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1.
We have studied the fluorescence of electronically excited OH*, H* and H2O+* dissociation fragments after VUV excitation ( h ν≥11.6 eV) of rare-gas clusters (Rg = Ne, Ar) doped with H2O molecules. In contrast to a free molecule, where Balmer H-series dominate the UV-visible spectra, only the OH * ( A 2 Σ + X 2 Π) emission band is observed in neon clusters. No emission of excited water ions has been observed. We find that while higher excitation energies (Ne vs. Ar) induce higher vibrational excitation of the OH* ( A ) fragment, the rotational temperature is lower. This effect is attributed to the difference in the geometric position of the H2O molecule on the surface or inside the Rg-cluster. The rotational relaxation in neon clusters is rapid while the vibrational relaxation is slow because of the coupling with the low energy matrix phonons. Received 7 March 2002 / Received in final form 27 May 2002 Published online 19 July 2002  相似文献   

2.
Magnetic measurements have been carried out in different LaNi1-xMnxO 3 + δ samples with 0.1 ⩽ x ⩽ 0.9. All these samples show two magnetic anomalies, one at relatively high temperature characteristic of a ferromagnetic ordering and the other at low temperature, typical of magnetic relaxation phenomena. Neutron diffraction patterns indicate that long-range ferromagnetic ordering is only achieved for x ≥ 0.5. Neutron patterns of LaNi0.5Mn0.5O 3 + δ samples show an ordered arrangement of Ni and Mn atoms in the perovskite lattice. LaNi0.5Mn0.5O 3 + δ is then, a double perovskite A2BB'O6 whereas Ni and Mn atoms are randomly distributed for the rest of the samples. X-ray magnetic circular dichroism experiments confirm the presence of collinear ferromagnetism in LaNi0.5Mn0.5O 3 + δ . The role of competitive magnetic interactions, structural disorder, magnetic anisotropy and magnetic disaccommodation is also discussed Received 19 July 2002 / Received in final form 23 October 2002 Published online 31 December 2002  相似文献   

3.
The most probable parameters of the pure, doped, and mixed GaSe1−xSx (x ≤ 0.4) crystals (solid solutions) are presented together with the results of investigations of their crystal structure and defects, optical and mechanical properties, and damage thresholds. __________ Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 6, pp. 35–40, June, 2007.  相似文献   

4.
By using heavy-ion induced fusion-evaporation reactions at the on-line mass separator of GSI, the decay properties of neutron-deficient isotopes between 56Ni and 100Sn were investigated. The experimental results will be presented and discussed in comparison with model predictions.  相似文献   

5.
We revisit the determination of α S (m τ 2) using a fit to inclusive τ hadronic spectral moments in light of (1) the recent calculation of the fourth-order perturbative coefficient K 4 in the expansion of the Adler function, (2) new precision measurements from BABAR of e+e annihilation cross sections, which decrease the uncertainty in the separation of vector and axial-vector spectral functions, and (3) improved results from BABAR and Belle on τ branching fractions involving kaons. We estimate that the fourth-order perturbative prediction reduces the theoretical uncertainty, introduced by the truncation of the series, by 20% with respect to earlier determinations. We discuss to some detail the perturbative prediction of two different methods: fixed-order perturbation theory (FOPT) and contour-improved perturbative theory (CIPT). The corresponding theoretical uncertainties are studied at the τ and Z mass scales. The CIPT method is found to be more stable with respect to the missing higher order contributions and to renormalization scale variations. It is also shown that FOPT suffers from convergence problems along the complex integration contour. Nonperturbative contributions extracted from the most inclusive fit are small, in agreement with earlier determinations. Systematic effects from quark-hadron duality violation are estimated with simple models and found to be within the quoted systematic errors. The fit based on CIPT gives α S (m τ 2)=0.344±0.005±0.007, where the first error is experimental and the second theoretical. After evolution to M Z we obtain α S (M Z 2)=0.1212±0.0005±0.0008±0.0005, where the errors are respectively experimental, theoretical and due to the evolution. The result is in agreement with the corresponding N3LO value derived from essentially the Z width in the global electroweak fit. The α S (M Z 2) determination from τ decays is the most precise one to date.  相似文献   

6.
Using an effective low-energy Hamiltonian derived from the first-principles electronic structure calculations for the narrow t 2g bands of YTiO3, LaTiO3, YVO3, and LaVO3, we evaluate the contributions of the correlation energy E c to the stability of different magnetic structures that can be realized in these distorted perovskite oxides. We consider two approximations for E c that are based on regular perturbation theory expansion around a nondegenerate Hartree-Fock ground state. One is the second order of perturbation theory, which allows comparing the effects of local and nonlocal correlations. The other is the local t-matrix approach, which allows treating some higher-order contributions to E c . The correlation effects systematically improve the agreement with the experimental data and additionally stabilize the experimentally observed G- and C-type antifer-romagnetic (AFM) structures in YVO3 and LaVO3, although the absolute magnitude of the stabilization energy is sensitive to the level of approximations and is somewhat smaller in the t-matrix method. The nonlocal correlations additionally stabilize the ferromagnetic ground state in YTiO3 and the C-type AFM ground state in LaVO3. Among two inequivalent transition-metal sites in the monoclinic structure, the local correlations are stronger at the sites with the least distorted environment. Limitations of the regular perturbation-theory expansion for LaTiO3 are also discussed. The text was submitted by the authors in English.  相似文献   

7.
Conduction-electron spin polarization dynamics achieved by pulsed optical pumping at room temperature in GaAs1−x N x alloys with a small nitrogen content (x = 2.1, 2.7, and 3.4%) is studied both experimentally and theoretically. It is found that the photoluminescence circular polarization determined by the mean spin of free electrons reaches 40–45% and this giant value persists within 2 ns. Simultaneously, the total free-electron spin decays rapidly with the characteristic time ≈ 150 ps. The results are explained by spin-dependent capture of free conduction electrons on deep paramagnetic centers resulting in the dynamical polarization of bound electrons. A nonlinear theory of spin dynamics in the coupled system of spin-polarized free and localized carriers has been developed which describes the experimental dependencies, in particular, the electron spin quantum beats observed in a transverse magnetic field. The text was submitted by the authors in English.  相似文献   

8.
In the framework of k t -factorization approach, the process of inclusive photoproduction of J/Ψ mesons at HERA conditions is considered. The spin density matrix elements are calculated, and the predictions are compared with recent experimental data. The article is published in the original.  相似文献   

9.
We show that D-branes in the Euclidean AdS 3 can be naturally associated to the maximally isotropic subgroups of the Lu–Weinstein double of SU(2). This picture makes very transparent the residual loop group symmetry of the D-brane configurations and gives also immediately the D-branes shapes and the σ-model boundary conditions in the de Sitter T-dual of the SL(2,C)/SU(2) WZW model.  相似文献   

10.
11.
We show that it is possible to construct a supersymmetric mechanics with four supercharges possessing not conformally flat target space. A general idea of constructing such models is presented. A particular case with Eguchi-Hanson target space is investigated in detail: we present the standard and quotient approaches to get the Eguchi-Hanson model, demonstrate their equivalence, give a full set of nonlinear constraints, study their properties and give an explicit expression for the target space metric. Presented at the International Colloquium “Integrable Systems and Quantum Symmetries”, Prague, 16–18 June 2005.  相似文献   

12.
Nanosized titanium dioxide (TiO2) powder was prepared by a laser-induced pyrolysis. Specific surface area of the as-grown powder measured by BET method was 109 m2/g. The grain size (14.5 nm) estimated from these data coincides well with the crystallite size (12.3 nm) determined by XRD measurements. The average grain size (∼35 nm) obtained from the subsequent SEM measurements refers to considerable agglomeration of nanoparticles. Raman spectroscopy has been used to investigate the structural properties of TiO2 nanopowder and its anatase structure is confirmed. The blueshift and broadening of the lowest frequency Eg Raman mode at temperature range ∼25–550 K have been analyzed using a phonon-confinement model. Dominant influence of the strong anharmonic effect at higher temperatures was demonstrated. PACS 81.07.Wx; 78.30.-j; 63.22.+m  相似文献   

13.
We investigate the solitons in the CP N model in terms of the decomposition of gauge potential. Based on the φ-mapping topological current theory, the charge and position of solitons is determined by the properties of the typical component. Furthermore, the motion and the bifurcation of multi-soliton is discussed. And the knotted solitons in high dimension is explored also.  相似文献   

14.
Powder neutron diffraction and Hi-Q neutron diffraction data have been recorded and analysed in order to obtain the local and long range order of Cu in Cudoped CeO2 with three doping levels of Cu. Rietveld method and MCGR techniques of data analysis for the two types of data reveal that the Cu ion is in the 2+ oxidation state and has a vacancy in its first coordination shell. These deductions from the data analysis fit well with the mechanism of catalysis we propose.  相似文献   

15.
Based on SU(3) flavor symmetry, many of the quark-graph amplitudes in two-body non-leptonic decays of charmed mesons can be extracted from experiment, which enable us to see the relevance and importance of weak annihilation topologies and to determine the complex parameters a1 and a2 to test the factorization approach. It is found that a 2 /a 1 in and can be different by a factor of 2, indicating that non-factorizable corrections to the latter are far more important than the former. The relative phase between a1 and a2 is about 150°. Weak annihilation topologies induced by nearby resonances via final-state rescattering can be described in a model-independent manner. Although the W-exchange contribution in decays is dominated by resonant final-state interactions (FSIs), its amplitude in VP decays (V: vector meson, P: pseudoscalar meson) receives little contributions from FSIs in the quark-antiquark resonance formation. As a consequence, the sign flip of the W-exchange amplitude in and decays, which is needed to explain the relatively real decay amplitudes of , remains unexplained. SU(3) symmetry is badly broken in some Cabibbo-suppressed modes and this can be accounted for by the accumulation of some modest SU(3) violation in individual quark-graph amplitudes. Received: 19 July 2002 / Published online: 20 November 2002  相似文献   

16.
We report results of the atomic and electronic structures of Al7C cluster using ab initio molecular dynamics with ultrasoft pseudopotentials and generalized gradient approximation. The lowest energy structure is found to be the one in which carbon atom occupies an interstitial position in Al7 cluster. The electronic structure shows that the recent observation [Chem. Phys. Lett. 316, 31 (2000)] of magic behavior of Al7C- cluster is due to a large highest occupied and lowest unoccupied molecular orbital (HOMO-LUMO) gap which makes Al7C- chemically inert. These results have further led us to the finding of a new neutral magic cluster Al7N which has the same number of valence electrons as in Al7C- and a large HOMO-LUMO gap of 1.99 eV. Further, calculations have been carried out on (Al7N)2 to study interaction between magic clusters. Received 28 July 2001  相似文献   

17.
The characteristics of the charged-current neutrino—nuclear interactions are investigated for the first time at E ν = 1–3 GeV using the data obtained with SKAT propane-freon bubble chamber irradiated in the neutrino beam at the Serpukhov accelerator. The E ν dependence of the mean multiplicities of different types of secondary particles and their multiplicity, momentum, and angular distributions are measured. The text was submitted by the authors in English.  相似文献   

18.
We calculate the leptonic constant for the pseudoscalar ground state of the B c meson in the framework of a QCD-motivated potential model taking into account the two-loop anomalous dimension for the heavy quark current in nonrelativistic QCD as matched with full QCD.  相似文献   

19.
 We prove estimates for the stationary state n-point functions at zero molecular diffusivity in the Kraichnan model [13]. This is done by proving upper bounds for the heat kernels and Green's functions of the degenerate elliptic operators M n that occur in the Hopf equations for the n-point functions. Received: 25 August 2001 / Accepted: 30 September 2002 Published online: 20 January 2003 Communicated by A. Kupiainen  相似文献   

20.
Transport properties of SrRuO3 thin films were studied as a function of the epitaxial strain. SrRuO3 films were grown on (100) SrTiO3 substrates by the Pulsed Laser Deposition technique equipped with Reflection High Energy Electrons Diffraction (RHEED). Samples thickness has been varied from a few unit cells to above 1000 ? while monitoring RHEED intensity oscillations. In thicker films epitaxial strain was found to be progressively relaxed. SrRuO3 relaxed films (thickness 1000 ?) show metallic behavior for the whole temperature range with a ferromagnetic ordering at about 150 K. For thinner films, ferromagnetic ordering occurs at progressively lower temperatures, until in films thinner than 400 ? it disappears. Films thinner than 80 ? show a semiconducting behavior at low temperatures. Our results provide direct evidence of the crucial role of the strain effect for conducting and magnetic properties of SrRuO3. Received 16 July 2001 and Received in final form 22 October 2001  相似文献   

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