Thermophoretic effects on nano-particle deposition in channel flow

In this study, deposition of particles with diameters of 3, 5, and 10 nm in a finite-length heated channel flow is numerically studied under both molecular diffusion and thermophoretic effects. Two types of thermal conditions were examined. The first condition involved various inlet temperatures with a fixed wall temperature. The second condition involved various wall temperatures and a fixed inlet temperature. For a finite channel length, higher particle deposition can be obtained for the various inlet temperature and fixed wall temperature cases. However, for the same temperature ranges, complete particle collection on the wall can only be achieved under various wall temperatures and fixed inlet temperature cases when the channel length is long enough. This is because a temperature gradient appears in these cases. The temperature gradient in the various inlet wall temperatures and fixed wall temperature cases is zero when the flow is thermally fully developed.     

Lie group analysis for thermophoretic and radiative augmentation of heat and mass transfer in a Brinkman-Darcy flow over a flat surface with heat generation

A boundary layer analysis is presented to investigate numerically the effects of radiation,thermophoresis and the dimensionless heat generation or absorption on hydromagnetic flow with heat and mass transfer over a flat surface in a porous medium.The boundary layer equations are transformed to non-linear ordinary differential equations using scaling group of transformations and they are solved numerically by using the fourth order Runge-Kutta method with shooting technique for some values of physical parameters.Comparisons with previously published work are performed and the results are found to be in very good agreement.Many results are obtained and a representative set is displayed graphically to illustrate the influence of the various parameters on the dimensionless velocity,temperature and concentration profiles as well as the local skin-friction coefficient,wall heat transfer,particle deposition rate and wall thermophoretic deposition velocity.The results show that the magnetic field induces acceleration of the flow,rather than deceleration(as in classical magnetohydrodynamics(MHD) boundary layer flow) but to reduce temperature and increase concentration of particles in boundary layer.Also,there is a strong dependency of the concentration in the boundary layer on both the Schmidt number and mass transfer parameter.     

Thermophoresis of nanoparticles hotter/colder than the surrounding dilute gases

Aerosol particles suspended in a diluted gas with non-uniform temperature distribution are expected to experience a thermophoretic force. In theoretical treatment of thermophoresis, it is usually assumed that the particle temperature is equal to the surrounding gas temperature. However, this might not always be the case. In some particular applications, the particle temperature can significantly differ from the gas temperature. In the present paper, we theoretically investigate the effect of the particle temperature on the thermophoresis of nanoparticles in the free molecule regime. Theoretical formulas for the thermophoretic force and thermophoretic velocity are obtained based on the gas kinetic theory. As examples, a spherical Ag nanoparticle suspended in a dilute He gas is considered, and the Rudyak–Krasnolutski potential is employed to model the gas–particle interaction. It is found that the influence of the particle temperature on the thermophoresis of nanoparticles can be significant. With increasing particle size, the error due to the equal gas–particle temperature assumption can be neglected.     

Effect of thermophoresis and other parameters on the particle deposition on a tilted surface

In this study a modified version of v2-f turbulence model (φ-α), is applied to simulate a non-isothermal air-flow. The φ-α model and a two-phase Eulerian approach complement each other to predict the rate of particle deposition on a tilted surface. The φ-α model can accurately calculate the normal fluctuations, which mainly represent the non-isotropic nature of turbulence regime near the wall. The Eulerian model was modified considering the most important mechanism in the particle deposition rate when compared to the experimental data. The model performance is examined by comparing the rate of particle deposition on a vertical surface with the experimental data in a turbulent channel flow available in the literature. The effects of lift force, turbophoretic force, thermophoreric force, electrostatic force, gravitational force and Brownian/turbulent diffusion were examined on the particle deposition rate. The results show that, using the φ-α model predicts the rate of deposition with reasonable accuracy. The results of modified particle model are in good agreement with the experimental data. This study highlights the paramount effect of thermophoretic force on the particle deposition rate and clearly shows that when the temperature difference exceeds a certain limit, the electrostatic force has insignificant effect on the particle deposition rate. Furthermore, it is indicated that even at small temperature differences, the effect of tilt angle on the particle deposition rate for intermediate-size particles is negligible.     

Graphite dust deposition in the HTR-10 steam generator

Graphite dust has an important effect on the safe operation of a high-temperature gas-cooled reactor (HTR). The present study analyzes temperature and flow field distributions in the HTR-10 steam generator. The temperature and flow field distributions are then used to study thermophoretic deposition and turbulent deposition. The results show that as the dust diameter increases, the thermophoretic deposition decreases, while the turbulent deposition first decreases and then increases. The thermophoretic deposition is higher at higher reactor powers, with turbulent deposition growing more rapidly at higher reactor power. For small particles, the thermophoretic deposition effect is greater than the turbulent deposition effect, while for large particles, the turbulent deposition effect is dominant.     

A stochastic Langevin model of turbulent particle dispersion in the presence of thermophoresis

Direct numerical simulation (DNS) and experimental data have shown that inertial particles exhibit concentration peaks in isothermal turbulent boundary layers, whereas tracer-like particles remain well mixed in the domain. It is therefore expected that the interactions between turbulence and thermophoresis will be strong in particle-laden flows where walls and carrier fluid are at significantly different temperatures. To capture turbulent particle dispersion with active thermophoresis, a coupled CFD-Lagrangian continuous random walk (CRW) model is developed. The model uses 3D mean flow velocities obtained from the Fluent 6.3 CFD code, to which are added turbulent fluid velocities derived from the normalized Langevin equation which accounts for turbulence inhomogeneities. The mean thermophoretic force is included as a body force on the particle following the Talbot formulation. Validation of the model is performed against recent integral thermophoretic deposition data in long pipes as well as the TUBA TT28 test with its detailed local deposition measurements. In all cases, the agreement with the data is very good. In separate parametric studies in a hypothetical cooled channel flow, it is found that turbulence strongly enhances thermophoretic deposition of particles with dimensionless relaxation times τ⁺ of order 1 or more. On the other hand, the thermophoretic deposition of very small inertia particles (τ⁺ < 0.2) in the asymptotic region far from the injection point tends to that which characterizes stagnant flow conditions, in agreement with the DNS results of Thakurta et al.     

Effects of thermophoresis on Brownian coagulation of spherical particles over the entire particle size regime

In many energy and combustion applications, particles experience large temperature gradients, which can affect the coagulation process due to thermophoresis. This study presents a rigorous theory of thermophoretically modified Brownian coagulation in the entire particle size regime. The theoretical derivations are based on the kinetic theory for the free-molecular regime and the harmonic mean method for the transition regime. The coagulation kernels in different size regimes can be expressed as the basic Brownian coagulation kernel times an enhancement factor. The enhancement factor represents the coagulation rate enhancement induced by thermophoresis and is a function of specific dimensionless numbers. Based on the enhancement factor, the thermophoretic enhancement effects on particle coagulation are further analyzed under a wide range of gas and particle conditions. The results show that thermophoretic enhancement effects are ignorable in the free-molecular regime, but need to be considered in the continuum regime and the transition regime. In addition, the enhancement effects increase significantly with increase of gas temperature and temperature gradient while decrease with increase of gas pressure. The present study can improve understanding of thermophoretic effects on Brownian coagulation in the entire size regime and provide a useful tool to calculate the coagulation rates in presence of thermophoresis.     

Numerische Berechnung des Partikeltransportes zu einer laminar angeströmten Kreisscheibe

Increasingly process steps become important, in which particles as product particles or contaminants are deposited on substrates out of the gas phase. In this paper the particles transport processes are investigated close to the surface of a circular plate surrounded by a laminar flow. The analogy between the governing equations of momentum, energy and mass is applied to the extended diffusion equation. In the nondimensional form the results of the numerical calculations give informations about velocity, temperature and particle concentration boundary layer thickness as well as their distributions. Especially the impact of external forces on particle concentration boundary layer thickness and profile is discussed. The transport of submicron particles to the surface due to convection, diffusion, gravity and thermophoretic forces acting independently is investigated. In the used normalized form the different forces are acting as one resulting force independently of their origin. Their resulting effect in comparison to the effect due to convective diffusive transport is important for particle deposition.     

Numerical study of particle deposition in a turbulent channel flow with transverse roughness elements on one wall

A numerical study is presented for the effect of wall roughness on the deposition of solid spherical particles in a fully developed turbulent channel flow based on large eddy simulation combined with a Lagrangian particle-tracking scheme. The interest is focused on particles with response times in wall units in the range of 2.5 ≤ τ_p⁺ ≤ 600 depositing onto a vertical rough surface consisting of two-dimensional transverse square bars separated by a rectangular cavity. Predictions of particle deposition rates are obtained for several values of the cavity width to roughness element height ratio and particle response time. It is shown that the accumulation of particles in the near wall region and their preferential concentration in flow areas of low streamwise fluid velocity that occur in turbulent flows at flat channels are significantly affected by the roughness elements. Particle deposition onto the rough wall is considerably increased, exhibiting a subtle dependence on the particle inertia and the spacing between the bars. The observed augmentation of deposition coefficient can be attributed to the flow modifications induced by the roughness elements and to the inertial impaction of particles onto the frontal deposition area of the protruding square bars.     

Thermophoresis in natural convection with variable properties

The present paper deals with thermophoresis in natural convection with variable properties for a laminar flow over a cold vertical flat plate. Variation of properties like density, viscosity and thermal conductivity with temperature is included in the formulation of the problem. Selection of components for the property ratio is made by fitting the property values between the desired temperature limits. For a selected fluid, Prandtl number variation with temperature is neglected and the Prandtl number corresponding to film temperature is used for the analysis. Solution is carried out by finite difference method. Variation of wall concentration and wall flux along the length of plate is studied. The effect of thermophoretic coefficient on wall concentration is also studied. Results are presented in the form of graphs. The result is compared with similarity solution by Runge-Kutta method and found to be accurate upto second decimal place. Received on 18 May 1998     

Conduction-radiation effect on transient natural convection with thermophoresis

This paper discusses the effect of thermophoretic particle deposition on the transient natural convection laminar flow along a vertical flat surface,which is immersed in an optically dense gray fluid in the presence of thermal radiation.In the analysis,the radiative heat flux term is expressed by adopting the Rosseland diffusion approximation.The governing equations are reduced to a set of parabolic partial differential equations.Then,these equations are solved numerically with a finite-difference scheme in the entire time regime.The asymptotic solutions are also obtained for sufficiently small and large time.The obtained asymptotic solutions are then compared with the numerical solutions,and they are found in excellent agreement.Moreover,the effects of different physical parameters,i.e.,the thermal radiation parameter,the surface temperature parameter,and the thermophoretic parameter,on the transient surface shear stress,the rate of surface heat transfer,and the rate of species concentration,as well as the transient velocity,temperature,and concentration profiles are shown graphically for a fluid(i.e.,air) with the Prandtl number of 0.7 at 20 C and 1.013 × 10 5 Pa.     

Particle deposition due to thermal force in a tube

Particle deposition in a tube with laminar flow is investigated. An analytical procedure is developed for predicting the particle deposition efficiency by incorporating the velocity of thermophoresis in the equation of conservation of particles. Effects of important parameters, such as temperature difference between the inlet gas and the tube wall, particle size and the Lewis number, on the particle precipitation efficiency are examined. Also considered in this work is the assumption of constant temperature gradient as a limiting case. It is found that particle precipitation efficiency predicted by using constant temperature gradient is much optimistic.     

A generalized mass transfer law unifying various particle transport mechanisms in dilute dispersions

A generalized mass transfer law for dilute dispersion of particles (or droplets) of any sizes suspended in a fluid has been described, which can be applied to turbulent or laminar flow. The generalized law reduces to the Fick’s law of diffusion in the limit of very small particles. Thus the study shows how the well-known and much-used Fick’s law of diffusion fits into the broader context of particle transport. The general expression for particle flux comprises a diffusive flux due to Brownian motion and turbulent fluctuation, a diffusive flux due to temperature gradient (thermophoresis plus stressphoresis) and a convective flux that arises primarily due to the interaction of particle inertia and the inhomogeneity of the fluid turbulence field (turbophoresis). Shear-induced lift force, electrical force, gravity, etc. also contribute to the convective flux. The present study includes the effects of surface roughness, and the calculations show that the presence of small surface roughness even in the hydraulically smooth regime significantly enhances deposition especially of small particles. Thermophoresis can have equally strong effects, even with a modest temperature difference between the wall and the bulk fluid. For particles of the intermediate size range, turbophoresis, thermophoresis and roughness are all important contributors to the overall deposition rate. The paper includes a parametric study of the effects of electrostatic forces due to mirror charging. The present work provides a unified framework to determine the combined effect of various particle transport mechanisms on mass transfer rate and the inclusion of other mechanisms not considered in this paper is possible.     

荷电颗粒在旋转环形通道内分离性能研究

为研究带电旋转环形通道内荷电颗粒的运动和沉积特性,本文使用计算流体力学两相流离散颗粒法对带电旋转环形通道内的荷电颗粒的运动过程进行了模拟。根据模拟结果分析了不同粒径、电压、入口雷诺数和通道长径比等参数对荷电颗粒运动和沉积的影响,研究了荷电颗粒在旋转通道内离心力与电场力之间的竞争关系,探索了离心力和电场力导致的荷电颗粒运动和沉积变化的规律。结果表明,单个不同粒径颗粒具有不同的颗粒逃逸电压区间,区间的大小随着颗粒粒径的增大而增大,且区间的宽度随着通道长径比的增大将会明显变小;多个颗粒的逃逸率曲线,不同粒径的颗粒将会有不同程度的交叉,随着长径比的增大,颗粒逃逸率曲线的高度与交叉会有明显的减小,而随着转速的增大,颗粒逃逸率曲线的交叉会有一定程度的减小,且高度不会有明显变化。     

Experimental studies on particle behaviour and turbulence modification in horizontal channel flow with different wall roughness

Detailed measurements in a developed particle-laden horizontal channel flow (length 6 m, height 35 mm, the length is about 170 channel heights) are presented using phase-Doppler anemometry for simultaneous determination of air and particle velocity. The particles were spherical glass beads with mean diameters in the range of 60 µm-1 mm. The conveying velocity could be varied between about 10 m/s and 25 m/s, and the particle mass loading could reach values of about 2 (the mass loading is defined as the ratio of particle to gas phase mass flow rates), depending on particle size. For the first time, the degree of wall roughness could be modified by exchanging the wall plates. The influence of these parameters and the effect of inter-particle collisions on the profiles of particle mean and fluctuating velocities and the normalised concentration in the developed flow were examined. It was shown that wall roughness decreases the particle mean velocity and enhances fluctuating velocities due to irregular wall bouncing and an increase in wall collision frequency, i.e. reduction in mean free path. Thereby, the larger particles are mainly more uniformly distributed across the channel, and gravitational settling is reduced. Both components of the particle velocity fluctuation were reduced with increasing mass loading due to inter-particle collisions and the momentum loss involved. Moreover, the effect of the particles on the air flow and the turbulent fluctuations was studied on the basis of profiles in the developed flow and turbulence spectra determined for the streamwise velocity component. In addition to the effect of particle size and mass loading on turbulence modulation, the influence of wall roughness was analysed. It was clearly shown that increasing wall roughness also results in a stronger turbulence dissipation due to two-way coupling.     

On the deposition of particles in liquid metals onto vertical ceramic walls

The deposition of non-metallic particles in liquid-metal flows is a serious industrial problem because the build-up of particles on ceramic walls clogs the flow path and interrupts the production, and this leads to large economic losses. This paper is an effort to extend the current state-of-the-art knowledge of particle deposition in air in order to predict particle deposition rates in liquid-metal flows using an improved Eulerian deposition model and considering Brownian and turbulent diffusion, turbophoresis and thermophoresis as transportation mechanisms. The model was used to predict the rate of deposition of particles in an air flow, and the predictions were compared to published measurements to demonstrate its performance. The model was then modified to take into account the differences in properties between air and liquid metals and thereafter applied to liquid-metal flows. Effects on the deposition rate of parameters such as steel flow rate, particle diameter, particle density, wall roughness and temperature gradient near the wall were investigated. It is shown that the steel flow rate has a very important influence on the rate of deposition of large particles, for which turbophoresis is the main deposition mechanism. For small particles, both wall roughness and thermophoresis have a significant influence on the particle deposition rate. Particle deposition rates under various conditions were successfully predicted.     

An experimental and theoretical study of particle deposition due to thermophoresis and turbulence in an annular flow

The paper describes an experimental and theoretical study of the deposition of small particles from a turbulent annular-flow with cross-stream temperature variation, focusing on the effects of thermophoresis. Various expressions for the thermophoretic force on a spherical particle are critically discussed. The well-known composite formula of Talbot et al. (1980) does not include the ‘second mechanism of thermophoresis’ and it is concluded that the more recent theoretical approach of Beresnev and Chernyak (1995) is probably more reliable. New experimental measurements of particle deposition from a turbulent flow with cross-stream temperature gradients are then presented. The measurement technique is similar to the method of Liu and Agarwal (1974) but in the test section the aerosol flows vertically downwards in an annular gap between two concentric pipes. By heating the outer pipe and cooling the inner it is possible to establish a substantial, near-constant temperature difference between the two walls and hence a thermophoretic force which varies only with radius. Numerical calculations provide a comparison of theory with experiment. The theory is based on the turbulent deposition models of Young and Leeming (1997) and Slater et al. (2003) modified to include thermophoresis and the annular geometry. The theory of Beresnev and Chernyak gives good agreement with the experimental measurements.     

Particle deposition on a channel wall in a turbulent disperse flow with gradient

Kinetic ideas about the motion of a set of particles (droplets) in a turbulent gas flow with gradient are used to derive a Fokker-Planck equation for the case of sufficiently large particles (more than few microns). This equation describes the process in which they are deposited on the wall of a channel. Satisfactory agreement has been obtained between the numerical solution to this equation for the deposition rate and the experimental data published in the literature. Under the assumption that the parameters of the carrier gaseous flow vary fairly slowly, a generalized equation is derived for particle diffusion in turbulent flow. This takes into account the intensity gradient of transverse pulsations in the velocity of the carrier gaseous flow.Translated from Izvestiya Akademii Nauk SSSR, Mekhanika Zhidkosti i Gaza, No. 4, pp. 57–63, July–August, 1985.     

Thermophoresis particle deposition in a non-Darcy porous medium under the influence of Soret, Dufour effects

Thermophoresis particle deposition in free convection on a vertical plate embedded in a fluid saturated non-Darcy porous medium is studied using similarity solution technique. The effect of Soret and Dufour parameters on concentration distribution, wall thermophoretic deposition velocity, heat transfer and mass transfer is discussed in detail for different values of dispersion parameters (Ra _γ, Ra _ξ) inertial parameter F and Lewis number Le. The result indicates that the Soret effect is more influential in increasing the concentration distribution in both aiding as well as opposing buoyancies. Also, the non-dimensional heat transfer coefficient and non-dimensional mass transfer coefficient changes according to different values of thermophoretic coefficient k.