激光诱导血红蛋白分子的多光子荧光

本文首次报道了血红蛋白吸收二个和四个1.06μm的光子后所发射的荧光特性,并分析了其产生的原因。     

Angular distribution of electrons in multiphoton ionisation of polarised Lithium atoms

The asymmetry of the angular distributions of photoelectrons in the photoionisation of polarised alkali atoms is investigated. The general formulas for the amplitude of the multiphoton ionisation of np-states are given. In these formulas the dynamical and kinematical factors are explicitly separated. Our calculations within Fues model potential approach demonstrate that, under the experimental conditions essentially similar to those employed in [M. Schuricke, Ganjun Zhu, J. Steinmann, K. Simeonidis, I. Ivanov, A. Kheifets, A.N. Grum-Grzhimailo, K. Bartschat, A. Dorn, J. Ullrich, Phys. Rev. A 83 (2011) 023413(11)], the relative magnitude of the linear magnetic dichroism in three-photon ionisation of Li can be as large as 30%.     

Laser-induced nonlinear resonances in the continuum at third-harmonic generation in Na vapor

A theoretical and experimental study of light-induced autoionizing-like resonance in the continuum at THG of λ=191 nm in sodium vapor is presented. A gain of the output THG power as much as 18 times due to autoionizing-like resonance has been obtained.     

Determination of structure parameters in molecular tunnelling ionisation model

We extracted the accurate structure parameters in a molecular tunnelling ionisation model (the so-called MO-ADK model) for 23 selected linear molecules including some inner orbitals. The molecular wave functions with the correct asymptotic behaviour are obtained by solving the time-independent Schrödinger equation with B-spline functions and molecular potentials numerically constructed using the modified Leeuwen–Baerends (LBα) model. We show that the orientation-dependent ionisation rate reflects the shape of the ionising orbitals in general. The influences of the Stark shifts of the energy levels on the orientation-dependent ionisation rates of the polar molecules are studied. We also examine the angle-dependent ionisation rates (or probabilities) based on the MO-ADK model by comparing with the molecular strong-field approximation calculations and with recent experimental measurements.     

Laser-induced reorientation effect and ripple structure in dye-doped liquid-crystal films

The effects of light-induced reorientation on a homeotropical dye-doped liquid crystal (DDLC) cell are discussed. The photoexcited azo dye Methyl Red (MR) is diffused and adsorbed onto the substrate, thus forming a ripple structure. The adsorbed dye and the laser-induced ripple structure then reorient the liquid-crystal molecules and induce a holographic grating. Initially, the liquid-crystal directors are reoriented primarily by the adsorbed dye. However, given a sufficiently large ripple groove amplitude, the torque imposed by the ripple grooves overcomes that which is due to the adsorbed dyes, and the liquid crystals are realigned along the groove direction.     

Laser-induced helical structure in the isotropic phase of nematic liquid crystal

We report on the first observation of laser-induced helical structure in the isotropic phase of a nematic liquid crystal. The helical structure was induced by two nearly counter-propagating waves circularly polarized in the same sense. Bragg reflection in the optical tunneling region was studied. We made an extensive investigation on the analogy between Bragg reflection from a cholesteric liquid crystal slab and four-wave mixing. It provides a deeper insight into the physics of the optical properties of cholesteric liquid crystal.     

Determination of cross sections and continuum phases of rubidium through complete measurements of atomic multiphoton ionization

We present a complete experimental determination of the atomic parameters necessary to unambiguously characterize two-photon ionization of atomic rubidium, i.e., the relative photoionization cross sections and the continuum wave function phase difference. We obtain these complete results through a single measurement, that of the two-photon photoelectron angular distribution using elliptically polarized light. While measured phase differences are in excellent agreement with expected values, the ratios of photoionization cross sections of the two D channels are not.     

Hadron structure on the lattice and in the continuum

Hadron structure physics has in recent years reached a level of precision which allows for a change of perspective. Model-based arguments are often quite unreliable. However, meanwhile they can be more and more replaced by controlled and systematic QCD approaches. The story of the strange electric form factor, which provided much of the motivation for the PAVI Conference series provides a typical example to illustrate this statement. However, high-precision theory is technically very challenging and progress is, therefore, unpleasantly slow. This fact and the present status in general is illustrated by a few typical examples.     

Underlying structure of continuum response functions in random phase approximation

It is shown that continuum-RPA results can be understood in terms of energy-dependent, complex RPA states. These states have finite widths which are direct escape widths. Calculations have been performed for a simple model of monopole resonance in ⁴⁰Ca, and the results are compared with those obtained by continuum-RPA and time-dependent Hartree-Fock methods.     

Antibunching in multiphoton processes

A Stokes-antiStokes-system of four Boson modes with hyper-scattering or similar four photon interaction is investigated with respect to the statistical behaviour of the common ground mode. The solution of Heisenberg equations in short time approximation opens the possibility of antibunching already with the terms linear in t. It is shown in how far antibunching can be remarked even at intensities which are not extremely small. Its characteristic time may be shifted over several orders of magnitude.     

Fractal structure of equipotential curves on a continuum percolation model

We numerically investigate the electric potential distribution over a two-dimensional continuum percolation model between the electrodes. The model consists of overlapped conductive particles on the background with an infinitesimal conductivity. Using the finite difference method, we solve the generalized Laplace equation and show that in the potential distribution, there appear quasi-equipotential clusters   which approximately and locally have the same values as steps and stairs. Since the quasi-equipotential clusters have the fractal structure, we compute the fractal dimension of equipotential curves and its dependence on the volume fraction over [0,1]$[0,1]$. The fractal dimension in [1.00, 1.246] has a peak at the percolation threshold _pc$p_c$.