Study of fusion and nucleon transfer channels in the <Superscript>197</Superscript>Au + <Superscript>6</Superscript>He reaction in an energy range of <Superscript>6</Superscript>He to 20 Mev/A

New data on the cross sections of reactions occurring during the interaction of ⁶He nuclei with ¹⁹⁷Au at energies of ⁶He from 40 to 120 MeV are presented. The experiments were performed in the ACCULINNA secondary beam separator of the Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research. To identify the reaction products, the activation method for measuring the gamma activity of the target assembly of thin foils was used. The excitation functions for fusion reactions involving the evaporation of up to ten neutrons from the compound nucleus as well as reactions with the emission of charged particles and nucleon transfer in the investigated energy region are obtained. Data analysis was carried out using two codes: ALICE-MP and NRV. The cross sections for the (⁶He, xn) reactions occurring through the compound nucleus are mostly in agreement with the results of model calculations based on the statistical approach. It is shown that, up to the energies of 114 MeV, the cross-section drop in the complete fusion reactions is negligible. The experimental excitation functions of reactions leading to the formation of isotopes of mercury and gold (transfer reaction) indicate that the main contribution to their formation is made by direct processes and that evaporation reactions (⁶He, pxn) and (⁶He, αxn) play a minor role, as is evidenced by a comparison of the measured cross sections with the calculation results.     

Pionic fusion study of the halo nucleus 6He, the reaction d+4He→6He+π + at CELSIUS

The halo nucleus ⁶He has been studied in a pionic fusion experiment at the CELSIUS storage ring facility in Uppsala. The ⁶He nuclei were produced in reactions with a deuteron beam incident on a ⁴He jet target 0.9–5.4 MeV above threshold in the center-of-mass frame. The ⁶He ions were detected in a ΔE-E solid-state detector telescope inserted into the CELSIUS ring. The aim of the experiment was to investigate, in particular, the high-momentum part of the halo wave function by measuring the total and differential cross sections of the reaction d+⁴He→⁶He+π ⁺.     

Excitation functions of191+193Ir,197Au(6Li,xn+yp) compound nuclear reactions at ELi=48–156 MeV

Excitation functions of the compound nuclear reactions^191+193Ir,¹⁹⁷Au(⁶Li,xn+yp) forx =3–13 andy=0–2 have been investigated by means of in-beamγ-ray spectroscopy at the 156 MeV⁶Li beam of the Karlsruhe Isochronous Cyclotron. The beam energy has been varied in the range of 48 to 156 MeV in steps of about 10 MeV by Be-absorber foils in the external beam line. Absolute cross sections have been determined by normalizing the measuredγ-ray intensities to the production cross sections ofK- X-rays in the target. The experimental excitation functions are discussed on the basis of predictions of the preequilibrium (hybrid) model. While in most cases the theoretical calculations fairly well reproduce energy position and shapes of the curves, strong discrepancies in the absolute scale of the cross sections are observed. The theoretical predictions overestimate the (⁶Li,xn) cross sections by a factor of about 6. Conspicuous anomalies have been detected when comparing the (⁶Li, xn+1(2)p) reactions with (⁶Li,xn) reactions. The reactions with emission of one or two protons are considerably enhanced. The discrepancies and anomalies observed are tentatively explained by the influence of direct reaction channels as the⁶Li break-up, which experimentally proved to be the dominant contribution to the total reaction cross section. The enhancement of the reactions with emission of protons may be a consequence of transfer reactions into highly excited states combined with compound nucleus formation thus implying a cluster effect in preequilibrium emission process.     

Cross sections of fusion and transfer reactions in interactions between 3He and Pt and 197Au nuclei in the subbarrier energy region

The reactions of complete and incomplete fusion, along with nucleon transfer reactions in the range of ³He energies from 10 to 24.5 MeV, are investigated by irradiating gold and platinum targets with an accelerated ³He ion beam on the U-120M cyclotron at the Institute of Nuclear Physics, Czech Academy of Sciences, ?e?. Activation is used to determine the yield of nuclides resulting from nuclear reactions. The γ-activity induced in the targets is measured using a with high-resolution HPGe detector. Despite the low binding energy of ³He and the reactions with positive Q values, the measured cross sections of fusion reactions exhibit no specific features, compared to reactions conducted using beams of other light stable particles. Transfer neutron reactions in the subbarrier energy region have relatively high cross sections. These cross sections continue to grow as the energy of ³He rises. When a neutron is captured by a nucleus of ³He, the cross sections of these reactions reach their maximum values in the Coulomb barrier region.     

Excitation functions for complete fusion and transfer reactions in the interaction of 6He with 197Au nuclei

The excitation functions for the fusion reactions with subsequent neutron evaporation, ¹⁹⁷Au(⁶He, xn)^{203 ? xn}Tl (x = 2?7), and the neutron transfer reactions with production of the ¹⁹⁶Au and ¹⁹⁸Au isotopes have been measured. Unusually high cross section of the ¹⁹⁸Au isotope production at energies below the Coulomb barrier has been observed. Possible mechanisms of production and decay of the transfer reaction products are considered.     

Fusion cross sections for 10,11B+12C at sub-Coulomb energies

Total fusion cross sections for the ¹⁰B + ¹²C and ¹¹B + ¹²C reactions have been determined over a 5 MeV (c.m.) energy range extending to ≈ 3 MeV below the Coulomb barrier. Absolute γ-ray yields for specific transitions in the de-excitation of the heavy products following compound nucleus decay were measured using a Ge(Li) detector. Statistical model calculations of the decay modes of the compound nucleus have been used to deduce, from the γ-ray data, cross sections for single proton, neutron and α-particle emission, and to determine total cross sections for compound nucleus formation. No evidence has been found for sub-Coulomb resonances in either reaction. The total reaction cross sections are compared with optical model calculations using different parameter sets and the observed trend in the very low energy cross sections is discussed relative to other reactions in the same mass region.     

Some peculiarities in the interaction of 6He with 197Au and 206Pb

Excitation functions were measured for fusion followed by the evaporation of neutrons in the reactions ²⁰⁶Pb(⁶He, 2 _n )²¹⁰Po and ¹⁹⁷Au(⁶He, xn)^203−xn T1, where x = 2−7, as well as for the transfer reactions on a ¹⁹⁷Au target with the formation of the ¹⁹⁶Au, ¹⁹⁸Au, and ¹⁹⁹Au isotopes. The experiment was carried out at the Dubna Radioactive Ion Beams (DRIBs) complex of FLNR, JINR. The ⁶He beam intensity was about 5 × 10⁶ pps, the maximum energy being (60.3 ± 0.4) MeV. A significant increase in the cross section was observed below the Coulomb barrier for the fusion reaction with the evaporation of two neutrons compared to statistical model calculations. Unusual behavior for the production of ¹⁹⁸Au is observed, whereas the cross section for the formation of ¹⁹⁹Au is very low. The analysis of the data in the framework of the statistical model for the decay of excited nuclei, which took into account the sequential fusion of ⁶He, has shown good agreement between the experimental and calculated values of the cross sections for the case of sub-Coulomb-barrier fusion in the ²⁰⁶Pb + ⁶He reaction. The text was submitted by the authors in English.     

Compound nucleus contribution and even-odd effect for (3He,p) reactions in the Ni region

The compound nucleus contributions to the proton spectra from 8 MeV and 10 MeV ³He induced (³He, p) reactions on even-A Ni isotopes were obtained. The relative cross sections for ⁵⁸Ni/⁶⁰Ni/⁶²Ni in the high excitation region are in fair agreement with predictions of statistical theory, but the absolute cross sections in the same region are smaller than the prediction by a factor of 3 to 8, and the shapes of the measured spectra for heavier isotopes do not agree with the prediction. These discrepancies between experiment and theory are in sharp contrast to the situation in (p, p′), (p, α), (α, p) and (α, α′), where good agreement was found.The proton spectra from (³He, p) reactions on nuclei in the A = 54–68 mass range have a systematic difference in slope between even-A targets and odd-A targets; it is similar to the systematic difference found previously in (p, p′) and (α, p) reactions, but none of these is readily explainable by theory.     

Excitation functions for complete-fusion and transfer reactions in <Superscript>4</Superscript>He interaction with <Superscript>197</Superscript>Au nuclei

Excitation functions are measured for the fusion reactions ¹⁹⁷Au(⁴He, xn)^201?xn Tl that are induced by alpha-particle interaction with gold nuclei in the energy range 14–36 MeV and in which x neutrons (0 ≤ x ≤ 3) are evaporated. The stack-activation technique was used to record and separate reaction products. Experimental data on the fusion reactions followed by evaporation of one to three neutrons agree with results of previous studies. For the radiative-capture reaction ¹⁹⁷Au(⁴He,γ)²⁰¹Tl, the upper limit on the cross section proved to be much lower. The excitation functions for the reactions subjected to measurements are compared with the results of calculations based on the statistical model and with the results of an experiment performed previously in a ⁶He beam.     

Fission of209Bi induced by6He ions

Secondary beams of⁴He and⁶He were produced through the transfer reactions with the 18.5 MeV/u¹¹B and 35.5 MeV/u⁷Li primary beams. The fusion-fission cross sections have been measured for the^4,6He +²⁰⁹Bi reactions at energies E_cm>1.5*B_fus. In the present experiment it was found that the fission excitation function for the neutron rich nuclei⁶He is significantly higher than for the⁴He nuclei.     

Resonant structure observed in the 3He(τ, γ)6Be capture reaction

The ³He(τ,γ)⁶Be capture reaction has been studied for ³He bombarding energies from 12 to 27, MeV. Transitions to the first excited state in ⁶Be(T = 1, 2⁺) are readily seen. Transitions to the ground state in ⁶Be (T = 1, 0⁺) are very weak and their presence could not be ascertained. The 90° excitation function for these transitions shows a broad maximum centered at E_τ = 23 ±1 MeV. This is interpreted as a resonance in the compound nucleus ⁶Be at E_x = 23.0±0.5 MeV with a configuration other than ³He+³He. These results are compared with other experimental work as well as with theoretical predictions.     

Cross sections of 43Sc, 44Sc, 46Sc isotopes formed in the 45Sc + 3He reaction

Reactions ⁴⁵Sc(³He, αn)⁴³Sc, ⁴⁵Sc(³He, α)⁴⁴Sc and ⁴⁵Sc(³He, 2p)⁴⁶Sc in the ³He energy range of 5 to 24 MeV are investigated in experiments performed with a ³He ion beam during the irradiation of U-120M cyclotron scandium targets. Activation is used to determine the yield of nascent Sc isotopes. The γ activity induced in targets is measured using a high-resolution HPGe detector. The character of the excitation function changes during the formation of these ions and differs from the excitation functions for deuterons, despite the low bond energy of ³He and the positive values of the Q reactions leading to the formation of ⁴⁴Sc and ⁴⁶Sc isotopes. The cross sections of ⁴⁴Sc formation reach their maximum value at the Coulomb barrier of the reaction, due to the stable ⁴He nucleus that accompanies the formation of ⁴⁴Sc. The contribution from different reaction mechanisms to the cross sections of ⁴³Sc, ⁴⁴Sc, and ⁴⁶Sc isotope formation are considered.     

Fusion and transfer cross sections of 3He induced reaction on Pt and Au in energy range 10–24.5 MeV

In experiments performed by accelerated ion ³He-beam irradiated gold and platinum targets on the cyclotron U-120M of the Nuclear Physics Institute of the Czech Academy of Sciences, ?e?, reactions of complete and incomplete fusion and nucleon transfer reactions in the ³He energy range from 10 to 24.5 MeV have been investigated. To determine the yield of the nuclides resulting from the nuclear reaction, the activation technique has been used. The obtained data are analyzed using models based on statistical calculations and compared with similar results for other light stable particles. Transfer reactions with positive Q values have relatively high cross sections in the energy range below the Coulomb barrier. These cross sections continue to grow with increasing ³He energy, and, in the case of capturing neutron from target nucleus by a nucleus of ³He, the excitation functions of these reactions reach their maximum almost at the Coulomb barrier of the reactions.     

Experimental investigation of highly excited states of the 5,6He and 5,6Li nuclei in the (6Li, 7Be) and (6Li, 7Li) one-nucleon pickup reactions

The (⁶Li, ⁷Be) and (⁶Li, ⁷Li) reactions on ⁶Li and ⁷Li nuclei were investigated in the angular interval 0°–20° in the laboratory system at a ⁶Li energy of 93 MeV. In addition to low-lying states of the ^5,6He and ^5,6Li nuclei, broad structures were observed near the t(³He)+d and t(³He)+t thresholds at the excitation energies of 16.75 (3/2⁺) and ～20 MeV (for ⁵He), 16.66 (3/2⁺) and ～20 MeV (⁵Li), 14.0 and 25 MeV (⁶He), and ～20 MeV (⁶Li). The angular distributions measured in the ⁷Li(⁶Li, ⁷Be)⁶He reaction for transitions to the ground state (0⁺) and excited states at E _x=1.8 MeV (2⁺) and 14.0 MeV of the ⁶He nucleus were analyzed by the finite-range distorted-wave method assuming the 1p-and 1s-proton pickup mechanism. The (⁶Li, ⁷Be) and (⁶Li, ⁷Li) reactions were shown to proceed predominantly through the one-step pickup mechanism, and the broad structures observed at high excitation energies are considered as quasimolecular states of the t(³He)+d and t(³He)+t types.     

The 28Si(3He,pp)29Si reaction induced by 33 MeV polarized 3He

Differential cross sections and analysing powers were measured for the ²⁸Si(³He, pp)²⁹Si reaction using a 33 MeV polarized ³He beam. The sequential breakup model successfully described the data as a function of both the emission angle and relative proton energy of the ²He cluster for several states in ²⁹Si. An unambiguous j-dependence of the analysing powers was observed and used to asign J^π values for some final states. A statistical analysis of the breakup continuum revealed that a large fraction of such events originate from a formation of the ³¹S compound system.     

Direct and compound nuclear contributions to the 13C(6Li,t) reaction at Elab = 25 MeV

The reaction ¹³C(⁶Li, t)¹⁶O has been studied in the incident energy range 24–26 MeV. Complete angular distributions have been measured at E_⁶Li, = 25 MeV in the angular range θ_lab = 8°–172°, with the reaction ⁶Li(¹³C, t)⁶O being used for the backward angle measurements. Cross sections for evaporation residues from the fusion of the ⁶Li + ¹³C system have been measured in the incident ⁶Li energy range 9.2–35.1 MeV. Compound nuclear contributions to the transfer cross sections have been calculated using the Hauser-Feshbach statistical theory with the assumption that the compound-nucleus formation cross section is equal to the measured fusion cross section. By comparison of the compound nuclear calculations with backward angle data it is found that the sharp cutoff approximation commonly used to represent the initial angular momentum distribution of the compound nucleus is not adequate for the ¹³C(⁶Li, t)¹⁶O reaction. Good fits to the backward angle data can be obtained by using a smooth cutoff approximation. The forward angle cross sections have been compared with exact finite-range distorted-wave Born approximation calculations to extract transferred angular momenta and spectroscopic strengths. The present results differ from those of an earlier study. These differences are due to the inclusion of forward angle data in the present study.     

Cross sections for the (n,n′), (n,p) and (n, 2n) reactions on 107Ag and 109Ag isotopes

The cross sections for (n, n′), (n, p) and (n, 2n) reactions on the target nuclei ¹⁰⁷Ag and ¹⁰⁹Ag were measured by the activation technique in the neutron energy range 13 to 18 MeV. The results are interpreted in terms of the compound nucleus and precompound emission models.     

Observation of deuteron D-state and compound nucleus effects in (d,p) reactions on 46Ti and 52Cr with a polarized deuteron beam

The cross section and the vector and tensor analyzing powers have been measured for ⁴⁶Ti(d, p)⁴⁷Ti at deuteron energies of 6 and 10 MeV and ⁵²Cr(d, p)⁵³Cr at 6 MeV. Transitions were observed to the states at E_x=0.159, 1.549 and 1.793 MeV in ⁴⁷Ti and the states at E_x=0.0, 0.564, 1.006 and 2.321 MeV in ⁵³Cr. In addition, the cross sections and vector analyzing powers for deuteron elastic scattering were measured for the same targets and deuteron energies and compared to optical model calculations. The choice of optical parameters for the DWBA analysis of the (d, p) reactions is discussed. Calculations made with the DWBA method show that the deuteron D-state must be included to reproduce even qualitatively the (d, p) tensor analyzing power measurements. The j-dependence of the tensor analyzing power T₂₂ is discussed. The validity of the local energy approximation (which was used to incorporate the deuteron D-state into the DWBA calculations) is evaluated by comparison to finite range calculations. The contribution of compound nucleus reactions to the measured cross sections and analyzing powers was investigated. In order to determine the compound cross section, the Ericson fluctuations in excitation functions of cross section and vector analyzing power were measured from 5 to 7 MeV on each target. The formulas used to calculate the polarization observables from the Hauser-Feshbach theory are presented.     

A detailed study of the 12C + 16O fusion reaction at Ecm = 19 to 24 MeV

Excitation functions of evaporation residues following the ¹²C + ¹⁶O reaction are investigated at E_cm = 19 to 24 MeV. At the resonances which have been previously identified in the ¹²C(¹⁶O, ⁸Be)²⁰Ne two-body channel, an order of magnitude larger resonance cross section is observed in the fusion channel than that in the two-body one and is shared among a few evaporation residues (²⁰Ne, ²³Na and ²⁴Mg). Here the resonance cross section is defined as the resonance part of the cross section on a resonance in an excitation function. It is found that for each resonance the relative intensity of the resonance cross sections of these residues is fairly well explained by assuming that they are coming from the decay of a compound nuclear resonance. It indiates that these intermediate resonances have a large probability to proceed to the formation of a more complicated configuration prior to its decay into exit channels. However, the resonant enhancement in the fusion channel is found to be weak at three energies (E_cm = 19.7, 22.0 and 22.6 MeV), where prominent resonant structures have been observed in inelastic channels. These distinct situations may be attributed to the magnitude of level density of the compound nucleus.     

Partial breakdown of the evaporation model and possible preequilibrium α-particle emission in heavy-ion fusion reactions

Relative cross sections for residual nuclei following fusion reactions were measured by γ-ray spectroscopy in the reactions ⁵²Cr+ ¹²C at 56.00 MeV and ⁴⁸Ti+ ¹⁶O at 57.74 MeV, in which the common “compound nucleus” ⁶⁴Zn was excited at the same energies and the relative distributions of the entrance spins were nearly identical. It is shown that ratios of the measured cross sections in both entrance channels can be precisely determined experimentally and are insensitive to small changes of the parameters in calculations based on the evaporation model. Using these particular quantities, we have shown that the evaporation process is not the sole mechanism producing the observed residues, especially those resulting from α-particle emission. The assumption of preequilibrium α-particle emission at high channel spins is shown to reproduce the present data fairly well.