Generation of harmonics of intense laser radiation in a transparent collisionless plasma

The spectral composition of a relativistically strong uniform nonlinear electromagnetic wave in a transparent collisionless plasma is analyzed. The vortex and potential components of the wave field are shown to contain only odd and even harmonics, respectively; in a transparent plasma, the wave remains quasi-monochromatic, since the intensities of the harmonics decrease exponentially with increasing harmonic number. An equation that includes diffraction effects is derived to describe the propagation of wavepackets. The results obtained are compared with experimental data.     

Generation of harmonics in a Compton laser

We have calculated the gain factor of the electromagnetic radiation at the harmonics, divisible by the scattering frequency, in a Compton laser for an electron beam with angular spread. We have also investigated polarization effects.     

Generation of higher harmonics in laser plasma formed on the surface of a silver target

The results of investigation of the higher harmonics (from the 21st to the 61st order) of radiation of a femtosecond laser (793 nm, 48 fs) that are generated in silver plasma are presented. The changes in the shape and spectra of harmonics for different chirps of the laser radiation are studied. It is found that the wavelengths of harmonics generated in the region of the plateaulike distribution of the converted radiation intensity can be tuned. It is shown that the conditions of phase matching between harmonics and laser radiation are different for different modulations of the femtosecond pulse spectrum. The tuning range of the spectrum of the converted radiation in the region of lower harmonics, which lie in the beginning region of the plateau, is shown to amount to 0.8 nm.     

Generation of higher harmonics of femtosecond radiation in clusters

The frequency conversion of laser radiation in cluster media is studied by the method of laser ablation of surfaces containing different nanoparticles (Cr₂O₃, In₂O₃, Ag, Sn, Au, and Cu). Using plasma that contains In₂O₃ nanoparticles as an example, it is shown that the resonant amplification of certain harmonics in the plateau-like distribution of harmonics, which is characteristic of the ablation of certain solid targets, is considerably modified in the case of targets that contain cluster formations. An increase in the conversion efficiency to harmonics in nanoparticle-containing media is discussed. In order to determine optimal characteristics of laser plasma with nanoparticles, their morphology is studied before and after laser ablation.     

Generation of whistler mode in a relativistic plasma

This paper contains the plasma maser interaction between high frequency nonresonant whistler R-mode and low frequency resonant ion acoustic mode in a relativistic plasma. It shows that the whistler R-mode grows through the plasma maser interaction between the relativistic electrons and the ion acoustic fluctuation.      

Generation of higher harmonics of laser radiation in plasma formed by pulses with a 1-kHz repetition rate

Studies of higher-order nonlinearities in plasma plumes by the method of higher-harmonic generation (HHG) upon laser ablation of different materials by pulses with a repetition rate of 1 kHz are reviewed. It is shown that an increase in the pulse repetition rate compared to the previous works on HHG in plasma using lasers with a pulse repetition rate of 10 KHz considerably increases the average power of converted radiation in the far-ultraviolet (FUV) region. The review considers the results of works on the interference of quantum trajectories of accelerated electrons, two-color pumping, HHG in graphite plasma, HHG in gases compared to HHG in plasma plumes, resonant enhancement of harmonics, and stabilization of the output parameters of radiation converted in plasma. It is shown that the new methods of optimization of the HHG process considerably increase the potential of the use of coherent FUV radiation owing to the improvement of some characteristics of harmonics in plasma generated by pulses with a high repetition rate.     

Selection of odd or even harmonics by a multi-color laser field with macroscopic phase-matching

We experimentally and theoretically demonstrate that the property(odd or even) of generated harmonics can be selected by manipulating the macroscopic phase-matching conditions based on a three-color laser field. Only odd or even harmonics can be made dominant by changing the focal position and adjusting the gas pressure. These results indicate that the odd-even property of the generated harmonics can be controlled by using the multi-color laser field with macroscopic phase-matching.     

High-order optical vortex harmonics generated by relativistic femtosecond laser pulse

Harmonics generated by an intense femtosecond Gaussian laser pulse normally incident on a spiral-shaped thin foil target were studied.By using two-dimensional(2D) particle-in-cell(PIC) simulation,we observed evident odd harmonics signals in the reflection direction and found that the reflected field has a helical structure determined by the target shape.This method provides a new way to generate an intense ultraviolet vortex with high-order topological charge by use of ultrahigh intense laser-driven harmonics.     

Generation of energetic electrons and ions by interaction of relativistic laser pulses with a supercritical plasma

Generation of hot electrons and fast ions under the action of a relativistic femtosecond laser pulse propagating through a supercritical-density plasma is studied in terms of the kinetic theory by constructing propagators for plasma particle distribution functions. Calculations are carried out for different laser pulse intensities, different sorts of multicharged ions, and different degrees of plasma inhomogeneity. Mechanisms of electron and ion acceleration in the plasma are explored.     

Polarization of the high harmonics of radiation in a laser plasma

The polarization of the high harmonics generated in plasmas by the bremsstrahlung of electrons oscillating under the influence of high-power plasma-heating electromagnetic radiation is described on the basis of a simple model of a cold plasma. It is shown that when the polarization of the heating radiation differs from plane polarization by a small but finite amount, the high harmonics are generated with almost perpendicular polarization, and the degree of circular polarization of the harmonics increases with the number of the harmonic. Pis’ma Zh. éksp. Teor. Fiz. 67, No. 5, 313–316 (10 March 1998)     

Generation of higher-order harmonics of chirped radiation from a titanium-sapphire laser in plasma generated by pulses of different durations

The frequency conversion of laser radiation in plasma created by pulses of different durations under conditions of the chirp variation of the radiation to be converted is investigated. It is shown that the chirp variation of the laser pulse during the generation of higher-order radiation harmonics of the femtosecond laser leads to a considerable change in the brightness, wavelength shift, and maximal order of generated harmonics. The long-and short-wavelength shifts of harmonics observed in these studies are attributed to the manifestation of a considerable concentration of free charge carriers in the plasma, as well as the self-modulation of the laser pulse. The generation of plasma by pulses whose durations vary from 160 fs to 20 ns is considered and it is shown that the generation efficiency of harmonics depends to a greater extent on the energy of the heating prepulse than on its intensity on the surface of a target to be ablated. The effect that the atomic number of the target has on the formation of optimal plasma at different delays between the heating prepulse and the femtosecond pulse to be converted is discussed.     

Generation of a continuum and stimulated Raman scattering harmonics during scattering of electromagnetic radiation of relativistic intensity

A theory of the propagation instability of plane, monochromatic, circularly polarized electromagnetic waves of relativistic intensity in matter is developed for a spatially three-dimensional geometry including arbitrary polarization of the scattered radiation. Harmonic generation owing to striction and relativistic nonlinearity is examined, as well as scattering owing to electron recoil, the decay instability of the harmonics with formation of scattered electromagnetic waves (Stokes components of the stimulated Raman scattering and plasmons), the interaction of electromagnetic waves in the plasma (antistokes stimulated Raman scattering), and the generation of a radiative continuum. The transition of the three-dimensional theory to a one-dimensional problem in the nonrelativistic limit is discussed. Zh. éksp. Teor. Fiz. 113, 2034–2046 (June 1998)     

On self-focusing of an ultrashort intense relativistic laser pulse in a plasma

The development of the spatiotemporal (filamentation) instability of a laser pulse upon excitation of a plasma wave is studied numerically and analytically. It is shown that first, as in a medium with inertialless cubic nonlinearity, the filamentation of radiation occurs and then filaments are attracted to each other. The following evolution differs weakly from the evolution of a smoothed wave beam in a medium with inertial nonlinear response.     

Electron impact ionization of atomic clusters in ultraintense laser fields

In this paper we report on inner ionization of Xe_n clusters (n = 55- 2171) in ultraintense Gaussian laser fields (peak intensity I = 10¹⁵- 10²⁰ Wcm^-2, pulse width τ= 25 fs, frequency 0.35 fs^-1). The cluster inner ionization process is induced by the barrier suppression ionization (BSI) mechanism and by electron impact ionization (EII), which occurs sequentially with the BSI. We address electron impact ionization of clusters, which pertains to inelastic reactive processes of the high-energy (100 eV–1 keV per electron) nanoplasma. We utilized experimental data for the energy dependence of the electron impact ionization cross-sections of Xe^j+ (j = 1-10) ions, which were fit by an empirical three-parameter Lotz-type equation, to explore EII in clusters by molecular dynamics simulations. Information was obtained on the yields and time-resolved dynamics of the EII levels (i.e., number n_imp of electrons per cluster atom) in the Xe_n clusters and their dependence on the laser intensity and cluster size. The relative long-time (t = 90 fs) yields for EII, n_imp/n_ii (where n_ii is the total inner ionization yield) are rather low and increase with decreasing the laser intensity. In the intensity range I = 10¹⁵-10¹⁶ Wcm^-2, n_imp/n_ii = 0.21 for n = 2171 and n_imp/n_ii = 0.09-0.14 for n = 459, while for I = 10¹⁸-10²⁰ Wcm^-2, n_imp/n_ii = 0.01-0.05. The difference Δn_imp between the EII yield at long time and at the termination of the laser pulse reflects on ionization dynamics by the nanoplasma when the laser pulse is switched off. For Xe₂₁₇₁ in the lower intensity domain, Δ n_imp = 0.9 at I = 10¹⁵ Wcm^-2 and Δn_imp = 0.4 at 10¹⁶ Wcm^-2, reflecting on EII by the persistent nanoplasma under “laser free” conditions, while in the higher intensity domain of I = 10¹⁷ - 10¹⁸ Wcm^-2, Δn_imp is negligibly small due to the depletion of the transient nanoplasma.     

Parametric generation of even polarization harmonics in a cubic nonlinear layer

The response of a cubic nonlinear medium to the action of a short-duration laser pulse is considered in the case in which the frequency of the optical radiation is close to the frequency of linear oscillators of the medium. It is shown that it is possible to realize parametric generation of even harmonics under the action of a high-intensity femtosecond pulse (with an amplitude exceeding some critical value), which leads to the formation of a supercontinuum at a certain duration and intensity of the incident pulse.     

Generation of the fifth and sixth harmonics of iodine laser pulses

High-power coherent radiation at 263 nm and 219 nm was generated by converting iodine laser pulses (λ = 1.315 μm) into fifth- and sixth-harmonic radiation. For 5ω-generation 3ω and 2ω were mixed in a KDP crystal. 6ω was produced by second-harmonic conversion of 3ω radiation in a KPB crystal.     

Features of femtosecond laser pulse reflection from a sharp boundary of relativistic laser plasma

The features of femtosecond laser pulse reflection from a plasma target of near-critical density were analytically and numerically studied in a wide range of laser pulse intensities and durations. Based on analytical calculations, it is shown that the pulse reflectance at a constant intensity decreases with decreasing pulse duration. Based of numerical simulation results, it is shown that, as a superintense femtosecond laser pulse is incident on a plasma layer with a concentration close to the critical one, a quasi-periodic electron-density structure is formed in the plasma bulk, which can both increase and decrease the the laser pulse reflectance.