Decay of149Gd and directional correlations of gamma cascades in149Eu

The decay of¹⁴⁹Gd(9.4d) to the levels of¹⁴⁹Eu has been studied using large volume high resolution Ge(Li) and NaI(Tl) detectors,γ-γ coincidence and directional correlation experiments have been performed. Newγ-rays at energies 131.9, 278.6, 384.7, 415.7, 599.2, 726.5, 734.7, 956.4 and 1,231.1 keV in¹⁴⁹Eu have been observed. Three new levels in¹⁴⁹Eu have been placed at 956.4, 1,082.0 and 1,231.1 keV. Spin-parity assignments have been made to some of the levels in¹⁴⁹Eu. Multipolarity assignments have been made for most of the electromagnetic transitions from the conversion coefficients obtained through the knowledge of ourγ-transition intensities and the published conversion-electron intensities. Based on the newγ-transitions observed in the singles and coincidence spectra, a revised level scheme has been proposed for¹⁴⁹Eu and compared with previously published level schemes. Radioactivity¹⁴⁹Gd; measuredT _1/2,T _γ,γγ coin, γγ(θ), I.C.C.,¹⁴⁹Eu deduced levels,J,γ-mixing,π. Enriched targets, Ge(Li) detectors.     

Experimental study of the decay of147Pr to levels in147Nd

The decay of¹⁴⁷Pr produced by (γ, p) reaction on enriched¹⁴⁸Nd has been studied with Ge(Li) detectors and gamma-gamma coincidence methods. Half-life determinations, and accurate energy and intensity measurements for 84 gamma transitions have been performed. A level scheme with 21 levels including 62 of the transitions was deduced. Beta branch intensities were estimated from measured gamma intensities. Tentative spin and parity assignments are given.     

Tentative level diagram of146Pm below 1.1 MeV

The level scheme of the doubly odd nucleus¹⁴⁶Pm was investigated by means of in-beam spectroscopy. The¹⁴⁶Nd(p, n) reaction in the 3.5–8 MeV proton energy interval on enriched targets has been used to populate the exited states of¹⁴⁶Pm. High resolutionγ-ray spectra using Ge(Li) and hyperpure Ge detectors and conversion electrons with a mini-orange spectrometer were measured. Withγ-exitation functions andnγ-coincidences usingnγ-discriminated NE231 neutron detectors transitions in¹⁴⁶Pm were identified,γγ-coincidences gave information aboutγ-cascades. With these data a level scheme of 38 levels below 1.1 MeV exitation energy has been deduced including 73 transitions. For 12 transitions experimental conversion coefficients have been evaluated, which agree with the expected values forM1/E2-transitions.     

The γ-ray spectrum following the β−-decay of147Nd

The still existing discrepancies in the γ-ray spectrum accompanying the β^?-decay of¹⁴⁷Nd could be cleared up by careful measurements with high-resolution Ge(Li)-detectors. It could be shown that these discrepancies are caused by radioactive impurities of^148m Pm thus excluding several energy levels and γ-ray transitions reported in earlier papers. The experimental level scheme is compared with the predictions of intermediate coupling theory.     

Decay of oriented149Nd and levels in theN=88149Pm nucleus

Levels in the¹⁴⁹Pm nucleus populated via¹⁴⁹Nd decay were studied using the low temperature nuclear orientation technique. The parent¹⁴⁹Nd nuclei were oriented in a gadolinium host. The normalized gamma-ray intensities were determined for twenty five transitions in the daughter¹⁴⁹Pm nucleus. The spins of the¹⁴⁹Pm levels at 288.2 and 425.3 keV were determined as 9/2 and 7/2, respectively, and for several other¹⁴⁹Pm levels the previous spin-assignments could be unambiguously confirmed. Substantial new information on multipole mixing ratios of gamma-transitions in¹⁴⁹Pm is presented. Low-energy level spacing in the¹⁴⁹Pm nucleus is found to be in reasonable agreement with recent particle-rotor model calculations including the variable moment of inertia.     

Der Zerfall des122Xe (T 1/2=20,l h) und des122J (T 1/2=3,6min)

Theγ spectra emitted in the decay of¹²²Xe and¹²²I have been investigated using Ge(Li) detectors and a Ge(Li)-NaI coincidence apparatus. 14γ transitions with energies between 61.8 and 416.9 keV have been identified in the decay of¹²²Xe, 44 transitions between 564.0 and 3,291.0 keV in the decay of¹²²I. Level schemes having 7 excited levels for¹²²I and 21 excited levels for¹²²Te are proposed.     

Level structure of149Nd. The decay of149Pr

The decay of¹⁴⁹Pr (T _1/2=2.2 min) has been studied using the two fission product separators JOSEF and LOHENGRIN to produce the¹⁴⁹Pr nucleus. A level scheme for¹⁴⁹Nd has been established. Theβ-branching and logft values for the excited levels were deduced from the analysis ofγ-intensity balances. Furthermore, the spins and parities for most of the excited states observed were obtained from the comparison between the present work, the neutron capture results and the pick-up reactions. The positive parity levels have been described with the Nilsson model with Coriolis andΔN=2 interactions included. The properties of the negative parity states cannot be explained as easily; however, it has been attempted to extract the structure of the ground state \((I^\pi = \tfrac{5}{2}^ - )\) and the first excited states \((I^\pi = \tfrac{7}{2}^ - and\tfrac{3}{2}^ - )\) .     

Structure of even-even138Nd from the decay of138Pm

The structure of¹³⁸Nd is investigated through theβ ⁺-decay of¹³⁸Pm, whose decay half-life is measured to be 3.24±0.05 min. A level structure comprising 27 excited states and 52 transitions is constructed. With the help of deducedft values and internal conversion coefficients, spin-parity assignments are made to many states in¹³⁸Nd and to the ground states of¹³⁸Pm. From the positron end-point energy measurement, the total decay energy is determined to be 5.4±0.2 MeV, which is compared with the predictions of several mass formulae and with the decay energy systematics of theN=77 isotones. The structure of¹³⁸Nd is discussed in the light of nuclear systematics of theN=78 isotones.     

Decay of193m Hg

The decay of^193m Hg to¹⁹³Au levels was investigated by means of Ge(Li) and Ge(Li)-NaI(Tl) coincidence spectrometers. In theγ-ray spectrum about 120 transitions were observed, about 80 of them being new. Forty coincidences betweenγ-transitions were observed. The level scheme of¹⁹³Au, including 12 earlier known levels as well as 17 new and corrected levels, has been constructed on the basis of the balance of energy sums and the observed coincidences. Possible multipolarities of 33 transitions were determined. Possible spins and parities of several levels were deduced from the determined multipolarities.     

Ground state properties and β-decay half-lives near 132Sn in a self-consistent theory

The level scheme of⁹⁵Tc has been investigated with Ge(Li)-detectors by observing the γ-rays after the decay of 1.65 h⁹⁵Ru. The energies and intensities of theγtransitions were extracted fromγ-singles andγγ-coincidence spectra. In the decay of⁹⁵Ru 88γ-transitions were observed; a scheme of⁹⁵Tc with 25 levels is proposed into which 86 transitions could be accomodated. Spin and parity assignments were made from log (ft) values andγ-ray branching ratios. The level structure of⁹⁵Tc is compared with that of the other odd Tc isotopes.     

Energy levels of136Pm and136Nd via beta decay of136Sm and136Pm

¹³⁶Pm and¹³⁶Nd were studied using theβ decay of¹³⁶Sm and¹³⁶Pm. The radioactive nuclei were produced by the⁹²Mo (⁴⁸Ti,xpyn) and¹¹²Sn (²⁸Si,xpyn) reactions. The UNISOR isotope separator enabled mass identification. The previously unknown level scheme of¹³⁶Pm was constructed and the half-life of¹³⁶Sm was determined to be 47±2 s. Six new levels and thirteen newγ-ray transitions have been added to the level scheme of¹³⁶Nd.     

The decay of143Sm to levels in143Pm

The beta decay of¹⁴³Sm was reinvestigated with the aid of a Ge(Li) detector. Levels of¹⁴³Pm at 271.8, 1,056.5, 1,173.4, 1,342.1, 1,403.2, 1,514.9, 1,752.8, 1,816.3, 1,853.6, (2,000), 2,009.0, 2,080.5, 2,344, 2,443, 2,463, 2,906 and (3,054) keV were established. Logft values for all observed beta transitions have been calculated. Spin and parity assignments have been made from electron capture and positon disintegration considerations and gamma branches. The experimental level scheme of¹⁴³Pm is compared with the results of 1 and 3 q.p. calculations forN=82 nuclei.     

On the decay of73Ga to levels in73Ge

Theγ-radiation following the β^? decay of⁷³Ga has been studied. Singlesγ andγγ coincidence spectra were recorded with Ge(Li)-detectors. 17γ-rays were assigned to transitions in⁷³Ge, where 11 excited levels are proposed. From logft values based onγ-transition intensities, spin and parity assignments for the levels were deduced. The half-life of⁷³Ga was measured to (4.86±0.03) h. From allowedβ-transitions the ground state of⁷³Ga was assigned 3/2^?.     

A high-resolution spectroscopic study of the gamma radiation from the decay of96Nb

The decay of 24h⁹⁶Nb has been studied with a Ge(Li) spectrometer and with a Ge(Li)-NaI(Tl) coincidence spectrometer. A total of 27 gamma-ray transitions were observed, their energies and intensities measured. All but one of these have been incorporated into the level scheme of⁹⁶Mo. The level at 1,625.9 keV reported recently in (n _th, γ) work on⁹⁵Nb has also been observed through the decay of⁹⁶Nb. No experimental evidence has been found for previously proposed levels at 2,657 and 2,791 keV in⁹⁶Mo.     

Gamma-gamma directional correlations and coincidence studies in154Gd

The intensities, placements andE2/M1 mixing ratios of transitions in the decay of¹⁵⁴Eu have been carefully studied to provide accurate data for microscopic calculations. Coincidence relationships in the decay of¹⁵⁴Eu have been studied extensively with a multiparameterγ-γ coincidence system with two large volume Ge(Li) detectors. Spectra in coincidence with twenty energy gates were analyzed. Twenty-nine new coincidence relationships were established and confirmed most, but not all, of several levels previously assigned by energy fits only. From an analysis of coincidence spectra and singles spectra with a 18% efficiency Ge(Li) detector new information on the gamma-ray intensities were obtained. Precise values of theE2/M1 mixing ratios of transitions from the gamma- and beta-vibrational bands to the g.s. band have been determined fromγ-γ directional correlation measurements with a NaI(Tl)-Ge(Li) detector coincidence system. Mixing ratios were obtained for a number of other transitions including those fromK ^π =0^? and 2⁺ bands from direct and skipped cascade correlations.     

States inN=80140Nd populated in the decay of140Pm

The level structure of theN=80,¹⁴⁰Nd has been investigated through the beta decay of^140m Pm and^140g Pm, whose decay half-lives were measured to be 5.95±0.05 min and 9.1±0.5 sec, respectively. Decay schemes for the two isomers have been constructed fromγ-ray measurements. With the help of the beta decayft values and internal conversion electron measurements, spins and parities were deduced for levels in¹⁴⁰Nd. Among the levels a 7^? state at 2222.0 keV and a 5^? state at 2273.3 keV are identified as two-neutron quasiparticle states. The (ie233-01) for^140m Pm and^140g Pm have been deduced as 7^? and 1⁺, respectively. From beta end-point measurements, the decay energies of the two isomers have been determined asQ _EC=6.48±0.07 MeV^140m (Pm) andQ _EC=6.08±0.10 MeV (^140gPm). The results are discussed in the light of nuclear systematics of theN=79 and 80 isotones.     

The Decay of130La to levels in130Ba

Theγ-radiation associated with the β⁺ decay of¹³⁰La to levels in¹³⁰Ba is studied. The level scheme is established on the basis of theγ-γ coincidence measurements emploing two Ge(Li) detectors. The available experimental data are compared to collective model calculations withγ-soft P.E.S. andγ-dependent inertial functions. To reproduce levels energyB _ββ value twice as large as other mass parameters is needed.Radioactivity: ¹³⁰La [from¹³⁰Ba(p, n),E _p=10MeV]; measuredE _γ,I _γ,γγ-coin.¹³⁰Ba deduced levels,J, π, logft. Enriched target, Ge(Li) detectors.     

Studies of γ-ray transitions in171Yb

The decay of¹⁷¹ Lu(t_1/2=8.2 day) to the levels of¹⁷¹Yb has been studied using large volume high resolution Ge(Li), x-ray Ge(Li) and NaI(Tl) detectors.γ-γ coincidence and directional correlation experiments have been performed. Spin-parity of 5/2^?, 7/2⁺, 5/2^?, 9/2⁺, 7/2^?, 7/2^?, 11/2⁺, 9/2^?, 9/2^? and 5/2^? have been assigned to the 75.87, 95.26, 122.37, 167.62, 208.00, 230.61, 259.02, 835.21, 948.37 and 1024.87 keV levels respectively. Several new coincidence relations have been observed in the present work. Two newγ-transitions at 141.45 and 821.30 keV observed and two levels at 766 and 944 keV been proposed. Multipolarity assignments have been made for most of theγ-transitions from theK-shell internal conversion coefficients obtained using the presentγ-ray intensities and the published conversion electron intensities. A revised level scheme for¹⁷¹Yb has been proposed and compared with published data. Radioactivity¹⁷¹Lu; measuredT _1/2,E _γ ,I _γ ,γγ coin,γγ (θ), I.C.C.,¹⁷¹Yb deduced levels,J, γ-mixing,π. Enriched targets, Ge(Li) detectors.     

Structure of140Pm from beta decay of140Sm

The structure of¹⁴⁰Pm is investigated through the beta decay of¹⁴⁰Sm, whose half-life is measured to be (14.7 ± 0.2) m. A level structure comprising 41 transitions among 17 excited states is constructed. Using the deduced ft values and measured internal conversion coefficients, spin-parity assignments to several states in¹⁴⁰Pm were made. From beta end-point measurement, the total decay energy is deduced to beQ _EC =3.4±0.3 MeV, which is compared with the predictions of several mass formulae. The systematics of the odd-Z, N=79 isotones are discussed.