基于飞秒光频梳的双频He-Ne激光器频率测量

利用光纤飞秒光频梳和外腔可调谐半导体激光器, 建立了一套双频He-Ne激光器频率测量系统. 选用铷钟作为系统的频率基准, 通过将外腔半导体激光锁定至光频梳使得其频率溯源至铷钟, 再利用外腔可调谐半导体激光与双频He-Ne激光器输出的正交偏振激光拍频, 同时测量两路正交偏振激光频率. 将可调谐半导体激光器锁定至光频梳第1894449个梳齿, 其绝对频率为473612190000.0±2.7 kHz, 相对不确定度为5.7×10^-12. 对商品双频He-Ne激光器进行频率测量实验, 双频He-Ne激光器水平方向偏振激光频率均值为473612229934 kHz, 竖直方向偏振激光频率均值为473612232111 kHz, 平均时间为1024 s的相对Allan标准差为5.2×10^-11, 频差均值为2.177 MHz, 标准偏差为2 kHz.     

High-resolution spectroscopy with a femtosecond laser frequency comb

The output of a mode-locked femtosecond laser is used for precision single-photon spectroscopy of 133Cs in an atomic beam. By changing the laser's repetition rate, the cesium D1 (6s 2S(1/2)-->6p 2P(1/2)) and D2 (6s 2S(1/2)-->6p 2P(3/2)) transitions are detected and the optical frequencies are measured with accuracy similar to that obtained with a cw laser. Control of the femtosecond laser repetition rate by use of the atomic fluorescence is also implemented, thus realizing a simple cesium optical clock.     

Combination of a continuous-wave optical parametric oscillator and a femtosecond frequency comb for optical frequency metrology

We combined a tunable continuous-wave optical parametric oscillator and a femtosecond Ti:sapphire laser frequency comb to provide a phase-coherent bridge between the visible and the mid-infrared spectral ranges. As a first demonstration of this new technique we performed a direct frequency comparison between an iodine-stabilized Nd:YAG laser at 1064 nm and an infrared methane optical frequency standard at 3.39 microm.     

Coherent multiwave heterodyne frequency measurement of a far-infared laser by means of a femtosecond laser comb

We demonstrate the possibility of using a femtosecond laser to measure with high accuracy the frequency of a far-infrared (FIR) monochromatic source, such as an optically pumped molecular laser, by generating in a suitable mixer a signal in the radio-frequency region at the frequency difference between n steps of a femtosecond comb and the FIR source. All the couples of modes lying a distance of n steps from one another contribute coherently to the heterodyne signal. The technique has been tested up to 670 GHz.     

Optical frequency measurement across a 104-THz gap with a femtosecond laser frequency comb

The frequency-domain mode comb of a Ti:sapphire femtosecond laser centered at 350 THz is broadened to 150 THz (full width at -30 dBc) by self-phase modulation in a single-mode optical fiber. By phase locking continuous-wave lasers to elements of the comb near 1064 and 778 nm, we measure the 104-THz frequency gap between these two lasers with a relative uncertainty of 2.7 x 10(-11) in 1 s.     

Stabilized frequency comb with a self-referenced femtosecond Cr:forsterite laser

A frequency comb is generated with a Cr:forsterite femtosecond laser, spectrally broadened through a highly nonlinear optical fiber to span from 1.0 to 2.2 ,m, and stabilized using the f-to-2f self-referencing technique. The repetition rate and the carrier-envelope offset frequency are stabilized to a hydrogen maser, calibrated by a cesium atomic fountain clock. Simultaneous frequency measurement of a 657-nm cw laser by use of the stabilized frequency combs from this Cr:forsterite system and a Ti:sapphire laser agree at the 10(-13) level. The frequency noise of the comb components is observed at 1064, 1314, and 1550 nm by comparing the measured beat frequencies between cw lasers and the supercontinuum frequency combs.     

Stabilizing the frequency of femtosecond Ti:sapphire comb laser by a novel scheme

We demonstrated a novel scheme for scanning the absolute frequencies of a femtosecond Kerr-lens mode-locked Ti:sapphire laser with the repetition rate unaffected, where the carrier-envelop phase of the pulse was controlled by slightly shifting pump beam and the repetition rate was phase locked to a stable radio-frequency oscillator. Since it was the first time to stabilize the frequency of a mode-locked laser by referring directly to the frequency of cesium two-photon-transition (TPT) stabilized diode laser, we evaluated the frequency instability and the frequency accuracy that showed the characteristic of being a comb laser. The feature of the comb laser in this report will be significant for multi-photon spectroscopy where the frequency difference between comb lines plays a key role. PACS  06.30.+v; 42.60.By     

飞秒钛宝石光学频率梳的精密锁定

经相位锁定后的飞秒钛宝石光学频率梳已经广泛用于绝对光频的测量，这是光频标领域一个革命性的突破.在自建的90MHz飞秒钛宝石激光器的基础上首先采用光子晶体光纤将其光谱展宽到一个光倍频程，接着利用锁相环技术分别将重复频率和载波包络频移同时高精度地锁定到一台稳定度为6×10^－14的Cs钟上，进而得到了稳定度相同的飞秒光学频率梳.     

Full phase stabilization of a Yb:fiber femtosecond frequency comb via high-bandwidth transducers

We present full phase stabilization of an amplified Yb:fiber femtosecond frequency comb using an intracavity electro-optic modulator and an acousto-optic modulator. These transducers provide high servo bandwidths of 580 kHz and 250 kHz for f(rep) and f(ceo), producing a robust and low phase noise fiber frequency comb. The comb was self-referenced with an f-2f interferometer and phase locked to an ultrastable optical reference used for the JILA Sr optical clock at 698 nm, exhibiting 0.21 rad and 0.47 rad of integrated phase errors (over 1 mHz-1 MHz), respectively. Alternatively, the comb was locked to two optical references at 698 nm and 1064 nm, obtaining 0.43 rad and 0.14 rad of integrated phase errors, respectively.     

Spectrally resolved optical frequency comb from a self-referenced 5 GHz femtosecond laser

We report a mode-locked Ti:sapphire femtosecond laser with 5GHz repetition rate. Spectral broadening of the 24 fs pulses in a microstructured fiber yields an octave-spanning spectrum and permits self-referencing and active stabilization of the emitted femtosecond laser frequency comb (FLFC). The individual modes of the 5 GHz FLFC are resolved with a high-resolution spectrometer based on a virtually imaged phased array spectral disperser. Isolation of single comb elements at a microwatt average power level is demonstrated. The combination of the high-power, frequency-stabilized 5 GHz laser and the straightforward resolution of its many modes will benefit applications in direct frequency comb spectroscopy. Additionally, such a stabilized FLFC should serve as a useful tool for direct mode-by-mode Fourier synthesis of optical waveforms.     

双飞秒激光频率梳光谱测量技术研究进展

双光梳光谱分析技术近年来凭借高分辨率、高灵敏度、宽光谱覆盖和快速测量的优势,在分子和原子光谱分析领域得到了快速发展.从双光梳光谱分析的原理出发,以使用泵浦光源数量为分类依据,对近年来国内外基于不同实现方案的多种双光梳光谱分析技术的原理进行了简要介绍,叙述了在不同数量泵浦光源条件下,不同实验小组提出的多种实验方案,介绍了...     

Diode-pumped Yb:KYW femtosecond laser frequency comb with stabilized carrier-envelope offset frequency

We describe the detection and stabilization of the carrier envelope offset (CEO) frequency of a diode-pumped Yb:KYW (ytterbium-doped potassium yttrium tungstate) femtosecond oscillator that is spectrally centered at 1033 nm. The system consists of a diode-pumped, passively mode-locked femtosecond laser that produces 290 fs pulses at a repetition rate of 160 MHz. These pulses are first amplified, spectrally broadened and temporally compressed to 80 fs, and then launched into microstructured fiber to produce an octave-spanning spectrum. An f-2f nonlinear interferometer is employed with the broadened spectrum to detect and stabilize the CEO frequency through feedback to the pump laser current. These results demonstrate that such a Yb-doped tungstate laser can provide an efficient, compact, high-repetition-rate optical frequency comb with coverage from 650–1450 nm.     

Frequency stability measurement of a transfer-cavity-stabilized diode laser by using an optical frequency comb

We report results of frequency stability measurements of an extended cavity diode laser (ECDL) whose frequency is stabilized by a non-evacuated scanning transfer cavity. The transfer cavity is locked to a commercial frequency stabilized helium–neon laser. Frequency stability is measured by use of an optical frequency comb. The environmental perturbations (variations of temperature, air pressure, and humidity) are also simultaneously measured. The observed frequency drift of the ECDL is well explained by environmental perturbations. An atmospheric pressure variation, which is difficult to control with a non-evacuated cavity, is mainly affected to the frequency stability. Thus we put the cavity into a simple O-ring sealed (non-evacuated) tube. With this simple O-ring sealed tube, the frequency drift is reduced by a factor of 3, and the Allan variance reaches a value of 2.4×10⁻¹⁰, corresponds to the frequency stability of 83 kHz, at the average time of 3000 s. Since the actual frequency drift is well estimated by simultaneous measurement of the ambient temperature, pressure, and humidity, a feed-forward compensation of frequency drifts is also feasible in order to achieve a higher frequency stability with a simple non-evacuated transfer cavity.     

基于飞秒锁模光纤激光脉冲基频光的差频产生红外光梳

报道了一种基于飞秒锁模光纤激光脉冲基频光的光纤型差频产生(DFG)红外光梳及其研制技术.基于自主研制的重频锁定200 MHz飞秒锁模掺铒光纤激光器,经啁啾脉冲光纤放大与超连续谱产生技术,优化近零色散OFS光纤(型号:OFS-980-20)长度,结合可调延时线,获得了精准同步的基频双色脉冲;以GaSe为非线性晶体,利用光整流技术,产生了可在6—10μm范围内宽带调谐的DFG红外光梳,光梳最大光谱宽度可达1.3μm.这种光纤型远红外光梳可望在分子光谱精密测量等领域发挥重要作用.     

Composite frequency comb spanning 0.4-2.4 microm from a phase-controlled femtosecond Ti:sapphire laser and synchronously pumped optical parametric oscillator

A repetition-rate-stabilized frequency comb ranging from the violet to the mid-infrared (0.4-2.4 microm) is obtained by phase locking a femtosecond Ti:sapphire laser and a synchronously pumped optical parametric oscillator to a common supercontinuum reference. The locking results have bandwidths lower than 3 kHz. By changing the locking frequencies, different relative and absolute offsets of the constituent frequency combs are achievable.     

Full stabilization of a microresonator-based optical frequency comb

We demonstrate control and stabilization of an optical frequency comb generated by four-wave mixing in a monolithic microresonator with a mode spacing in the microwave regime (86 GHz). The comb parameters (mode spacing and offset frequency) are controlled via the power and the frequency of the pump laser, which constitutes one of the comb modes. Furthermore, generation of a microwave beat note at the comb's mode spacing frequency is demonstrated, enabling direct stabilization to a microwave frequency standard.     

Improved stabilization of a 1.3 microm femtosecond optical frequency comb by use of a spectrally tailored continuum from a nonlinear fiber grating

We report significant enhancement (+24 dB) of the optical beat note between a 657 nm cw laser and the second-harmonic generation of the tailored continuum at 1314 nm generated with a femtosecond Cr:forsterite laser and a nonlinear fiber Bragg grating. The same continuum is used to stabilize the carrier-envelope offset frequency of the Cr:forsterite femtosecond laser and permits improved optical stabilization of the frequency comb from 1.0 to 2.2 microm. Using a common optical reference at 657 nm, a relative fractional frequency instability of 2.0 x 10(-15) is achieved between the repetition rates of Cr:forsterite and Ti:sapphire laser systems in 10 s averaging time. The fractional frequency offset between the optically stabilized frequency combs of the Cr:forsterite and Ti:sapphire lasers is +/-(0.024 +/- 6.1) x 10(-17).     

Absolute frequency measurement in the 28-THz spectral region with a femtosecond laser comb and a long-distance optical link to a primary standard

A new frequency chain was demonstrated to measure an optical frequency standard based on a rovibrational molecular transition in the 28-THz spectral region accessible to a CO₂ laser. It uses a femtosecond-laser frequency comb generator and two laser diodes at 852 nm and 788 nm as intermediate oscillators, with their frequency difference phase locked to the CO₂ laser. The rf repetition rate of the femtosecond laser was compared with a 100-MHz signal from a hydrogen maser, located at BNM-SYRTE. The 100-MHz signal is transmitted by amplitude modulation of a 1.55-m laser diode through a 43-km telecommunication optical fibre. As a first example, the absolute measurement of a saturation line of OsO₄ in the vicinity of the P(16) laser line of CO₂ is reported with a relative uncertainty of 10^-12, limited by the CO₂/OsO₄ frequency day-to-day reproducibility. The current limit on the stability of the frequency measurement is 4×10^-13 at 1 s. PACS 06.20.-f; 42.62.Eh; 06.30.Ft