Non-collinear phase of a singlet–triplet magnet

The spin subsytem of copper oxides within the model of polar singlet–triplet Jahn–Teller centers is described by the Hamiltonian of a singlet–triplet magnet with multiparametric (non)collinear spin arrangements. Using the modified mean-field approximation we analyze the conditions of an appearance of the non-collinear phase. Certain static and dynamic properties of the new phase are considered.     

Effect of in-plane magnetic field on spin polarization in the presence of the Dresselhaus spin–orbit effect

In this paper, we theoretically study the effect of the in-plane magnetic field on spin polarization in the presence of the Dresselhaus spin–orbit effect. It is shown that the large spin polarization can be achieved in such a nanostructure due to the effects of both the Dresselhaus spin–orbit term and the in-plane magnetic field, but the latter plays a main role in the tunneling process. It is also shown that with the increase of in-plane magnetic field, the degree of spin splitting obviously becomes larger.     

Thermally induced spin polarization and thermal conductivities in a spin–orbit-coupled two-dimensional electron gas

The thermal conductivities and spin polarization induced by the temperature gradient are investigated in a Rashba spin–orbit-coupled two-dimensional electron gas. In this spin–orbit-coupled system in the presence of nonmagnetic or magnetic electron–impurity scattering, the Wiedemann–Franz law still holds. However, the spin polarization induced by the temperature gradient strongly depends on the property of impurities. The components of spin accumulation both perpendicular and parallel to the direction of the temperature gradient, and the thermally induced charge Hall conductivity may be nonzero for magnetic disorders.     

Theory of spin polarization in mesoscopic spin–orbit coupling systems

We establish a general formalism of the bulk spin polarization (BSP) and the current-based spin polarization (CSP) for mesoscopic ferromagnetic and spin–orbit interaction (SOI) semiconducting systems. Based on this formalism, we reveal the basic properties of BSP and CSP and their relationships. The BSP describes the intrinsic spin polarized properties of devices. The CSP depends on both intrinsic parameters of device and the incident current. For the non-spin-polarized incident current with the in-phase spin-phase coherence, CSP equals to BSP. We give analytically the BSP and CSP of several typical nanodevice models, ferromagnetic nanowire, Rashba nanowire and rings. These results provide basic physical behaviors of BSP and CSP and their relationships.     

Saturation recovery electron spin–lattice relaxation studies on benzene anion radical and its derivatives: application of Kivelson–Orbach mechanism of electron spin relaxation

The role of low-lying excited states on the spin–lattice relaxation times (T₁) of organic radicals has been investigated. To test the applicability of Kivelson's electric field fluctuation model (D. Kivelson, J. Chem. Phys. 45, 1324 (1966)), based on the Orbach mechanism of spin relaxation, the T₁s of the anion radicals of benzene, benzene-1-d, toluene, ethyl benzene, isopropyl benzene, t-butyl benzene, p-xylene, 1,2,4-trimethyl benzene and 1,3,5-trimethyl benzene in liquid solutions, with potassium cation as the counter ion, have been measured by the pulse saturation recovery technique. The energy gap between the ground and the first excited electronic states changed with the substitutions to different extent. The spin–lattice relaxation rates showed correlation with this energy gap. Anion radicals of benzene and benzene-1-d showed the shortest T₁ among the radicals studied here. A small but measurable energy splitting due to the deuterium substitution in benzene-1-d radical was obtained from the temperature dependence of T₁. Spin–lattice relaxation times of benzene anion measured here decreased monotonically in the range of ?60 to ?125 °C, in contrast to some reported claims of very unusual temperature dependence, based on the continuous wave microwave power saturation studies. Our results also showed that the ion pairing between benzene anion and potassium cation did not significantly influence the spin–lattice relaxation times.     

Intrinsic electron spin relaxation due to the D'yakonov–Perel' mechanism in monolayer MoS2

Intrinsic electron spin relaxation due to the D'yakonov–Perel' mechanism is studied in monolayer Molybdenum Disulphide. An intervalley in-plane spin relaxation channel is revealed due to the opposite effective magnetic fields perpendicular to the monolayer Molybdenum Disulphide plane in the two valleys together with the intervalley electron–phonon scattering. The intervalley electron–phonon scattering is always in the weak scattering limit, which leads to a rapid decrease of the in-plane spin relaxation time with increasing temperature. A decrease of the in-plane spin relaxation time with the increase of the electron density is also shown.     

Gate control of quantum dot-based electron spin–orbit qubits

We investigate theoretically the coherent spin dynamics of gate control of quantum dot-based electron spin–orbit qubits subjected to a tilted magnetic field under electric-dipole spin resonance (EDSR). Our results reveal that Rabi oscillation of qubit states can be manipulated electrically based on rapid gate control of SOC strength. The Rabi frequency is strongly dependent on the gate-induced electric field, the strength and orientation of the applied magnetic field. There are two major EDSR mechanisms. One arises from electric field-induced spin–orbit hybridization, and the other arises from magnetic field-induced energy-level crossing. The SOC introduced by the gate-induced electric field allows AC electric fields to drive coherent Rabi oscillations between spin-up and -down states. After the crossing of the energy-levels with the magnetic field, the spin-transfer crossing results in Rabi oscillation irrespective of whether or not the external electric field is present. The spin–orbit qubit is transferred into the orbit qubit. Rabi oscillation is anisotropic and periodic with respect to the tilted and in-plane orientation of the magnetic field originating from the interplay of the SOC, orbital, and Zeeman effects. The strong electrically-controlled SOC strength suggests the possibility for scalable applications of gate-controllable spin–orbit qubits.     

Electron–electron interaction induced spin thermalization in quasi-low-dimensional spin valves

We study the spin thermalization, i.e., the inter-spin energy relaxation mediated by electron–electron scattering in small spin valves. When one or two of the dimensions of the spin valve spacer are smaller than the thermal coherence length, the direct spin energy exchange rate diverges and needs to be regularized by the sample dimensions. Here we consider two model systems: a long quasi-1D wire and a thin quasi-2D sheet.     

Theoretical study of the intensity of chemically induce dynamic electron polarization of radical-triplet pairs

Considering the interaction between encited triplet molecule and cloublet radical,based on the second-order perturbation theroy and the motion equation of density matrix,the polarzation intersity of RTPM were theoretically calculated with the overpopulated doublet spin states and quartet spin states of radical0triplet paris as initial conditions the radical result from the zero-field-splitting(zfs)and the multiplet A/E and E/A polarization result from hyperfine (hf) interactions of the triplet molcule,The hyperfine ralated A A/E or E E/A CIDEP on the radical were the overpopulation of the net abscrptive or emissive polarization and multiple A/E or E/A polarization.     

Progress of hidden spin polarization in inversion-symmetric crystals

Hidden spin polarization refers to that doubly degenerate bands protected by combined inversion and time-reversal symmetry in nonmagnetic inversion-symmetric crystals could have opposite non-zero local spin polarizations, which are spatially separated in two real-space sectors paired by the inversion symmetry. Since its first prediction from ab initio calculation, hidden spin polarization has inspired tremendous interest and has been observed experimentally due to its intriguing fundamental properties as well as the great potential for applications. Moving forward, the search for moment-dependent spin splitting has also been extended to antiferromagnets even without considering spin-orbit coupling. This paper systematically reviews recent works in this field with a focus on basic concepts and material realization. It also details several remaining bottlenecks and suggests possible avenues for future research.     

NMR probing of the spin polarization of the ν=5/2 quantum Hall state

Resistively detected nuclear magnetic resonance is used to measure the Knight shift of the 75As nuclei and determine the electron spin polarization of the fractional quantum Hall states of the second Landau level. We show that the 5/2 state is fully polarized within experimental error, thus confirming a fundamental assumption of the Moore-Read theory. We measure the electron heating under radio frequency excitation and show that we are able to detect NMR at electron temperatures down to 30 mK.     

Control of electron spin–orbit anisotropy in pyramidal InAs quantum dots

We investigate the electron spin–orbit interaction anisotropy of pyramidal InAs quantum dots using a fully three-dimensional Hamiltonian. The dependence of the spin–orbit interaction strength on the orientation of externally applied in-plane magnetic fields is consistent with recent experiments, and it can be explained from the interplay between Rashba and Dresselhaus spin–orbit terms in dots with asymmetric confinement. Based on this, we propose manipulating the dot composition and height as efficient means for controlling the spin–orbit anisotropy.     

The NMR indirect nuclear spin–spin coupling constant of the HD molecule

We present new calculated and experimental values of the NMR indirect nuclear spin–spin coupling constant in HD. In the quantum-chemical ab initio calculations, the full configuration-interaction (FCI) method is used, yielding an equilibrium value of 41.22?Hz in the basis-set limit. Adding a calculated zero-point vibrational correction of 1.89?Hz and a temperature correction of 0.20?Hz at 300?K, we obtain a total calculated spin–spin coupling constant of J _FCI(HD)?=?43.31(5)?Hz at 300?K. This result is within the error bars of the experimental gas-phase NMR value, J _exp(HD)?=?43.26(6)?Hz, obtained by extrapolating values measured in HD–He mixtures to zero density.     

Renormalization of the contribution of the electron—electron interaction to the conductivity of two-dimensional electron systems

The contribution of the electron—electron interaction to the conductivity of the two-dimensional electron gas in an In_x Ga_1-x As single quantum well with different disorder strengths was experimentally studied. It is shown that the data are described well within the framework of the one-loop approximation of the renormalization group theory so long as the conductivity of the system remains higher than around 15e ²/μh.     

Percolation and the electron–electron interaction in an array of antidots

A square lattice of microcontacts with a period of 1 μm in a dense low-mobility two-dimensional electron gas is studied experimentally and numerically. At the variation of the gate voltage V _g , the conductivity of the array varies by five orders of magnitude in the temperature range T from 1.4 to 77 K in good agreement with the formula σ(V _g ) = (V _g ?V _g ^* (T))^β with β = 4. The saturation of σ(T) at low temperatures is absent because of the electron–electron interaction. A random-lattice model with a phenomenological potential in microcontacts reproduces the dependence σ(T, V _g ) and makes it possible to determine the fraction of microcontacts x(V _g , T) with conductances higher than σ. It is found that the dependence x(V _g ) is nonlinear and the critical exponent in the formula σ ∝ ? (x - 1/2) ^t in the range 1.3 < t(T, V _g ) < β.     

Snowballs of radioactive ions — nuclear spin polarization of core ions

Short-lived ions¹²B (beta-radioactive, T_1/2=20.3 ms) sustaining nuclear spin polarization were introduced into superfluid helium at 1.7 K. It was found that the¹²B ions were transported as charged entities under a static electric field and that the nuclear polarization was maintained throughout the lifetime of¹²B nuclei. Polarization of¹²B was determined through beta-NMR method. Snowball, a singly charged microcluster of helium atoms formed around an impurity ion, is responsible for the behaviour and thus constitutes a suitable environment for preserving nuclear polarization of the core ions¹²B. In a separate experiment snowballs were produced by implanting⁸Li (T_1/2=830 ms) into liquid helium and detected by means of alpha particles from the core ions to guarantee that the snowballs survive longer than the lifetime of¹²B.