Rapid Preparation of Large-Area Densely Packed Plasmonic Hot-Spots for Reliable Sers Sensing

A facile, efficient and time-saving strategy is proposed to obtain large-area and reliable surface-enhanced Raman scattering (SERS) substrates via artificial heat-treatment of Au nanoparticles or ultrathin Au films sputtered on the silica substrates. Excellent Raman enhancements with the detection limitation down to 10^–9 mol/L are obtained due to the highly-dense plasmonic hot-spots and strong plasmons near-field coupling. Decreased intensity of Raman peaks with the increased sputtering time of Au nanoparticles or ultrathin films mainly originates from the excited and hybridized coupling of multiple surface plasmons. The simple fabrication strategy and superior performance make these substrates promising candidates for the development of inexpensive and reliable SERS substrates.

     

量子通信中单光子探测器的实验研究

为了提高单光子探测系统的灵敏度,实验采用InGaAs/InP雪崩光电二极管作为量子通信中的单光子探测器件,以门控脉冲模式实现了更高精度的单光子探测器的偏压生成电路、单光子信号放大电路、单光子信号检测电路和温度控制模块,并通过选用高精度前置放大器OP37和精密比较器AD8561,将量子效率提高到18.3%,暗计数控制小于4.1%×10~(-6)/ns.     

原向反射式大面积三角形探测光幕灵敏度分布

分体式大靶面测试系统的探测光幕灵敏度直接影响飞行弹丸速度测量的精度。可在散布不大的情况下,使用反射膜与激光器代替矩形大面积测试系统中的人工光源,简化测试系统。对新建的三角形探测光幕的灵敏度进行了分析,综合考虑激光器在不同传播距离处的光强度衰减、空间的非均匀性分布及反射膜逆反射系数和镜头离轴效应等因素,采用数值仿真和实弹试验的方法,将同一弹径的弹丸穿过光幕不同位置时的灵敏度等效到同一基准点进行归一化分析。结果显示,镜头离轴效应对灵敏度影响最大,激光器空间非均匀性分布影响最小。在3.5 m×2 m(宽×高)的直角三角形探测光幕区域进行实弹试验,其结果与仿真结果一致,距镜头越近,灵敏度越高;反之越低。研究结果可为类似原向反射式大面积探测光幕的工程设计提供参考。     

Direct observation of depolarization shift of the intersubband resonance

We have studied the intersubband resonance of GaAs/AlGaAs multi-quantum-well systems by comparing photon drag and absorption spectra obtained by in-plane photocurrent and photoconduction measurements. The peak absorption at room temperature is found to be blueshifted from the photon drag resonance by as much as 33 cm(-1). We argue that this difference gives directly the depolarization shift, since the resonant photon drag current is driven by the Doppler effect, which is a k-vector dependent single particle process.     

Features of the electron-photon drag effect in a spiral ribbon in the external magnetic field

The features of the photon drag effect in a spiral two-dimensional ribbon, which are associated with an asymmetric electron energy spectrum in a longitudinal magnetic field, have been studied theoretically. The effect of the anisotropic transfer of the photon momentum to the electron system in a spectral dependence of the photon drag current density has been revealed.     

Quantitative luminous efficiency determination for large-area light-emitting devices

During recent decades organic light-emitting devices became of increasing interest in many fields of applications. A broad spectrum of available organic molecules can be used to fabricate organic light-emitting diodes (OLEDs) emitting at various photon energies. One of the commonly used quality criteria to specify the light output of OLEDs is the luminous efficiency. The standard measurements are based on the assumption of a point source, which is not applicable in the case of large-area devices, or can be achieved only approximately by long distances between emitter and detector. Therefore, we developed a data evaluation procedure, taking into account the extended area of the emitter as well as the geometry of the detector and its spectral sensitivity. This mathematical model delivers correction factors for the luminous efficiency as a function of the distance between a large-area emitter and a detector. The model was tested experimentally for rectangular-shaped OLED structures and delivered accurate results for three different standard types of detectors.     

Large-area fabrication: The next target of perovskite light-emitting diodes

Perovskite materials show exciting potential for light-emitting diodes (LEDs) owing to their intrinsically high photoluminescence efficiency and color purity. The research focusing on perovskite light-emitting diodes (PeLEDs) has experienced an exponential growth in the past six years. The maximum external quantum efficiency of red, green, and blue PeLEDs has surpassed 20%, 20%, and 10%, respectively. Nevertheless, the current PeLEDs are still in the laboratory stage, and the key for further development of PeLEDs is large-area fabrication. In this paper, we briefly discuss the similarities and differences between manufacturing high-quality and large-area PeLEDs and perovskite solar cells. Especially, the general technologies for fabricating large-area perovskite films are also introduced. The effect of charge transport layers and electrodes on large-area devices are discussed as well. Most importantly, we summarize the advances of large-area (active area ≥ 30 mm²) PeLEDs reported since 2017, and describe the methods for optimizing large-area PeLEDs reported in the literature. Finally, the development perspective of PeLEDs is presented for the goal of highly efficient and large-area PeLED fabrication. It is of great significance for the application of PeLEDs in future display and lighting.     

用于位置灵敏型中子探测器的6LiF/ZnS（Ag）闪烁体性能研究

研究了掺杂6LiF的ZnS(Ag)闪烁体对中子、γ射线的发光特性和EJ426闪烁体样品的热中子探测效率、出射光产额和γ灵敏度。EJ426的热中子探测效率为32.4%,出射光产额为8.01×103光子/中子,70 mV阈值时的γ灵敏度小于10-7,表明EJ426是较理想的闪烁体型位置灵敏中子探测器材料。     

基于单光子探测及脉冲位置调制的激光通信关键技术研究

为了实现高灵敏度的空间激光通信,并提高传输信道的抗干扰能力,将单光子探测技术和脉冲位置调制技术相结合,采用门控电路与反馈淬灭电路相结合的方式淬灭单光子探测器雪崩,设计了插入帧头法用于脉冲位置调制解调。用现场可编程门阵列进行了脉冲位置调制解调过程的仿真,验证了插入帧头法的有效性与可行性。在此基础上搭建了1 550 nm的脉冲位置调制激光通信实验,同时测试了单光子探测器在不同参数下的性能。结果表明,当探测效率为25%,触发延时为8.00 ns,门宽为5.0 ns,死时间为0.1μs时,单光子探测器性能最佳。最后测试了不同调制速率下单光子探测器的探测灵敏度,结果表明,当通信码速率为1 Mbps时,通信灵敏度为-51.8 dBm;当通信码速率为4 Mbps时,通信灵敏度为-41.0 dBm,实现了高灵敏度的空间激光通信。     

基于深紫外激光-光发射电子显微技术的高分辨率磁畴成像

基于磁二色效应的光发射电子显微镜磁成像技术是研究薄膜磁畴结构的一种重要研究手段,具有空间分辨率高、可实时成像以及对表面信息敏感等优点.以全固态深紫外激光(波长为177.3 nm;能量为7.0 eV)为激发光源的光发射电子显微技术相比于传统的光发射电子显微镜磁成像技术(以同步辐射光源或汞灯为激发源),摆脱了大型同步辐射光源的限制;同时又解决了当前阈激发研究中由于激发光源能量低难以实现光电子直接激发的技术难题,在实验室条件下实现了高分辨磁成像.本文首先对最新搭建的深紫外激光-光发射电子显微镜系统做了简单介绍.然后结合超高真空分子束外延薄膜沉积技术,成功实现了L10-FePt垂直磁各向异性薄膜的磁畴观测,其空间分辨率高达43.2 nm,与利用X射线作为激发源的光发射电子显微镜磁成像技术处于同一量级,为后续开展高分辨磁成像提供了便利.最后,重点介绍了在该磁成像技术方面取得的一些最新研究成果:通过引入Cr的纳米"台阶",成功设计出FePt的(001)与(111)双取向外延薄膜;并在"台阶"区域使用线偏振态深紫外激光观测到了磁线二色衬度,其强度为圆二色衬度的4.6倍.上述研究结果表明:深紫外激光-光发射电子显微镜磁成像技术在磁性薄膜/多层膜体系磁畴观测方面具备了出色的分辨能力,通过超高真空系统与分子束外延薄膜制备系统相连接,可以实现高质量单晶外延薄膜制备、超高真空原位传输和高分辨磁畴成像三位一体的功能,为未来磁性薄膜材料的研究提供了重要手段.     

Performance of photon drag and photon drag-optical rectification detectors in the 2 to 33 μm range

Previous studies of the spectral response of p-Ge photon drag and n-Gap photon drag-optical rectification detectors have been extended. Measurements have also been made of the spectral response of p-Si photon drag, p-GaP photon drag-optical rectification and p-GaAs photon drag-optical rectification detectors. The wavelength range of main interest is between 2 and 11 μm, (HF, HCl, HBr, H₂O vapour and CO₂ lasers), but some measurements have also been made at 28 and 33 μm, (H₂O vapour laser).     

Transverse MIR fast response in PbSe films

Under lightening, anisotropic semiconductor or semimetal films can show large transverse voltage. PbSe and PbS films have a room temperature intense sub nsec response ( V/MW) in the 10µm region due to free carrier photon drag, but the effective direct matched response on a 50 impedance is lower ( 0.1 V/MW for 1 cm² film) because of the high film resistance (> KW). CO₂ 500ps mode locked pulses are easily detected in the scope limit.     

Application of gain-modulated avalanche photodiodes in phase-sensitive fluorescence spectroscopy

Phase and modulation fluorometry experiments at frequencies up to 875 MHz and lifetime-selective fluorescence detection with picosecond resolution are reported. A high-frequency gain-modulated silicon avalanche photodiode is used as an opto-electronic crosscorrelator which permits 10 ps time resolution and 1 photon per laser period sensitivity. Application of the correlator to fluorescence rejection from Raman spectra is proposed.     

Drag effect of one-dimensional electrons upon photoionization of D<Superscript>(−)</Superscript> centers in a longitudinal magnetic field

A theory is elaborated for the impurity photon drag effect in a semiconductor quantum wire exposed to a longitudinal magnetic field B directed along the axis of the quantum wire. The phonon drag effect is associated with the transfer of the longitudinal photon momentum to localized electrons in optical transitions from D^(?) states to hybrid-quantized states of the quantum wire, which is described by a confinement parabolic potential. An analytical expression for the drag current density is derived within the model of a zero-range potential in the effective mass approximation, and the spectral dependence of the drag current density is examined at different magnitudes of B and parameters of the quantum wire upon electron scattering by a system of impurities with short-range potentials. It is established that the spectral dependence of the drag current density exhibits a Zeeman doublet with a clear beak-shaped peak due to optical transitions of electrons from D^(?) states to states with the magnetic quantum number m=1. The possibility of using the photon drag effect in a longitudinal magnetic field for the development of laser radiation detectors is analyzed.     

Anomalous polarization dependence of the photon drag and optical rectification fields inn-type gallium phosphide

The photon drag and optical rectification response fromn-type gallium phosphide containing 2.4×10¹⁶ electrons cm^–3 has been studied using laser sources at 10.61 and 2.83m. By using different contact configurations, the existence of an additional electric field term in the propagation direction has been deduced. This field is shown to arise from the spatial derivatives of the photon drag and optical rectification field components caused by absorption of the radiation. The importance of this effect in detector design is considered.     

高光电探测效率CMOS单光子雪崩二极管器件

基于0.18μm CMOS工艺技术,制作了单光子雪崩二极管,可对650~950nm波段的微弱光进行有效探测.该器件采用P~+/N阱结构,P~+层深度较深,以提高对长光波的光子探测效率与响应度;采用低掺杂深N阱增大耗尽层厚度,可以提高探测灵敏度;深N阱与衬底形成的PN结可有效隔离衬底,降低衬底噪声;采用P阱保护环结构以预防过早边缘击穿现象.通过理论分析确定器件的基本结构参数及工艺参数,并对器件性能进行优化设计.实验结果表明,单光子雪崩二极管的窗口直径为10μm,器件的反向击穿电压为18.4V左右.用光强为0.001 W/cm~2的光照射,650nm处达到0.495A/W的响应度峰值;在2V的过偏压下,650~950nm波段范围内光子探测效率均高于30%,随着反向偏压的适当增大,探测效率有所提升.     

Photon-drag effect in a two-dimensional electron gas in high magnetic fields

We present the first measurements concerning the photon drag effect in a two-dimensional electron gas based on intersubband transitions in high magnetic fields. It is shown that the excitation mechanism of the drag voltage in a magnetic field differs obviously from the case of zero magnetic field. The longitudinal as well as the Hall drag voltage show strong oscillations around zero when the magnetic field is swept. Both consist of a B-symmetrical and an antisymmetrical part with the same periodicity in B as the magnetoresistanceR_xx. The drag voltage oscillations are strongly correlated to the relative position of Fermi energy and Landau levels and are independent of the photon energy in the range of usable laser lines.     

Spin photocurrents and the circular photon drag effect in (110)-grown quantum well structures

The study of spin photocurrents in (110)-grown quantum well structures is reported. The investigated effects comprise the circular photogalvanic effect and so far not observed circular photon drag effect. The experimental data can be described by an analytical expression derived from a phenomenological theory. A microscopic model of the circular photon drag effect is developed demonstrating that the generated current has a spin dependent origin. The text was submitted by the authors in English.     

Resonant Photon Drag of Dipolar Excitons

The theory of the photon drag of dipolar excitons in double-quantum-well nanostructures is presented. It is shown that the exciton-drag flux density features a resonant behavior if the photon frequency is close to some transition frequency in the discrete exciton spectrum. When the structure is irradiated with polarized light, the resonant enhancement of the drag current occurs when the photon energy coincides with the energy of an excited level of the exciton internal motion and the components of the angular momentum of internal motion in the initial and final states differ by one. The proposed effect can be used to control exciton transport in nanostructures based on a two-dimensional exciton gas.     

Towards higher sensitivity and lighter elements by collinear laser spectroscopy at isolde

New resonance detection mechanisms based on atom or ion counting instead of fluorescence photon detection have been introduced in collinear laser spectroscopy at ISOLDE. This increased the sensitivity by several orders of magnitude and allowed measurements on short-lived isotopes very far from stability, which are available in minor quantities only (≤10³ ions per second). Results of recent measurements on the medium mass and light elements Sr, Kr, Ca and Li are presented.