Nonlocal theory of stimulated Raman backscattering in a strongly magnetized plasma

A nonlocal theory of stimulated Raman backscattering (BSRS) parametric instability of a large amplitude electromagnetic (EM) mode in a strongly magnetized plasma e.g., one encountered in a plasma filled backward wave oscillator, is reported. The EM mode is unstable to parametric instability in a magnetized plasma and decays into a Trivelpiece-Gould (TG) mode and a sideband EM mode. The growth rate of instability (Γ) scales proportional to three-fourth power of plasma density. For a typical BWO the growth rate is ∼10⁸ s^-1     

Increase of the backward Raman reflectivity caused by the langmuir decay instability in an inhomogeneous plasma: the loss of gradient stabilization

We investigate the nonlinear evolution of the backward stimulated Raman scattering (BSRS) in the regime where the nonlinear saturation mechanism is the Langmuir decay instability resulting from the coupling of the BSRS-generated Langmuir wave with the ion acoustic waves. We present numerical results obtained with a fluid-type code in one- and two-dimensional spatial dimensions, in the case of an inhomogeneous plasma. The plasma density is under quarter-critical and depends linearly on the longitudinal spatial coordinate, in the regime where the Rosenbluth gain factor for the amplitude, denoted as G(Ros), is in the range pi/2< or =G_(Ros)< or =6. We observe that the Langmuir decay instability is able to suppress the gradient stabilization and restore the absolute nature of BSRS, thus leading to a significantly increased BSRS reflectivity.     

Effect of a fluorescing impurity on the characteristics of stimulated Raman scattering from acetone

Asymmetry in the intensities between backward and forward stimulated Raman scattered radiations (BSRS and FSRS respectively) in acetone is investigated in the presence of a fluorescing impurity (rhodamine 6G). In the case of pure acetone above a threshold pump power, BSRS becomes more intense than FSRS. On the other hand intensity of BSRS decreases with concentration of the fluorophore in solution, while that of FSRS is found to increase. It is observed that absorption saturation also affects the asymmetry between FSRS and BSRS.     

Stimulated Raman adiabatic passage via the ionization continuum in helium: Experiment and theory

We experimentally demonstrate coherent population transfer, driven by stimulated Raman adiabatic passage (STIRAP) between two bound quantum states, coupled via a continuum of states. We present extended numerical and experimental investigations on population transfer from the metastable state 2s ¹S₀ to the excited state 4s ¹S₀ in metastable helium atoms. While techniques based on incoherent excitation do not permit any population transfer via rapidly decaying continuum states, our data indicate a maximum transfer efficiency of 20% in coherent excitation by STIRAP. We study the transfer efficiency with respect to the relevant experimental parameters.     

探测大气中CO2的Raman激光雷达

基于大气激光后向散射光谱，研究和设计了探测大气CO₂浓度的Raman激光雷达,其发射机采用Nd∶YAG激光的三倍频354.7nm作为工作波长,发射的单脉冲能量350mJ,重复频率20Hz；接收机采用了光电倍增管(量子效率25%)和光子计数器(计数速率200MHz),探测CO₂的Raman散射371.66nm(频移1285cm^-1)信号,(1小时累加)近地面2.5km以内信噪比不小于8.采用组合滤光片来抑制强的354.7nm Mie-Rayleigh后向散射和氧气375.4nm Raman后向散射对信号的严重干扰. 比较分别来自大气CO₂和参考气体N₂的Raman后向散射回波,可反演出大气中CO₂的相对浓度. 关键词： 大气光学 激光雷达 Raman散射光谱 参考气体 Mie-Rayleigh散射     

Measurement of the gravitational acceleration of an atom with a light-pulse atom interferometer

Velocity sensitive stimulated Raman transitions have been used to measure the gravitational acceleration, g, of laser cooled sodium atoms in an atomic fountain geometry. By using an improved scheme to drive the Raman transitions, we have demonstrated a resolution of 3×10^–8 g after 2×10³ seconds of integration time. In addition to presenting recent experimental results, we review the theory of stimulated Raman transitions as it applies to atom interferometers and discuss the prospects of an atom interferometer-based gravimeter with better than 10^–10 g absolute accuracy.     

Diagnostics of skin pathologies based on spectral analysis of backward and raman scattering

A mathematical model of the interaction of optical radiation with skin tissues is developed taking into account stimulated Raman scattering. Numerical experiments show that the backscattering spectra possess specific features typical of skin pathologies. It is shown that the pathology type can be determined from an analysis of the differential ratios of the Raman scattering intensities at 1271 and 1663 cm^?1 to the intensity in the region of 1454 cm^?1. It is found that the difference in the differential ratios of the Raman scattering intensities for pathologically changed and normal layers may exceed 40%.     

Transient enhancement and detuning of laser-driven parametric instabilities by particle trapping

Kinetic simulations of backward stimulated Raman scattering (BSRS), where the Langmuir wave coherence time is greater than the bounce time for trapped electrons, yield transient reflectivity levels far above those predicted by fluidlike models. Electron trapping reduces the Langmuir wave damping and lowers the Langmuir wave frequency, and leads to a secular phase shift between the Langmuir wave and the BSRS beat ponderomotive force. This phase shift detunes and saturates BSRS and a similar effect, due to ion trapping, is the saturation mechanism for backward stimulated Brillouin scattering. Competition with forward SRS is discussed.     

Small-stokes-shift frequency conversion in single-mode birefringent fibers

We report experimental observation of nondegenerate four-photon mixing (FPM) via a new phase-matched process in birefringent fibers. This phase-matching process is characterized by relatively long coherence lengths, and by small pump-to-Stokes frequency shifts (of the order of 100 cm^-1 in high birefringence fibers) that are directly proportional to the fiber birefringence. Pump-to-Stokes energy conversion efficiencies of over 40 percent have been obtained with moderate pump powers (≈1 kW) from a visible cw mode-locked dye laser coupled into single-mode polarization-preserving high-birefringence fibers of a few meters length. In addition, we report the first observation of a totally non-degenerate phase-matched four-photon process in a fiber; this invokes mixing of the original FPM Stokes component with the pump and stimulated Raman radiation.     

Temperature measurements in condensed phases using non‐resonant femtosecond stimulated Raman scattering

We have previously demonstrated the capability of femtosecond stimulated Raman scattering (FSRS) data to measure the temperature (T) of condensed matter at the molecular vibrational level. [Phys. Rev. Lett. 2011, 107, 43001] In this paper, we expand the theory for the FSRS temperature dependence by considering the effects of an isolated change of T as well as a coupled change of T and chemical concentration. We point out that the origin of the temperature sensitivity of the Stokes to anti‐Stokes ratio of FSRS lies in the exponential nonlinearity of the gain and loss. We establish that FSRS of two Raman modes can be used to simultaneously determine the vibrational temperature and the change in concentration of the species contributing to those two modes. Single‐shot experimental results using FSRS are presented to demonstrate over four orders of magnitude higher efficiency than spontaneous Raman in small volume samples with picosecond resolution. Copyright © 2012 John Wiley & Sons, Ltd.     

Redshifts in space caused by stimulated Raman scattering in cold intergalactic Rydberg matter with experimental verification

The quantized redshifts observed from galaxies in the local supercluster have recently been shown to be well described by stimulated Stokes Raman processes in intergalactic Rydberg matter (RM). The size of the quanta corresponds to transitions in the planar clusters forming the RM, of the order of 6 × 10^?6 cm^?1. A stimulated Stokes Raman process gives redshifts that are independent of the wavelength of the radiation, and it allows the radiation to proceed without deflection, in agreement with observation. Such redshifts must also be additive during the passage through space. Rydberg matter is common in space and explains the observed Faraday rotation in intergalactic space and the spectroscopic signatures called unidentified infrared bands (UIBs) and diffuse interstellar bands (DIBs). Rydberg matter was also recently proposed to be baryonic dark matter. Experiments now show directly that IR light is redshifted by a Stokes stimulated Raman process in cold RM. Shifts of 0.02 cm^?1 are regularly observed. It is shown by detailed calculations based on the experimental results that the redshifts due to Stokes scattering are of at least the same magnitude as observations.     

Origin of the Raman mode at 379 cm−1 observed in ZnO thin films grown on sapphire

In this work, we present a detailed Raman scattering study to clarify the origin of the mode at 379 cm⁻¹ which is observed in Raman spectra of the ZnO films grown on c‐sapphire substrates and generally attributed to the A₁‐transverse optical (A₁‐TO) mode of ZnO. The studied ZnO films were deposited by metal‐organic chemical vapor deposition on c‐sapphire and (0001) ZnO substrates. In the z(−,−)z̄ backscattering configuration, the A₁‐TO mode is forbidden, while the 379 cm⁻¹ peak is still observed in the as‐deposited film grown on sapphire substrate. However, this mode is not observed in Raman spectra of the as deposited film grown on ZnO substrate. We suggest that the peak at 379 cm⁻¹ is the E_1g mode of the sapphire substrate which is allowed in z(−,−)z̄ backscattering configuration. The effects of annealing, the substrate and the collection cross‐section on Raman active modes were analyzed. Copyright © 2011 John Wiley & Sons, Ltd.     

Nonlinear spectral signatures and spatiotemporal behavior of stimulated Raman scattering from single laser speckles

Simulations are reported of the Thomson scatter spectrum of electrostatic waves (ESWs) excited in single laser hot spots by backward stimulated Raman scattering (BSRS). Under conditions similar those in the recent experiments of Kline et al. [Phys. Rev. Lett. 94, 175003 (2005)], a spectral streak, resulting from the trapping-induced frequency shift of the ESW, is found for high wave-number ESWs, similar to the observations. This shift and parametric frequency matching lead to isolated BSRS pulses. Modes with acoustic dispersion, resulting from the trapping-modified electron velocity distribution, can enhance the frequency range of the streak.     

Observation of stimulated raman scattering in CVD-diamond

We report the first experimental observation of a nonlinear laser effect, stimulated Raman scattering (SRS), in manmade diamond grown from the gaseous phase by the chemical vapor deposition (CVD) technique. Multiple Stokes and anti-Stokes generation in the visible and near-IR ranges was excited under nanosecond and picosecond pumping in a 350-μ-thick plate. All the registered Raman-induced lasing wavelengths were identified. We classify the CVD-diamond as a promising χ⁽³⁾-active material for Raman laser converters in a record wide spectral range.     

分子间费米共振增强二元溶液体系的受激拉曼散射研究

研究了液芯光纤内不同体积比的甲苯和间二甲苯二元混合溶液的受激拉曼散射.实验结果表明:在不同的体积比之下二元溶液的环呼吸振动模式1002 cm^-1,甲基的CH伸缩振动模式2920 cm^-1 以及芳香环CH对称伸缩振动模式3058 cm^-1的拉曼带同时产生受激拉曼辐射,并且2920 cm^-1 和 3058 cm^-1 拉曼带的一阶受激拉曼散射阈值要低于1002 cm^-1拉曼带的二阶 关键词： 分子间费米共振 二元溶液 受激拉曼散射 拉曼散射截面     

New far infrared laser lines in optically pumped CD3F

Summary Using a high pressure CO₂-laser we have studied laser action in¹²CD₃F stimulated by R-branch pumping. We used an arrangement with low-feedback mirrors as suitable for Raman laser action. However, no Raman laser action has been observed in¹²CD₃F though similar experimental conditions were met as for¹²CH₃F and¹³CH₃F. The reason for the different behavior of the gases is not yet clear.Instead of Raman laser action we found 15 FIR resonant laser lines with 13 of them unknown up to now in the frequency range from 50 cm^–1 to 68 cm^–1. We reached FIR pulse energies up to 900 J, corresponding to a photon conversion efficiency of 12%. For our arrangement the optimum operation pressure varied from 40 torr at low J values (J=36) to 70 torr at high J values (J=49).     

氧离子辐照二氧化钛单晶后的结构与磁性

氧离子辐照二氧化钛单晶可以诱发其铁磁性．辐照后在室温下也能观察到二氧化钛的铁磁性,且对温度依赖性较小．结合X射线衍射实验、卢瑟福背散射/沟道实验、拉曼散射实验谱、电子自旋共振实验谱、超导量子干涉仪实验、单位原子随沟道位移实验,测定了晶格的损伤随辐照流强的增加而增加．发现在氧离子辐照二氧化钛时出现了Ti³⁺替代氧空位(O_V)的缺陷复合体,即形成Ti³⁺-OV复合体．这种缺陷复合体导致了局部(TiO_6-x)的拉曼模式的伸展．说明了Ti³⁺结合一个未成对的3d电子是二氧化钛局部铁磁性的起源.     

光纤维中的喇曼混频

我们在656厘米^-1到1343厘米^-1的频率范围研究了光纤维的调谐喇曼混频(RM)效应。在实验中观察到下列现象:相干反斯托克斯喇曼散射(CARS)的大小与逆喇曼吸收(VRA)的大小成反比;RM对受激喇曼散射(SRS)的强度分布有强烈影响。除了观测到相干斯托克斯(CSRS)和CARS辐射,还观测到二级相干斯托克斯(SOCSRS)和相干反斯托克斯(SOCARS)辐射。对实验结果进行了讨论。 关键词：     

Cooperative and quantum phenomena in experiments involved in the study of ordinary and stimulated Raman scattering of light

Results are presented of experimental studies of Raman scattering (RS) of light and of stimulated Raman scattering (SRS) of light, in which the quantum and cooperative properties of these phenomena are manifested. Experiments are described, revealing for the first time ever the connection between the integral intensity of the RS and SRS spectra and Brownian motion of molecules in condensed media. A number of experimental properties of RS and SRS are interpreted as results of collective behavior of molecules in condensed media. Spatial energy quantization of SRS energy is observed for the first time following excitation by 10^–9- and 10^-12-sec pulses. The experimental results are discussed in the Conclusion in light of the existing theoretical premises. New properties of RS and SRS are demonstrated and an explanation of their physical nature is proposed.Optics Division, lebedev Physics Institute. Translated from Preprint No. 103, Lebedev Physics Institute, Academy of Sciences of the USSR, Moscow, 1991.     

Raman study of InAs/GaAs quantum dot solar cells

We report polarized and resonant Raman study of InAs/GaAs quantum dot solar cell (QDSC) structures. Raman spectra obtained from the top surfaces of the samples suggested that the formation of InAs QDs induced tensile strain in the overgrown GaAs layers. Furthermore, a longitudinal optical phonon-plasmon (LPP) coupled modes were observed in the p-type GaAs layers. The tensile strain was increased with an increase in the QD size. The hole concentrations estimated by fitting the individual LPP coupled modes were in the range of 2.4–3.5 × 10¹⁸ cm^?3. Resonant Raman spectra obtained from the cleaved sides, where the QDs were located, showed a 225 cm^?1 mode in parallel polarization configurations. Based on accurate analysis, this mode was identified as the LA(X) phonon of GaAs.