3 GHz, fundamentally mode-locked, femtosecond Yb-fiber laser

We demonstrate a fundamentally mode-locked Yb-fiber laser with 3?GHz repetition rate and ～206 fs pulse duration. The laser incorporates two enabling technologies: a 1?cm heavily Yb-doped phosphate glass fiber as the gain medium and a high-dispersion (-1300 fs²) output coupler to manage cavity dispersion. The oscillator self-starts and generates up to 53?mW average power.     

Spectral features of the interaction of femtosecond light pulses of different frequencies near the boundary of a Kerr medium

The interaction of probe ultraviolet (UV) and intense infrared (IR) pump pulses with a duration of 150 fs in a thin 2-mm-long sample of fused silica has been studied theoretically and experimentally. The spectra of UV radiation at the output of the sample have been measured depending on the time delay between the pulses at the sample input. The maximum shifts of the spectrum, attaining up to 0.22 nm for an IR power density of 3 × 10¹¹ W/cm², have been observed under conditions of coincidence of the pulses at the sample input and output, which corresponds to a predominant interaction of the probe radiation with the leading and trailing edges of the pump pulse near the boundary of the medium. The observed dependences are interpreted as a manifestation of the cross-phase modulation due to the Kerr nonlinearity of the medium and the dispersion of the group velocities of the UV and IR pulses. The numerical simulations performed taking into account these effects agree well with the experimental data.     

Nuclear fusion induced by a super-intense ultrashort laser pulse in a deuterated glass aerogel

A SiO₂ aerogel with absorbed deuterium is proposed as a target for the fusion reaction d + d → He³ + n induced by a superintense ultrashort laser pulse. The multiple inner ionization of oxygen and silicon atoms in the aerogel skeleton occurs in the superintense laser field. All the formed free electrons are heated and removed from the aerogel skeleton by the laser field at the front edge of the laser pulse. The subsequent Coulomb explosion of the deuterated charged aerogel skeleton propels the deuterium ions up to kinetic energies of ten keV and higher. The neutron yield is estimated at up to 10⁵ neutrons per laser pulse for ～200–500 ps if the peak intensity is 10¹⁸ W/cm² and the pulse duration is 35 fs.     

X-ray spectroscopic diagnostics of ultrashort laser-cluster interaction at the stage of the nonadiabatic scattering of clusters

X-ray spectroscopic diagnostics of laser-cluster interaction at the stage of nonadiabatic scattering of clusters and formation of a spatially uniform plasma channel has been performed. The experimental investigations have been carried out on a Ti:Sa laser setup with a pulse duration of about 65 fs and an energy up to 600 mJ. It has been shown that, within 10 ps from the beginning of a laser femtosecond pulse, the laser-cluster interaction forms a uniform plasma channel with a length of 0.4 to 1 mm with the parameters N _e ～ 10¹⁹?10²⁰ cm^?3 and T _e ～ 100 eV.     

SEM and Raman spectroscopy analyses of laser-induced periodic surface structures grown by ethanol-assisted femtosecond laser ablation of chromium

The effect of fluence and pulse duration on the growth of nanostructures on chromium (Cr) surfaces has been investigated upon irradiation of femtosecond (fs) laser pulses in a liquid confined environment of ethanol. In order to explore the effect of fluence, targets were exposed to 1000 pulses at various peak fluences ranging from 4.7 to 11.8?J?cm^–2 for pulse duration of ～25?fs. In order to explore the effect of pulse duration, targets were exposed to fs laser pulses of various pulse durations ranging from 25 to 100?fs, for a constant fluence of 11.8?J?cm^–2. Surface morphology and structural transformations have been analyzed by scanning electron microscopy and Raman spectroscopy, respectively. After laser irradiation, disordered sputtered surface with intense melting and cracking is obtained at the central ablated areas, which are augmented with increasing laser fluence due to enhanced thermal effects. At the peripheral ablated areas, where local fluence is approximately in the range of 1.4–4?mJ?cm^–2, very well-defined laser-induced periodic surface structures (LIPSS) with periodicity ranging from 270 to 370?nm along with dot-like structures are formed. As far as the pulse duration is concerned, a significant effect on the surface modification of Cr has been revealed. In the central ablated areas, for the shortest pulse duration (25?fs), only melting has been observed. However, LIPSS with dot-like structures and droplets have been grown for longer pulse durations. The periodicity of LIPSS increases and density of dot-like structures decreases with increasing pulse duration. The chemical and structural modifications of irradiated Cr have been revealed by Raman spectroscopy. It confirms the formation of new bands of chromium oxides and enol complexes or Cr-carbonyl compounds. The peak intensities of identified bands are dependent upon laser fluence and pulse duration.     

Behaviour of scintillators under XUV free electron laser radiation

Free electron lasers (FEL) are new generation accelerator-based short wavelength light sources providing high pulse intensity and femtosecond pulse duration, which enable investigation of interaction of elementary excitations in solids under extreme conditions. Using the FLASH facility of HASYLAB at DESY (Hamburg, Germany), we investigated the response of different materials with scintillating properties based on intrinsic emissions to the 25.6 and 13.8 nm FEL radiation by means of time-resolved luminescence spectroscopy. FLASH delivered single pulses of 25 fs duration having energy per pulse up to 30 μJ resulting in power densities of ～10¹² W/cm² on crystals. As a function of excitation density we observed the shortening of lifetime and non-exponential behaviour of emission decays in CaWO₄, while the emission spectra recorded are comparable to those obtained at conventional excitation sources.     

Generation of superintense femtosecond pulses by the Cr:forsterite laser system

A repetitively pulsed chromium-forsterite laser system is created. High-power femtosecond light pulses are generated at the fundamental (1.24 μm) and second-harmonic (0.62 μm) wavelengths. Theoretical analysis is performed to optimize the output pulse energy. Laser pulses with a duration of 110 fs, an energy of 1 mJ, and a repetition rate of 1–50 Hz are generated. The intensity of the focused beam is greater than 10¹⁶ W/cm². High-efficiency radiation conversion into the second harmonic is used to increase the energy contrast of the generated pulses. Original Text ? Astro, Ltd., 2006.     

Femtosecond ring all-fiber Yb laser with combined wavelength-division multiplexer-isolator

An original scheme of an all-fiber all-normal-dispersion ring mode-locked Yb laser is proposed and experimentally studied. A single fiber element serves as a wavelength-division multiplexer for the pumping radiation, an optical isolator, and a spectrally selective element for the radiation of the Yb laser. The output pulse duration is 900 fs, and the intracavity compression yields the pulses with a duration of 200 fs. The maximum laser power is 35 mW at a wavelength of 1070 nm.     

Generation of fast ions in femto-and picosecond laser plasmas at low intensities of the heating radiation

X-ray spectra from Teflon targets irradiated by laser pulses with a duration of 60 fs to 1 ps have been investigated experimentally. It is shown that, when the contrast of the laser pulse is sufficiently low, the effect of self-focusing of the main laser pulse in the plasma produced by the prepulse can significantly enhance the generation efficiency of fast particles. In this case, ions with energies as high as ～1 MeV are observed at relatively low laser intensities, q _las ≈ (4–6) × 10¹⁶ W/cm².     

Ar气中超连续谱产生的研究

采用中心波长为800nm,脉宽30fs的超快激光在Ar气池中产生了200—1000nm宽范围的超连续谱.通过改变激光脉冲的初始啁啾量、单脉冲能量、气体压强以及聚焦长度等条件,详细研究了获得稳定的超宽频谱的条件.结果表明,单脉冲能量为20mJ,附带29×10⁴fs²正色散的啁啾脉冲用f=50mm的凹面镜在15m长,23×10⁵Pa的Ar气中聚焦,得到稳定的频谱宽度达10³THz的超连续谱.还测量了光斑 关键词： 非线性效应 超连续谱 初始啁啾 光斑远场模式     

High-power Kerr-lens mode-locked Yb:YAG thin-disk oscillator in the positive dispersion regime

We demonstrate a self-starting Kerr-lens mode-locked (KLM) Yb:YAG thin-disk oscillator operating in the regime of positive intracavity group-delay dispersion (GDD). It delivers 1.7?ps pulses at an average power of 17?W and a repetition rate of 40?MHz. Dispersive mirrors compress the pulses to a duration of 190?fs (assuming sech² shape; Fourier limit: 150?fs) at an average power level of 11?W. To our knowledge, this is the first KLM thin-disk oscillator with positive GDD. Output powers of up to 30?W were achieved with an increased output coupler transmission and intracavity GDD. We demonstrate increase of the pulse energy with increasing positive intracavity GDD, limited by difficulties in initiating mode-locking.     

Dynamics of the strong field of a few-cycle optical pulse in a dielectric medium

The dependence of the conditions for the dominance of different physical factors in the self-action of few-cycle optical pulses in dielectrics on the intensity, duration, and spectrum of radiation has been theoretically analyzed. It is shown that the larger the pulse width and the central wavelength, the stronger the effect of plasma nonlinearity. For example, for a quartz glass in the field of pulses with a duration of 10 fs and a central wavelength of 780 nm, this nonlinearity mechanism is dominant at intensities exceeding 3 × 10¹³ W cm^?2.     

Femtosecond optical parametric converter in the 168–182-nm range

Femtosecond pulses continuously tunable in the vacuum ultraviolet (VUV) spectral range between 168 and 182 nm were generated using four-wave frequency mixing in an argon-filled capillary. The pulse energy reached 200 nJ at a pump-to-VUV conversion efficiency of 1%. The bandwidth at 181 nm was up to 27 THz corresponding to a transform limited duration of 17 fs. The upper limit in the shortest measured pulse duration was 75 fs.     

基于交叉偏振波产生的脉冲净化技术研究与应用

本文利用交叉偏振波产生技术(XPW)对800 nm波段钛宝石飞秒激光器输出的激光脉冲进行时域净化, 提高脉冲时域对比度, 并测量验证了10¹¹对比度的脉冲, 达到测量仪器的动态范围极限, 比初始脉冲时域对比度有三个量级的提高, XPW的效率为22%. 同时发现净化后脉冲光谱宽度也得到一定展宽, 进一步利用啁啾镜对和补偿片对净化后的脉冲进行色散补偿, 得到25 fs脉宽的脉冲. 利用该净化后的激光脉冲作为种子注入已有的太瓦级钛宝石啁啾脉冲放大系统中, 在输出脉冲能量250 mJ, 宽度50 fs, 对应峰值功率5 TW的情况下, 在主脉冲前100 ps以外的范围内测量验证了10¹¹的脉冲对比度.     

End-pumped Tm,Ho:NaY(WO<Subscript>4</Subscript>)<Subscript>2</Subscript> crystal laser at 2.07 μm

We presented an infrared laser output at 2.07 μm with Tm,Ho:NaY(WO₄)₂ crystal end-pumped by 795 nm laser diode at room temperature. The crystal was grown by the Czochralski method with the concentrations of 5 at % Tm³⁺ and 1 at % Ho³⁺. The highest output power was up to 2.7 W corresponding to the crystal temperature being controlled at 283 K. The overall optical conversion efficiency was 5.4% and the slop efficiency was 26%. The output characteristics and the laser threshold affected by the pulse duration and temperature have been studied. We found the stability of the output power was correlative with the crystal temperature heavily. In addition, the wider pulse duration of pump could promote the output power efficiently.     

Femtosecond laser ablation of cadmium tungstate for scintillator arrays

Ultrafast pulsed laser ablation has been investigated as a technique to machine CdWO₄ single crystal scintillator and segment it into small blocks with the aim of fabricating a 2D high energy X-ray imaging array. Cadmium tungstate (CdWO₄) is a brittle transparent scintillator used for the detection of high energy X-rays and γ-rays. A 6 W Yb:KGW Pharos-SP pulsed laser of wavelength 1028 nm was used with a tuneable pulse duration of 10 ps to 190 fs, repetition rate of up to 600 kHz and pulse energies of up to 1 mJ was employed. The effect of varying the pulse duration, pulse energy, pulse overlap and scan pattern on the laser induced damage to the crystals was investigated. A pulse duration of ≥500 fs was found to induce substantial cracking in the material. The laser induced damage was minimised using the following operating parameters: a pulse duration of 190 fs, fluence of 15.3 J cm⁻² and employing a serpentine scan pattern with a normalised pulse overlap of 0.8. The surface of the ablated surfaces was studied using scanning electron microscopy, energy dispersive X-ray spectroscopy, atomic force microscopy and X-ray photoelectron spectroscopy. Ablation products were found to contain cadmium tungstate together with different cadmium and tungsten oxides. These laser ablation products could be removed using an ammonium hydroxide treatment.     

Radiative characteristics of nitrogen upon excitation by volume discharge initiated by runaway electron beam

The amplitude, time, spectral, and energetic characteristics of a volume (diffuse) discharge at an elevated pressure (up to 5 atm) in a gap with an inhomogeneous electric field without an additional preionization source are studied. The concentration and temperature of electrons in the discharge plasma are mea-sured by spectral methods. The effective lifetime of the C ³Π _u state of the nitrogen molecule at the trailing edge of the radiation pulse is shown to be determined by radiative and collisional quenchings. For transitions of the second positive system of nitrogen, a plasma discharge radiation power into the complete solid angle is obtained to be ～120 kW, with a specific radiation power of up to ～50 kW/cm³.     

High-power pulse-periodic Nd3+-YAG laser with combined pumping by diode arrays

Output characteristics of the pulse-periodic solid-state laser pumped by diode arrays at a pump pulse repetition rate of 8...512 Hz were studied. Three pump types are used: longitudinal raster-lightguide, transverse, and combined ones. Diode arrays with a pulse power of ～800 W, emitting area sizes of 5 × 25 mm², and radiation divergence along two mutually perpendicular axes equal to 4° and 15°, respectively, were used as a pump source. The pump current pulse duration was varied within 100–350 µs. Three operating modes were studied: (i) free generation, (ii) passive Q-switch, and (iii) acousto-optic Q-switch ones. The lasing peak pulse power was (i) ～2 kW(free generation mode), (ii) ～1.5 MW (passive Q-switch mode), and (iii) ～100 kW (acousto-optic Q-switch mode). The highest average lasing power was 150 W at a pump pulse repetition rate of 512 Hz. The highest pulsed lasing energy was 0.65 J.     

Femtosecond oscillator on Yb:KYW crystal pumped by laser diode with fiber output

A femtosecond laser based on an Yb:KYW crystal with direct longitudinal pumping by a high-power semiconductor injection laser with a fiber output is described. Femtosecond pulses were generated in the self-longitudinal-mode-locking operating condition due to the use of a semiconductor saturable absorber. The average power of the oscillator was as high as 3.5 W at a central wavelength of 1035 nm, the pulse length and pulse repetition rate being 200 fs and 85.5 MHz, respectively. The product of the pulse length and the radiation spectrum width was 1.3 times higher than the theoretical limit for the pulse shape described by the function sech². The designed master oscillator can be also used as a stand-alone source of femtosecond radiation pulses for material microprocessing and primary source for femtosecond laser amplification systems.     

Generation of high-contrast and high-intensity laser pulses using an OPCPA preamplifier in a double CPA, Ti:sapphire laser system

We demonstrate a high-contrast, high-intensity double chirped-pulse amplification (CPA) Ti:sapphire laser system using an optical parametric chirped-pulse (OPCPA) pre- amplifier. By injecting cleaned microjoule seed pulses into the OPCPA, a temporal contrast greater than 10¹⁰ within picosecond times before the main femtosecond pulse is demonstrated with an output pulse energy of 1.7 J and a pulse duration of 30 fs, corresponding to a peak power of 60 TW at a 10 Hz repetition rate. This system uses a cryogenically-cooled Ti:sapphire final amplifier and generates focused peak intensities in excess of 10²⁰ W/cm².