A novel-high energy pulse compression system: generation of multigigawatt sub-5-fs pulses

Received: 28 February 1997 / Revised version: 2 May 1997     

Generation of subpicosecond infrared pulses tunable between 5.2 μm and 18 μm at a repetition rate of 76 MHz

2 (2 mm thick) and GaSe (1 mm thick) crystals are applied as nonlinear media. GaSe has a larger tuning range and is more efficient in the whole spectral range than AgGaS₂. The average IR power reaches up to 2.0 mW at 8.5 μm when the GaSe crystal is used, and up to 1.3 mW at the same wavelength when AgGaS₂ is applied for the frequency conversion. Received: 17 February 1997/Revised version: 14 July 1997     

All-reflective interferometric autocorrelator for the measurement of ultra-short optical pulses

We have developed a novel interferometric autocorrelator composed of only reflective elements, which functions as a beam splitter and an optical delay line. Analytical expressions are derived to give second-order autocorrelation functions and deconvolution factors for various conditions. The measurement of femtosecond laser pulses by interferometric autocorrelation is demonstrated in the visible region. The results are compared with those by calculation. Received: 9 December 2002 Revised version: 18 February 2003 / Published online: 5 May 2003 RID="*" ID="*"Present address: Department of Physics, Tokai University, 1117 Kitakaname, Hiratsuka, Kanagawa 259-1207, Japan RID="**" ID="**"Corresponding author. Fax: +81-48/462-4682, E-mail: asuda@postman.riken.go.jp     

Low-threshold high-dynamic-range optical limiter for ultra-short laser pulses

We demonstrate an optical limiter for ultra-short (∼100-fs) laser pulses. The device has a dynamic range (= damage energy/onset-of-limiting energy) of more than 10000 and an onset-of-limiting energy of only ∼10 nJ. The output-pulse energy is kept below 1.3 μJ. The limiting mechanism is based on two-photon absorption and refractive nonlinearities in a 20-mm piece of ZnSe. We discuss the importance of the different nonlinearities, damage issues, and guidelines for the construction of the device. Received: 20 December 2001 / Revised version: 25 March 2002 / Published online: 8 May 2002     

High-dynamic-range pulse-front steepening of amplified femtosecond pulses by third-order dispersion

Received: 9 June 1998/Revised version: 4 November 1998     

Temporal behavior of a high repetition rate infrared optical parametric oscillator based on periodically poled materials

The temporal behavior of a nanosecond pulsed singly resonant periodically poled lithium niobate optical parametric oscillator has been studied both theoretically and experimentally. Taking into account the cylindrical symmetry of the system, a numerical model based on the Hankel transform has been developed. Good agreement is obtained between experiment and simulation. Moreover, the computation time is reduced roughly by a factor of 60 compared to the usual simulation software. Received: 23 April 2001 / Published online: 19 September 2001     

Ionization spectrum broadening and frequency blue-shift of high-intensity femtosecond laser pulses in gas-filled capillary tubes

. We report on the experimental and theoretical study of spectrum transformation and frequency blue-shift of femtosecond laser pulses with intensities up to 2×10¹⁶ W/cm², propagating in glass capillary tubes under gas ionization. Monomode optical guiding with 45% transmission efficiency is demonstrated in a 100-μm-diameter, 20-cm length capillary. A broadening of the initial spectrum as much as several initial spectrum widths is achieved. Besides the broadening, the mean frequency of the output radiation in the spectrum experiences a blue-shift of up to several initial spectrum widths, caused by the non-stationary, non-linear process of gas ionization. Our numerical simulations, in the form of a simple one-dimensional model for the propagation of intense laser pulses in gas-filled capillaries, are in good qualitative agreement with the experimental results. These simulations show the possibility of significant compression of an output pulse in a simple compression scheme (e.g. a piece of silica glass with normal dispersion), which is very important for obtaining laser pulses with few optical cycles at the millijoule energy level. Received: 25 September 2001 / Revised version: 6 December 2001 / Published online: 25 September 2002 RID="*" ID="*"Corresponding author. Fax: +7-8312/363-792, E-mail: dekart@ufp.appl.sci-nnov.ru     

A dispersionless Michelson interferometer for the characterization of attosecond pulses

A novel application of a free-standing transmission grating as a beam splitter in a Michelson-type interferometer is described. The arrangement can operate in the XUV and soft X-ray spectral region and, therefore, it is well suited for the characterization of attosecond pulses. Using ray-tracing codes, we have analyzed three different setups in which spherical mirrors are employed in conjunction with the transmission grating and have investigated in detail their dispersive characteristics. It is shown that such an arrangement can be made to exhibit group-delay dispersion of ∼1 as² while it provides two co-propagating and converging beams. Received: 12 October 2001 / Revised version: 17 December 2001 / Published online: 7 February 2002     

All-solid-state cavity-dumped sub-5-fs laser

Received: 19 March 1997/Revised version: 9 May 1997     

Generation of tunable sub-picosecond pulses in the UV with a travelling wave dye laser

Received: 22 June 1998/Revised version: 3 August 1998     

Adaptive shaping of two-cycle visible pulses using a flexible mirror

We present a double-pass non-collinear optical parametric amplifier (NOPA) that delivers 4-fs visible–near-infrared pulses. The paper discusses geometrical and temporal properties of the NOPA configuration, which allow us to broaden the gain band of simultaneous parametric amplification in excess of 250 THz. The key elements of the bandwidth enhancement include (i) the use of a broadband second-harmonic pump, (ii) optimization of the incidence angle of all monochromatic spectral components of the pump in order to produce a favorable offset of the corresponding phase-matching curves, and (iii) selection of the chirp rate and time delay between the stretched pump and seed pulses. We next devise a two-stage compressor that incorporates a flexible mirror for adaptive pulse shaping and develop a simple and trustworthy feedback loop based on a one-dimensional spectral measurement. Our rapid numerical algorithm for adaptive control of the flexible membrane is found superior to more complex search routines that are less resistant to the fluctuations of the laser intensity. The automated optimization procedure results in the generation of two-cycle pulses with a carrier wavelength at ∼600 nm. The absence of deep modulation on the parametrically amplified spectrum in combination with the adaptive phase correction lead to a high quality of the temporal profile and allow concentrating 90% of the pulse energy within only a 7.5-fs time window. Received: 8 April 2002 / Revised version: 26 June 2002 / Published online: 25 September 2002 RID="*" ID="*"Present address: Institut für Photonik, Technische Universit?t Wien, Gusshausstrasse 27, 1040 Vienna, Austria RID="**" ID="**"Corresponding author. Fax: +81-3/5841-4165, E-mail: kobayashi@phys.s.u-tokyo.ac.jp     

SPM-induced spectral compression of picosecond pulses in a single-mode Yb-doped fiber amplifier

In a fiber amplifier, spectral compression due to self-phase modulation is demonstrated for ultrashort pulses. We report the generation of near-transform-limited picosecond pulses with peak powers of several kW at a repetition rate of 74 MHz and diffraction-limited beam quality in a Yb-doped fiber amplifier when seeding with a negative chirped pulse. Received: 17 September 2001 / Revised version: 22 November 2001 / Published online: 17 January 2002     

Harmonic repetition-rate femtosecond optical parametric oscillator

We report on a femtosecond optical parametric oscillator (OPO) with a repetition rate of 1 GHz, which is 12 times that of the pump laser used. We also introduce a novel method for operating an OPO with a high harmonic repetition rate which is not determined by the cavity length of the OPO, but rather the cavity length difference between the OPO and its pump laser. Operation of an OPO at 4-times the harmonic repetition rate has been carried out to show the feasibility of this method. The new approach paves the way for constructing a femtosecond OPO working at repetition rates of 10 GHz, or higher, when the pump laser used has a relatively low repetition rate. Received: 26 October 2001 / Revised version: 11 Januar 2002 / Published online: 14 March 2002     

High-power sub-10-fs Ti:sapphire oscillators

Received: 10 March 1997/Revised version: 16 April 1997     

Generation of high average power, 7.5-fs blue pulses at 5 kHz by adaptive phase control

The spectral width of a 5-kHz Ti:sapphire laser system was broadened by spectral control in a regenerative amplifier consisting of broadband chirped mirrors. The dispersion over the wide spectral range was compensated by a deformable mirror along with a genetic algorithm, resulting in a pulse width of 15 fs. The pulse width is the shortest, to our knowledge, in chirped pulse amplification systems with a regenerative amplifier. The phase distortion of broadband frequency doubling in addition to the Ti:sapphire laser was compensated by using the self-diffraction intensity in sapphire as the feedback signal into the genetic algorithm, resulting in a pulse width of 7.5 fs. The average power of the second harmonic was 1 W with a fundamental input of 7 W.     

Generation of femtosecond pulses by two-photon pumping supercontinuum-seeded collinear traveling wave amplification in a dye solution

Visible femtosecond (fs) laser pulses have been obtained in a dye solution with a very simple traveling wave collinear configuration. A femtosecond Ti:sapphire laser (790 nm) pumps the dye solution by two-photon absorption and simultaneously generates supercontinuum, which seeds a light-amplification mechanism. Cross-correlation frequency-resolved optical gating measurements reveal a chirped structure in the dye pulse. The shortest pulse duration achieved is 170 fs and the overall energy efficiency of the process is typically 25%. Received: 22 March 2001 / Revised version: 4 July 2001 / Published online: 19 September 2001     

Spectral broadening of 40-fs Ti:sapphire laser pulses in photonic-molecule modes of a cobweb-microstructure fiber

Photonic-molecule modes of a cobweb-microstructure fiber allow efficient nonlinear optical spectral broadening of nanojoule femtosecond light pulses. Spectral widths of approximately 200 nm are achieved at the output of a 6-cm sample of such a fiber for 40-fs Ti:sapphire laser pulses with an energy of a few nanojoules coupled into photonic-molecule modes. Higher values of the group index and a lower group-velocity dispersion, attainable with higher-order photonic-molecule modes, allow the efficiency of spectral broadening of femtosecond laser pulses to be increased relative to the efficiency of spectral broadening in the fundamental photonic-molecule mode. Received: 9 June 2002 / Revised version: 29 June 2002 / Published online: 22 November 2002 RID="*" ID="*"Corresponding author. Fax: +7-095/939-3959, E-mail: zheltikov@top.phys.msu.su     

Semiconductor saturable absorber mirrors supporting sub-10-fs pulses

Received: 18 March 1997/Revised version: 12 May 1997     

Concatenation of plasma filaments created in air by femtosecond infrared laser pulses

We report the first observation of the attachment of two single plasma filaments created collinearly in the atmosphere by IR femtosecond laser pulses. The linked filamentary structure is electrically conductive and emits sub-THz radiation over its entire length. Concatenation is achieved only for a specific time ordering between the two initial laser pulses. The pulse producing the filament closer to the laser source must be retarded with respect to the other pulse. This special time ordering is attributed to the acceleration of light in a self-guided pulse. Received: 4 March 2003 / Published online: 14 May 2003 RID="*" ID="*"Corresponding author. Fax: +33-1/6931-9996, E-mail: stzortz@ensta.fr     

Time-resolved two photon photoemission electron microscopy

Femtosecond, time-resolved two photon photoemission has been used to map the dynamics of photo-excited electrons at a structured metal/semiconductor surface. A photoemission microscope was employed as a spatially resolving electron detector. This novel setup has the potential to visualize variations of hot electron lifetimes in the femtosecond regime on heterogeneous sample surfaces and nanostructures. Received: 22 October 2001 / Revised version: 10 January 2002 / Published online: 7 February 2002