Time-resolved STM light emission from an evaporated Au film

STM (scanning tunneling microscope) light emission from an evaporated Au film irradiated by pico second laser pulses has been investigated for various bias voltages of the STM. The observed emission consists of two components. The first component that has the same duration as the incident laser pulse is excited by laser induced tunneling electrons. The second component that has a longer duration than that of the laser pulse is emitted from surface polariton plasmons excited non-linearly by the laser pulse.     

Reflection and transmission of an ultrashort electromagnetic pulse incident normal to a flat plasma layer

The process of reflection and transmission of ultrashort pulses incident normal to a flat plasma layer of finite thickness and on a step barrier is calculated within an exact mathematical approach for various parameters (barrier width and duration and carrier frequency of a corrected Gaussian pulse) of the problem.     

Q-switched and mode-locked diode-pumped Nd:YVO4 laser with an intracavity composite semiconductor saturable absorber

We have demonstrated a passively Q-switched and mode-locked Nd:YVO₄ laser with an intracavity composite semiconductor saturable absorber (ICSSA). Stable Q-switched and mode-locked pulses with Q-switched envelope pulse duration of 180 ns and pulse repetition rate of 72 KHz have been obtained. The maximum average output power was 1.45 W at 8 W incident pump power. The repetition rate of the mode-locked pulses inside the Q-switched envelope was 154 MHz. Experimental results revealed that this ICSSA was suitable for Q-switched and mode-locked solid-state lasers.     

Analysis of laser-diode end-pumped intracavity frequency-doubled,passively Q-switched and mode-locked Nd:YVO<Subscript>4</Subscript> laser

Simultaneous Q-switching and mode locking in a laser-diode end-pumped intracavity frequency-doubled Nd:YVO₄/KTP green laser using a Cr⁴⁺:YAG saturable absorber with 81% initial transmission is experimentally demonstrated. At an incident pump power of 6 W, 300 mW of average green power was obtained, which is around four times higher than the cw green power obtained without the Cr⁴⁺:YAG crystal. The repetition rate of the mode-locked green pulses was 400 MHz and the individual mode-locked pulse width was measured to be 500 ps. The repetition rate of the Q-sw itched envelope of the mode-locked pulses was 15 kHz at 6 W of incident pump power. The energy of the mode-locked pulse at the peak of the Q-sw itched envelope was estimated to be 1 J and the peak power was estimated to be 2.4 kW. The measured width and the total energy of the Q-sw itched envelope of the mode-locked pulses was 47 ns and 21 J, respectively, at the maximum incident pump power. An analysis of the system by incorporating a nonlinear loss term due to the intracavity second-harmonic generation to the general recurrence relation for the mode-locked pulses under the Q-sw itched envelope at the fundamental wavelength has been presented. Using a hyperbolic secant square function to model the mode-locked pulse, the temporal shape of a single Q-sw itched pulse at the second-harmonic wavelength has been reconstructed. The theoretical calculations of the pulse parameters like pulse energy, peak power, pulse width and pulse-symmetry factor have shown fairly good agreement with the experimental results. PACS 42.55.Rz; 42.55.Xi; 42.60.By     

Interference and dispersion effects on tunneling time

We study the interplay between pulse width, interference and tunneling for a wave packet incident upon a barrier and, within the context of tunneling time, we offer a complementary insight into the origin of the Hartman effect. We find that interference together with momentum spread lower (increase) the transmission (reflection) tunneling time thereby `breaking the symmetry between transmission and reflection times'. But, within the limits of our method, we are unable to confirm that negative tunneling time can be obtained.     

Analysis of a laser-diode end-pumped intracavity frequency-doubled passively Q-switched and mode-locked Nd:GdVO<Subscript>4</Subscript>/KTP laser with a semiconductor saturable absorber

A diode-pumped passively Q-switched mode-locked (QML) intracavity frequency-doubled Nd:GdVO₄/KTP green laser with a semiconductor saturable absorber is presented. Nearly 100% modulation depth for the mode-locked green pulses can be achieved at any pump power over 1.92 W. The width of the mode-locked green pulse was estimated to be about 150 ps. The mode-locked pulse interval within the Q-switched envelope of 320 ns and the repetition rate of 97.5 kHz were obtained, at an incident pump power of 4.4 W. The repetition rate of the mode-locked green pulses inside the Q-switched envelope was 140 MHz.     

Effect of Lorentz local field correction on propagation of ultrashort laser pulse in one-dimensional para-nitroaniline (PNA) molecules

This paper investigates the effect of Lorentz local field correction (LFC) on the propagation of ultrashort laser pulses in a para-nitroaniline molecular medium under resonant and nonresonant conditions by solving numerically the full-wave Maxwell-Bloch equations beyond slowly-varying envelope approximation and rotating-wave approximation. The effect of the LFC is considerably obvious when pulses with large areas propagate in the dense molecular medium. In the case of resonance,the group velocity of the sub-pulses split from the incident pulse along propagation is severely decreased by the LFC,especially for the latest sub-pulse. However,in the case of nonresonance,the influence of the LFC on the temporal evolution of the pulse is less obvious and lacks homogeneity with an increase in incident pulse area,propagation distance and molecular density.     

Thermoacoustic Method for Detection of Powerful Microwave Pulses

We propose a method for detection of the envelope of a microwave nanosecond pulse, which is based on the effect of generation of sound pulses resulting from absorption of electromagnetic waves. We show that to reproduce exactly the envelope shape of a short microwave pulse, it is necessary that the wave be absorbed in a layer of thickness much less than the product of the sound speed and the pulse duration. In searching for conditions ensuring this, we study the process of thermoacoustic generation in thin metal films deposited on quartz substrates. Measurements performed at a wavelength of 8 mm show that the absorption coefficient is maximum if the aluminum-film thickness is 22–25 Å. The maximum absorption coefficient amounts to 49% if the wave is incident from the quartz-substrate side. It is important that in this case, the wave reflection coefficient does not exceed 44%, whereas an aluminum plate reflects almost completely (99.8%) the incident-wave power. The phenomena observed in thin metal films are explained theoretically in terms of the anomalous skin effect. An experimental setup for a study of generation of ultrasonic signals by powerful microwave pulses is described.     

Dynamics of ultrashort pulse focusing

The method for studying the transformation of an ultrashort pulse of a spherical wave in the vicinity of the focus was developed. It was shown that the impulse response of the circular aperture contains two components: the transmitted one “cut” by the aperture from the incident wave and the toroidal edge one. Simple algebraic relations describing the propagation process were derived and corresponding software was developed. An example of a change in the pulse shape with Gaussian envelope is given. It was shown that pulses propagating with velocity ν > c, one of which overtakes the primary wave, are formed on the system axis.     

Passively Q-switched and mode-locked diode-pumped Nd:YVO4 laser with LT-GaAs output coupler

We have demonstrated an efficient and compact passively Q-switched and mode-locked (QML) 1064 nm Nd:YVO₄ laser by using a low temperature grown GaAs (LT-GaAs) saturable absorber as well as an output coupler. Stable QML with envelope duration as short as 10 ns and Q-switched repetition rate of 36 kHz was obtained. It is the shortest envelope duration as far as we know, and it is so short that it can be used as Q-switching pulses directly. At 6.9 W of the incident pump power, average output power of 1.24 W was achieved and the corresponding peak power and energy of a single Q-switched pulse were 3.44 kW and 34.4 μJ, respectively. The mode-locked pulses inside the Q-switched pulse envelope had a repetition rate of 780 MHz.     

Broadband Terahertz Wave Generation from Monolayer Graphene Driven by Few-Cycle Laser Pulse

We theoretically investigate the characteristics of terahertz(THz) radiation from monolayer graphene exposed to normal incident few-cycle laser pulses, by numerically solving the extended semiconductor Bloch equations. Our simulations show that the THz spectra in low frequency regions are highly dependent on the carrier envelope phase(CEP) of driving laser pulses. Using an optimal CEP of few-cycle laser pulses, we can obtain broadband strong THz waves, due to the symmetry breaking of the laser-graphene system. Our results also show that the strength of the THz spectra depend on both the intensity and central wavelength of the laser pulses. The intensity dependence of the THz wave can be described by the excitation rate of graphene, while wavelength dependence can be traced back to the band velocity and the population of graphene. We find that a near single-cycle THz pulse can be obtained from graphene driven by a mid-infrared laser pulse.     

熔合反应中动力学势垒的研究

用改进的量子分子动力学模型研究了与入射能量相关的重离子熔合势垒. 随着 入射能的降低可以观察到动力学势垒的最低值, 这个最低动力学势垒与绝热势垒 非常接近；动力学势垒随着入射能的增加而升高, 最终接近于静态势垒(非绝热势垒). 基于动力学势垒的研究, 对于重离子熔合反应的额外推动(extra-push)给出了微观理解,对势垒贯穿给出了一种新的解释. 为进一步理解动力学势垒, 还研究了颈部的形成和体系的动力学形变, 分析了动力学势垒降低的原因.     

Diode-pumped passively Q-switched and mode-locked Nd:Lu<Subscript>0.15</Subscript>Y<Subscript>0.85</Subscript>VO<Subscript>4</Subscript> laser with a GaAs saturable absorber

By using a-cut Nd:Lu_0.15Y_0.85VO₄ mixed crystal as laser gain medium, a diode-pumped passively Q-switched and mode-locked (QML) laser with a GaAs saturable absorber in a Z-type folded cavity is demonstrated for the first time. The Q-switched mode-locked laser pulses with about 90% modulation depth are obtained as long as the pump power reached the oscillation threshold. The repetition rate of the passively Q-switched pulse envelope ranges from 50 to 186 kHz as the pump power increases from 0.915 to 6.520 W. Under an incident pump power of 6.52 W, the QML pulses with the largest average output power of 694 mW, the shortest pulse width of 200 ns and the highest pulse energy of 3.73 μJ are obtained. The mode-locked pulse width inside the Q-switched envelope is estimated to be about 275 ps. The experimental results show that Nd:Lu_0.15Y_0.85VO₄ is a promising mixed crystal for QML laser.     

Tunneling time in magnetic barrier structures

We adopt the group velocity approach to the issue of tunneling time in two configurations of magnetic barrier structures, which are arranged with identical or unidentical building blocks. The effects of an external electric field are also taken into account. The tunneling time in magnetic barrier structures is found to be strongly dependent on the magnetic configuration, the applied bias, the incident energy as well as the longitudinal wave vector. The results indicate that for electrons with equal energy but different incident angles, the tunneling processes are significantly separated in time within the same magnetic barrier structure. In the configuration arranged with unidentical building blocks, there exists obvious asymmetry of tunneling time in two opposite tunneling directions. Such a discrepancy of the tunneling time varies distinctly with the longitudinal wave vector and the applied bias. Received 4 March 2002 / Received in final form 22 May 2002 Published online 17 September 2002     

Definitions and control of the CEP and CEO

The definitions of the carrier to envelope phase (CEP) and carrier to envelope offset (CEO) arc reviewed. It is pointed out that a unique separation of the field of an ultrashort pulse in a “carrier” and “envelope” is not always possible for ultrashort pulses. Another definition is proposed for pulses of a few optical cycles, that is not dependent on the notion of “carrier” and “envelope.” The carrier to envelope offset (CEO) is a frequency, generally defined as the ratio of the change in CEP between pulses, to the pulse (temporal) spacing. It is shown that the CEO exists for trains of long pulses, for which the CEP cannot be measured. Methods of measuring the CEO of a mode-locked laser are proposed. It is shown that MQW have a locking tendency on the CEO of two pulse trains.     

Generation of multiple femtosecond pulses by step gratings

A simple method for generating multiple isolated femtosecond pulses by step gratings is presented, and a criterion for judging whether or not an incident pulse is just split into multiple independent pulses is obtained. The dependences of multiple pulses on the structural parameters of the step gratings are explored. The results show that an incident pulse can split into multiple isolated similar diffraction pulses for enough step height, and the pulse repetition interval increases with the increasing of the step height.     

Carrier Envelope Phase Description for an Isolated Attosecond Pulse by Momentum Vortices

As a crucial parameter for a few-cycle laser pulse, the carrier envelope phase(CEP) substantially determines the laser waveform. We propose a method to directly describe the CEP of an isolated attosecond pulse(IAP) by the vortex-shaped momentum pattern, which is generated from the tunneling ionization of a hydrogen atom by a pair of time-delayed, oppositely and circularly polarized IAP-IR pulses. Superior to the angular streaking method that characterizes the CEP in terms of only one streak, our method describes the CEP of an IAP by the features of multiple streaks in the vortex pattern. The proposed method may open the possibility of capturing sub-cycle extreme ultraviolet dynamics.     

Optical and photocurrent spectroscopy with picosecond strain pulses

This paper gives an overview of optical experiments using picosecond strain pulses. The strain pulses, which propagate with the sound velocity, are incident on a semiconductor nanostructure and induce an ultrafast shift of the exciton resonance energy by an amount, that exceeds the spectral width of the corresponding optical transition. When the duration of the high-amplitude strain pulse is long enough compared with the coherence time of the optical resonance, modulation of the resonance takes place adiabatically and exciton energy can be accurately defined at each momentary position. If the coherence time exceeds the characteristic time of the strain pulse, a non-adiabatic regime is realized and the exciton cannot be related to an optical transition with a specific photon energy. In more detail, we describe the recent experiments on the gating of photocurrent in a tunneling p-i-n device and the generation of THz polariton sidebands in an optical microcavity strongly coupled to the excitons in an embedded quantum well. These two experiments represent, respectively, examples of adiabatic and non-adiabatic behaivior of excitons in the presence of the high-amplitude picosecond strain pulse.     

Carrier envelope phase noise in stabilized amplifier systems

At present most laser systems for generating phase-stabilized high-energy pulses are chirped pulse amplifier systems that involve the selection and subsequent amplification of pulses from a phase-stabilized seed oscillator. We investigate the effect of the picking process on the carrier envelope phase stability and how the phase noise of the picked pulse sequence can be estimated from the phase noise properties of the seed oscillator. All noise components from the original pulse train above the picking frequency are aliased into the picked pulse train and therefore cannot be neglected.