裂变产物产额数据的评价

以中子诱发235U裂变产生的135Xe 的累积产额数据为例, 利用了所有可利用的实验数据, 介绍了裂变产物产额数据的评价方法, 包括数据的收集、 修正、 评价、 误差调整和数据处理, 特别是协方差数据的评价、 半经验模型理论计算数据的应用和相关数据的处理, 给出了135Xe热能点产额的推荐值以及0～20 MeV产额-能量关系曲线。 Takeing 135Xe produced by neutron induced fission of 235U as an example, the evaluation method for fission yield was introduced using the all experimental data available. The evaluation procedure includes the experimental data collection, correction, evaluation, error assessment and data analysis. The study of the uncertainty covariance, application of semi empirical theoretical calculation and the yield energy dependence of 135Xe in the incident energy range 0~20 MeV were emphasized in this work.     

n+233U裂变碎片质量分布的唯象模型研究

本模型基于裂变多通道无规颈断裂模型,考虑宏观液滴能、壳效应能以及壳效应与温度的关系,得到参数化的势能表示形式。通过拟合不同测量方法得到的实验数据(经过评价) 获得3 组模型参数。3 组参数计算的碎片质量分布均很好地再现了不同能点的实验数据,除了基于动能法实验数据得到的参数外,其14 MeV的计算结果与实验数据符合较差。研究发现,不同入射中子能量的裂变碎片质量分布有4 个主要交叉点,在叉点之上的产额随入射中子能量增加减少,之下的产额则随入射中子能量上升;内侧(或外侧) 的两个交叉点质量数之和近似等于裂变复合核的质量数;不同裂变系统的重峰左侧的交叉点都保持在132 附近。Present model was based upon Brosa model, where macro energy,shell effect energy and its decreasing with system temperature were considered and parameterized. 3 sets of model parameters were obtained by fitting to 3 groups of evaluated experimental data, respectively, where the groups were classified by measured method: radiochemistry (RA) method, double kinetic energy (KE) method, and both (ALL). All the 3 sets of parameters could well reproduce themeasured mass distributions on different energies, except the KE set on 14 MeV. The result shows the mass distributions mainly had 4 trend turning points, above which the yield decreasing and below which the yield increasing with energy.The sum of the 1st and 4th (or 2nd and 3rd) point positions was equal to the compound nuclei mass approximately. And the 3rd point was kept at ~132 constantly for different fission systems n+233 U, n+235U, n+233Pu.     

轻中等质量核非对称裂变研究的新进展

介绍了轻中等质量核非对称裂变研究的新进展.通过对64,58Ni+12C和78,82,86Kr+12C反应复杂碎片的激发函数测量,发现流行的转动液滴模型和转动有限力程模型均不能复现实验的非对称裂变位垒数据.The excitation functions were measured for complex fragments with atomic number Z=4—25 emitted from the compound nuclei~(70,76)Se and~(90,94,98)Mo produced in the reactions~(64,58)Ni+~(12)C and~(78,82,86)Kr+~(12)C. The extracted mass asymmetric fission barriers have been compared with those calculated from macroscopic nuclear models.     

中子诱发232Th裂变初始碎片质量及动能分布Monte-Carlo研究

随着第四代反应堆以及先进核能利用系统的发展,对中子核数据提出了高精度、多核素、宽能区的新要求.目前,中国核数据评价库(CENDL库)中相关核裂变的数据较缺失,不足以满足当前核能发展的需求.因此,建立面向中子核数据需求的可靠计算方法和工具变得极为重要.本文基于Monte-Carlo方法建立了裂变碎片质量动能计算模型,研究了中低能中子诱发²³²Th(n,f)反应发射中子前裂变碎片的分布特性.对于裂变碎片质量分布,本模型计算结果与实验值最大偏差约1%,与GEF, TALYS程序计算结果 (与实验值最大偏差约2%)相比具有一定优势.对于发射中子前裂变碎片动能分布,本模型计算结果与实验数据一致.结果表明,所发展的计算模型能够较好地预测²³²Th(n,f)反应发射中子前裂变碎片数据,为中子诱发锕系核裂变反应计算提供一种新思路.     

238U(n,f)短寿命产物核累积产额的评价(英文)

为满足堆内或核爆中链式反应过程的燃耗值的计算需要，对裂变谱中子和14MeV中子诱发238U裂变的短寿命产物核的累积产额进行了评价。评价利用了所有可利用的实验数据， 经物理分析后， 使用AVERAGE程序加权平均， 用ZOTT程序进行同时评价， 给出了所要求能点的唯一最佳推荐数据， 并将评价结果与ENDF/B-VII， JEF-2.2， JENDL-3.2和CENDL-2的推荐数据进行了比较。 评价结果将用于CENDL-2的更新与升级。For reliable and consistent nuclear calculation, the cumulative yields for short lived fission products are evaluated based on the available experimental data for 238U fission induced by fission spectrum neutrons and ~14 MeV neutrons. The data are processed using codes AVERAGE for weighed average and ZOOT for simultaneous evaluation. The evaluated data are compared with those in the major international nuclear data libraries, including ENDF/B-VII, JEF-2.2, JENDL-3.2 and CENDL-2. The present evaluation will be used to improve and update the CENDL-2 library.     

Gammasphere上裂变丰中子核核结构若干前沿领域的新进展(Ⅰ:第一和第二部分)(英文)

(第一和第二部分):使用Gammasphere多探测器系统对252Cf裂变源瞬发γ射线进行γ-γ-γ和γ-γ(θ)符合测量,裂变丰中子原子核核结构若干前沿领域的深入研究获得了新的进展。高达5.7×1011以上的三重和更高重符合事件的数据统计,以及更少压缩的三维数据为宽广未知丰中子核区的寻找和研究提供了有利的条件。在具有重要物理意义的若干丰中子核区首次建立,或显著扩展了一批包括转晕态和转晕附近能态的高自旋能级纲图。在偶-偶丰中子核110,112Ru和108Mo中鉴别出了手征对称破缺结构。丰中子110,112Ru附近核的三轴形变基态具有最低的能量,在它们之中已确认了接近最大值的三轴形变。在这些Ru和Mo同位素中观察到的手征双线能带展示出手征破缺的一切特征,特别是其理想的能量简并,表明它们在迄今已报道的手征破缺结构中,具有最好的手征特性。研究了手征结构从具有γ软度的108Ru到具有大三轴形变的110,112Ru的过渡。斜轴推转(TAC)和随机相近似(RPA)理论计算成功地拟合了在这些偶-偶丰中子核中观察到的手征双线能带的特性,并指定其为软手征振动态。在这些偶-偶核中观察到的手征破缺不可能归纳为奇-奇核中那样的简化的几何图像。前者来自闭壳外所有中子的相互作用。对双幻核132Sn附近N=83同中素链的系统研究为这个极富吸引力的核区提供了大量新的谱学信息。N=83同中素135Te(Z=52),136I(Z=53),137Xe(Z=54),138Cs(Z=55)和139Ba(Z=56)的最新能级信息,特别是首次建立的138Cs高自旋能级纲图和壳模型理论计算表明,Z=50质子闭壳外少数g7/2价质子激发同N=82中子闭壳外之唯一f7/2价中子的耦合对该核区能级结构具有关键作用。观察到了132Sn和208Pb附近核区谱学信息的相似性和相对应的三粒子和五粒子态。在135Te中观察到了磁转动,这是在双幻核132Sn附近观察到的首例磁转动。     

Subbarrier Complete Fusion-Fission Reactions of 16)O+232Th

We have succeeded in isolating the complete arising from complete fusion-fission in terms of the fragment folding angle technique,and measured complete fusion-fission cross sections and fragment angular distributions for the ¹⁶O+²³²Th system in the center-of-mass energies between 72.61 and 80.11 MeV.The observed fission excitation function is in quite good agreement with the expectation of the coupled-channels theory.However,the measured fragment angular distributions are more anisotropic than the predictions of both the saddle-point transition-state model and scission model.     

CHARGE DISTRIBUTION IN THE FISSION OF 232Th BY 14MeV NEUTRON

Independent yields of ⁸²Br, ⁹⁶Nb, ¹¹²Ag, ¹³⁰I,¹³²I, ¹³⁴I, ^134mCs, ^135mCs, ¹³⁶Cs and upper limitof independent yield for ¹⁴⁰La in the fission of ²³²Th induced by neutrons of 14 MeVwere determined with nuclear chemistry techniques. The correlation of the fractionalindependent yields in the high yield mass chains with a Gaussian curve of charge dis-tribution has been investigated using various mass formulae and charge distributionhypotheses. The results indicate that the hrpothesis of minimum potential energy witha shell-effected mass equation gives the best fit to the data. The width parameter Cof the charge distribution is found to be 0.80. The large deviations of ³²Br and ¹¹²Ag from the Gaussian curve seem to show that the low yield in very asymmetric fissioncan be attributed to a narrower width of charge distribution, whereas the high yield insymmetric fission may correlate with a wider width. The trends have been explainedqualitatively in terms of a liquid drop model. There is no evidence for 40-proton subshell effect on the fission yield.     

Identification of New Isotope 238Th

Unreported heavy neutron-rich nuclide ²³⁸Th has been produced via a multinucleon transfer reaction by 60MeVIu ¹⁸0 ions bombardment of natural uranium.Thorium was radiochemically separated from the mixture of uranium and reaction products. ²³⁸Pa as a daughter nucleus of ²³⁸Th has been identified according to the growth and decay of ²³⁸Pa γ rays which has been observed. The half-life of ²³⁸Th was determined to be (9.4 + 2.0) min. At the same time, a new γ ray of (89.0 + 0.3) keV with T_1/2= (8.9 + 1.5)min was found in the γ spectrum gated with the K_α1, X ray of Pa and assigned to ²³⁸Th decay based on the measurements of its transition energy and the half-life.

     

A New Heavy Neutron-rich Isotope 238Th

A new nuclide ²³⁸Th has been produced via multinucleon transfer reaction induced by 60MeV/u ¹⁸O ion irradiation of natural uranium. The thorium was radiochemically separated from the mixture of uranium and its reaction products. The activity of thorium was measured by using a HPGe detector and a planar HPGe detector. The ²³⁸Th has been identified for the first time by measuring the growth and decay of the γ-rays from its daughter ²³⁸Pa. The half-life of 238Th was determined to be (9.4±2.0)min. In addition,a new (89.0±0.3)keV γ-ray with T_1/2=(8.9±1.5)min was observed and assigned to ²³⁸Th decay based on the measurement of transition energy and half life.     

Temporal variation of fundamental constants in 229Th transition

If is there enhanced sensitivity to variations of fine structure constant, nucleon mass and meson masses in the transition between the low energy and long-lived nuclear isomer and ground states? To answer this open problem, we investigate the transition between the long-lived 7.6±0.5 eV isomer and ground states in ²²⁹Th based on the formulae derived from both the Nilsson model and Feynman-Hellmann theorem. Consistent conclusions are drawn by these two method. The sensitivity to relative variation of fine structure constant could be enhanced by 3—4 orders of magnitude, and to variations of nucleon mass and meson masses are enhanced by about 5—6 orders of magnitude in the ²²⁹Th transition.     

46.7MeV/u 12C轰击159Tb、197Au和209Bi的裂变测量及分析

用46.7MeV/u~(12)C轰击~(159)Tb、~(197)Au、~(209)Bi,测量关联裂片的速度和角度,研究了线性动量转移(LMT)、质量和出平面角分布,提取了核温度,应用级联两体统计衰变理论进行了拟合与解释,结果表明:在～50MeV/u入射能的中能重离子碰撞中,以非完全熔合方式形成了核温度高达4～5MeV的类复合核,其后通过裂变、蒸发级联统计两体衰变而退激。 The velocities and angles of fission partners emitted from reactions in ~(12)C+~(159)Tb, ~(197)Au,~(209)Bi systems with bombarding energy of 46.7MeV/u are measured. The linear momentum transferfrom projectile to target、mass and out-of-reaction plane angle distributions of fission fragments arestudied, and the temperatures of the target residues are extracted. These results have been explained by statistical binary decay model. It seems that the compound-likesystem with high temperature...     

Possible Mechanisms of Ternary Fission in the 197Au+197Au System at 15 A MeV

Ternary fission in ^197Au＋^197Au collisions at 15 A MeV is investigated by using the improved quantum molecular dynamical （ImQMD） model. The experimental mass distributions for each of the three fragments are reproduced for the first time without any freely adjusting parameters. The mechanisms of ternary fission in central and semicentral collisions are dynamically studied. In direct prolate ternary fission, two necks are found to be formed almost simultaneously and rupture sequentially in a very short time interval. Direct oblate ternary fission is a very rare fission event, in which three necks are formed and rupture simultaneously, forming three equally sized fragments along space-symmetric directions in the reaction plane. In sequential ternary fission a binary division is followed by another binary fission event after hundreds of fm/c.     

Measurement of L X-Ray Intensity Ratios for^92U and ^90Th Elements Using Photoionization in an External Magnetic Field

L x-ray intensity ratios Le/Lγ, Lα/L7 and Lβ/Lγ for ^92U and ^90Th are measured by using 59.5keV incident photon energy at 110° and 125° scattering angles. The samples are located in the external magnetic field of intensities ±0.15T, ±0.30T, ±0.45T, ±0.60T and ±0.75T. The experimental results obtained for B = 0 are compared with the theoretical values calculated using Scofield＇s tables based on the Hartree Slater theory. The contribution to the alignment of the external magnetic field is discussed. It is observed that the L x-ray intensity ratios decrease with the increasing magnetic field intensity.