Nonlinear forward scattering of resonant laser light from excited neon systems

We investigate forward scattering induced by a powerful single mode dye laser interacting with excited neon systems. We present experimental data obtained with the three transitions: 1s ₄(J=1)-2p ₃(J=0), 1s ₂(J=1)-2p ₁(J=0), and 1s ₅(J=2)-2p ₄(J=2). The lineshape dependences on the gas pressure, the laser power and the laser field fluctuations are discussed in the context of published theories. Our data resemble the calculated lineshapes in which fluctuations in the interaction processes between atoms and laser fields are taken into account. In atomic systems having more complex level degeneracies [1s ₅(J=2)-2p ₄(J=2)] signal structures expected from higher order nonlinear coherences can occur. To theoretically reproduce these lineshapes a simple J=1J=0 model is fully appropriate provided that the level with J=1 has a narrow width.     

四能级原子系统中非线性电磁感应吸收的理论研究

在n型四能级原子系统中,研究了电磁感应吸收的非线性理论.结果表明:探测光的拉比频率和衰减分配系数A影响非线性吸收,进而影响介质吸收.当探测光光强较弱时,介质吸收和线性吸收一致,均表现为电磁感应吸收特征;当探测光光强增大时,介质吸收和线性吸收不再一致,介质吸收曲线将会呈现出烧孔现象;当探测光光强增大到控制光(或信号光)光强时,介质吸收表现出很大的增益现象.同时,非线性吸收受到衰减分配系数A的影响,即使在探测场很弱的条件下,随着A值的减小,介质吸收由电磁感应吸收现象表 关键词： 电磁感应吸收 非线性吸收 增益现象 n型四能级原子系统     

Dark resonances for ground-state transfer of molecular quantum gases

One possible way to produce ultra-cold, high-phase-space-density quantum gases of molecules in the rovibronic ground state is given by molecule association from quantum-degenerate atomic gases on a Feshbach resonance and subsequent coherent optical multi-photon transfer into the rovibronic ground state. In ultra-cold samples of Cs₂ molecules, we observe two-photon dark resonances that connect the intermediate rovibrational level |v=73,J=2〉 with the rovibrational ground state |v=0,J=0〉 of the singlet X ¹ Σ _g ⁺ ground-state potential. For precise dark resonance spectroscopy we exploit the fact that it is possible to efficiently populate the level |v=73,J=2〉 by two-photon transfer from the dissociation threshold with the stimulated Raman adiabatic passage (STIRAP) technique. We find that at least one of the two-photon resonances is sufficiently strong to allow future implementation of coherent STIRAP transfer of a molecular quantum gas to the rovibrational ground state |v=0,J=0〉.     

Local scaling transformation function and atomic shell structure in density functional theory

The method of local scaling transformation in density functional theory calculates a transformation function (TRF) in order to generate an optimized atomic N-electron wave function from a trial density and a reference density/wave function. The TRFsf(r) for several atomic systems are studied and it is observed that the number of minima in df(r)/dr equals the number of atomic shells, except whenρ=ρ ₀ andf=r.     

Nonclassical effects in a highly nonlinear generalized homogeneous Dicke model

An intensity dependent nonlinear coupling model of N two-level atoms (generalized Dicke model) interacting dispersively with a bimodal cavity field via two-photon transitions is investigated in a scenario where the rotating wave approximation is assumed. The model becomes homogeneous in the sense that the spin transition frequency is the same for all atoms and the coupling constants emerging from the collective interactions of the atomic system with the cavity field depend only on the particular radiation field mode. This allows us to represent the Dicke Hamiltonian entirely in terms of the total angular momentum J. It is assumed that, initially, the atomic system and the field are in a disentangled state where the field modes are in Glauber coherent states and the atomic system is a superposition of states |JM〉 (Dicke states). The model is numerically tested against simulations of normal squeezing variance of the field, squeezing factors based on the Heisenberg uncertainty principle, along with the statistical properties of the light leading to the possible production of nonclassical effects, such as degree of second-order coherence in the modes, degree of intermode correlation, as well as violation of the Cauchy–Schwartz inequality. Analytical expression of the total density operator matrix elements at t>0 shows the present nonlinear model to be strongly entangled, which is reflected in the time evolution of the linear entropy, where the superposition states are reduced to statistical mixtures. Thus, the present generalized Dicke model does not preserve the modulus of the Bloch vector. The computations, performed in the weak coupling and strong field limits, were conducted via second-order Dyson perturbative expansion of the time evolution operator matrix elements for the totality of the angular momentum states of the atomic system.     

Localization of atoms in light fields: Optical molasses,adiabatic compression and squeezing

We present a theoretical study of the localization1 of atoms with an angular momentumJ _g=3 toJ _e=4 transition (e.g., chromium atoms) in quantized optical molasses created by two counterpropagating linearly polarized laser beams. We study the localization as a function of the potential depth, the angle between the polarizations and the interaction time with the molasses in the low-intensity limit, and discuss the possibility of adiabatic compression and squeezing of the atomic distribution.Dedicated to H. Walther on the occasion of his 60th birthday     

Raman heterodyne Ramsey spectroscopy in a Samarium atomic beam

A novel optical heterodyne technique for Raman Ramsey spectroscopy of atomic radio-frequency resonances in an atomic beam is reported. The method relies on coherent resonance Raman transitions to optically excite and probe sublevel coherence in atomic ground states using two separated atom-field interaction regions. First experimental results obtained with the use of Zeeman sublevels in the Samarium =570.68 nm (J=1)–(J=0) transition are discussed.     

Surface optical waves at the boundary with a nonlinear Kerr medium

A rigorous solution consistent with a plane wave approximation is given to the boundary problem for Maxwell’s equations for surface optical waves at the boundary with a nonlinear Kerr medium. Exact formulas for the flux intensity (J ₀) and energy density (W ₀) of these waves are derived depending on the parameters of the adjacent media and the propagation constant (ξ). It is shown that these variables as functions of ξ have minima. Thus, J ₀ and W ₀ increase sharply as the propagation constant deviates from the minimum value ξ_min. Their values are greater, the larger the difference between the dielectric constants of the linear and nonlinear media is. An expression for the propagation velocity of a nonlinear surface wave is also obtained.     

非等同双原子与双模腔场相互作用模型中原子布居的时间演化

研究了两个非等同二能级原子与双模腔场耦合系统中原子能级布居的时间演化规律. 并详细讨论了两个原子与双模腔场的相对耦合常数(R=g₁/g₂)和腔场的初态对原子能级布居数反转的影响. 关键词： 双模腔场 双原子体系 原子布居     

Exotic Isomers in Deformed Atomic Nuclei

Excited states of atomic nuclei can have long half lives, due to the angular-momentum couplings of unpaired nucleons. Such isomeric states provide opportunities for exploring novel nuclear physics, astrophysics and physics at the atomic/nuclear interface. This review focuses on the properties of isomers in deformed nuclei, and emphasises the importance of axial symmetry in preserving the integrity of the K quantum number. A region of neutron-rich nuclei around ¹⁸⁸Hf (Z=72, N=116) is predicted to have exceptional isomer properties, and experimental advances are now opening up this region to detailed investigation. This revised version was published online in July 2006 with corrections to the Cover Date.     

Optical nutation and photon echo by phase or amplitude shift of light waves

Optical nutation and photon echo caused by phase shift of a light wave incident on a resonant medium are considered. The case of simultaneous ultrashort perturbation of phase and amplitude is also treated. It is shown that a change of linear to circular polarization of incident light waves gives rise to an increase of the period and the decay time of optical nutation on the resonant atomic transitions J→J. On the contrary, the above mentioned period and decay time in the same situation are decreased on the resonant atomic transitions with the moment change J?J+1. This law in optical nutation can be taken as a base of the method for experimental identification of the atomic and molecular transitions. Moreover, the comparison of the theoretical and experimental optical nutation curves allows the probability of spontaneous emission to be determined.     

On light supernuclei

The possible existence of charmed analogues of the YN and light hypernuclear systems are investigated using phenomenological one-boson-exchange potential and the SU(4) symmetry. Bound light supernuclei such as C₁N (I=3/2, J=0) and C₁NN(I=2, J=1/2) C₀NN (I=1, J=1/2, and I=0, J=1/2 or 3/2) are predicted with reasonable binding energies using Faddeev formalism for the three body systems.     

Rovibrational laser control targeting a dark state in acetylene. Simulation in the Ns = 1, Nr = 5 polyad

Optimal control theory in the Liouville space is used to perform rovibrational control by means of a laser pulse in a polyad of acetylene in order to populate a dark vibrational state. The initial mixed state is a truncated Boltzmann distribution of rotational levels from J=27 to J=31 of the ground vibrational state. The target state is a rotational equidistribution of levels ranging from J=28 to J=32 of the first excited vibrational dark state including quanta of energy in each bending modes, with positive vibrational angular momenta. The simulation is performed by using a manifold of eigenstates of a full-dimensional Hamiltonian calibrated by high precision spectroscopy known as the global acetylene Hamiltonian [B. Amyay et al., J. Chem. Phys. 131, 114301 (2009)]. The control is successful as an Uhlmann's fidelity of 0.98 is reached.     

Two dimension selective coherent population trapping controlled by a phase shift

Two-dimensional laser cooling based on velocity-selective coherent population trapping is investigated theoretically for the J _g=1J _e=0 atomic transition. Wavevectors and polarizations of three laser beams are chosen to realize a coherent superposition of three degenerate ground states. For the first time in laser cooling, use is made of the electric field phases to realize coherent population trapping selective in two dimensions. Numerical solutions and analytic estimates are presented for laser cooling of helium atoms.     

Modulated Phase of a Potts Model with Competing Binary Interactions on a Cayley Tree

We study the phase diagram for Potts model on a Cayley tree with competing nearest-neighbor interactions J ₁, prolonged next-nearest-neighbor interactions J _p and one-level next-nearest-neighbor interactions J _o . Vannimenus proved that the phase diagram of Ising model with J _o =0 contains a modulated phase, as found for similar models on periodic lattices, but the multicritical Lifshitz point is at zero temperature. Later Mariz et al. generalized this result for Ising model with J _o ≠0 and recently Ganikhodjaev et al. proved similar result for the three-state Potts model with J _o =0. We consider Potts model with J _o ≠0 and show that for some values of J _o the multicritical Lifshitz point be at non-zero temperature. We also prove that as soon as the same-level interactionJ _o is nonzero, the paramagnetic phase found at high temperatures for J _o =0 disappears, while Ising model does not obtain such property. To perform this study, an iterative scheme similar to that appearing in real space renormalization group frameworks is established; it recovers, as particular case, previous work by Ganikhodjaev et al. for J _o =0. At vanishing temperature, the phase diagram is fully determined for all values and signs of J ₁,J _p and J _o . At finite temperatures several interesting features are exhibited for typical values of J _o /J ₁.     

Calculation of the E.S.R. spectrum shape of the dynamic biradical system

The E.S.R. spectrum shape of a dynamic biradical system is calculated by means of the density spin-matrix formalism. The biradical is treated as a system which has two conformations characterized by the different values of the exchange integrals J=J ₁ and J=J ₂ and the lifetimes τ₁ and τ₂ respectively. The influence of both the rate and the strength of exchange interactions on the shape of the spectrum is discussed. Criteria to distinguish the spectra of the cases of both slow and fast exchange are discussed.     

Optical surface <Emphasis Type="Italic">TM</Emphasis>-waves at the boundary of a nonlinear Kerr-type medium

Solutions for a nonlinear system of Maxwell’s equations and for a corresponding boundary problem describing the propagation of a surface TM-wave (p-polarization) along an interface with an optically nonlinear Kerr-type medium are presented. An analytical expression for the intensity of an integrated flux J₀ carried by such a wave along the interface between two media has been derived as a function of both the wave propagation constant ξ and the optical characteristics of the adjacent media. It is shown that flux intensities corresponding to the same values of the propagation constant ξ are much smaller for p-polarization than for s-polarization.     

Reflection and refraction of light by a system of interfering atomic states

The boundary problem of nonlinear optics was investigated for a trial wave reflected (refracted) by an excited region of a nonlinear medium considered as a system of multilevel atoms in the spectrum of which there are two closely-spaced energy levels excited by a powerful quasi-resonant radiation. It is shown that under interference conditions of the atomic states in the field of the trial and resonance waves there exist three types of waves: an inverse wave and two polarization waves. By way of extension of the Ewald-Oseen procedure to this case a formula for the complex refractive index of a nonlinear medium for the three types of waves as well as a generalized extinction theorem have been obtained. It is shown that the trial wave can be amplified without inversion of the interfering atomic states and that the refractive index can be markedly changed at certain concentrations of atoms in the medium. General formulas for the amplitudes of the reflected and refracted waves have been obtained. Ul’yanovsk State University, 42, Tolstoi Str., Ul’yanovsk, 432700, Russia. Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 65, No. 4, pp. 568–575, July–August, 1998.     

Manifestation of higher polarization moments in the dipole emission under conditions of stepwise excitation and anisotropic collisions

The induction of higher polarization moments-the octupole orientation and the hexadecapole alignment—in the case of two-step excitation of atoms through dipole transitions and their manifestation in the polarization of dipole emission under conditions of anisotropic collisions are studied. For all channels of the two-step excitation process J ₀→J ₁ J, the efficiencies of production of higher polarization moments with integer and half-integer angular momenta from J=2 to J=7 through the absorption of linearly or circularly polarized light are calculated. The rates of collisional relaxation and interconversion of higher polarization moments, for both orientation and alignment, as functions of frequency detuning of the laser line from the center of the Doppler profile are calculated. The theory is illustrated by an example of two channels of excitation of the atomic state J=2 by circularly polarized light: J ₀=0→J ₁=1J=2 and J ₀=3→J 1=2 (or 3)→J=2. In the first case, the octupole orientation enhances or attenuates the signal of circular polarization depending on the laser frequency detuning. In the second case, it represents the only source producing orientation and circular polarization of the emitted light.