Polarization and phase shifts in 9Be(p,p)9Be from 0.8 TO 2.7 MeV and the structure of 10B

Angular distributions of the analyzing power in ${}^9\text{Be(}\text{p}\text{,p)}{}^9$Be have been measured to an accuracy of about ±0.03 at 21 energies from 0.9 to 2.7 MeV with a target thickness of 20 keV at 1 MeV. These data and the cross section measurements of others are reproduced well in the region from 0.8 to 1.6 MeV by a set of phase shifts that vary reasonably with energy. The ³S₁, ⁵S₂, ⁵P₁, and ⁵P₂ phases suffice to describe the data, although channel spin and s-d mixing are required. Three levels satisfy the data: at 0.980±0.010 MeV are two levels, a 1⁺ of width 0.10 MeV and a 2^? of width 0.11 MeV; at 1.37±0.02 MeV is a 1^? level of width 0.30 MeV. The 1⁺ and 1^? states do not agree with earlier assignments. Outside of the energy region from 0.8 to 1.6 MeV a satisfactory set of phases could not be obtained, owing to inadequate data. These regions were studied in the analysis, however, and the results are discussed.     

Observation of the π(1800) and (1880) mesons in decay

A partial-wave analysis of the reaction π⁻p→ηηπ⁻p at 18 GeV/c has been performed on a data sample of approximately 4000 events obtained by Brookhaven experiment E852. The J^PC=0⁻⁺π(1800) state is observed in the a₀(980)η and f₀(1500)π decay modes. It has a mass of 1876±18±16 MeV/c² and a width of 221±26±38 MeV/c². The J^PC=2⁻⁺π₂(1880) meson is observed decaying through a₂(1320)η. It has a mass of 1929±24±18 MeV/c² and a width of 323±87±43 MeV/c². Both states are potential candidates for non-exotic hybrid mesons.     

A combined analysis of the hadronic and leptonic decays of the Z

We report on a measurement of the mass of the Z⁰ boson, its total width, and its partial decay widths into hadrons and leptons. On the basis of 25 801 hadronic decays and 1999 decays into electrons, muons or taus, selected over eleven energy points between 88.28 GeV and 95.04 GeV, we obtain from a combined fit to hadrons and leptons a mass of M_z=91.154±0.021 (exp)±0.030 (LEP) GeV, and a total width of Γ_z=2.536±0.045 GeV. The errors on M_z have been separated into the experimental error and the uncertainty due to the LEP beam energy. The measured leptonic partial widths are Γ_ee=81.2±2.6 MeV, Γ_μμ=82.6± 5.8 MeV, and Γ_ττ=85.7±7.1 MeV, consistent with lepton universality. From a fit assuming lepton universality we obtain Γ_ℓ⁺ ℓ⁻ = 81.9±2.0 MeV. The hadronic partial width is Γ_had=1838±46 MeV. From the measured total and partial widths a model independent value for the invisible width is calculated to be Γ_inv=453±44 MeV. The errors quoted include both the statistical and the systematic uncertainties.     

Measurement of the mass of the Λb baryon

In a data sample of four million hadronic Z decays collected with the ALEPH detector at LEP, four Λ_b baryon candidates are exclusively reconstructed in the Λ_b → Λ_c⁺π⁻ channel, with the Λ_c⁺ decaying into pK⁻π⁺, , or Λπ⁺π⁺π⁻. The probability of the observed signal to be due to a background fluctuation is estimated to be 4.2 × 10⁻⁴. The mass of the Λ_b is measured to be 5614±21 (stat.) ± 4 (syst.) MeV/c².     

Study of in flight

An analysis of data on is presented at beam momenta 600 to 1940 MeV/c. There is evidence for an I=1, J^PC=2⁻⁺ resonance in ηηπ⁰ with mass M=1880±20 MeV and width 255±45 MeV, decaying strongly to a₂(1320)η; it is too strong to be explained as the high mass tail of π₂(1670)→a₂(1320)η. There is tentative evidence also for weak decays to f₀(1500)π. It makes a natural partner to the η₂(1860).     

Measurement of the WWγ cross section and direct limits on anomalous quartic gauge boson couplings at LEP

The process e⁺e⁻→W⁺W⁻γ is analysed using the data collected with the L3 detector at LEP at a centre-of-mass energy of 188.6 GeV, corresponding to an integrated luminosity of 176.8 pb⁻¹. Based on a sample of 42 selected W⁺W⁻ candidates containing an isolated hard photon, the W⁺W⁻γ cross section, defined within phase-space cuts, is measured to be: σ_WWγ=290±80±16 fb, consistent with the Standard Model expectation. Including the process , limits are derived on anomalous contributions to the Standard Model quartic vertices W⁺W⁻γγ and W⁺W⁻Zγ at 95% CL: −0.043 GeV⁻²<a₀/Λ²<0.043 GeV⁻², −0.08 GeV⁻²<a_c/Λ²<0.13 GeV⁻², −0.41 GeV⁻²<a_n/Λ²<0.37 GeV⁻².     

Isoscalar quadrupole strength in Ca from the (p,p′α0) reaction at Ep = 100 MeV

The ⁴⁰Ca(p,p′ α) reaction has been studied at an incident proton energy E_p = 99.5 MeV for proton laboratory scattering angles Θ_p^lab = 17°, 23° and 27°. Emission of α particles coincident with the scattered proton has been measured for an angular range Θ_α 0° − 180° relative to the recoil axis. A multipole decomposition for the α₀-decay channel to the ³⁶Ar ground state has been performed from the angular-correlation functions. The energy distribution of the dominating E2 strength deduced in the excitation energy range E_x = 11–21 MeV agrees reasonably well with the results from electron and α-induced α₀-decay investigations. The exhaustion of the E2 energy-weighted sum rule in this channel up to an energy of 17 MeV is 16.1(4.0)%, in accord with the study of the (α, α′ α₀) reaction. However, this value is twice what is found in the (e,e′ α₀) experiment in the same energy region. Thus, the puzzling discrepancy in the E2 strengths derived from electromagnetic and hadronic probes remains unsolved.     

Preparation and electrical properties of the 0,37Li2S-0,18P2S5-0,45LiI glass

A new lithium vitreous electrolyte has been found in the LiI---Li₂S---P₂S₅ system. LiI concentration in the glass, 45% moles, is close to the solubility limit of LiI in 2Li₂S---P₂S₅ glass.The activation energy is of the order of 7.2 Kcal.mole⁻¹ and the conductivity value is 10⁻³ (ohm cm)⁻¹ at 25°C. The conduction is ionic and assured by Li⁺ ions.     

Study of the (9.46) meson in electron-positron annihilations

New data for the reaction e⁺e⁻→(9.46) have been obtained using the DASP detector at the DORIS storage ring. The electronic width Γ_ee is (1.5±0.4) keV. The branching ratio for the decay into muon pairs is (2.5 ± 2.1)%. Energy spectra for inclusive production of hadrons are given.     

Rotational absorption spectrum of methylene fluoride in the 20–100 cm region

The pure rotational spectrum of CH₂F₂ was recorded in the 20–100 cm⁻¹ spectral range and analyzed to obtain rotation and centrifugal distortion constants. Analysis of the data yielded rotation constants: A = 1.6392173 ± 0.0000015, B = 0.3537342 ± 0.00000033, C = 0.3085387 ± 0.00000027, τ_aaaa = −(7.64 ± 0.46) × 10⁻⁵, τ_bbbb = −(2.076 ± 0.016) × 10⁻⁶, τ_cccc = −(9.29 ± 0.12) × 10⁻⁷, T₁ = (4.89 ± 0.20) × 10⁻⁶, and T₂ = −(1.281 ± 0.016) × 10⁻⁶cm⁻¹.     

Coherent Raman and Infrared Studies of Sulfur Trioxide

High-resolution (0.001 cm⁻¹) coherent anti-Stokes Raman scattering (CARS) was used to observe the Q-branch structure of the IR-inactive ν₁ symmetric stretching mode of ³²S¹⁶O₃ and its various ¹⁸O isotopomers. The ν₁ spectrum of ³²S¹⁶O₃ reveals two intense Q-branches in the region 1065–1067 cm⁻¹, with surprisingly complex vibrational–rotational structure not resolved in earlier studies. Efforts to simulate this with a simple Fermi-resonance model involving ν₁ and 2ν₄ states do not reproduce the spectral detail, nor do they yield reasonable spectroscopic parameters. A more subtle combination of Fermi resonance and indirect Coriolis interactions with nearby states, 2ν₄(1=0, ±2), ν₂+ν₄(1=±1), 2ν₂(1=0), is suspected and a determination of the location of these coupled states by high-resolution infrared measurements is under way. At medium resolution (0.125 cm⁻¹), the infrared spectra reveal Q-branch features from which approximate band origins are estimated for the ν₂, ν₃, and ν₄ fundamental modes of ³²S¹⁸O₃, ³²S¹⁸O₂¹⁶O, and ³²S¹⁸O¹⁶O₂. These and literature data for ³²S¹⁶O₃ are used to calculate force constants for SO₃ and a comparison is made with similar values for SO₂ and SO. The frequencies and force constants are in excellent agreement with those obtained by Martin in a recent ab initio calculation.     

No pre-critical enhancement observed in C(π, γ)N(g.s.) at q 2mπ

The cross section and angular distribution for the reaction ¹³C(π⁺, γ)¹³N(g.s.) have been measured from 37 to 85° in the laboratory, at a pion energy of 115.5 MeV. The observed cross section ranges from 320 to 660 nb/sr. These results do not show the large magnitude and wide-angle peaking expected if pre-critical effects due to nascent pion condensation were present. In addition, the observed cross section is less than one-half of the predictions of available theoretical calculations which do not include the pre-critical effect. Data on the reaction ¹H(π⁻, γ)n at T_π = 116.6 MeV were also obtained for calibration purposes. These data agree with expectations based on knowledge of the inverse reaction and previous measurements.     

Interaction of oxovanadium(IV) with carboxylic ligands in aqueous solution: A thermodynamic and visible spectrophotometric study

The hydrolysis of VO²⁺ and the complex with sulfate were studied potentiometrically, spectrophotometrically and calorimetrically, in NaCl aqueous solution (0 < I ≤ 1 mol L^− 1) and at t = 25 °C. The formation of two hydrolytic species VO(OH)⁺ and VO₂(OH)₂²⁺ and one complex with sulfate was found, with log β = − 5.65 for the reaction VO²⁺ + H₂O = VO(OH)⁺ + H⁺, log β = − 7.02 for the reaction 2VO²⁺ + 2H₂O = (VO)₂(OH)₂²⁺ + 2H⁺ and log K = 1.73 for VOSO₄⁰ species (at I = 0.1 mol L^− 1 and t = 25 °C). For these species, using calorimetric data, ΔH and TΔS values were also obtained. By using the above values, interactions of VO²⁺ with acetate (ac), malonate (mal), succinate (suc), 1,2,3-propanetricarboxylate (tca) and 1,2,3,4-butanetetracarboxylate (btc) ligands were studied potentiometrically and spectrophotometrically. The formation of ML⁺, ML₂⁰ and MLOH⁰ for ac; ML⁰, MLH⁺, ML₂²⁻ and ML₂H⁻ for mal; ML⁰, MLH⁺ and MLOH⁻ for suc; ML⁻ and MLH⁰ for tca and ML²⁻, MLH⁻ and MLH₂⁰ for btc were found. Formation constants are reported at I = 0.1 mol L^− 1, together with SIT parameters for the dependence on ionic strength. By visible spectrophotometric measurements, λ_max and ε_max values for the relevant species in solution were determined.     

Line Positions and Intensities of the ν1+ ν2+ 3ν3, ν2+ 4ν3, and 3ν1+ 2ν2Bands of Ozone

Using a Fourier transform spectrometer, we have recorded the spectra of ozone in the region of 4600 cm⁻¹, with a resolution of 0.008 cm⁻¹. The strongest absorption in this region is due to the ν₁+ ν₂+ 3ν₃band which is in Coriolis interaction with the ν₂+ 4ν₃band. We have been able to assign more than 1700 transitions for these two bands. To correctly reproduce the calculation of energy levels, it has been necessary to introduce the (320) state which strongly perturbs the (113) and (014) states through Coriolis- and Fermi-type resonances. Seventy transitions of the 3ν₁+ 2ν₂band have also been observed. The final fit on 926 energy levels withJ_max= 50 andK_max= 16 gives RMS = 3.1 × 10⁻³cm⁻¹and provides a satisfactory agreement of calculated and observed upper levels for most of the transitions. The following values for band centers are derived: ν₀(ν₁+ ν₂+ 3ν₃) = 4658.950 cm⁻¹, ν₀(3ν₁+ 2ν₂) = 4643.821 cm⁻¹, and ν₀(ν₂+ 4ν₃) = 4632.888 cm⁻¹. Line intensities have been measured and fitted, leading to the determination of transition moment parameters for the two bands ν₁+ ν₂+ 3ν₃and ν₂+ 4ν₃. Using these parameters we have obtained the following estimations for the integrated band intensities,S_V(ν₁+ ν₂+ 3ν₃) = 8.84 × 10⁻²²,S_V(ν₂+ 4ν₃) = 1.70 × 10⁻²², andS_V(3ν₁+ 2ν₂) = 0.49 × 10⁻²²cm⁻¹/molecule cm⁻²at 296 K, which correspond to a cutoff of 10⁻²⁶cm⁻¹/molecule cm⁻².     

Elementary reactions of formyl (HCO) radical studied by laser photolysis—transient absorption spectroscopy

Several elementary reactions of formyl radical of combustion importance were studied using pulsed laser photolysis coupled to transient UV–Vis absorption spectroscopy: HCO → H + CO (1), HCO + HCO → products (2), and HCO + CH₃ → products (3). One-pass UV absorption, multi-pass UV absorption as well as cavity ring-down spectroscopy in the red spectral region were used to monitor temporal profiles of HCO radical. Reaction (1) was studied over the buffer gas (He) pressure range 0.8–100 bar and the temperature range 498–769 K. Reactions (2a), (2b), (2c), (3a) and (3b) as well as the UV absorption spectrum of HCO, were studied at 298 and 588 K, and the buffer gas (He) pressure of 1 bar. Pulsed laser photolysis (308, 320, and 193 nm) of acetaldehyde, propionaldehyde, and acetone was used to prepare mixtures of free radicals. The second-order rate constant of reaction (1) obtained from the data at 1 bar is: k₁(He) = (0.8 ± 0.4) × 10⁻¹⁰exp(−(66.0 ± 3.4) kJ mol⁻¹/RT) cm³ molecule⁻¹ s⁻¹. The HCO dissociation rate constants measured in this work are lower than those reported in the previous direct work. The difference is a factor of 2.2 at the highest temperature of the experiments and a factor of 3.5 at the low end. The experimental data indicate pressure dependence of the rate constant of dissociation of formyl radical 1, which was attributed to the early pressure fall-off expected based on the theory of isolated resonances. The UV absorption spectrum of HCO was revised. The maximum absorption cross-section of HCO is (7.3 ± 1.2) × 10⁻¹⁸ cm² molecule⁻¹ at 230 nm (temperature independent within the experimental error). The measured rate constants for reactions (2a), (2b), (2c), (3a) and (3b) are: k₂ = (3.6 ± 0.8) × 10⁻¹¹ cm³ molecule⁻¹ s⁻¹ (298 K); k₃ = (9.3 ± 2.3) × 10⁻¹¹ cm³ molecule⁻¹ s⁻¹(298 and 588 K).     

The rotational-vibrational spectra of HNCS and DNCS : An analysis of the high resolution spectra

Ro-vibrational spectra of HNCS and DNCS have been obtained in the spectral range 300–4000 cm⁻¹ with a practical resolution limit of 0.06 cm⁻¹ in the region 350–1200 cm⁻¹ and 0.15 cm⁻¹ in the region 1200–4000 cm⁻¹. The observed fine structure permitted definitive assignments for some of the ^PQ_K, ^QQ_K, and ^RQ_K branches in both molecules, and yielded sets of rotational constants in substantial agreement with those obtained from recent microwave and far-infrared studies. Precise estimates of the band origins have been obtained and there is evidence of second-order Coriolis coupling between the three bending modes in each molecule. The isolation of the out-of-plane bending modes has lead to a re-assignment of ν₃, ν₄, ν₅, and ν₆ for each molecule. The band origins, uncorrected for Coriolis interaction, are for HNCS and DNCS, respectively. v₁:3538.6 ±0.3, 2644.5±0.5cm⁻¹;v₂:1989.0 ±0.3, 1944.3±0.5cm⁻¹;v₃:857.0 ±0.6, 851.0±0.1cm⁻¹;v₄:615.0 ±0.5, 549.1±0.2cm⁻¹;v₅:469.2 ±0.1, 365.8 ±0.2cm⁻¹;v₆:539.2 ±0.5, 481.0±0.1cm⁻¹;     

Electrical conductivity of Ag/Na ion-exchanged titanosilicate glasses

The Ag₂O–TiO₂–SiO₂ glasses were prepared by Ag⁺/Na⁺ ion-exchange method from Na₂O–TiO₂–SiO₂ glasses at 380–450 °C below their glass transition temperatures (T_g), and their electrical conductivities were investigated as functions of TiO₂ content and the ion-exchange ratio (Ag/(Ag+Na)). In a series of glasses 20R₂O·xTiO₂·(80−x)SiO₂ with x=10, 20, 30 and 40 in mol%, the electrical conductivities at 200 °C of the fully ion-exchanged glasses of R=Ag were in the order of 10⁻⁵ or 10⁻⁴ S cm⁻¹ and were 1 or 2 orders of magnitude higher than those of the initial glasses of R=Na. The glass of x=30 exhibited the highest increase of conductivity from 3.8×10⁻⁷ to 1.3×10⁻⁴ S cm⁻¹ at 200 °C by Ag⁺/Na⁺ ion exchange among them. When the ion-exchange ratio was changed in 20R₂O·30TiO₂·50SiO₂ system, the electrical conductivity at 200 °C exhibited a minimum value of 7.6×10⁻⁸ S cm⁻¹ around Ag/(Ag+Na)=0.3 and increased steeply in the region of Ag/(Ag+Na)=0.5–1.0. When the ion-exchange temperature was changed from 450 to 400 °C, the conductivity of the ion-exchanged glass of x=30 decreased. The infrared spectroscopy measurement revealed that the ion-exchange temperature of 450 °C induced a structural change in the glass of x=30. The T_g of the fully ion-exchanged glass of x=30 was 498 °C. It was suggested that the incorporated silver ions changed the average coordination number of titanium ions to form higher ion-conducting pathway and resulted in high conductivity in the titanosilicate glasses.     

The Fe(α, γ)Ni reaction at excitation energies in the region of the giant dipole resonance

Excitation functions for the ⁵⁶Fe(α, γ₀)⁶⁰Ni and ⁵⁶Fe(α, γ₁)⁶⁰Ni reactions have been measured at 90° to the beam direction over the bombarding energy range 8.0–17.6 MeV. Gamma-ray angular distributions were measured at ten bombarding energies. Excitation functions for the ⁵⁹Co(p, γ₀)⁶⁰Ni and ⁵⁹Co(p, γ₁)⁶⁰Ni reactions were measured over the range E_x = 16.58–16.92 MeV and compared with the (α, γ) data. The angular distribution data indicate that the (α, γ₀) and (α,γ₁) reactions proceed through 1⁻, and 1⁻ and 3⁻ states, respectively. The (α, γ) excitation functions are discussed with respect to isospin splitting of the ⁶⁰Ni giant dipole resonance. The fine structure observed in the excitation functions is shown to be most probably due to Ericson fluctuations. The gross (α, γ) cross sections are shown to be in reasonable agreement with the results of calculations made using the theory of Hauser and Feshbach assuming excitation of the giant dipole resonance.     

Determination of the Splitting of the 6a0 and 6b0 Bands of C-Hexadeuterobenzene in a Supersonic Jet

By using resonance-enhanced two-photon ionization, rotationally resolved spectra of the 6¹₀ band of ¹²C₆D₆ and (¹³C¹²C₅D₆ molecules have been obtained for the first time at a rotational temperature of 0.7 K in a pulsed supersonic beam. From the former, the values of B″ = 0.1573 ± 0.0008 cm⁻¹, B′ = 0.1508 ± 0.0008 cm⁻¹, and ξ′ = −0.412 ± 0.050 have been derived for rotational and Coriolis constants in the lower and upper levels of ¹²C₆D₆. Also, the spectra corresponding to ¹²C₆H₆ and ¹³C¹²C₅H₆ have been measured and the values B″ = 0.1892 ± 0.0008 cm⁻¹, B′ = 0.1815 ± 0.0008 cm⁻¹, and ξ′ = −0.586 ± 0.050 have been obtained for ¹²C₆H₆, in agreement with previous results. Rotational constants of ¹³C labeled benzene molecules have been geometrically deduced from the constants obtained. Experimental isotopic shifts of the vibronic origins of the 6a¹₀ and 6b¹₀ bands have been determined. There is agreement with previous ¹³C-benzene-h₆ data. The present results are −0.91 ± 0.05 and 3.09 ± 0.05 cm⁻¹ for ¹³C¹²C₅D₆ and −1.64 ± 0.05 and 2.64 ± 0.05 cm⁻¹ for ¹³C¹²C₅H₆. The splittings of vibrational modes 6b and 6a in the ¹B_2u state are 4.00 ± 0.10 cm⁻¹ for ¹³C¹²C₅D₆ and 4.28 ± 0.10 cm⁻¹ for ¹³C¹²C₅H₆.     

Direct measurement of the pseudoscalar decay constant

The absolute branching fraction for the decay D⁺→μ⁺ν has been directly measured based on a data sample of about 33 pb⁻¹ collected around with the BES-II detector at the BEPC collider. A total of 5321±149±160 D⁻ mesons are reconstructed in nine hadronic decay modes. In the system recoiling against these singly tagged D⁻ mesons, 2.67±1.74 purely leptonic decay events of D⁺→μ⁺ν_μ are observed. Those yield the branching fraction of , and a corresponding value of the pseudoscalar decay constant .