He(I) and He(II) populations in the Nagoya TPD plasma machine

A collisional-radiative model is used to explain the He(I) population densities observed by Otsuka, Ikee and Ishii in their TPD plasma machine. It is shown that a plasma model, which is partially optically thick to He(II) Lyman radiation, can explain the experimentally observed He(II) population density at T_e=3.17 eV. The agreement between the experimental and calculated He(II) population densities observed by Otsuka and others is shown to be due to an error in their calculations.     

The reaction3He(d,p)4He with a polarized target

The left-right asymmetry for the³He(d, p)⁴He reaction has been measured with a polarized³He target at a bombarding energy of 12 MeV. The experimental results are compared with proton polarization measurements for unpolarized target and beam. The construction of the optically pumped³He target is described. A special design has been chosen to overcome the difficulty that the target contamination caused by the bombarding particles destroys the polarization. The target can easily be purified without removing it from the experimental set-up.     

Microscopic study of the low-energy3He(3He, 2p)4He and3H(3H, 2n)4He fusion cross sections

We have calculated the³He(³He, 2p)⁴He and³H(³H, 2n)⁴He reaction cross sections at low energies within the microscopic multichannel resonating group method. For both reactions, we find good agreement with experiment. For the³H(³H, 2n)⁴He reaction, our calculated energy dependence reproduces that of each individual low-energy experimental data set, except for a normalization constant. Using this fact, we derive at a low-energy³H(³H, 2n)⁴He rate by taking the averaged mean of these fits.This work has been supported in part by the National Science Foundation, Grants PHY86-04197 and PHY88-17296.     

Ab initio many-body calculations of the (3)H(d,n)(4)He and (3)He(d,p)(4)He fusion reactions

We apply the ab initio no-core shell model combined with the resonating-group method approach to calculate the cross sections of the (3)H(d,n)(4)He and (3)He(d,p)(4)He fusion reactions. These are important reactions for the big bang nucleosynthesis and the future of energy generation on Earth. Starting from a selected similarity-transformed chiral nucleon-nucleon interaction that accurately describes two-nucleon data, we performed many-body calculations that predict the S factor of both reactions. Virtual three-body breakup effects are obtained by including excited pseudostates of the deuteron in the calculation. Our results are in satisfactory agreement with experimental data and pave the way for microscopic investigations of polarization and electron-screening effects, of the (3)H(d,γn)(4)He bremsstrahlung and other reactions relevant to fusion research.     

Large-space cluster model calculations for the 3He(3He,2p)4He and 3H(3H,2n)4He reactions

The ³He(³He,2p)⁴He and ³H(³H,2n)su4He reactions are studied in a microscopic cluster model. We search for resonances in the ³He+³He and ⁴He + p + p channels using methods that treat the two- and three-body resonance asymptotics correctly. Our results show that the existence of a low-energy resonance or virtual state, which could influence the ⁷Be and ⁸B solar neutrino fluxes, is rather unlikely. Our calculated ³He(³He,2p)⁴He and ³H(³H,2n)⁴He cross sections are in a good general agreement with the experimental data.     

Theoretical interpretation of photoelectron spectra for transition metal compounds. The He(I) and He(II) spectra of MF2 molecules (M = Co,Ni and Cu)

Calculated vertical ionization energies (VIEs) and relative intensities (RIs) have been used in interpreting He(I) and He(II) photoelectron spectra of MF₂ molecules, M being Co, Ni and Cu. VIEs have been obtained by the Green's function technique applying the semiempirical CNDO-UHF method. Within the framework of the Gelius-Siegbahn model, but utilizing the theoretical atomic cross-sections, the molecular photoionization cross-sections (and the corresponding relative intensities of spectral bands) have been calculated for He(I) and He(II) spectra of MF₂ molecules. A comparison of the theoretical and experimental VIEs and RIs shows that the procedure is useful in ascribing photoemission peaks at particular binding energies of He(I) and He(II) spectra to the set of molecular orbitals.     

On pressure broadening of the ammonia inversion spectrum by inert gases (He,Ar)

We have calculated the linewidths of the inversion spectrum of NH₃ perturbed by inert gases (He, Ar) using a convergent theory proposed by Cattani. We have employed the Herman and Tipping potential for the dispersion interaction. Our theoretical results and those obtained from the Anderson and Tsao and Curnutte second and third approximations are compared with experimental results.     

The He(1s, 2s) + Ne interaction potential

A well depth D = 0.79 meV at R = 11.56 au is calculated for the excited He(1s, 2s) atom interacting with Ne by using a non-local pseudopotential method in good agreement with the experimental values. The pseudopotential I use also contains polarization effects in an adiabatic form. The contribution of the polarization to the well depth is calculated to be 0.42 meV.     

Stability of (3)He(2)(4)He(n) and (3)He(3)(4)He(n) L=0 clusters

We have studied the stability of mixed (3)He/(4)He clusters in L=0 states by the diffusion Monte Carlo method, employing the Tang-Toennies-Yiu He-He potential. The clusters (3)He(4)He(N) and (3)He(2)(4)He(N) are stable for N>1. The lighter atoms tend to move to the surface of the cluster. The minimum number of 4He atoms able to bind three 3He atoms in a L=0 state is nine. Two of three fermionic helium atoms stay on the surface, while the third one penetrates into the cluster.     

He(I) and He(II) photoelectron spectra of iron tetracarbonyl-olefin complexes

The He(I) and He(II) photoelectron spectra of a series of iron tetracarbonyl—olefin complexes (olefin = acrolein, crotonaldehyde, methyl acrylate, acrylic acid, dimethyl maleate and some dihalogenated ethylenes) are reported. Assignments are proposed, based on differences in intensity between the He(I) and He(II) spectra, in comparison with related compounds and the results of extended CNDO calculations. The electronic structure of the coordinated olefins is discussed.     

On the diffraction of He by a Ni(110) surface

The diffraction of low-energy He atoms by a Ni(110) surface is studied using hard and soft wall models for the elastic scattering. The effects of thermal vibrations and inelastic processes on the He intensities are estimated. It is shown that the experimental spectra imply a corrugation height along the [001] direction that is maximally 0.12 au. A value of 0.30 au, calculated recently within a scheme that assumes the repulsive interaction to be proportional to the electron density of unperturbed Ni(110), leads to “double rainbow” diffraction patterns qualitatively different from those observed.     

Microscopic calculation of six-body inelastic reactions with complete final state interaction: photoabsorption of (6)He and (6)Li

Six-body inelastic reactions are calculated microscopically including the full six-nucleon final state interaction. The total cross sections of gamma+ (6)He ( (6)Li)-->X are considered as examples. The Lorentz integral transform method and the effective interaction approach for the hyperspherical formalism are employed. While (6)Li has a single broad giant resonance peak, there are two well separated peaks for (6)He corresponding to the breakup of the neutron halo and the alpha core, respectively. The comparison with the few available experimental data is discussed.     

类氦离子Cr~(22 ) 精细结构能级和光谱跃迁的相对论多组态计算

采用相对论多组态自洽场方法,计算了类氦Cr22 离子的精细结构能级,能级宽度,激发态寿命和光谱跃迁参数。计算中考虑了核的有限体积效应,Breit修正,QED修正和轨道极化效应。所得结果与文献的实验值和计算值进行了比较     

光泵Ba/He系统582.8nm碰撞诱导荧光辐射及其弛豫振荡

观察到光泵Ba/He混合物产生的582.8nm碰撞诱导荧光新谱线及其弛豫振荡.进行理论分析和计算,结果与实验相符合.     

He(I) and He(II) photoelectron spectra of some substituted ethylenes

The He(I) and He(II) photoelectron spectra of acrolein, acrylic acid, methyl acrylate, vinyl acetate, acrylamide and some of their methyl-substituted analogues are reported. Detailed assignments are proposed, mainly based on differences in intensity between the He(I) and He(II) spectra, on sum rule considerations and on the results of modified CNDO/S calculations.The assignment criteria are critically evaluated.     

Atom-surface interaction in inelastic scattering: He/Ag(111)

The amplitude of inelastic He scattering from Rayleigh waves on a Ag(111) surface is calculated in the framework of the distorted wave Born approximation (DWBA) for a two-body exponential potential. Using the potential parameters recently obtained by Bortolani et al. from a quantum mechanical calculation, agreement is obtained with the experimental data. Simple explicit formulas are presented both in the DWBA and in the eikonal approximation. The essential factor in both cases describes an approximate exponential decay of the intensity for increasing parallel momentum transfer.     

Ionization of metastable He(1s2s) atoms by alkalated surfaces

We calculate the ionization probability for singlet and triplet metastable He(1s2s) atoms scattered from potassium covered surfaces, on the basis of the resonant tunnelling process. We do not assume the trajectory approximation, but we do assume classical motion on the potential energy curves, with crossing between neutral and ionic curves at a given point calculated from electronic tunnelling probabilities. Energy spectra of the He⁺ ions are also calculated. The results are found to be somewhat sensitive to tunnelling probability as a function of distance from the surface. Results are compared with experimental ionization probabilities measured by Roussel. The agreement is found to be fair if the tunneling rate is parameterized according to the theory of Janev et al. A simple interpretation is given.     

_(18)Ar~(q~ )(q=3,4)与H和He碰撞的电荷剥离截面

采用二体碰撞近似和托马斯 -费米近似计算了多电荷离子18Arq ( q =3,4 )与中性原子H和He碰撞的电荷剥离截面以及Arq 的势函数和电子动量分布 ,计算结果与文献 [4]中的数据符合得较好。所导出的计算公式和编制的计算程序可以计算任何一个多电荷离子Aq 与H或He碰撞的电荷剥离截面。因而具有一定的普适性。     

Polarization of 4He(23S1) by optically pumped Rb

The Zeeman resonance in He(2³S₁) has been observed with narrow linewidth, ～350 Hz, using a technique involving spin-dependent Penning collisions with optically pumped Rb. This linewidth is 100 times narrower than previously reported in determination of g_J(⁴He, 2³S₁).     

Measurements of the strong-interaction widths of the kaonic (3)He and (4)He 2p levels

The kaonic (3)He and (4)He X-rays emitted in the [Formula: see text] transitions were measured in the SIDDHARTA experiment. The widths of the kaonic (3)He and (4)He 2p states were determined to be [Formula: see text], and [Formula: see text], respectively. Both results are consistent with the theoretical predictions. The width of kaonic (4)He is much smaller than the value of [Formula: see text] determined by the experiments performed in the 70's and 80's, while the width of kaonic (3)He was determined for the first time.