Dephasing processes as studied by two pulse photon echoes and photochemically accumulated echoes: The question of spectral diffusion in a doped organic polymer matrix

Two pulse photon echoes (2PPE) and photochemically accumulated stimulated photon echoes (PASPE) were measured under identical conditions for the system octaethylporphin in a polystyrene matrix. Experiments at 1.9 K show that both echoes have a different decay behavior. Whereas the 2PPE-signal decays with a time constant of 1300 ps, the PASPE-signal decays faster with a time constant of 600 ps. The different temporal behavior of both signals is tentatively attributed to spectral diffusion.     

强电磁脉冲信号激励下复杂目标的散射

 用时域有限差分法仿真了某飞行器缩比模型及该模型涂敷雷达吸波材料的散射特性,得到了鼻锥方向、侧向和后向ns级脉冲激励下模型的时域响应和频域雷达散射截面;并在外场用ns级脉冲源进行了该金属模型的探测实验。仿真与外场实验结果均得到了模型的鼻锥方向回波幅度最小,侧向最大;鼻锥方向回波脉宽最宽,侧向最窄的结论。研究结果表明：外形隐身和材料隐身对ns或亚ns级窄脉冲的隐身效果不明显,ns或亚ns级窄脉冲能发现和识别隐身目标。     

Electron spin-echo experiments in photo-excited triplet states in an external magnetic field

Electron spin-echo experiments in the photo-excited triplet states of quinoxaline-d₆ and naphthalene-d₈ at 1·2 K in an external magnetic field are presented. These include two-pulse Hahn echoes, three-pulse stimulated echoes and Carr-Purcell pulse-echo trains. The decay of the Hahn and stimulated echoes as a function of pulse interval yields measures of the spin relaxation times. Furthermore, the Hahn echo is used to obtain E.P.R. line shapes and the dynamics of the triplet sublevel populations. The angular dependence of the Hahn echo is also investigated. The Hahn echo decay time and decay modulation suggest the kind of role played by nuclear spins in the loss of electron spin phase coherence. Some promising characteristics of the pulse method are discussed.     

Multiple Nonlinear Stimulated Echoes

Three-pulse sequences in the presence of magnetic field gradients at high magnetic fields produce multiple nonlinear stimulated echoes (NOSE) at timesnτ₁after the third pulse, wherenis an integer and τ₁the interval between the first two pulses. These phenomena are due to the demagnetizing field produced by the spatial modulation of the nuclear magnetization arising in the sample after the first two pulses. The theory is presented and compared with experiments. The dependence of the NOSE amplitudes on the flip angles and on the pulse intervals is described. Implications for multidimensional NMR experiments based on sequences of three or more pulses in the presence of field gradients are discussed.     

Femtosecond primary and stimulated photon echoes in a dye-doped polymer film at room temperature

The signals of both primary and stimulated femtosecond photon echoes are observed and investigated in a dye-doped polymer film at room temperature using a modernized femtosecond echo-spectrometer. It should be noted that stimulated photon echo in the solid-state sample is observed for the first time at such a high temperature. Experimentally obtained decay curves of these signals have a nonexponential character. The spectra of these echo signals are also measured. It is found that the spectrum of the primary photon echo is short-wave shifted with respect to the spectrum of excitation. This can be used for the coherent laser cooling of a sample. The spectrum of the stimulated photon echo is also shifted to the short-wave range relative to the spectrum of excitation, but its shift is much less than that of the primary photon echo. The experiment shows that the femtosecond echo signals at room temperature are excited via the phonon-side band of the absorption line.     

Double PGSE NMR with Stimulated Echoes: Phase Cycles for the Selection of Desired Encoding

When two pairs of position-encoding pulses are used in a pulsed gradient spin echo (PGSE) NMR experiment, it is possible to examine velocity fluctuations. The one-dimensional version of double PGSE NMR uses identical pulse pairs whose amplitudes are stepped simultaneously. In the two-dimensional version (VEXSY) the pulse pairs are stepped independently, resulting in a velocity exchange spectrum. A key limitation in such experiments is transverse relaxation, so that stimulated echoes are often used as the method of choice. It is shown here that the use of stimulated echoes results in a superposition of signals arising from different magnetization pathways such that the spin phases may reflect both the sum and difference of displacements over the pulse pair encoding times, as well as the displacement over the exchange time between the pulse pairs. A phase cycle scheme that selects desired encodings as required is demonstrated.     

双侧回波联合的合成孔径声呐运动补偿算法

利用单侧回波可估计合成孔径声呐基阵的斜距误差,但无法区分横荡误差和升沉误差。针对此问题,提出了一种双侧回波联合的运动补偿方法。该方法首先根据双侧基阵运动误差的几何关系,建立了双侧基阵的运动误差模型,再结合偏移相位中心算法估计基阵的横荡误差和升沉误差,最后利用所估计的运动误差对不同掠射角上的回波进行运动补偿。仿真结果表明:该方法能精确估计双侧基阵的运动误差,其估计值与实际值的偏差为10-4 m左右,估计结果的标准差接近克拉美罗下界;对回波进行运动补偿后,能获得比基于单侧回波运动补偿方法更好的成像效果。水下球串目标的湖试数据的成像结果显示,与基于单侧回波的运动补偿方法相比,所提方法能更好地抑制图像的散焦现象。      

Studies of phase characteristics of various photon echoes with a phase sensitive detection method

Various optical coherent transient signals in ruby have been examined by using an optical phase sensitive detection (PSD) technique. The PSD is performed by comparing the phase of the heterodyne beat signals obtained by the Stark switching technique with that of a local oscillator whose frequency is equal to the heterodyne beat frequency. The optical FID, two-pulse photon echoes, radiation locked echoes and notched echoes have been detected as υ-mode signals with small u-mode signals probably due to the asymmetry of the inhomogeneous broadening. The dependence of the phase of the radiation locked and notched echoes upon the driving pulses is also examined. The experimental results are in good agreement with theoretical predictions based on Bloch equations.     

Millimeter-Wave Signal Generation and Harmonic Upconversion Through PM-IM Conversion in Chirped Fiber Gratings

A novel technique for generating millimeter-wave signals through phase-to-intensity modulation conversion in chirped fiber gratings is proposed and demonstrated. Experimental results on generating a 28 G Hz signal using harmonics orders from 7th to 10th are provided. Excellent phase-noise performance (87 dBc Hz @ 10KHz) is demonstrated. It is also demonstrated that this technique may be efficiently used for harmonically upconverting intermediate frequency signals to the millimeter-wave band. Bit-error-rate measurements for different modulation format (QPSK MQAM) signals, which were upconverted employing the PM-IM conversion technique, show very good performance (< 10 ^{- 9}) and transparency to the modulation format.     

Categories of coherence pathways for the CPMG sequence

The CPMG sequence has been extremely useful for efficient measurements of NMR signal, spin-spin relaxation, and diffusion, particularly in inhomogeneous magnetic fields, such as when samples are outside the magnet and RF coil. Due to the inaccuracy of the pulses and the off-resonance effects, the CPMG echoes have contributions from the Hahn echo as well as signals that are similar to stimulated echoes. The systematic understanding of the CPMG pulse sequence requires decomposing the magnetization dynamics into different coherence pathways. In this paper, we describe a method to classify the CPMG coherence pathways and illustrate the nature of these types of pathways. This classification shows that direct echo and stimulated echoes are the major contribution to the CPMG signal. It also provides a clear understanding of the effect of restricted diffusion in porous media.     

On the problem of field-gradient NMR measurements of intracrystalline diffusion in small crystallites--water in NaA zeolites as an example

Necessary conditions for measuring intracrystalline diffusion in small crystal size systems via field-gradient NMR are discussed. As an illustrative case self-diffusion coefficients of water adsorbed in NaA zeolites (average crystal diameter about 1 μm) have been measured by ¹H-NMR stimulated echoes in static magnetic field gradients of up to 180 T/m in the temperature range of 254–344 K. Obtaining intracrystalline diffusion coefficients necessitates a sufficiently high spatial resolution only provided by such large field gradients.     

浅海双基地有源探测调频信号直达波消除

双基地有源探测常采用长脉宽探测信号以获取更高的时间增益,容易导致回波弱信号被强直达波信号掩蔽而影响回波检测.针对长调频信号直达波的干扰,提出基于分数阶傅里叶变换(FrFT)的直达波消除方法.该方法利用调频信号在时频分布上的稀疏性,通过对接收信号进行分数阶傅里叶变换分离直达波和回波信号然后在变换域对直达波信号进行去除.远...     

Parametric multiecho proton spectroscopic imaging: Application to the rat brain in vivo

A parametric multiecho variant of proton spectroscopic imaging (SI) is presented using a multiecho SI sequence with uniform phase-encoding of all echoes within each echo train. The acquisition of SI data sets at different echo times (TE) increases the amount of information obtained within the same total measuring time as in standard SI measurements. The gain in information can be used: (a) to choose the most appropriate TE for each metabolite signal with respect to T₂, spin coupling, or problems caused by peak overlap; (b) to measure the relaxation time T₂ of metabolite signals with high spatial resolution; or (c) to improve the signal-to-noise ratio for metabolite signals with long T₂ values by adding spectra calculated from consecutive echoes. The method was tested in vivo on healthy rat brain and applied to study metabolic changes in rat brain lesions.     

Measuring sound scattering coefficients of uneven surfaces in a reverberant workplace – Principle and validation of the method

In workplaces, wall facings are often based on periodic or aperiodic sound scattering surfaces. It is necessary to develop acoustic characterization methods for these kinds of walls to predict the acoustic pressure cartography in the room in order to improve the acoustical treatment. However, this characterization is quite difficult because of the partially reverberant conditions. We developed a measurement system which determines in situ the sound scattering coefficients of relief surfaces. The measurement method, originally operating in free-field conditions, was adapted for indoor use. To overcome problems of parasite echoes coming from reverberation and from noisy sources present on the site, we developed a dedicated emission/reception system. An acoustic antenna with constant directivity over the full frequency range allows spatial filtering of the parasite echoes and an impulsive sound source enables the use of a broad temporal window, resulting in adequate time separation of the different signals received by the antenna. Measurements of the sound scattering coefficient of a corrugated panel were carried out for several incidence angles in free-field and in a noisy workshop and allowed the in situ validation of this system.     

Reconfigurable photonic differentiators based on all-optical phase modulation and linear filtering

We theoretically propose a novel scheme to implement two types of optical differentiators using all-optical phase modulation and linear filtering. Differences between the two differentiators rely on whether the differentiated signals are formed on the optical intensity or optical field of the output signal, which in turns depends on the relative shift between the probe wavelength and the closest notches of a linear filter. A proof-of-concept experiment is carried out using a semiconductor optical amplifier and a fiber-based delay interferometer (DI). Both differentiators are obtained for periodical Gaussian pulses and pseudo random non-return-to-zero signals at various data rates. Defined as the mean absolute deviation of the measured waveform from the ideal one, total average errors of less than 18% are observed in all cases. The impact of probe wavelength on the total average errors is investigated. Due to periodical feature of the DI spectrum, we also demonstrate the capability of multi-channel differentiation.     

The influence of stimulated echoes on contrast in fast spin-echo imaging

Tissue contrast obtained using fast spin-echo (FSE) and conventional spin-echo (SE) sequences is not identical and a number of mechanisms are thought to contribute to these contrast differences. The effect of stimulated echoes has previously been apparently ruled out as a contributing mechanism. Signal-to-noise ratios of single-slice matched FSE and conventional SE sequences were compared in aqueous solutions of CuSO₄, Cr₂(SO₄)₃ and MnSO₄ with various T₁ and T₂ values. Enhancement of the FSE signal was observed in short T₂ solutions and the effect was greater in samples where the T₁ to T₂ ratio was high. Reducing the refocusing pulse flip angle to increase the contribution from stimulated echoes also resulted in slightly increased enhancement. Experimental results were verified by computer simulations. Our results show that stimulated echoes do contribute to the contrast differences between FSE and conventional SE images and may be significant in the imaging of brain hemorrhage.     

Nuclear magnetic resonance in inhomogeneous magnetic fields

The response of the spin system has been investigated by numerical simulations in the case of a nuclear magnetic resonance (NMR) experiment performed in inhomogeneous static and radiofrequency fields. The particular case of the NMR-MOUSE was considered. The static field and the component of the radiofrequency field perpendicular to the static field were evaluated as well as the spatial distribution of the maximum NMR signal detected by the surface coil. The NMR response to various pulse sequences was evaluated numerically for the case of an ensemble of isolated spins (1/2). The behavior of the echo train in Carr-Purcell-like pulse sequences used for measurements of transverse relaxation and self-diffusion was simulated and compared with the experiment. The echo train is shown to behave qualitatively differently depending on the particular phase schemes used in these pulse sequences. Different echo trains are obtained, because of the different superposition of Hahn and stimulated echoes forming mixed echoes as a result of the spatial distribution of pulse flip angles. The superposition of Hahn and stimulated echoes originating from different spatial regions leads to distortions of the mixed echoes in intensity, shape, and phase. The volume selection produced by Carr-Purcell-like pulse sequences is also investigated for the NMR-MOUSE. The developed numerical simulation procedure is useful for understanding a variety of experiments performed with the NMR-MOUSE and for improving its performance. Copyright 2000 Academic Press.     

Modulated spatial transmission signals in the photonic bandgap

This paper describes the spatial transmission of electromagnetically induced transparency and four-wave mixing signals in the photonic bandgap structure, which are modulated using the adjustable parameters of light fields. The spatial transmission patterns of the relevant signals are experimentally investigated with respect to the optical nonlinear Kerr effect that occurs in the modulation process. The experimental results reveal the spatial transmission patterns of the probe transmission and the four-wave mixing signals, such as focusing, defocusing, shifting, and spatial splitting. This study explains how the tunable parameters of light fields and their interactions with each other can regulate the spatial transmission of the light fields by changing the refractive indices of media, which provides a new research perspective and a degree of experimental technology support for more efficient all-optical communications.     

基于双边带调制的频率扫描干涉型激光测距技术

提出并论证了一种基于双边带调制的双扫频干涉测距技术,利用电-光双边带调制产生的-1和+1阶边带分别作为扫描方向相反的两个扫频信号,在接收端各获得一个频率与相对距离相关的拍频信号,通过将这两个拍频信号相乘的方式来减小由光路中扰动引起的测量误差.利用Optisystem软件进行系统仿真,结果表明,该方法能够有效抑制由于光路中扰动产生的测量误差.设计了实验验证系统,在光路中引入小幅振动作为扰动时,该方法对扰动的抑制比超过14dB,有效地提升了测距准确度.     

Femtosecond photon echo in a dye-doped polymer film and the possibility of coherent optical cooling

The signals of primary and stimulated femtosecond photon echoes are investigated in a dye-doped polymer film at room temperature. The homogeneous S ₀ → S ₁ spectral line width, which is due to the interaction between the impurity molecules and the quasi-local low-frequency modes, is estimated (≈5 × 10¹² Hz). Special attention is paid to the study of spectra of femtosecond echo signals. The short-wave shifts of these spectra, with respect to the spectrum of femtosecond exciting pulses, are observed. These shifts indicate that the anti-Stokes regime of femtosecond pulse emission is realized. Therefore, the coherent regime of laser cooling of solids appears to be possible. The prospects of using of this new cooling regime in the function of a solid-state optical refrigerator are discussed.