Activation cross-sections of titanium isotopes at neutron energies of 13.5–14.8 MeV

The cross-sections for ~(46) Ti(n,2 n)~(45) Ti, ~(46) Ti(n,p)~(46 m+g) Sc+~(47) Ti(n,d*)~(46 m+g) Sc, ~(46)Ti(n,p)~(46 m+g) Sc, ~(47) Ti(n,p)~(47) Sc+~(48) Ti(n,d*)~(47) Sc, ~(47) Ti(n,p)~(47) Sc, ~(48) Ti(n,p)~(48) Sc+~(49) Ti(n,d*)~(48) Sc,~(48) Ti(n,p)~(48) Sc, and ~(50) Ti(n,α)~(47) Ca reactions were investigated around neutron energies of 13.5–14.8 Me V by means of the activation technique. Fast neutrons were produced by the~3 H(d,n)~4 He reaction. Neutron energies from different directions in the measurements were obtained in advance using the method of cross-section ratios for ~(90) Zr(n,2 n)~(89 m+g) Zr and ~(93) Nb(n,2 n)~(92 m) Nb reactions. The results obtained are analyzed and compared with the experimental data provided by the literature and verified nuclear data in the JEFF-3.3,CENDL-3.1, ENDF/B-VIII.0 libraries, as well as results calculated by Talys-1.9 code.     

Study of even-mass Ba nuclei by the (p,t) reaction

The (p, t) reaction on the nuclei ^{134, 136, 138}Ba has been studied at a bombarding energy of 52 MeV. Angular distributions of emitted tritons were obtained between 6° and 60°. The following six negative-parity states were strongly excited by the (p, t) reaction: 5^?(2.121 MeV) and 7^?(2.482 MeV) in ¹³²Ba, 5^?(1.998 MeV) and 7^?(2.274 MeV) in ¹³⁴Ba, and 5^?(2.139 MeV) and 7^?(2.031 MeV) in ¹³⁶Ba. DWBA calculations using the code DWUCK successfully reproduce these angular distributions. The 0⁺ assignment to the 1.761 MeV level in ¹³⁴Ba is confirmed. Intensities of the (p, t) reaction for low-lying states are discussed.     

Selectivity of the 16O(7Li, α) reaction and states with (sd)3 and (sd)2(fp)1 configurations in 19F

The ¹⁶O(⁷Li, α)¹⁹F reaction has been studied at 35 MeV up to 11 MeV excitation energy. Comparison with the ¹⁶O(⁶Li, ³He)¹⁹F and ¹⁶O(⁶Li, t)¹⁹Ne reactions shows very good agreement up to 5.5 MeV excitation energy and large differences at higher excitation energies which can be explained by different angular momentum matching conditions in the different reactions. The identification of mirror states in A = 19 and of states with (sd)³ and (sd)² (fp)¹ configurations in ¹⁹F are discussed.     

Nuclear-matter radii of 7Be and 7Li and astrophysical S-factors for radiative alpha-capture reactions

The nuclear-matter radii of ⁷Be and ⁷Li measured in high-energy heavy-ion reactions have been calculated and applied to the estimate of astrophysical S-factors for the ³He(α,γ)⁷Be and ³G(α,γ)⁷Li reactions. The absolute S(O) values in the KeV b are constrained to be 0.36<S(0)<0.63 and 0.083<S(0)<015 for the ³He(α,γ)⁷Be and ³H(α,γ)⁷Li reactions, respectively.     

Cross sections for proton induced reactions on 41K and for the reaction 62Ni(α, p)65Cu

Excitation functions have been measured for ⁶²Ni(α, p)⁶⁵Cu in the energy range 6.5–9.0 MeV, for ⁴¹K(p, α)³⁸Ar in the range 0.8–2.6 MeV, for ⁴¹K(p, γ)⁴²Ca, ⁴¹K(p, αγ)³⁸Ar, ⁴¹K(p, nγ)⁴¹Ca, and ⁴¹K(p, p'γ)⁴¹ in the range 0.6–4.0 MeV, and for ⁴¹K(p, n)⁴¹Ca from threshold to 3.0 MeV. Cross sections have been extracted from the data and these are compared with statistical-model calculations based on global optical model parameters. Alternative parameter sets have been tried for the ⁶²Ni(α, p)⁶⁵Cu data and published data for ⁶²Ni(α, γ)⁶⁶Zn and ⁶²Ni(α, n)⁶⁵Zn, and both these and the global parameters have been used in statistical-model calculations of ⁶⁵Cu(p, γ)⁶⁶Zn, ⁶⁵Cu(p, n)⁶⁵Zn and ⁶⁵Cu(p, α)⁶²Ni cross sections, which are compared with published data for these reactions. Both the global and the alternative parameters lead to very good agreement with experiment for all six reactions. Alternative parameters have been tried for the ⁴¹K + p reactions also. The global parameters lead to agreement to within a factor of 2 and the alternative parameters lead to agreement to within a factor of 1.3. The ⁴¹K + p alternative parameters are used in calculations of ⁴¹Ca(n, γ)⁴²Ca, ⁴¹Ca(n, p)⁴¹K and ⁴¹Ca(n, α)³⁸Ar cross sections, and these and the experimental ⁴¹K + p data are used in calculations of thermonuclear reaction rates under stellar conditions for the ⁴¹Ca + n and ⁴¹K + p reactions.     

Ground and γ-vibrational bands in even Os isotopes (A = 182–188) studied by (α, χnγ) and (p, χnγ) reactions

Gamma rays following ¹⁸²W(α, 2n)¹⁸⁴Os, ¹⁸⁴W(α, 2n)¹⁸⁶Os, ¹⁸⁶W(α, 2n)¹⁸⁸Os, ¹⁸⁵Re (p, 2n)¹⁸⁴Os, ¹⁸⁵Re(p, 4n)¹⁸²Os, ¹⁸⁷Re(p, 2n)¹⁸⁶Os and ¹⁸⁷Re(p, 4n)¹⁸⁴Os reactions have been measured to study the ground and γ-vibrational bands in even Os isotopes (A = 182–188). In addition to the ground-state levels the γ-vibrational bands have been identified up to the 5⁺ members. The K = 4 band head is proposed in ¹⁸⁶Os and ¹⁸⁸Os.     

Spectroscopy of 166W and 167W and alignment effects in very neutron-deficient tungsten nuclei

High-spin states in ¹⁶⁶W and ¹⁶⁷W were populated by the reactions ¹⁴²Nd(²⁸Si,4n)¹⁶⁶W, ¹⁴²Nd(²⁸Si,3n)¹⁶⁷W and ¹⁴⁷Sm(²⁴Mg,4n)¹⁶⁷W. From the γ-decay the yrast band and a side band (with assumed negative parity) were identified to high spins. There is evidence for a second side band in ¹⁶⁷W. The observed backbend of the yrast sequences and band-crossing anomalies in the side bands are discussed in conjunction with cranked-shell-model calculations. A systematic comparison is made between the yrast bands of ^166,167,168W in order to understand the structure of the second backbend in ¹⁶⁸W.     

Excitation functions for 44Sc, 46Sc, and 47Sc radionuclides produced in the interaction of 45Sc with deuterons and 6He

Experimental excitation functions are presented for ⁴⁵Sc(d, p)⁴⁶Sc, ⁴⁵Sc(d, t)⁴⁴Sc, ⁴⁵Sc(⁶He, ⁵He*)⁴⁶Sc and ⁴⁵Sc(6He, α)⁴⁷Sc reactions at projectile energies near the Coulomb barrier. The obtained excitation functions for reactions ⁴⁵Sc(d, p)⁴⁶Sc and ⁴⁵Sc(⁶He, ⁵He*)⁴⁶Sc have similar behavior and have a maxima near the Coulomb barriers of these reactions. The compilation of the available experimental data, obtained at deuteron- and ⁶He-energies near the Coulomb barrier, showed that the values of the cross sections at the maxima of the excitation functions obtained in (d, p) reactions and the reactions for one-neutron pickup from the ⁶He projectiles have a different Z-dependence.     

Luminescent properties of cobalt-doped α-ZnAl2S4 spinel type single crystals

The absorption and luminescent properties of α-ZnAl₂S₄:Co spinel type crystals grown by chemical transport reactions method are investigated. The spectra are assigned to the electronic transitions of Co²⁺ ions located in tetrahedral sites. It is shown, that the revealed four radiative spectral components are caused by the ²A(²G)→⁴T₁(⁴F), ⁴T₁(⁴P)→⁴T₂(⁴F), ²E(²G)→ ⁴T₂(⁴F) and ²E(²G)→⁴T₁(⁴F) transitions.     

Rotational bands in 181Ta

High-spin states in ¹⁸¹Ta have been studied via the ¹⁷⁶Yb(¹¹B,α2n) reaction at 52 MeV using the PEX array and at 57 MeV using the NORDBALL array, with α-particle detection. The previously known, K^π=(7/2)⁺ ground state band and K^π=(9/2)⁻ band have been extended to spins (29/2)⁺ and (31/2)⁻, respectively. Two new one-quasiparticle bands, the K^π=(5/2)⁺ band built on the known (5/2)⁺ isomer and a K^π=((1/2)⁻) band have been observed. Two other rotational bands with three-quasiparticle structure, K^π=(15/2)⁻ and ((19/2)⁺ with π(7/2)[404]ν²(1/2)[510](9/2)[624] and π(9/2)[514]ν²(1/2)[510](9/2)[624] configurations, respectively, have been newly observed. The half-life of the K^π=((19/2)⁺) bandhead which decays to the head of the (15/2)⁻ band has been measured to be 140(36) ns. However, transitions from the ((19/2)⁺) state to the (15/2)⁻ band have not been observed. Received: 26 August 1998     

Perturbations in the A1Π, v = 0 state of 12C18O investigated via complementary spectroscopic techniques

The A¹Π(v = 0) level of ¹²C¹⁸O has been reinvestigated using three different high-resolution spectroscopic methods: (1) 2 + 1′ resonance-enhanced multiphoton ionisation of the A¹Π ? X¹Σ⁺(0, 0) band using narrowband lasers in a Doppler-free geometry; (2) Fourier-transform emission spectroscopy in the visible range probing the B¹Σ⁺ ? A¹Π(0, 0) band in a discharge; (3) Fourier-transform absorption spectroscopy in the vacuum-ultraviolet range measuring the A¹Π ? X¹Σ⁺(0, 0) and B¹Σ⁺ ? X¹Σ⁺(0, 0) bands at multiple temperatures ranging from 90 to 900 K. An effective-Hamiltonian analysis of A¹Π, v = 0 levels was performed up to J = 44 which quantitatively addresses perturbations by the e?³Σ^?(v = 1), d³Δ(v = 4), a′³Σ⁺(v = 9), D?¹Δ(v = 0), and I?¹Σ^?(v = 0, 1) levels.     

High resolution study of the reactions 54, 56, 58Fe(16O, 12C)58, 60, 62Ni and a comparison with (6Li,d) α-transfer spectroscopy

Spectra and angular distributions for the reactions ^{54, 56, 58}Fe(¹⁶O, ¹²C)^{58, 60, 62}Ni (E_x = 0.0–4.5 MeV) have been measured at 50 MeV with an energy resolution of 45–80 keV using a Q3D spectrograph. The selectivity of the (¹⁶O, ¹²C) reaction is found to be very similar to the (⁶Li, d) reaction. The close correspondence recently noted between the (⁶Li, d) spectra and levels strongly excited in (t, p) and (³He, n) two-nucleon transfer reactions is also observed to be present for the (¹⁶O, ¹²C) reaction. Relative α spectroscopic factors for (¹⁶O, ¹²C) and (⁶Li, d) obtained in a DWBA analysis assuming direct one-step α-cluster transfer are in very good quantitative agreement. Unnatural parity states, whose excitation is forbidden in the DWBA α-cluster approximation, are observed to be very weakly populated. These results, together with previous work on s-d shell and Ni targets, strongly suggest that the spectroscopic information provided by the (¹⁶O, ¹²C) and (⁶Li, d) reactions is essentially the same and that this information may be reliably extracted by DWBA analysis.     

Search for superheavy hydrogen isotopes <Superscript>4,5</Superscript>H in reactions of pion absorption by <Superscript>10,11</Superscript>B nuclei

The results of searching for production of superheavy hydrogen isotopes ^4,5H in reactions of absorption of stopped π^? mesons by ^10,11B nuclei are reported. A peak near 3 MeV was observed in the missing mass spectra measured in the reactions ^10,11B(π^?, t⁴He)X, ¹⁰B(π^?, d⁴He)X, and ¹⁰B(π^?, t³He)X. A structure caused by two ⁵H states with the resonance energies E _R = 5.2 and 10.4 MeV was observed in the missing mass spectra measured in the reactions ¹¹B(π^?, d⁴He)X, ¹¹B(π^?, t³He)X, and ¹⁰B(π^?, d³He)X.     

Investigation of one-nucleon transfer reactions between complex nuclei at incident energies between 3 and 8

Angular distributions of the ground state transitions in the reactions ¹¹B(¹⁴N, ¹⁵O)¹⁰Be, ¹¹B(¹⁴N, ¹³C)¹²C, ¹²C(¹¹B, ¹²C)¹¹B and ¹³C(¹²C, ¹³C)¹²C have been measured with a magnetic spectrometer as an identification system. The first two reactions (angular momentum transfer l = 2) measured at 41, 77 and 113 MeV show a clear damping of the oscillatory structures in the angular distributions. This effect was qualitatively reproduced by DWBA calculations which take into account a recoil phase, thus showing that the damping of the structures is due to the recoil of the transferred particle on the system. The reaction ¹¹B(¹²C, ¹¹B)¹²C (l = 2) at 87 MeV with Q = 0 is well reproduced by the calculations, whereas the ¹³C(¹²C, ¹³C)¹²C reaction as the only l = 0 transition is in complete disagreement with theoretical expectations.     

A study of the 26Mg(12C, 12B)26Al charge-exchange reaction

The reaction ²⁶Mg(¹²C, ¹²B)²⁶A1(5⁺, 3⁺) has been studied using a beam of 102 MeV of ¹²C. Shell-model, microscopic direct model and finite-range coupled reaction channel (CRC) calculations including recoil effects, have been performed, for comparison with the experimental data. DWBA calculations were performed for the intermediate states of interest in the ¹¹B + ²⁷Al and in the ¹³C + ²⁵Mg channels and these results were also compared with the experimental ones. The dominant reaction mechanism for ²⁶Mg(¹²C, ¹²B)²⁶Al(5⁺, 3⁺) appears to be the sequential mode.     

S?(12)群表示的填充与强衰变

本文讨论了(3/2)^-,(1/2)^-,(7/2)⁺等共振态在S?(12)群表示中的填充及其强衰变,发现16016,35100两个表示中的(3/2)^-粒子不能衰变到(1/2)⁺和0^-.通过改变运动方程质量项的符号使表示的宇称改变,就能将((3/2)^-,8)和((1/2)^-,1)填在572表示中,从而使它们能衰变到(1/2)⁺和0^-。但是,((3/2)^-,1)和(7/2)⁺仍然不能通过S?(12)对称的有效顶点衰变,本文还详细分析了S?(12)在基本粒子分类和强衰变中的成功之处与局限性,并讨论了这种局限性产生的原因。     

Gamma rays from thermal-neutron capture in natural and K enriched potassium

Gamma rays following thermal-neutron capture in natural and in ³⁹K enriched potassium have been investigated with a Ge(Li) and a Ge(Li)-NaI spectrometer. In the ³⁹K(n,γ)⁴⁰K reaction 222 γ-rays were found, of which 187 could be fitted into the level scheme of ⁴⁰K. Fifteen γ-rays could be ascribed to the ⁴¹K(n, γ)⁴²K reaction. Excitation energies of 54 levels in ⁴⁰K and of 9 levels in ⁴²K have been determined with 0.2−1.0 keV errors. The Q-values of the ³⁹K(n, γ)⁴⁰K and ⁴¹K(n, γ)⁴²K reactions are Q = 7799.7 ±0.8 keV and 7533.9±1.2 keV, respectively.     

On the mechanism of the (3He,t) reaction

The (³He, t) reactions are investigated by means of the second-order perturbation method with the (³He-α-t) process and the ordinary DWBA term. The analyses are performed on the data of ⁴⁸Ca(³He, t)⁴⁸Sc(0⁰⁺, 2⁺, 4⁺, 6⁺), ⁹⁰Zr(³He, t)⁹⁰Nb(2⁺, 4⁺, 6⁺, 8⁺) and ^{46, 48, 50}Ti(³He, t)^{46, 48, 50}V(0⁺. The results show that the (⁺He-α-t) process is an important process in these reactions and a very good agreement between observed and calculated cross sections is obtained. The energy dependence of the cross section of the ⁹⁰Zr(³He, t)⁹⁰Nb(O⁺) reaction is also discussed.     

Rotationally resolved state-to-state photoelectron study of zirconium monoxide cation (ZrO+)

Using two-colour visible (Vis)–ultraviolet (UV) photoionisation and pulsed field ionisation–photoelectron (PFI–PE) methods, we have obtained cleanly rotationally resolved photoelectron spectra for ZrO⁺(X ²Δ_3/2,5/2; v⁺ = 0, 1, and 2). The rotation assignment of these state-to-state Vis–UV–PFI–PE spectra has allowed the unambiguous determination of the ground state term symmetry for ZrO⁺(X) to be ²Δ_3/2, and the adiabatic ionisation energy of ⁹⁰Zr¹⁶O, IE(⁹⁰Zr¹⁶O) = 54,948.3(8) cm^?1 [6.81272(10) eV]. The symmetry of the ionic ZrO⁺(X ²Δ_3/2) ground state determined here disagrees with that reported in previous experiments. The rotational and vibrational constants determined in this experiment for the ionic ⁹⁰Zr¹⁶O⁺(X ²Δ_3/2) ground state are: B_e⁺ = 0.4343(8) cm^?1 and α_e⁺ = 0.0019(5) cm^?1, and ω_e⁺ = 991.2(8) cm^?1 and ω_e⁺x_e⁺ = 3.5(8) cm^?1; and those for the ionic ⁹⁰Zr¹⁶O⁺(X ²Δ_5/2) excited spin-orbit state are: B_e⁺ = 0.4357(6) cm^?1 and α_e⁺ = 0.0022(4) cm^?1, and ω_e⁺ = 991.9(8) cm^?1 and ω_e⁺x_e⁺ = 3.6(8) cm^?1, respectively. Based on the latter B_e⁺ value, the equilibrium bond distances are determined to be r_e⁺ = 1.691(2) Å for ⁹⁰Zr¹⁶O⁺(X ²Δ_3/2) and r_e⁺ = 1.688(1) Å for ⁹⁰Zr¹⁶O⁺(X ²Δ_5/2). The IE(ZrO) along with the spectroscopic constants obtained here are valuable for benchmarking the ab initio quantum chemical calculations for energetic and structural predictions of ZrO/ZrO⁺.