Femtosecond surface plasmon resonance dynamics and electron-electron interactions in silver nanoparticles

Femtosecond excitation and relaxation of nonequilibrium electrons are investigated in silver clusters using a two color pump-probe technique with resonant excitation of the surface plasmon resonance and off resonant probing. The excitation process is shown to be identical to that in metal films, and permits creation of a strongly athermal single electron excitation in a time scale shorter than the duration of the pulses (25-30 fs), in agreement with the free-electron absorption model. Following the time evolution of the nonequilibrium distribution yields information on the internal energy redistribution dynamics of the conduction electrons and of its modification by confinement in metal clusters. Received 1st December 2000     

Pattern dynamics in an annular laser

Competition among modes in an annular CO₂ laser has been experimentally and numerically analyzed. During the coexistence of different patterns, each of them resulting from the interaction of two transverse modes with opposite angular momentum, chaos has been experimentally detected. A numerical model, derived from the Maxwell-Bloch equations and including symmetry breaking terms, enables the interpretation of the main experimental features. Received 10 March 2000     

Time-resolved photoluminescence study of Ga In P alloys

The time-resolved photoluminescence spectra of ordered and disordered Ga_0.52In_0.48P alloys were studied at room temperature and at 77 K liquid nitrogen, respectively. The ordered samples have well fitted two exponential processes decay curves and the time constants are sample dependent and have little relationship with the ordering degree. The decay curve of disordered sample shows that it has single exponential process and its lifetime has a tendency of reduction with the decrease of excitation intensity. The photoluminescence spectra with different delay time at 77 K show that the ordered samples exhibit about 6 ∼ 10 meV blue-shift of PL peak energy with the delay time. Received 13 December 2001 Published online 19 July 2002     

Pattern selection and stabilization in an annular CO laser

The formation and stabilization of spatio-temporal patterns in an annular CO₂ laser is studied. We give experimental and numerical evidence of the role of a small spatial perturbation (consisting of a thin metallic wire inserted in the optical cavity) in the selection and stabilization of patterns. Received 15 December 1999     

Phase locking and chaotic synchronization in an array of three lasers

A linear array of three lasers that are coupled mutually in space is investigated. It is shown that the phase of the laser fields is locked with intermediate coupling while the laser intensities are totally chaotic and chaotically synchronized. When the intensities of lasers reenter the regime of chaotic synchronization at smaller coupling constant, the laser fields show low degree of phase locking. The phase differences in the fields between three lasers show rich patterns when the coupling is changed. Received 3 August 2001 and Received in final form 27 September 2001     

Light-induced instabilities driven by competing helical patterns in long-pitch cholesterics

We study theoretically the dynamical reorientation phenomena when a long-pitch cholesteric liquid-crystal film with homeotropic alignment is illuminated by a circularly polarized lightwave. In the present case, the natural cholesteric pitch is of the order of (or larger than) the film thickness. The helical cholesteric structure is thus frustrated by the boundary conditions without illumination. However, above a light intensity threshold reorientation occurs and the bifurcation scenario depends strongly on the natural cholesteric pitch. Recalling that a long-pitch cholesteric is achieved in practice by adding a small amount of chiral agents in a nematic liquid crystal, the observed dynamics can be viewed as the result of the competition between intrinsic and extrinsic unidimensional helical patterns. The intrinsic part consists of the helical deformations induced by the chirality of the dopant, whereas the extrinsic part is related to the chirality induced by the optical field through the non-uniform angular momentum transfer of light to a nematic. The all-optical analog in the case of a pure nematic (without chiral dopant), is also discussed.     

Statistical properties for a class of nonlinear squeezed states

Theoretical investigations of dynamical behavior in optical parametric oscillators (OPO) have generally assumed that the cavity detunings of the interacting fields are controllable parameters. However, OPOs are known to experience mode hops, where the system jumps to the mode of lowest cavity detuning. We note that this phenomenon significantly limits the range of accessible detunings and thus may prevent instabilities predicted to occur above a minimum detuning from being evidenced experimentally. As a simple example among a number of instability mechanisms possibly affected by this limitation, we discuss the Hopf bifurcation leading to periodic behavior in the monomode mean-field model of a triply resonant OPO and show that it probably can be observed only in very specific setups.     

Electron impact single and double ionization of argon

Stable two-mode, and three-mode oscillations due to the spatial hole burning effect were observed experimentally with the increase of the pump power ratio in a laser-diode pumped sub-nanosecond microchip Cr,Yb:YAG self-Q-switched multimode laser. The stability of the output pulse trains was attributed to the mode coupling through antiphase dynamics between different modes. Modified multimode rate equations including the spatial hole-burning effect in the active medium and the non-linear absorption of the saturable absorber were proposed. Numerical simulations of the antiphase dynamics of such a laser were in good agreement with the experimental data, and the antiphase dynamics were explained by the evolution of the inversion population and the bleaching and recovery of the inversion population of the saturable absorber.     

Thermomechanical effects in uniformly aligned dye-doped nematic liquid crystals

We show theoretically that thermomechanical effects in dye-doped nematic liquid crystals when illuminated by laser beams, can become important and lead to molecular reorientation at intensities substantially lower than that needed for optical Fréedericksz transition. We propose a 1D model that assumes homogenous intensity distribution in the plane of the layer and is capable to describe such a thermally induced threshold lowering. We consider a particular geometry, with a linearly polarized light incident perpendicularly on a layer of homeotropically aligned dye-doped nematics.     

On the role of athermal electrons in non-linear photoemission from Ag(100)

The non-linear photoelectron spectra obtained by short laser pulses from a Ag(100) surface show a high-energy electron emission due to an athermal electron distribution created by the laser pulse. By comparing the photoemission at normal and non-normal emission geometry it is possible to evidence the independence of the hot electron photoemission on the parallel momentum and on different final-state configurations. A photoemission correlation measurement evidences that non-photoelectric effects, as tunneling or thermally assisted photoemission, do not contribute to the electron yield. Various theoretical models are discussed on the basis of the present data.     

A novel mechanism for spin dephasing due to spin-conserving scatterings

A new spin dephasing mechanism is proposed for semiconductors with carrier momentum-dependent transition energies (inhomogeneous broadening) between spin states. In the presence of this inhomogeneous broadening of the spin transitions, spin-conserving (SC) scatterings lead to irreversible spin dephasing in a complete analogy to the optical dephasing of inhomogeneously broadened optical transitions. This phenomenon is demonstrated for the case when the g-factor becomes electron-energy dependent. Received 29 June 2000     

Bistable behaviour in squeezed vacua: I. Stationary analysis

A time-independent theoretical and numerical analysis of an optical bistable model of two-level atoms in a ring cavity, driven by a coherent field and in contact with a squeezed vacuum field is presented in the two cases of absorptive and dispersive optical bistability (OB). In the former case, a suitable choice of the phase of the squeezed vacuum field reduces the threshold for OB to occur compared with the normal vacuum case. In the latter case, regions of OB are identified as one or two disconnected simple closed curves depending on the cooperation parameter [0pt] : is the maximum possible value of the critical value of C at fixed values of the squeezed vacuum field parameters. Phase switching effects between different (output) states of the system is investigated in detail. In the absorptive case, one- or two-way optical switching is possible depending on [0pt] . We also present results which demonstrate more complicated switching behaviour in the dispersive case. Received 12 March 1999 and Received in final form 20 August 1999     

Intermolecular and diffusive dynamics of pure acetonitrile isotopomers studied by depolarized Rayleigh scattering and femtosecond optical kerr effect

The relaxation dynamics of pure acetonitrile isotopomers has been investigated in the temperature range 8 to 75 ^° C. The overall response of the liquid is measured either recording directly the decay of the optical Kerr signal with heterodyne detection (OHD-OKE) and Fourier transforming the depolarized Rayleigh scattering spectra (DRS). The OHD-OKE signals show a decay that can be described by a bi-exponential law. At some temperatures, stressing to a maximum level the sensitivity of the OHD-OKE experimental set-up, a damped oscillation is observed on top of the fast decay component. The two techniques provide same results with a high level of reproducibility, as far as the slow component is concerned. This latter is described by an exponential law with the time constants ranging in the interval 2.0 to 0.85 ps in the light and approximately in the same interval in the deuterated molecule. The decays are, at all temperatures, well reproduced by the extended diffusion J-model. The fast component, better observed with the OHD-OKE experiments in a restricted temperature range, has time constants ranging from 550 to 350 fs. After the subtraction of the curve due to the slower decay component, the data have also been analyzed by Fourier transforming the fast part of the decay. The spectrum then consists of a broad (approximately 80 cm^-1 wide) band centered at 50 cm^-1. This band is interpreted as the manifestation of intermolecular vibrational motions. Received 21 July 2002 Published online 1st October 2002 RID="a" ID="a"e-mail: foggi@colonnello.lens.unifi.it     

Comparison of different switching techniques in a cavity soliton laser

We compare three different switching techniques for the control of cavity solitons in a VCSEL-based cavity soliton laser, one incoherent and the other two semicoherent with different injection frequencies. We show that the switching dynamics and energies can be very different depending on the type of injection.     

The pulse shape of a passively Q-switched microchip laser

The shape of the intensity pulse of a passively Q-switched microchip laser is investigated numerically and analytically. Our analysis is motivated by independent microchip laser experiments exhibiting nearly symmetric pulses in the case of a semiconductor saturable absorber and asymmetric pulses in the case of a solid state saturable absorber. Asymptotic methods are used to determine limiting behaviors of the pulse shape for both symmetric and asymmetric pulses. In the first case, we determine a sech² solution parametrized by one parameter which can be determined by solving two coupled nonlinear algebraic equations. In the second case, the pulse solution is decomposed into two distinct approximations exhibiting different amplitude and time scales properties. We review earlier approximations of the repetition rate and the pulse width. Received 2 August 1999     

Carrier scattering by Auger mechanism in a single quantum wire

We report on time-resolved microphotoluminescence experiments in a single GaAs/GaAlAs V-shaped quantum wire as a function of optical excitation intensity. At low pump power we observe that excitons are localized in quantum boxes formed by the local potential minima existing along the wire axis. As the pump power is increased, state filling of the lowest lying levels of the boxes appears. When two carriers occupy the first excited level of the box, a very efficient Auger scattering occurs, leading to a transfer of carriers from one box to another neighbouring one. The intradot Auger scattering time has been measured and is of the same order of magnitude as the LA-phonon emission rate. Received 5 February 2001     

General plasma behavior in the energy relaxation of electrons in highly p-doped semiconductors

We present a systematic study of the dependence of the energy relaxation of photo-excited minority electrons on the doping concentration in highly p-doped GaAs. A nonmonotonic dependence is found in the region where the characteristics of the carrier-carrier interaction changes from plasmon-mediated to quasistatically screened. Using a detailed Monte-Carlo study we are able to attribute this observation to a general property of plasmas at high density. Received: 1st April 1998 / Revised: 6 May 1998 / Accepted: 18 May 1998     

Combination of two basic types of synchronization in a coupled semiconductor laser system

Combination of two basic types of synchronization, anticipatory synchronization and lagged synchronization, is investigated numerically between two coupled semiconductor lasers. It is found that lagged synchronization produced by a backward coupling with a suitable delay can combine with the originally hidden anticipatory synchronization and produce a type of synchronization overcoming the original lagged synchronization produced by a forward coupling. We study the combination synchronization phenomenon when the delay of the backward coupling is different from that of the original anticipatory synchronization. Our results suggest that the synchronization combination phenomenon might allow an interpretation of an experimental observation by Sivaprakasam et al. [Phys. Rev. Lett. 87, 154101 (2001)] that the anticipating time is irrespective of the external-cavity round trip time, which to date remains to be understood.     

Nonlinear lensing mechanisms in a cloud of cold atoms

We present an experimental study of nonlinear lensing of near-resonant light by a cloud of laser-cooled rubidium atoms, specifically aimed at understanding the role of the interaction time between the light and the atomic vapor. We identify four different nonlinear mechanisms, each associated with a different time constant: electronic nonlinearity, Zeeman optical pumping, hyperfine optical pumping and radiation pressure. Our observations can be quite accurately reproduced using a simple rate equation model which allows for a straightforward discussion of the various effects. The results are important for planning more refined experiments on transverse nonlinear optics and self-organization in samples of cold atoms.