Entrance channel potentials in the synthesis of the heaviest nuclei

Entrance channel potentials in nucleus-nucleus collisions, relevant for the synthesis of superheavy elements, are systematically studied within a semi-microscopic approach, where microscopic nuclear densities of the colliding spherical or deformed nuclei are used in semi-classical expressions of the energy-density functional. From experimental data on fusion windows evidence is found that the existence of pockets in the entrance channel potentials is crucial for fusion. Criteria for the choice of the best collision systems for the synthesis of superheavy elements are discussed. Received: 14 May 2002 / Accepted: 6 June 2002 / Published online: 26 November 2002 RID="a" ID="a"e-mail: v.denisov@gsi.de, denisov@kinr.kiev.ua RID="b" ID="b"e-mail: w.nrnbrg@gsi.de Communicated by P. Schuck     

Energy dependence of Lévy stability and multi-fractal spectrum in e<Superscript>+</Superscript>e<Superscript>−</Superscript> collisions

Various nuclear reactions like quasi-fission, fusion-fission or particle and cluster evaporation from excited compound nuclei were studied in heavy-ion reactions at the velocity filter SHIP of GSI. The velocity filter offers the possibility to detect all reaction products under zero degree relative to the beam direction. Together with the measurement of the product velocity distribution this allows for an identification of the underlying reaction mechanism. This article is focussed on reactions of ²⁵Mg and ⁶⁴Ni beams on ^{206, 207}Pb targets at energies of 5.9×AMeV and 8.7×AMeV . Besides evaporation residues from ²⁵Mg + ²⁰⁶Pb collisions we found evidence for rotation and quasi-fission of nuclear molecules formed in the entrance channel after the capture stage. The break-up of the systems showed a preferred clustering leading to isotopes in the region 84 ⩽ Z ⩽ 88 and 122 ⩽ N ⩽ 127 of the chart of nuclei.     

Fusion cross-section of the 7Li + 11B reaction

The ⁷Li + ¹¹B reaction has been investigated in the energy range 5.5 MeV < E _lab < 19MeV, by detecting γ-ray resulting from the de-excitation of evaporation residues. Statistical compound-nucleus calculations have been performed in order to extract both the cross-sections of individual exit channels and the fusion cross-section of the system. The total angular momentum that the compoundn ucleus ¹⁸O can support has been deduced and is seen to exhibit saturation for a limiting value of 8.5ħ at the high-energy extreme. The results are discussed in terms of the entrance channel and statistical yrast line limitations.     

Fusion-fission dynamics in the superheavy nucleus production

The fusion-fission reaction mechanism leading to the massive nucleus formation is studied. We investigate the superheavy nucleus formation in heavy-ion induced reactions by analysing the evaporation residue (ER) production in order to study the fusion dynamics and the decay properties of nuclei close to the stability island at Z=114. We consider the ⁶¹Ni+²⁰⁸Pb, ⁴⁸Ca+²³⁸U and ⁴⁸Ca+²⁴⁴Pu reactions that lead to the Z=110, 112 and 114 superheavy elements respectively. By using the dinuclear system (DNS) concept of the two interacting nuclei we calculate the quasifission-fusion competition in the entrance channel and the fission-evaporation competition along the de-excitation cascade of the compound nucleus. The dynamics of the entrance channel allows us to determine the beam energy window which is favorable to the fusion, while the dynamic evolution of the compound nucleus on the shell correction to the fission barrier and the dissipative effects influence the fission-evaporation competition in order to obtain the residue nuclei from the superheavy nucleus formation. We also calculate the τ _n /τ_tot ratio at each step of the de-excitation cascade of the compound nucleus and we present a systematics of τ _n /τ_tot (at first step of the cascade) for many reactions that lead to nuclei with Z=102–114.     

The role of the entrance channel in the fusion of massive nuclei

The role of the entrance channel in the fusion-fission reactions leading to nearly the same superheavy compound nucleus is studied in the framework of dynamic model. The calculations are done for ⁴⁸Ca +²⁴⁴Pu and ^74,76Ge +²⁰⁸Pb reactions which could lead to formation of superheavy element Z = 114. It is shown that for these reactions there is an energy window for the values of the bombarding energy at which a capture probability is sufficiently large. Together with the restriction coming from the intrinsic barrier for fusion, it helps to find an optimal value of the bombarding energy for a given projectile--target combination. Received: 15 July 1998     

Partial breakdown of the evaporation model and possible preequilibrium α-particle emission in heavy-ion fusion reactions

Relative cross sections for residual nuclei following fusion reactions were measured by γ-ray spectroscopy in the reactions ⁵²Cr+ ¹²C at 56.00 MeV and ⁴⁸Ti+ ¹⁶O at 57.74 MeV, in which the common “compound nucleus” ⁶⁴Zn was excited at the same energies and the relative distributions of the entrance spins were nearly identical. It is shown that ratios of the measured cross sections in both entrance channels can be precisely determined experimentally and are insensitive to small changes of the parameters in calculations based on the evaporation model. Using these particular quantities, we have shown that the evaporation process is not the sole mechanism producing the observed residues, especially those resulting from α-particle emission. The assumption of preequilibrium α-particle emission at high channel spins is shown to reproduce the present data fairly well.     

GSI experiments on synthesis and nuclear structure investigations of the heaviest nuclei

Isotopes of elements up to Z = 113 have been synthesized using medium heavy projectiles and target nuclei around doubly magic ²⁰⁸Pb. Synthesis of still heavier elements in reactions of ⁴⁸Ca projectiles with actinide target nuclei has been reported. To obtain more information about production mechanism of transfermium isotopes nuclear reaction studies including investigations of massive transfer were resumed at SHIP, GSI. Nuclear structure investigations at SHIP have been concentrated so far mainly on systematic investigations of low lying Nilsson levels in odd-mass nuclei. Recently this field has been extended to decay studies of isomeric states in nobelium nuclei at E^* > 1 MeV.     

Excitation functions of fusion reactions and neutron transfer in the interaction of 6He with 197Au and 206Pb

Excitation functions for evaporation residues in the reactions ¹⁹⁷Au(⁶He, xn)^203-xnTl, x = 2-7, and ²⁰⁶Pb(⁶He, 2n)²¹⁰Po, as well as for neutron transfer reactions for the production of ¹⁹⁶Au and ¹⁹⁸Au in the interaction of ⁶He with ¹⁹⁷Au were measured. The ⁶He beam was obtained from the accelerator complex for radioactive beams DRIBs (JINR). The maximum energy of the beam was about 10AMeV and the intensity reached 2×10⁷pps. The stacked-foil activation technique was used directly in the beam extracted from the cyclotron or in the focal plane of the magnetic spectrometer MSP-144. The identification of the reaction products was done by their radioactive γ- or α-decay. The fusion reaction with the evaporation of two neutrons was characterized by an increase in the cross-section compared to statistical model calculations. The analysis of the data in the framework of the statistical model for the decay of excited nuclei, which took into account the sequential fusion of ⁶He has shown good agreement between the experimental and the calculated values of the cross-sections in the case of sub-Coulomb-barrier fusion in the ²⁰⁶Pb + ⁶He reaction. An unusually large cross-section was observed below the Coulomb barrier for the production of ¹⁹⁸Au in the interaction of ⁶He with ¹⁹⁷Au. Possible mechanisms of formation and decay of transfer reaction products are discussed.     

Does break-up affect 9Be +209Bi fusion at the barrier?

The ⁹Be +²⁰⁹Bi fusion cross sections were measured in the 36.0 MeV ≤ E_lab≤ 50.0 MeV range, down to 0.6 mb, with high accuracy via in-beam detection of the ground state α-decay of the evaporation residues produced. The elastic scattering cross sections around 150° and 135° were also obtained with moderate angular resolution. The cross sections below the barrier are reproduced by coupled channel calculations which include only one break-up channel with a moderate strength and a phenomenological renormalization of the potential depth. These simple calculations overestimate the cross sections above the barrier most likely due to the fact that the ⁹Be break-up process becomes much stronger. The barrier distributions extracted do not have evident break-up signature since they show one-barrier structure. Received: 22 February 1999 / Revised version: 26 March 1999     

Calculation of the Coulomb potential between spherical-deformed and deformed-deformed nuclei using the Monte Carlo method

The Coulomb potential between spherical-deformed and deformed-deformed nuclei has been calculated using the Monte Carlo simulation. The results obtained for the Coulomb potential in the ¹⁶O$ + $²³⁸U and ²⁷Al$ + $⁷⁰Ge reactions are in good agreement with those obtained using the double-folding method. The simulation technique employed here has the ability of calculating the Coulomb potential taking into account the finite diffuseness parameter, all the possible deformation degrees of freedom, and different orientations of the symmetry axes of the target and the projectile nuclei with respect to each other. The accuracy of this simulation technique is high and the computer time taken to do these calculations is much less than those of the double-folding method.     

Analytical calculation of fusion cross-sections

We analyse the fusion cross-sections, calculated by using two different analytical parameterisations and compare them with the experimental data. Both the parameterisations are based on ion-ion potentials calculated within the framework of Skyrme energy density formalism. In the first case, the ion-ion potential (including the spin-density term) was parameterised and then, by adding the Coulomb potential, one could compute the fusion barrier analytically. In the second case, the calculated fusion barrier heights and positions were parameterised directly. Both of these (previously) reported parameterisations are used here to calculate the fusion barriers and fusion excitation functions for more than 50 reactions belonging to the s-d and f-shell nuclei. A detailed comparison of these parametrisations with the experimental and several other theoretical results shows that both of these parameterisations are able to reproduce the experimental data equally well. As the (second) direct parameterisation depends only on the charges and masses of colliding nuclei, it is very useful for predicting/ understanding the fusion process in low energy heavy-ion reactions. Received: 24 February 1999 / Accepted: 16 March 2000     

Isotopic dependence of neutron emission from dinuclear system

Using the statistical approach, we study the isotopic dependence of the de-excitation of dinuclear systems formed in the entrance channel of heavy-ion reactions. The probabilities of neutron emission from the dinuclear systems ^62-73Ni + ²⁰⁸Pb are estimated and a possible experiment for the observation of this emission is discussed.     

Precompound charged particle emission (PCE) — a mechanism beyond element production by complete fusion

Complete fusion reactions (xn-channels) using actinide targets are observed for values of the effective fissilities x _eff ∼ 0.80 in the sub-pb range of production cross sections. The elements produced at this limit are Z = 108–112. Beyond complete fusion, heavier elements might still be produced by reaction mechanisms releasing part of the nuclear charge before an equilibrated compound system might have been reached. Precompound Charged particle Emission (PCE) is proposed as a possible mechanism following complete fusion. A scheme delivering isotopes of elements Z = 110–115 is discussed, and experimental evidence for such a process is presented. Compound systems, the atomic numbers of which are smaller than in complete fusion reactions, might be produced in ⁴⁸Ca induced reactions on actinides with larger cross sections than those at the limits of complete fusion. Besides complete fusion, the PCE-mechanism should be considered as an alternative to interpret the ⁴⁸Ca-induced reactions on actinides.     

Isotopic dependence of fusion probabilities for neutron-deficient and -rich colliding nuclei

Isotopic dependence of the fusion dynamics is studied by analyzing the collision of a large number of isotopes of Ca and Ni with 0.6 N/Z 2. This study, which results from the Skyrme energy density formalism, reveals that the addition of neutrons favors fusion of reacting partners, whereas the reverse happens with the removal of neutrons. The fusion barrier heights and positions follow a non-linear second-order dependence on ( -1 ), whereas fusion cross-sections can be parameterized by a straight line.-1     

Fusion around the barrier in 11,9Be +209Bi

The ⁹Be +²⁰⁹Bi fusion cross sections were measured in the range 37.5 MeV ≤ E _lab ≤ 45.0 MeV at the Munich Tandem via the observation of ground state α-decay of the evaporation residues. Fusion cross sections of ²⁰⁹Bi with the “halo”¹¹Be unstable projectile in the region around the Coulomb barrier were deduced from an experiment done with the same technique at the RIKEN Ring Cyclotron. Above the Coulomb barrier the ¹¹Be cross sections are larger than the ⁹Be ones in agreement with theoretical predictions based on the larger ¹¹Be halo radius. Also below the barrier these theories foresee the same behavior in disagreement with the experimental results, since the two cross sections are rather similar. Received: 2 April 1998     

Discrete structures in fusion-barrier distributions for vibrational nuclei

We obtain a closed-form expression for the distribution of fusion barriers for vibrational nuclei using a generalization of Dasso, Landowne, and Winther's model, which represents the nuclear surface vibrations as a number of harmonic oscillators, and allows the excitation of an arbitrary number of phonons in the target and/or projectile. We find that this expression is in reasonable agreement with the average trends of the empirical distributions for the fusion of ¹⁶O with ⁹²Zr, ¹⁴⁴Sm and ²⁰⁸Pb, but fails to reproduce the double peaking of the distribution for the ¹⁴⁴Sm target. Only when we restrict the number of excited phonons to a limited number, we are able to reproduce such discrete structures. We show that limiting the number of coupled channels, particularly in the case of strong coupling, increases the spacings between the channel eigenvalues that determine the positions of the peaks of the barrier distribution and modifies their heights. Received: 6 March 2000 / Accepted: 31 January 2001     

Fission and ternary cluster decay of hyper-deformed 56Ni

Coincidences between two heavy fragments have been measured from the fission of ⁵⁶Ni compound nuclei formed in the ³²S + ²⁴Mg reaction at E _lab( ^32S ) = 165.4 MeV. A unique experimental set-up consisting of two large-area position-sensitive (x, y) gas detector telescopes has been used allowing the complete determination of the observed fragments and their momentum vectors. In addition to binary fission events with subsequent particle evaporation, narrow out-of-plane correlations are observed for two fragments emitted in purely binary events and in events with a missing charge consisting of 2α - and 3α -particles (¹²C). These events are interpreted as ternary cluster decay from ⁵⁶Ni nuclei at high angular momenta through hyper-deformed shapes.     

Measurement of fusion excitation functions of 27, 29, 31Al + 197Au

A systematic study of the sub-barrier fusion reactions with neutron-rich projectiles has been carried out for three isotopes ^27,29,31Al bombarding a ¹⁹⁷Au target. A target chamber equipped with a target stack and sets of MWPC was employed in order to enhance the efficiency of the radioactive beam experiment. Coupled-channel calculations including the quadrupole excitations do not well fit the measured fusion excitation functions, whereas flat barrier distributions to represent the coupling to the neutron transfer largely account for the observed enhancement of the sub-barrier fusion cross-sections. Received: 13 March 2001 / Accepted: 27 April 2001