecule (model calculations)

The third-order non-linear susceptibility, ⁽³⁾(; , , –), describing the phase conjugation by degenerate four-wave mixing (DFWM) is calculated for a three-level polar system under a two-photon resonance (TPR) condition. The part of the susceptibility expressed only by the transitional dipole moments and the part resulting from the permanent dipole moments are distinguished. The spectra of ⁽³⁾(; , , –), as well as the DFWM power-reflection and power-transmission spectra near to the TPR, are modelled for polar molecules. The effect of enhanced reflectivity of TPR-DFWM is obtained numerically.     

Rate equations in the hopping transport

The usual kinetic equations for the site occupation probabilities in an external field are solved exactly in a simple one-dimensional periodic model with two kinds of atoms using a) free boundary conditions and order of limitsN, 0 needed for a proper treatment of the dc conductivity here b) boundary conditions with metallic contacts and order of limitsN, 0 and c) the same boundary conditions but reversed order of limiting processes 0,N typical of e.g. numerical and percolation treatments. (N and are the number of sites and frequency.) It is demonstrated that though the bulk dc conductivity is the same in all three cases, local bulk properties of the material are strongly dependent on the régime used. The role of the order of all three limiting processes 0,N+ andn+ (N–n+) for local shifts of the chemical potential _n in the dc limit is examined (n is the number of the relevant site calculated from a boundary of the chain). It is shown especially that the rate equation treatment (régime a) on the one hand and numerical or percolation treatments (régime c) on the other hand never yield the same bulk values of _r.     

Excited-state absorption and third-order optical nonlinearities in symmetric π-electron organic molecules

Excited-State Absorption (ESA), Two-Photon Absorption (TPA) and the third-order polarizability (;,, – ) have been investigated for a model dichloride derivative of a symmetrically substituted benzylidene analine (SBAC), using a multielectron configuration-interaction procedure. The calculations indicate that SBAC exhibits ESA across the visible region of the spectrum, but that it is not as extensive as for molecules such as the phthalocyanines. The magnitude of the third-order polarizability is dominated by resonance enhancement from a very strongA _g B _u one-photon absorption. The calculated off-resonance value for (;,, – ) suggests that SBAC is a potential candidate for ultrafast switching applications.     

Calculation of the dispersion of the third-order optical nonlinearity in C60 films

Using wave functions determined from ground-state local-density calculations, we have calculated the wave-dispersed free response of the optical nonlinear polarizability ⁽³⁾(–3;,,), for the C₆₀ molecule and ⁽³⁾(–3;,,) i.e. Third-Harmonic Generation (THG) for films using a sum-over-states approach. The influence of screening was determined by applying an external static electric field in separate selfconsistent calculations to evaluate induced dipole moments which was used to determine the static linear and nonlinear polarizabilities. The polarizabilities calculated in the static limit were used to determine an effective screening parameter which was, in turn, used together with an RPA approach to calculate screened wave-dispersed, third-order nonlinear optical properties such as ⁽³⁾(–3;,,) and ⁽³⁾(–3;,,). Comparing evaluated polarizabilities with experimental values we found that the non-resonant free polarizability compares well in absolute magnitude with experimental results. Inclusion of screening results in a polarizability about two orders of magnitude below the experimental values.Paper presented at the 129th WE-Heraeus-Seminar on Surface Studies by Nonlinear Laser Spectroscopies, Kassel, Germany, May 30 to June 1, 1994     

Flow of an elastico-viscous fluid past an oscillating plate

An exact solution for the flow of an elastico-viscous fluid (Walters' liquid B') due to an oscillating infinite plate has been derived. It has been observed that forgwt=0, ( — frequency,t — time) the flow near the plate may become unstable with increasing whereas fort>0, the velocity increases with increasing. The shearing stress decreases with increasing.I wish to thank the referee for his useful comments which led to the improvement of this paper.     

On the spectrum of Schrödinger operators with a random potential

We investigate the spectrum of Schrödinger operatorsH of the type:H =–+q _i ()f(x–x _i + _i ())(q _i () and _i () independent identically distributed random variables,i ^d ). We establish a strong connection between the spectrum ofH and the spectra of deterministic periodic Schrödinger operators. From this we derive a condition for the existence of forbidden zones in the spectrum ofH . For random one- and three-dimensional Kronig-Penney potentials the spectrum is given explicitly.     

Vacuum ultraviolet 178.7 nm emission in sodium vapour under two-photon resonance excitation

We have observed a fixed wavelength emission at 178.7 nm in sodium vapour under 578.7 nm two-photon resonance excitation. The proposed non-linear wave mixing scheme is described by _{178.7 nm} = 2_L + _{465.7 nm}; where _178.7 is the 178.7 nm photon frequency, _L is the laser-photon frequency, and _465.7 is the 465.7 nm photon frequency. This 465.7 nm emission comes from another six-wave mixing process involving two hyper-electronic Raman scattering photons. The excitation spectrum of the 178.7 nm emission has a typical multiwave mixing pattern with a competing effect appearing at higher temperatures under two-photon resonance excitation. Numerical analysis indicates that this vacuum ultraviolet emission has a poor phase-match condition that will depress the emission intensity to a certain extent. This makes the observation more difficult compared with other reported four-wave mixing generated emissions. Fortunately, on the one hand, it is enhanced by quasi-auto-ionization resonance when the 3s–5s transition is coupled to the sodium continuum by a 330.2 nm photon. On the other hand, its wavelength sits so close to the sodium Cooper minimum that weak absorption will not suppress this vacuum ultraviolet emission further.     

The proper formula for relative entropy and its asymptotics in quantum probability

Umegaki's relative entropyS(,)=TrD (logD –logD ) (of states and with density operatorsD andD , respectively) is shown to be an asymptotic exponent considered from the quantum hypothesis testing viewpoint. It is also proved that some other versions of the relative entropy give rise to the same asymptotics as Umegaki's one. As a byproduct, the inequality TrA logAB TrA(logA+logB) is obtained for positive definite matricesA andB.     

Four-wave mixing in CO via the C 1Σ+ (υ′=0) state

Coherent vacuum ultraviolet (VUV) radiation was generated by four-wave difference frequency mixing (_VUV=2₁–₂) of pulsed dye laser radiation in carbon monoxide (CO). The frequency ₁ was tuned to the C ¹⁺(=0)X ¹⁺(=0) two-photon transition, while the dye laser frequency ₂ was scaned around 17650 cm^–1 which corresponds to the A ¹(=7)«C ¹⁺(=0) transition energy. The VUV intensity was found to be strongly wavelength dependent. The analysis of the spectrum revealed (i) that the VUV intensity was enhanced by the rotational levels of the A ¹(=7) state and (ii) that the off-resonance excitation in the C ¹⁺(=0)X ¹⁺(=0) two-photon transition greatly contributed to the present four-wave mixing process. The effects of pumping laser detuning, saturation and foreign gases are briefly discussed.     

Linear and non-linear ac response of the stochastic classical model for sliding charge density waves

A comprehensive study of the ac response properties of the classical stochastic model for sliding charge density waves (CDW) in quasi one-dimensional metals is made by numerically solving the associated Fokker-Planck equation. Above the conductivity threshold a noise mechanism is indispensable to give finite line widths to the resonances of the applied ac signal of frequency with the narrow band noise frequency _OSC inherent in the model. In the present investigation a current noise of strengthT _N proportional to the CDW current is used in the Fokker-Planck equation in order to model the broad band current noise frequently observed above threshold. The present model thus incorporates three characteristic frequency scales: _OSC,T _N ,and a crossover frequency _OSC. Results are evaluated for the ac conductivity (;E ₀,E ) as function of frequency , dc bias electric fieldE ₀ and ac signal field strengthE . ForE 0 the linear ac response is obtained by a separate treatment of the Fokker-Planck equation. The resonances near =_OSC are studied in detail. Strong ac signals reduce the response at the fundamental resonance and lead to a harmonic interference structure nearn=_OSC. The overall agreement of the present results with recent measurements of the linear ac response is not good. In reality our results seem to be superimposed on a background not reproduced by the classical model with one cross over frequency. However, the peak in Im (;E ₀,E =0) vs.E ₀, when the narrow band noise frequency is near , is well reproduced. The spectral width of this peak which corresponds to the inductive dip in the susceptibility is studied as function of current noise strengthT _N .The results stress the need for a complete Fokker-Planck treatment sinceT _N is not simply related to the line width.     

Generation of more than 40 laser emission lines from the ultraviolet to the visible regions by two-color stimulated raman effect

An intense and monochromatic laser beam consisting of more than 40 vibrational and rotational lines is generated by the stimulated Raman effect, when two-color laser beams separated by 590 cm^–1 are tightly focused into pressurized hydrogen. This phenomenon is reasonably explained by four-wave mixing; one beam is used for two-step excitation (₁+₁) to an imaginary level and another beam (₂) acts as a seed beam, generating a fourth beam (2₁–₂). Through cascade processes, so many laser emissions appear with a frequency difference of (₁–₂) in entire ultraviolet and visible regions.