Effect of infra-red irradiation on holographic recording in Bismuth silicon oxide

In this paper we discuss the effect of preliminary infrared (IR) irradiation on holographic recording in Bi₁₂SiO₂₀. The lighting has been found to give rise to an unusual dynamics of the diffraction efficiency. The diffraction efficiency of the hologram, recorded in the preliminary illuminated sample at low spatial frequencies (up to 1500 lines/mm) is eight times higher than that of the hologram, recorded without preliminary IR irradiation. At high spatial frequencies above 2000 lines/mm this additional lighting leads to an increase of the holographic sensitivity.     

Resonant Brillouin scattering via free and bound excitons in CdSe

We report resonant Brillouin scattering results in CdSe. Enhancements in Brillouin scattering have been observed at both the I₂ bound exciton and the free exciton. As a result of the spatial dispersion of the exciton-polariton, the Brillouin frequencies vary with the polariton energy. From this variation of the Brillouin frequencies, we deduced the following parameters in CdSe: transverse exciton frequency =14713 cm^?1, splitting between longitudinal and transverse exciton frequencies = 4cm^?1 and exciton effective mass (perpendicular to the c-axis) =0.40 times free electron mass. The Brillouin linewidths were found to vary with polariton energies in qualitative agreement with the theory of Brenig, Zeyher and Birman.     

Nonlinear interaction of moving space-charge and photoconductivity gratings in Bi<Subscript>12</Subscript>SiO<Subscript>20</Subscript> crystal

A nonlinear interaction of moving space-charge and photoconductivity gratings is experimentally investigated. In the presence of a dc electric field, a crystal is irradiated with an oscillating interference pattern with a spatial frequency K and an oscillation frequency ω. An ac electric field with a frequency \gM is also applied to the sample. At certain frequencies ω and \gM, the crystal exhibits two types of interacting oscillations: the space-charge grating moving with velocity |ω−Ω|/K and the photoconductivity grating moving with velocity −ω/K. The effect is studied using the method of the nonstationary photoelectromotive force in a photorefractive Bi₁₂SiO₂₀ crystal.     

Highly efficient hologram enhancement in Bi12TiO20 fibre-type crystal

Experimental results for two-wave mixing experiments in a single Bi₁₂TiO₂₀ fibre-type crystal at a wavelength of 632.8 nm under transverse a.c. electric field are reported. An exponential gain factor =4.7 cm^-1, which is much higher than the absorption coefficient (0.6 cm^-1), is obtained. It is observed that the signal beam enhancement is in fact signal beam depletion for spatial frequencies higher than F _B, which is determined by fibre geometry. An unusually strong dependence of response time on the recording beams intensities ratio reflects the nonlinearities of the multi-two-wave mixing process.     

A comparative study of FMR and Brillouin light scattering on amorphous Fe40Ni40B20

It is shown that magnetic surface mode frequencies in the amorphous ferromagnet Fe₄₀Ni₄₀B₂₀ measured using Brillouin light scattering depend upon the incident laser light intensity: presumably due to local heating of the specimen due to the concentration of the light flux into a focal spot only a few microns in diameter. Surface mode frequencies extrapolated to zero light intensity are shown to be consistent with magnetic parameters measured using ferromagnetic resonance at 35.731 GHz to within ±0.5 GHz for specimens of amorphous Fe₄₀Ni₄₀B₂₀. 0.5 GHz corresponds to a change of 0.17 kG in the saturation magnetization, 4πM_s.     

Effective room-temperature broad-band recording of 3D dynamic holograms in CdF<Subscript>2</Subscript>:Ga crystals

Photochromic CdF₂:Ga crystals with bistable impurity centers were effectively used for the dynamic recording of holograms and readout over the visible and near IR spectral regions at spatial frequencies of up to 5000 mm^?1 at room temperature. The diffraction efficiency of the dynamic holograms was as high as 60% at maximum and exceeded 1% when the beams’ intensities were in the ratio 1:100. As one goes from the low temperatures (≤200 K) to 300 K, the peak diffraction efficiency of the dynamic holograms decreases approximately by a factor of 1.5, while the speed of their response and photosensitivity in the long-wavelength spectral region increases by more than an order of magnitude. For the sake of comparison, the dynamic holograms were recorded under the same conditions as the widely used electrooptical SBN crystals. Comparative analysis ascertained a unique combination of the useful features offered by CdF₂:Ga crystals in holography.     

Spatial frequency dependence of the energy transfer in two-wave mixing experiments with BSO crystals

Energy transfer between two beams interfering in an electrooptic Bi₁₂SiO₂₀ crystal is analyzed as a function of the spatial frequency of the recorded hologram. We report high coefficients in a wide range of low spatial frequencies $\text{(Λ}{}^{-1}\text{?44 mm}{}^{-1}\text{)}$, when the drift length of the photocarriers becomes comparable to the fringe spacing. Exponential gain coefficients of Γ = 7 cm^-1 have been reached for high intensity beams ratio (β > 10⁴) and an optimized fringe displacement speed (moving grating recording). Application to coherent image amplification (×20) is shown.     

Josephson coupling and Fiske dynamics in ferromagnetic tunnel junctions

We report on the fabrication of Nb/AlO _x /Pd_0.82Ni_0.18/Nb superconductor/insulator/ferromagnetic metal/superconductor (SIFS) Josephson junctions with high critical current densities, large normal resistance times area products, high quality factors, and very good spatial uniformity. For these junctions a transition from 0- to π-coupling is observed for a thickness d _F @\simeq 6 nm of the ferromagnetic Pd_0.82Ni_0.18 interlayer. The magnetic field dependence of the π-coupled junctions demonstrates good spatial homogeneity of the tunneling barrier and ferromagnetic interlayer. Magnetic characterization shows that the Pd_0.82Ni_0.18 has an out-of-plane anisotropy and large saturation magnetization, indicating negligible dead layers at the interfaces. A careful analysis of Fiske modes provides information on the junction quality factor and the relevant damping mechanisms up to about 400 GHz. Whereas losses due to quasiparticle tunneling dominate at low frequencies, the damping is dominated by the finite surface resistance of the junction electrodes at high frequencies. High quality factors of up to 30 around 200 GHz have been achieved. Our analysis shows that the fabricated junctions are promising for applications in superconducting quantum circuits or quantum tunneling experiments.     

EPR lineshape study of the incommensurate phase in γ-irradiated K2SeO4

The temperature dependence of the SeO^4-₄ EPR frequencies and the asymmetric broadening of the EPR lines in the incommensurate phase of K₂SeO₄ can be explained by an incommensurate spatial modulation of the g tensors which corresponds to the “broad” phase soliton limit. A comparison between the experimental and calculated lineshape shows a ≈1% volume fraction of commensurate regions in the middle of the incommensurate phase at 110 K.     

Collective electronic excitations in a semiconductor superlattice in the Landau and Wannier-Stark ladder regime

Using a mean-field approximation, we have developed a systematic treatment of collective electronic modes in a semiconductor superlattice (SL) in the presence of strong electric and magnetic fields parallel to the SL axis. The spectrum of collective modes with zero wavevector along the SL axis is shown to consist of a principle magnetoplasmon mode and an infinite set of Bernstein-like modes. For non-zero wavevector along the SL axis, in addition to the cyclotron modes, extra collective modes are found at the frequencies |Nω _c±Mω _s|, which we call cyclotron-Stark modes (ω _c and ω _s are respectively the cyclotron and Stark frequencies, N and M are integer numbers). The frequencies of the modes propagating in “oblique” direction with respect to the SL axis show oscillatory behavior as a function of electric field strength. All the modes considered have very weak spatial dispersion and they are not Landau damped. The specific predictions made for the dispersion relations of the collective excitations should be observable in resonant Raman scattering experiments. Received 29 August 2002 / Received in final form 25 February 2003 Published online 4 June 2003 RID="a" ID="a"e-mail: 612033@inbox.ru     

Anomalous temperature dependence of the low-frequency vibrational density of states in vitreous B2O3

Inelastic neutron-scattering measurements of v-B₂O₃ reveal an upshift in energy of the first moment of the vibrational density of states for frequencies below ≈ 15 meV as temperature increases from 20 to 300 K. Such a stiffening is at odds with predictions based on some current approaches. Instead, the present result and related anomalies in specific heat and other microscopic and transport properties can be understood in terms of anharmonic motions at low frequencies. The atomic origin of the anharmonicity, and its consequence for the thermodynamical behavior are examined by molecular-dynamics simulations.     

In situ FTIR investigation of adsorption properties of sub-micron Cu2O-doped RuO2 sensing electrode of planar potentiometric pH sensor

In situ Fourier transform infrared spectroscopy (FTIR) was used to study adsorption properties of 20?mol% Cu₂O-doped RuO₂ sensing electrode (SE) screen-printed on the platinised alumina substrate of the planar electrochemical pH sensor and subsequently sintered at 800?°C. Morphology and properties of developed SEs were characterized by X-ray diffraction, scanning electron microscopy, atomic force microscopy and FTIR techniques. It was shown that both Cu₂O doping and changes in the sintering condition of the SE affected morphology and adsorption spectra of 20?mol% Cu₂O-doped RuO₂. Fundamental vibration frequencies of ruthenium?Coxygen bond at a temperature of 23?°C as well as region above fundamental frequencies for the sub-micron 20?mol% Cu₂O-doped RuO₂-SE were identified.     

Dielectric permittivity and AC conductivity investigations of the structural phase transitions in (NH3)2(CH2)7CdCl2Br2

The AC dielectric permittivity as a function of temperature (100–400 K) at different frequencies (between 80 Hz and 20 kHz) for the layered alkylene diammonium insulator containing Cd, namely, [(NH₃)₂(CH2)₇CdCl₂Br₂] has been measured. The formation of the compound was confirmed by microchemical analysis and IR absorption spectrometry. X-ray powder diffraction indicates an orthorhombic unit cell of dimensions: a = 10.219(2) Å, b = 9.168(2) Å and c = 38.694(4) Å. The AC conductivity ([sgrave]) is presented as a function of temperature and frequency. The conductivity and permittivity results indicate the presence of first-order phase transitions at 317 and 345 K. This has been confirmed by thermal analysis techniques. The activation energies were of values ranging between 0.15 and 0.62 eV depending upon the temperature range and the applied frequencies.     

Anomalies of elastic properties of layered materials

Acoustic investigations of layered crystals KY(MoO₄)₂ and glassy alloys Si₂₀Te₈₀ (with inclusions of nanocrystallites) are performed with the purpose of elucidating the character of binding forces in layered materials. The absorption and velocity of sound, as well as the spatial evolution of the spectrum of acoustic fluxes in various directions in wide ranges of temperatures (90–300 K), frequencies (14–1800 MHz), and intensities (0.04–100 W/cm²) of sound, are measured. Acoustooptical and pulse-echo methods were used for the measurements. A theoretical analysis of the data obtained has revealed anomalously large values of the nonlinear elastic coefficients and anharmonicity constants of longitudinal phonon modes that are determined by the anharmonicity of binding forces across the layers and at boundaries with nanocrystallites. It is shown that the anisotropy of the mechanical strength of layered crystals is to a large extent determined by the anharmonicity of binding forces.     

High frequency behaviours and Mssbauer study of field annealed FeCuNbSiB alloy ribbons

This paper investigates the high frequency behaviours and magnetic anisotropy of rapidly solidified FINEMET (Fe73.5Si13.5B9Nb3Cu1) alloy ribbons annealed in an applied magnetic field. It finds that the ribbons annealed with the applied magnetic field show much higher resonance frequencies and have even higher permeability at higher frequencies than the samples annealed without the magnetic field and the non-annealed ribbons. Mssbauer spectroscopy had been employed to study the spatial distribution of the magnetic moments of five selected FINEMET alloy ribbons in different heat-treated conditions. The results show that an easy plane has been established after annealling in the magnetic field, while for the other ribbons this effect is not significant. Hence, the relationship between magnetic field annealing and high frequency property has been bridged by the bianisotropic theory.     

Nonlinear interactions and scattering of space charge waves in sillenites

For the first time the effects of overall doubling, spatial doubling, and overall rectification of space charge waves in a photorefractive crystal (Bi₁₂GeO₂₀, BGO) have been detected and theoretically studied. The effects of overall doubling and overall rectification resemble second-harmonic generation and rectification of light in nonlinear optics. A good agreement between theory and experiment is found for the effect of spatial doubling, while for overall doubling and overall rectification effects only a qualitative agreement between theory and experiment has been established until now. Received: 13 July 2001 / Published online: 10 October 2001     

Photoacoustic study of the energy conversion in silicon photodiode

Conclusion Photoacoustic allows simple nondestructive and noncontact measurement of the photovoltaic energy conversion efficiency and internal quantum efficiency of the photodiode. We can also determine the responsivity of the photodiode.Using different frequencies we can obtain information about spatial distribution of heat generation and consequently about the processes within the sample.We also showed that the presented theory is valid only for low modulation frequencies (below 20 Hz).The frequency photoacoustic study concerning spatial distribution of heat sources in photodiodes is in progress and will be published separately later.We are very grateful to Petr Sladký for helpful discussions.     

Photorefractive Fourier transform profilometer for the measurement of 3-D object shapes

In the present work dynamic moiré-like fringe patterns, produced by photorefraction with low spatial frequencies, applied for profile determination of small objects is proposed. Basically, a Fourier transform profilometry technique is developed for an automated profile determination. This means, as far as we know, a new experimental procedure that exploits the real time holographic two wave mixing in Bi₁₂TiO₂₀ crystal sample. Besides, the mainly advantages of this procedure are, comparatively to the classical fringe projection method using the Michelson interferometer, best fringe pattern contrast, less speckle noise, absence of noises produced by spurious reflections and, the most significant, a pure sinusoidal shape obtained by dynamic holographic moiré-like process using photorefraction.     

Holographic digital data storage using phase-modulated pixels

We propose and demonstrate the use of phase images for holographic data storage. Use of phase images as input leads to uniform diffraction efficiency of multiplexed data pages. Use of binary phase-based data pages with 0 and π phase changes produces uniform spectral distribution at the Fourier plane. This in turn facilitates better recording of higher spatial frequencies. We experimentally demonstrate a phase-based holographic data storage system using shift multiplexing in a Fe:LiNbO₃ crystal, and use it for associative retrieval. Preliminary studies indicate high discrimination capabilities of phase-based holographic data storage system over the amplitude-based system in a content-addressable memory.     

Frequency dependent kinetics of the cw CO2 laser induced reaction of CF3Br

Kinetics of the decomposition of CF₃Br at 20 torr by a cw CO₂ laser have been studied over the range of laser frequencies 1043–1085 cm^-1. At constant translational temperature the change in the rate constant with laser frequency over the frequency range is a factor of 500, comparable to the effect previously observed in CF₂ClCF₂Cl and CF₃CF₂Cl. Arrhenius plots show an activation energy of 64.9 kcal/mole, independent of frequency. The laser induced optical absorption of CF₃Br exhibits a hysteresis effect at the lower laser frequencies.