Simultaneous generation of ultrashort pulses at 158 and 198?nm in a single filamentation cell by cascaded four-wave mixing in Ar

Ultrashort 198- and 158-nm pulses are generated simultaneously by cascaded four-wave mixing of the second and third harmonics of a 80-fs Ti:Sapphire laser in filamentation propagation through a single Ar gas cell. The energies of the 198- and 158-nm pulses are 7.6?μJ and 600?nJ, respectively. The duration of 198-nm pulse is determined to be ca. 45?fs by transient-grating frequency-resolved optical grating, which indicates that the pulse is intrinsically transform limited and chirped by the rear window of the gas cell. The spectral bandwidths of 198- and 158?nm support the transform limited pulse durations of 40 and 28?fs, respectively.     

Enhanced four-wave mixing in a hollow-core photonic-crystal fiber

Hollow-core photonic-crystal fibers are shown to substantially enhance four-wave mixing (FWM) of laser pulses in a gas filling the fiber core. Picosecond pulses of Nd:YAG fundamental radiation and its second harmonic are used to generate a signal at the frequency of the third harmonic by the FWM process 3omega = 2omega + 2omega - omega. The efficiency achieved for this process in a 9-cm-long, 13-microm-hollow-core-diameter photonic-crystal fiber, designed to simultaneously transmit a two-color pump and the FWM signal, is shown to be approximately 800 times higher than the maximum FWM efficiency attainable with the same laser pulses in the tight-focusing regime.     

Generation of tunable octave-spanning mid-infrared pulses by filamentation in gas media

The continued development of femtosecond mid-infrared (IR) sources with ultrabroad spectral width is critical for probing and controlling complex molecular structural dynamics on an ultrafast timescale. We report on a sub-20 fs, coherent mid-IR source with an octave-spanning spectral bandwidth (>2000 cm(-1)) tunable from 2-8 micrometers (37.5-150 THz), with energy >0.4 μJ/pulse at 1 kHz. The mid-IR pulses are generated by four-wave mixing during the filamentation of intense 800 nm and 400 nm pulses in various gas media. Spectral tunability is achieved by the choice of gas, pressure and input 800 nm pulse energy.     

Hollow-fiber compression of visible, 200 fs laser pulses to 40 fs pulse duration

We demonstrate the use of a very simple, compact, and versatile method, based on the hollow-fiber compression technique, to shorten the temporal length of visible laser pulses of 100-300 fs to pulse durations shorter than approximately 50 fs. In particular, 200 fs, frequency-doubled, Nd:glass laser pulses (527 nm) were spectrally broadened to final bandwidths as large as 25 nm by nonlinear propagation through an Ar-filled hollow fiber. A compact, dispersive, prism-pair compressor was then used to produce as short as 40 fs, 150 microJ pulses. A very satisfactory agreement between numerical simulations and measurements is found.     

Generation of femtosecond vacuum-ultraviolet pulses

High power femtosecond pulses in the Vacuum Ultra Violet (VUV) have been generated through the nonlinear interaction of femtosecond KrF pulses with xenon and argon gas. Under near resonant two photon excitation of xenon by a femtosecond KrF laser, parametric four wave mixing processes lead to VUV pulses at 147 and 108 nm with pulse energies in the 10 µJ range. Tuning is demonstrated by mixing the KrF pulse with a 500 fs dye laser pulse at 497 nm, resulting in 165 nm emission. In argon, a three photon resonance leads to third harmonic generation at 83 nm and micro joule level pulses near 127 nm generated by a six wave mixing process. Since the spectra of the VUV pulses show an ionization-induced blue shift with increasing KrF laser intensity, the VUV pulses can be shown to have temporal duration less than the pulse width (450 fs) of the KrF laser. Blue shifting of the third harmonic of the KrF laser in argon is dominated by a reduction in the neutral gas density rather than by an increase in the electron density.     

Tunable Supercontinuum Generated in a Yb~(3+)-Doped Microstructure Fiber Pumped by Ti:Sapphire Femtosecond Laser

We experimentally demonstrate that a tunable supercontinuum(SC) can be generated in a Yb3+-doped microstructure fiber by the concept of wavelength conversion with a Ti:sapphire femtosecond(fs) laser as the pump.Experimental results show that an emission light around 1040 nm in an anomalous dispersion region is first generated and amplified by fs pulses in the normal dispersion region. Then, SC spectra from 1100 to 1380 nm and 630 to 840 nm can be achieved by combined effects of higher-order soliton fission and Raman soliton self-frequency shift in the anomalous dispersion region and self-phase modulation, dispersive wave, and four-wave mixing in the normal dispersion region. It is also demonstrated that the 20 nm change of pump results in a 280 nm broadband shift of soliton and the further red-shift of soliton is limited by OH-absorption at 1380 nm.     

Bandwidth scaling and spectral flatness enhancement of optical frequency combs from phase-modulated continuous-wave lasers using cascaded four-wave mixing

We introduce a new cascaded four-wave mixing technique that scales up the bandwidth of frequency combs generated by phase modulation of a continuous-wave (CW) laser while simultaneously enhancing the spectral flatness. As a result, we demonstrate a 10?GHz frequency comb with over 100?lines in a 10?dB bandwidth in which a record 75?lines are within a flatness of 1?dB. The cascaded four-wave mixing process increases the bandwidth of the initial comb generated by the modulation of a CW laser by a factor of five. The broadband comb has approximately quadratic spectral phase, which is compensated upon propagation in single-mode fiber, resulting in a 10?GHz train of 940?fs pulses.     

Four-wave mixing in hollow photonic-crystal fibers

A radical enhancement of four-wave mixing in hollow-core photonic-crystal fibers is experimentally demonstrated. An enhancement ratio of about 800 relative to the regime of tight focusing is achieved for the four-wave mixing process 3ω=2ω+2ω?2ω, where ω and 2ω are the frequencies of fundamental radiation and the second harmonic of picosecond Nd:YAG laser pulses.     

孤子光脉冲的产生及其应用研究

利用非线性偏振旋转技术实现自起振被动锁模.在掺铒光纤环形腔激光器中产生了中心波长为1563.3 nm、重复频率为12.5 MHz、脉冲宽度为352.0 fs、3 dB光谱宽度为7.8 nm的孤子光脉冲.采用该孤子光脉冲作为抽运光源，经掺铒光纤放大器放大后，输入到101 m长的高非线性光子晶体光纤中，获得了20 dB带宽约为240 nm的超连续激光光谱.实验详细观测了光脉冲随抽运功率的变化及超连续激光光谱的形成过程，分析了其形成机理.研究表明：当抽运功率较低时，光谱加宽主要由高阶孤子的分裂引起；随着抽运功率的增加，高阶孤子分裂成基本孤子的数目逐渐增大，光谱进一步加宽；当抽运功率增加到受激拉曼散射的阈值时，受激拉曼散射成为光谱展宽的主要原因；抽运功率进一步增加时，受激拉曼散射、参量四波混频等非线性的共同作用将使光谱进一步加宽且变得光滑. 关键词： 孤子光纤激光器 超连续 光子晶体光纤     

Generation of high-energy broadband femtosecond deep-ultraviolet pulses by highly nondegenerate noncollinear four-wave mixing in a thin transparent solid

We present a simple and efficient technique for the generation of ultrashort deep-ultraviolet pulses based on four-wave mixing of noncollinear laser pulses in a thin solid. Sub-30-fs pulses (Fourier-limit of 13 fs) centered at 270 nm, with energies up to 6 μJ, were obtained by mixing the fundamental and the second harmonic of a Ti:sapphire amplifier in fused silica. Temporal characterization was performed with a dispersionless self-diffraction FROG setup. Spectra as broad as 20 nm were also obtained that can in principle support sub-4-fs deep-ultraviolet pulses.The results are well described by two-dimensional numerical simulations.     

Generation of 11 fs pulses by using hollow-core gas-filled fibers at a 100 kHz repetition rate

Using self-phase modulation in a hollow-core fiber filled with xenon, we were able to produce 2.3 microJ laser pulses with a duration of 10.9 fs at a repetition rate of up to 100 kHz. We started with 45 fs, 4.4 microJ, 800 nm pulses generated by a Coherent RegA Ti:sapphire regenerative amplifier system, then spectrally broadened the 30 nm bandwidth to more than 100 nm. Dispersion compensation was achieved with two pairs of chirped mirrors. This is believed to be the first time this type of compression was achieved at a repetition rate as high as 100 kHz. This brings the advantages of few-cycle laser pulses to experiments that require high-repetition-rate, low-energy laser systems, for example, coincidence experiments.     

Femtosecond optical parametric converter in the 168–182-nm range

Femtosecond pulses continuously tunable in the vacuum ultraviolet (VUV) spectral range between 168 and 182 nm were generated using four-wave frequency mixing in an argon-filled capillary. The pulse energy reached 200 nJ at a pump-to-VUV conversion efficiency of 1%. The bandwidth at 181 nm was up to 27 THz corresponding to a transform limited duration of 17 fs. The upper limit in the shortest measured pulse duration was 75 fs.     

Intense self-compressed, self-phase-stabilized few-cycle pulses at 2 microm from an optical filament

We report the compression of intense, carrier-envelope phase stable mid-IR pulses down to few-cycle duration using an optical filament. A filament in xenon gas is formed by using self-phase stabilized 330 microJ 55 fs pulses at 2 microm produced via difference-frequency generation in a Ti:sapphire-pumped optical parametric amplifier. The ultrabroadband 2 microm carrier-wavelength output is self-compressed below 3 optical cycles and has a 270 microJ pulse energy. The self-locked phase offset of the 2 microm difference-frequency field is preserved after filamentation. This is to our knowledge the first experimental realization of pulse compression in optical filaments at mid-IR wavelengths (lambda>0.8 microm).     

Parametric amplification of few-cycle carrier-envelope phase-stable pulses at 2.1 microm

We demonstrate an optical parametric chirped-pulse amplifier producing infrared 20 fs (3-optical-cycle) pulses with a stable carrier-envelope phase. The amplifier is seeded with self-phase-stabilized pulses obtained by optical rectification of the output of an ultrabroadband Ti:sapphire oscillator. Energies of -80 microJ with a well-suppressed background of parametric superfluorescence and up to 400 microJ with a superfluorescence background are obtained from a two-stage parametric amplifier based on periodically poled LiNbO3 and LiTaO3 crystals. The parametric amplifier is pumped by an optically synchronized 1 kHz, 30 ps, 1053 nm Nd:YLF amplifier seeded by the same Ti:sapphire oscillator.     

Generation of 2.5 μJ vacuum ultraviolet pulses with sub-50 fs duration by noncollinear four-wave mixing in argon

Generation of sub-50fs vacuum UV pulses with more than 2.5μJ energy at a 1kHz repetition rate is reported. The pulses at 160nm are produced using noncollinear difference-frequency four-wave mixing between the fundamental and third harmonics of an amplified Ti:sapphire laser in argon. While the pulse duration is maintained by increasing the phase-matching pressure, noncollinear interaction improves the conversion efficiency by 1 order of magnitude in comparison with the previous results in collinear geometry.     

Pump-depleting four-wave mixing in supercontinuum-generating microstructure fibers

Four-wave mixing processes are shown to provide a high efficiency of non-linear optical frequency conversion and spectral transformation of ultrashort pulses in supercontinuum-generating microstructure fibers. Pump-depleting conversion of 800-nm radiation to the spectral range around 500 nm is achieved by phase-matching the parametric four-wave mixing process for 80-fs Ti:sapphire-laser pulses. The ways to use microstructure fibers for generating frequency-tunable radiation through four-wave mixing with the maximum efficiency of pump-field frequency conversion are discussed. PACS 42.65.Wi; 42.81.Qb     

Generation of femtosecond anti-stokes pulses through phase-matched parametric four-wave mixing in a photonic crystal fiber

Phase-matched parametric four-wave mixing in higher-order guided modes of a photonic crystal fiber is shown to result in an efficient decay of 40-fs 800-nm Ti:sapphire laser pump pulses into an anti-Stokes signal with a central wavelength around 590-600 nm and a Stokes signal centered at 1.25 microm. The photonic crystal fiber is designed in such a way as to minimize the group-velocity dispersion at the pump wavelength, phase match the parametric four-wave-mixing process, and reduce the group delay between the pump and the anti-Stokes pulses. The duration of the anti-Stokes pulse under these conditions, as shown by cross-correlation frequency-resolved optical gating measurements, is less than 200 fs.     

Sub-20 fs visible pulses with 750 nJ energy from a 100 kHz noncollinear optical parametric amplifier

We demonstrate the operation of a 100 kHz noncollinear optical parametric amplifier that is pumped by just a few microjoules of 800 nm pulses with 50 fs duration. The device delivers sub-20 fs pulses tunable from 460 nm to beyond 1 microm and pulse energies up to 750 nJ when it is pumped with 7 microJ of energy. The design of the single-stage amplifier has been carefully optimized, and the design considerations are discussed.     

Multikilohertz optical parametric chirped pulse amplification in periodically poled stoichiometric LiTaO3 at 1235 nm

We demonstrate, for the first time to our knowledge, multikilohertz operation of a double-stage optical parametric chirped pulse amplifier with periodically poled stoichiometric LiTaO3 crystals, seeded by a homemade Cr:forsterite oscillator operating at 1235 nm. The repetition rate of the amplifier could easily be tuned without the use of electro-optic modulators by using a repetition-rate-tunable kilohertz pump laser operating at 532 nm and a time-synchronization unit. Amplified total (signal+idler) energies of 55.9 and 36.2 microJ were achieved at 1 and 5 kHz, respectively. After recompression, the pulse width of amplified idler pulses at 1235 nm amounted to 530 fs.     

Compression of high-energy laser pulses below 5 fs

High-energy 20-fs pulses generated by a Ti:sapphire laser system were spectrally broadened to more than 250 nm by self-phase modulation in a hollow fiber filled with noble gases and subsequently compressed in a broadband high-throughput dispersive system. Pulses as short as 4.5 fs with energy up to 20-microJ were obtained with krypton, while pulses as short as 5 fs with energy up to 70 microJ were obtained with argon. These pulses are, to our knowledge, the shortest generated to date at multigigawatt peak powers.