Energy calibration of tagged photons by the d(γ,π~-pp) reaction

The energy of tagged photons, which were provided from the internal photon tagging system of the Laboratory of Nuclear Science, Tohoku University, has been calibrated using the d(γ,π-pp) reaction. Charged pions and protons in the final state were detected with the Neutral Kaon Spectrometer (NKS2). Photon energies were obtained from the reaction of d(γ,π-pp). The derived photon energy was consistent with the design of the tagger system and the previous measurement using electron-positron pair production. The consistency demonstrates the performance of NKS2 and the capability of the photon energy calibration using d(γ,π-pp).     

Energy calibration of tagged photons by the d（γ,π~-pp） reaction

The energy of tagged photons, which were provided from the internal photon tagging system of the Laboratory of Nuclear Science, Tohoku University, has been calibrated using the d（γ,π-pp） reaction. Charged pions and protons in the final state were detected with the Neutral Kaon Spectrometer （NKS2）. Photon energies were obtained from the reaction of d（γ,π-pp）. The derived photon energy was consistent with the design of the tagger system and the previous measurement using electron-positron pair production. The consistency demonstrates the performance of NKS2 and the capability of the photon energy calibration using d（γ,π-pp）.     

Study of Charged Pion Photoproduction on Deuteron with Tagged Photons

The reactions γd→π~- pp and γd→npπ~+π~- have been studied in an energy range from 0.8 to 1.1 GeV at the tagged photon facility of Laboratory of Nuclear Science,T ohoku University.Charged pions and protons in the final state were measured by using the Neutral Kaon Spectrometer (NKS2).The analysis of the γd→π~- pp was mainly used to check the acceptance of the NKS2 and to calibrate the tagged photon energy.The photoproduction of the Δ~(++)Δ~- was identified in the γd→npπ~+π~- reaction.Since the data analyses are still in progress,we issue an interim report and preliminary results.     

Energy diffusion controlled reaction rate in dissipative Hamiltonian systems

In this paper the energy diffusion controlled reaction rate in dissipative Hamiltonian systems is investigated by using the stochastic averaging method for quasi Hamiltonian systems. The boundary value problem of mean first-passage time (MFPT) of averaged system is formulated and the energy diffusion controlled reaction rate is obtained as the inverse of MFPT. The energy diffusion controlled reaction rate in the classical Kramers bistable potential and in a two-dimensional bistable potential with a heat bath are obtained by using the proposed approach respectively. The obtained results are then compared with those from Monte Carlo simulation of original systems and from the classical Kramers theory. It is shown that the reaction rate obtained by using the proposed approach agrees well with that from Monte Carlo simulation and is more accurate than the classical Kramers rate.     

High spin states in stable nucleus ~(84)Sr

High spin states of 84Sr were populated through the reaction 70Zn(18O,4n)84Sr at 75 MeV beam energy.Measurement of excitation function,γ-γ coincidences,directional correlation from oriented state (DCO) ratios and γ-transition intensities were performed using eight anticompton HPGe detectors and one planar HPGe detector.Based on the measured results,a new level scheme of 84Sr was established in which 12 new states and nearly 30 new γ-transitions were identified in the present work.The positive-parity states of the new level scheme were compared with the results from calculations in the framework of the projected shell model (PSM).One negative-parity band was extended to spin Iπ=19-and it can be found that in the high spin states,the γ-transition energies show the nature of signature staggering.The negative-parity band levels are in good agreement with deformed configuration-mixing shell model (DCM) calculations.     

Isomeric ratio of the 181Ta(γ,3n)178m,gTa reaction products at energy Eγmax up to 95 MeV

The photoneutron reaction¹⁸Ta(y,3m)(178m,g)Ta was investigated with the beam from the NSC KIPT electron linear accelerator LUE-40.The measurements were performed using the residual y-activity method.The bremsstrahlung flux-averaged cross sections((E_γmax)>.(r(E_γmax)>m.γmax)g and the isomerie ratio of the re-action products d(E_γmax)were measured.The theoretical values of the averaged cross-sections and isomeric ratio were calculated using the partial cross-sections from the TALYS1.95 code for different level density models LD 1-6..The obtained experimental d(E_γmax)agree with the data in the lterature,but differ from the theoretical values in ab-solute magnitude and the behavior of the energy dependence.A comparison of the determined averaged cross-sec-tions with the calculated cross sections showed the best agreement for the case of the LD 5 model.     

Measurement of 59Co(ai,x)reaction cross sections with the fast neutrons based on the 9Be(p,n)reaction

The cross sections of the ⁵⁹Co(n,x)reaction in the average energy range of 15.2-37.2 MeV were meas-ured using activation and an off-line γ-ray spectrometric technique.The neutrons were generated from the ⁹Be(p,n)reaction with proton beam energies of 25-45 MeV at the MC-50 Cyclotron facility of the Korean Institute of Radi-ological and Medical Sciences(KIRAMS).Theoretical cal lculations of neutron-induced reactions on ⁵⁹Co were per-formed using the nuclear model code TALYS-1.9.The results for the ⁵⁹Co(n,x)reactions were compared with the theoretical values obtained using TALYS-1.9 and the literature data provided in EXFOR and the TENDL 2019 nuc-lear data library.The theoretical values obtained using TALYS-1.9 with adjusted parameters are comparable to the experimental data.The measured reaction cross sections of a few radionuclides are new,and the others are compar-able to the literature data,and thus,they can strengthen the database.The present study on cross sections leads to useful insight into the mechanisms of ⁵⁹Co(n,x)reactions.     

Isospin Effect of Charged Particle Multiplicity in Intermediate Energy Heavy Ion Collisions

The dependences of He and intermediate mass fragments (IMF) production rates in the reactions 55 MeV/u ^40Ar ^58,64 Ni on the isospin, impact parameter and primary excitation energy of the reaction nuclear system were studied by using the 4π charged particle multi-detector array system (MUDAL). For the mentioned two reaction systems, the measured He particle contribution in the total charged particle multiplicity increases with increasing the total charged particle multiplicity but for the contribution of IMFs in the total charged particle multiplicity increases with increasing the total charged particle multiplicity at lower total charged particle multiplicities, and latter on it drops down with further increasing of the total charged particle multiplicities (see Fig.l). The experimental results of these two reaction systems with the same nuclear charge indicate that the contribution of He and IMFs in the total charged particle multiplicities are obviously isospin dependent.     

Measurements of differential and angle-integrated cross sections for the ~(10)B(n, α)~7Li reaction in the neutron energy range from 1.0 eV to 2.5 MeV

Differential and angle-integrated cross sections for the ~(10)B(n,α)~7 Li,~(10)B(n,α_0) ~7 Li and ~(10)B(n,α_1) ~7 Li~*reactions have been measured at CSNS Back-n white neutron source.Two enriched(90%) ~(10)B samples 5.0 cm in diameter and～85.0 μg/cm~2 in thickness each with an aluminum backing were prepared,and back-to-back mounted at the sample holder.The charged particles were detected using the silicon-detector array of the Light-charged Particle Detector Array(LPDA) system.The neutron energy En was determined by TOF(time-of-flight) method,and the valid a events were extracted from the E_n-Amplitude two-dimensional spectrum.With 15 silicon detectors,the differential cross sections of a-particles were measured from 19.2°to 160.8°.Fitted with the Legendre polynomial series,the(n,a) cross sections were obtained through integration.The absolute cross sections were normalized using the standard cross sections of the ~(10)B(n,α) ~7 Li reaction in the 0.3-0.5 MeV neutron energy region.The measurement neutron energy range for the ~(10)B(n,α) ~7 Li reaction is 1.0 eV≤E_n 2.5 Me V(67 energy points),and that for the ~(10)B(n,α_0) ~7 Li and~(10)B(n,α_1) ~7 Li~*reactions is 1.0 eV≤E_n1.0 MeV(59 energy points).The present results have been analyzed by the resonance reaction mechanism and the level structure of the ~(11)B compound system,and compared with existing measurements and evaluations.     

Precise measurement of the e~+e~- →π~+π~-(γ) crosssection with the initial state radiation method at BABAR

We present a precise BABAR measurement on the cross section of the process e+e-→π+π-(γ) from threshold to an energy of 3 GeV with the initial state radiation(ISR) technique,using 232 fb-1 of data collected with the BABAR detector at e+e-center-of-mass energies near 10.58 GeV.The ISR luminosity is determined from a study of the leptonic process e+e-→μ+μ-γ(γ).The leading-order hadronic contribution to the muon magnetic anomaly calculated using the ππ cross section measured from threshold to 1.8 GeV is(514.1±2.2(stat)±3.1(syst))×10-10.     

New empirical formula for(γ, n) reaction cross section near GDR peak for elements with Z ≥ 60

A new empirical formula has been developed that describes the(7,n) nuclear reaction cross sections for isotopes with Z ≥ 60.The results were supported by calculations using TALYS-1.6 and EMPIRE-3.2.2 nuclear modular codes.The energy region for incident photon energy has been selected near the giant dipole resonance(GDR) peak energy.The evaluated empirical data were compared with available data in the experimental data library EXFOR.The data produced using TALYS-1.6 and EMPIRE-3.2.2 are in good agreement with experimental data.We have tested and presented the reproducibility of the present new empirical formula.We observe the reproducibility of the new empirical formula near the GDR peak energy is in good agreement with the experimental data and shows a remarkable dependency on key nuclei properties:the neutron,proton and atomic number of the nuclei.The behavior of nuclei near the GDR peak energy and the dependency of the GDR peak on the isotopic nature are predicted.An effort has been made to explain the deformation of the GDR peak in(γ,n) nuclear reaction cross sections for some isotopes,which could not be reproduced with TALYS-1.6 and EMPIRE-3.2.2.The evaluated data have been presented for the isotopes ~(180)W,~(183)W,~(202)Pb,~(203)Pb,~(204)Pb,~(205)Pb,~(231)Pa,~(232)U,~(237)U and ~(239)Pu,for which there are no previous measurements.     

Measurement of(n,α)and(n,2n)reaction cross sections at a neutron energy of 14.92±0.02 MeV for potassium and copper with uncertainty propagation

Experimentally measured neutron activation cross sections are presented for the ⁶⁵Cu(n,0)^62mCu,⁴¹ K(n,a)^38Cl,and ⁶⁵Cu(n.2n)⁶⁴Cu reactions with detailed uncertainty propagation.The neutron cross secions were measured at an incident energy of 14.92±0.02 MeV,and the neutrons were based on the(d,n)a fusion reaction.The ²⁷ Al(n,a)²⁴Na reaction was used as a reference reaction for the normalization of the neutron flux.The pre-calib-rated lead-shielded HPGe detector was used to detect the residues'γ-ray spetra.The data from the measured cross sections are compared to the previously measured cross sections from the EXFOR database,theoretically calculated cross sections using the TALYS and EMPIRE codes,and evaluated nuclear data.     

Isomeric pair 95m,gNb in the photonuclear reactions on natMo at the bremsstrahlung end-point energy of 38–93 MeV

The ^natMo(γ,xnp)^95m,g Nb photonuclear reaction was studied using the electron beam from the NSC KIPT linear accelerator LUE-40.The experiment was performed using the activation and off-line γ-ray spectrometric technique.The experimental isomeric yield ratio(IR) was determined for the reaction products ^95m,gNb at the bremsstrahlung end-point energy E_γmax range of 38-93 MeV.The obtained values of IR are in satisfactory agreement with the results of other...     

Chemical Effect Analyses of 3dElements by Study of X-Ray Fluorescence Spectra

Spectra of K X-rays emitted from pure 3d transition metals and their oxide and sulfate compounds were measured using a single crystal wavelength dispersive X-ray spectroscopy (WDXRF). The measurements were performed using a ZSX-100e sequential spectrometer equipped with an Rh X-ray tube operated. An accurate analytical representation of each line was obtained by a fit to a Lorentz function. The spectra were analyzed in order to examine the K X-ray peak parameters such as asymmetry index, peak energy and relative intensity ratios. The energy shifts and relative intensities weredetermined tobetter understand the chemical effect.     

Combined multi-level quantum mechanics theories and molecular mechanics study of water-induced transition state of OH~- + CO_2 reaction in aqueous solution

The presence of a solvent interacting with a system brings about qualitative changes from the corresponding gasphase reactions. A solvent can not only change the energetics along the reaction pathway, but also radically alter the reaction mechanism. Here, we investigated the water-induced transition state of the OH~- + CO_2→ HCO_3~- reaction using a multi-level quantum mechanics and molecular mechanics method with an explicit water model. The solvent energy contribution along the reaction pathway has a maximum value which induces the highest energy point on the potential of mean force. The charge transfer from OH~- to CO_2 results in the breaking of the OH~- solvation shell and the forming of the CO_2 solvation shell. The loss of hydrogen bonds in the OH~-solvation shell without being compensated by the formation of hydrogen bonds in the CO_2 solvation shell induces the transition state in the aqueous solution. The calculated free energy reaction barrier at the CCSD(T)/MM level of theory, 11.8 kcal/mol, agrees very well with the experimental value, 12.1 kcal/mol.     

π~0 Photoproduction on Deuteron for Photon Energies from 0.6 to 1.15 GeV

Differential and total cross sections of the γp→π~0 p and the γp→π~0 pn reaction were measured for photon energies between 640 and 1 150 MeV.The data have been compared with SAID and MAID model calculations.π~0 photoproduction on the deuteron shows a strong suppression of the 2nd resonance which is clearly seen in the γp→π~0 p reaction.     

Ultrasensitive Detection of Infrared Photon Using Microcantilever: Theoretical Analysis

We present a new method for detecting near-infrared, mid-infrared, and far-infrared photons with an ultrahigh sensitivity. The infrared photon detection was carried out by monitoring the displacement change of a vibrating microcantilever under light pressure using a laser Doppler vibrometer. Ultrathin silicon cantilevers with high sensitivity were produced using micro/nano-fabrication technology. The photon detection system was set up. The response of the microcantilever to the photon illumination is theoretically estimated, and a nanowatt resolution for the infrared photon detection is expected at room temperature with this method.     

Measurement of 85Rb（n, 2n） 84Rb reaction cross-section from 12 MeV up to 19.8 MeV

The cross-section data of the 85Rb(n,2 n)84Rb reaction have been measured with the neutron energies of 12 MeV to 19.8 MeV using the activation technique and the relative method.The 85Rb samples were irradiated on the surface of a two-ring orientation assembly with neutrons produced from the 3H(d,n)4He reaction at the 5SDH-21.7-MV Tandem accelerator in China.Theoretical model calculations were performed with the TALYS-1.9 code.The present data were compared with previously obtained experimental data and the available evaluated data.     

Measurements of neutron energy spectra of 9Be(d,n)10B reaction with a thick beryllium target

Novel measurements of the neutron energy spectra of the 9Be(d,n)10B reaction with a thick beryllium target are performed using a fast neutron time-of-flight(TOF)spectrometer for the neutron emission angles θ=0°and 45°,and the incident deuteron energies are 250 and 300 keV,respectively.The neutron contributions from the 9Be(d,n)10B reaction are distributed relatively independently for the ground state and the first,second,and third excited states of 10B.The branching ratios of the 9Be(d,n)10B reaction for the different excited states of 10B are obtained for the neutron emission angles θ=0°and 45°,and the incident deuteron energies are 250 and 300 keV,respectively.The branching ratio of the 9Be(d,n)10B reaction for the third excited state decreases with increase in the incident deuteron energy,and the branching ratios for the ground state and the second excited state increase with increase in the neutron emission angle.     

Determination of neutron capture cross sections of ~(232)That 14.1 MeV and 14.8 MeV using the neutron activation method

The ~(232)Th(n,γ)~(233)Th neutron capture reaction cross sections were measured at average neutron energies of 14.1 MeV and 14.8 MeV using the activation method.The neutron flux was determined using the monitor reaction~(27)Al(n,α)~(24)Na.The induced gamma-ray activities were measured using a low background gamma ray spectrometer equipped with a high resolution HPGe detector.The experimentally determined cross sections were compared with the data in the literature,and the evaluated data of ENDF/B-Ⅶ.1,JENDL-4.0u+,and CENDL-3.1.The excitation functions of the ~(232)Th(n,γ)~(233)Th reaction were also calculated theoretically using the TALYS1.6 computer code.