Generation of picoseconds stimulated Raman scattering in a BaWO4 crystal and frequency up-conversion by difference-frequency generation in BBO

The characters of stimulated Raman scattering of BaWO₄ crystal excited by a picoseconds laser at 1064 nm are studied based on optical parametric amplification (OPA). Up to six-order Stokes components and five-order anti-Stokes components are observed. The SRS components are amplified by an OPA and the wavelength tunable range from 411 to 2594 nm is achieved with a maximum conversion efficiency of 38% using the OPA stage.     

Tunable diode laser spectroscopy of benzene near 1684 nm with a low-temperature VCSEL

We describe the application of a long-wavelength vertical-cavity surface-emitting laser (VCSEL) with extended tuning range to the detection of benzene vapor at atmospheric pressure. A benzene absorption feature centered at 1684.24 nm was accessed by reducing the heat sink temperature of a VCSEL designed for room-temperature operation to −55°C. This allowed us to increase the injection current and thus to extend a single-scan tuning interval up to 46.4 cm⁻¹ or 13.2 nm around a central wavelength of 1687.4 nm. Five absorption lines of methane in the 5903–5950 cm⁻¹ range could be acquired within single laser scans at a repetition rate of 500 Hz. A benzene absorption feature between 5926 and 5948 cm⁻¹ was recorded for concentration measurements at atmospheric pressure using a single-pass 1.2 m absorption cell. A 50 ppmv mixture of CH₄ in N₂ was introduced into the cell along with benzene vapor to calibrate benzene concentration measurements. Benzene mixing ratios down to ∼90 ppmv were measured using a direct absorption technique. The minimum detectable absorbance and detection limit of benzene were estimated to be ∼10⁻⁴ and 30 ppmv, respectively. Using the wavelength modulation technique, we measured a second harmonic sensor response to benzene vapor absorption in air at atmospheric pressure as a function of modulation index. We conclude that a low-temperature monolithic VCSEL operating near 1684 nm can be employed in compact benzene sensors with a detection limit in the sub-ppm range.     

Generation of 100 μJ pulses at 82.8 nm by frequency tripling of sub-picosecond KrF laser radiation

. Investigations of the efficient generation of powerful coherent radiation at 82.8 nm by frequency tripling of short-pulse KrF laser radiation are presented. Argon gas is selected as nonlinear medium due to the resonantly enhanced 3rd-order susceptibility χ⁽³⁾(-3ω,ω,ω,ω). Pulse energies of 100 μJ at 82.8 nm have been measured for a pump pulse energy of 14 mJ. An upscaling to more than 500 μJ is expected with available more powerful pump lasers. Features of this XUV source and possible applications are discussed. Received: 26 July 2002 / Published online: 15 November 2002 RID="*" ID="*"Corresponding author. Fax: +49-511/7622211, E-mail: reinhardt@iqo.uni-hannover.de     

Ultrashort-pulse laser irradiation of metal films: the effect of a double-peak laser pulse

The optical properties of blue-violet InGaN light-emitting diodes under normal and reversed polarizations are numerically studied. The best light-emitting performance under normal and reversed polarization is obtained in a single quantum-well structure and double quantum-well structure, respectively. The key factors responsible for these phenomena are presumably the carrier concentration distribution and the amount of carriers in quantum wells. The turn-on voltage of light-emitting diodes under reversed polarization is lower than that of light-emitting diodes under normal polarization, due mainly to lower potential heights for electrons and holes in the active region.     

Absolute frequency measurement of the iodine-stabilized He-Ne laser at 633 nm

The absolute frequency of an iodine-stabilized He-Ne laser at 633 nm stabilized on the i (or a₁₃) component of the 11-5 R(127) hyperfine transition of the ¹²⁷I₂ molecule is measured using a femtosecond optical comb generator and an iodine-stabilized Nd:YAG laser standard at 1064 nm. We link the measured absolute frequency to the current internationally adopted value via frequency intercomparison between JILA and the Bureau International des Poids et Mesures (BIPM), leading to the determination of the absolute frequency of the BIPM-4 standard laser. The resulting absolute frequency f_i(BIPM) of the BIPM-4 standard laser is f_i(BIPM)=473612214711.9±2.0 kHz, which is 6.9 kHz higher than the value adopted by the Comité International des Poids et Mesures (CIPM) in 1997. Received: 29 May 2000 / Revised version: 13 September 2000 / Published online: 22 November 2000     

Raman spectroscopic differentiation of beef and horse meat using a 671 nm microsystem diode laser

A non-invasive Raman spectroscopic approach for meat species identification and quality detection was successfully demonstrated for the two closely related species beef and horse. Fresh beef and horse muscles were cut and ice-stored at 5 °C, and time-dependent Raman measurements were performed daily up to 12 days postmortem. Applying a 671 nm microsystem diode laser and a laser power of 50 mW, spectra were recorded with integration times of 1–4 s. A pronounced offset of the Raman spectra was observed between horse and beef, with high fluorescence background for horse compared to beef for all days of storage. Principal components analysis was applied for data evaluation revealing a clear distinction between beef and horse meat which can be attributed to differences in the myoglobin content of both species. Furthermore, separations according to aging and spoilage for the two species could be identified simultaneously. Therefore, Raman spectroscopy might be an efficient test method for meat species identification in combination with spoilage detection.     

Numerical study of the expansion of metallic vapor plasma by a nanosecond laser pulse

The interaction between a laser-produced aluminum plasma and the ambient air, at a pressure of 173.3 Pa, is studied at the plasma thermalization stage. A two-dimensional approach is developed to solve the Navier–Stokes equations, where a finite volume discretization allows for obtaining a numerical solution. The simulation runs over a time representing 10 μs of plasma expansion. It is shown that the shock and drag models are good approximations for the two successive regimes after the initial strong expansion stage, and the calculation makes evident the plume sharpening on the axial direction before its confinement by the ambient gas, which is in good agreement with the experimental observation.     

Influence of Z-pinch evolution on laser pulse duration at 46.9 nm in Ne-like Ar ions

A capillary discharge 46.9 nm Ne-like Ar laser is achieved with peak current of 20–23 kA. The variation of laser pulse duration with initial Ar pressure and rise-time of main current is reported. Measurements show that the laser pulse durations slightly increase with the increased pressure and increased rise-time of current. A comparison of the experimental results with the calculation of snow-plow model indicates that the increase of laser pulse duration is the result of decreased Z-pinch velocity at the pinch time when the radius of plasma is minimal.     

Study of characteristics of ultrasound pulse generated by a laser pulse

I.IntroductionThegenerationofacousticpulsebylaserirradiationofametalsurfacewasfirstsuggestcdbyWhitein1963[1l.SincethatdateLaserU1trasoundtechniquchasbeendcvclopedrapidly.Becausethistechniquehasanumberoftechnicalfcatures,suchasnon-contact,highbandwidth,highhme-spacia1resolution,quantitativeteshng,generationoflongitudinal,shcarandRay1cighwaves(simu1taniously),andsoon,ithasbccnwidelyapp1icdtomcasurementsofmatcrialproperties,detectionofdefects,andcalibrationoftransd.ccrsl'-'o].Inordertodcve1opth…     

Q-switched operation of an in-band-pumped Ho:LuAG laser with kilohertz pulse repetition frequency

We report continuous-wave (CW) and repetitively Q-switched operation of an in-band-pumped Ho:LuAG laser at room temperature. End-pumped by a Tm:YLF solid-state laser with emission wavelength of 1.91 μm, the CW Ho:LuAG laser generated 5.4-W output at 2100.7 nm with beam quality factor of M ²～1.03 for an incident pump power of 14.1 W, corresponding to slope efficiency of 67% with respect to absorbed pump power. Up to 1.5-mJ energy per pulse at pulse repetition frequency (PRF) of 3 kHz and 4.5-W average power with FWHM pulse width of 28 ns at 5 kHz were demonstrated in repetitively Q-switched operation.     

Generation of 7-fs laser pulse directly from a compact Ti:sapphire laser with chirped mirrors

A compact femtosecond Ti:sapphire laser resonator consisting of three chirped mirrors and one output coupler was designed. By accurately balancing the intra- cavity dispersions between Ti:sapphire crystal, air and chirped mirrors, we directly generated the laser pulse shorter than 7 fs at the average power of 340 mW with 3.1 W pump. The repetition rate of the laser oscillator is 173 MHz at the centre wavelength of 791 nm, and the ultrabroaden spectrum covers from 600 nm to 1000 nm. To the best of our knowledge, this is the simplest laser resonator capable of generating sub-10 fs laser pulse.     

Frequency shifting of sub-100 fs laser pulses by stimulated Raman scattering in a capillary filled with pressurized gas

The technique of Raman conversion of sub-100 fs laser pulses based on excitation of active medium by two orthogonally polarized pulses has been developed for Raman lasers with a glass capillary. 52 fs Stokes pulse at the wavelength of 1200 nm has been generated by stimulated Raman scattering of 48 fs Ti:sapphire laser pulse at the wavelength of 800 nm in hydrogen. 13% energy conversion efficiency has been achieved at pulse repetition rate up to 2 kHz.     

Generation and measurement of complex laser pulse shapes in the SG-Ⅲ laser facility

The generation and measurement of complex ultraviolet laser pulse shapes is demonstrated in the SG-III laser facility. Relatively high contrast ratio of 300∶1 required by the physics experiment is achieved and successfully measured. Two continuous main shots validate the reproduction and the stability of the pulse shape, which provide solid foundation for precise physics experiment and laser power balance.     

High-efficiency eye-safe intracavity Raman laser at 1531 nm with SrWO4 crystal

A high-efficiency diode-end-pumped Q-switched eye-safe linearly-polarized intracavity Raman laser at 1531 nm is demonstrated, with Nd:YVO₄ as the laser medium and SrWO₄ as the Raman crystal. The highest average power of 1.93 W is achieved, with an incident pump of 15.6 W and a repetition rate of 35 kHz. The narrowest pulse duration of 4.9 ns and the highest peak power of 32.2 kW are obtained at a repetition rate of 5 kHz.     

Generation of cavity-birefringence-dependent multi-wavelength bright–dark pulse pair in a figure-eight thulium-doped fiber laser

We experimentally demonstrated a stable multi-wavelength bright–dark pulse pair in a mode-locked thulium-doped fiber laser(TDFL). The nonlinear polarization rotation(NPR) and nonlinear optical loop mirror(NOLM) were employed in a figure-eight cavity to allow for multi-wavelength mode-locking operation. By incorporating different lengths of high birefringence polarization-maintaining fiber(PMF), the fiber laser could operate stably in a multi-wavelength emission state. Compared with the absence of the PMF, the birefringence effect caused by PMF resulted in rich multi-wavelength optical spectra and better intensity symmetry and stability of the bright–dark pulse pair.     

Generation of an ultrashort optical pulse by four-wave Raman mixing in deuterium cooled at 77 K

When a 100-fs Ti:sapphire laser is focused into molecular deuterium cooled at 77 K, rotational stimulated Raman emission is generated based on four-wave Raman mixing. By phase locking the emission lines, the laser pulsewidth was reduced to 40 fs, when a nearly transform-limited pulse was utilized as a fundamental laser. The pulsewidth was further reduced to 20 fs, when a positively chirped pulse was employed. Computer simulation suggests that the Raman emission is strongly chirped and a train of pulses with lower intensities are formed when a chirp pulse is used as a fundamental laser. PACS 42.65.Dr; 42.55.Ye; 42.50-p     

Absolute frequency measurements of wavelength standards 532 nm, 543 nm, 633 nm and 1540 nm

This paper describes the results of absolute frequency measurements of primary wavelength standards 633 nm, 543 nm, 532 nm, (iodine stabilized) and 1540 nm (acetylene stabilized) in CMI. The values obtained with Menlo Systems femtosecond frequency comb in CMI are compared with previous measurements of the same standards in BIPM, BEV and MPQ. Measured sub-Doppler linewidths and relative intensities of several hyperfine spectral components of iodine molecule are also presented.     

465 nm laser sources by intracavity frequency doubling using a 49-edge-emitters laser bar

A compact blue laser was generated by intracavity frequency doubling based on quasi-phase-matched second-harmonic generation (SHG) in a MgO-doped periodically poled lithium niobate bulk crystal. A 49 single-transverse-mode edge-emitters laser bar with antireflective coating was used as a pump source. An optical output power of 1.2?W SHG of blue lights at 465?nm is generated at 45?A injection current, equivalent to an overall wall-plug efficiency of 1.33%.