共查询到20条相似文献,搜索用时 11 毫秒
1.
Tao Huang Peng He Ranran Wang Siwei Yang Jing Sun Xiaoming Xie Guqiao Ding 《Advanced functional materials》2019,29(45)
Wearable textile strain sensors that can perceive and respond to human stimuli are an essential part of wearable electronics. Yet, the detection of subtle strains on the human body suffers from the low sensitivity of many existing sensors. Generally, the inadequate sensitivity originates from the strong structural integrity of the sensors because tiny external strains cannot trigger enough variation in the conducting network. Inspired by the rolling friction where the interaction is weakened by decreasing interface area, porous fibers made of graphene decorated with nanoballs are prepared via a prolonged phase‐separation process. This novel structure confers the graphene fibers with high gauge factors (51 in 0–5% and 87 in 5–8%), which is almost 10 times larger than the same structures without nanoballs. A low detection limit (0.01% strain) and good durability (over 6000 circles) are obtained. By the virtue of these qualities, these fiber‐based textile sensors can recognize a pulse wave and eyeball movement in real‐time while keeping comfortable wearing sense. Moreover, by weaving such fibers, the electronic fabrics with a specially designed structure can distinguish the multilocation in real time, which shows great potential as wearable electronics. 相似文献
2.
Yan Wang Li Wang Tingting Yang Xiao Li Xiaobei Zang Miao Zhu Kunlin Wang Dehai Wu Hongwei Zhu 《Advanced functional materials》2014,24(29):4666-4670
Sensing strain of soft materials in small scale has attracted increasing attention. In this work, graphene woven fabrics (GWFs) are explored for highly sensitive sensing. A flexible and wearable strain sensor is assembled by adhering the GWFs on polymer and medical tape composite film. The sensor exhibits the following features: ultra‐light, relatively good sensitivity, high reversibility, superior physical robustness, easy fabrication, ease to follow human skin deformation, and so on. Some weak human motions are chosen to test the notable resistance change, including hand clenching, phonation, expression change, blink, breath, and pulse. Because of the distinctive features of high sensitivity and reversible extensibility, the GWFs based piezoresistive sensors have wide potential applications in fields of the displays, robotics, fatigue detection, body monitoring, and so forth. 相似文献
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Strain Sensors: Large‐Area Ultrathin Graphene Films by Single‐Step Marangoni Self‐Assembly for Highly Sensitive Strain Sensing Application (Adv. Funct. Mater. 9/2016) 下载免费PDF全文
Xinming Li Tingting Yang Yao Yang Jia Zhu Li Li Fakhr E. Alam Xiao Li Kunlin Wang Huanyu Cheng Cheng‐Te Lin Ying Fang Hongwei Zhu 《Advanced functional materials》2016,26(9):1488-1488
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Facile Synthesis of Graphene Quantum Dots from 3D Graphene and their Application for Fe3+ Sensing 下载免费PDF全文
Arundithi Ananthanarayanan Xuewan Wang Parimal Routh Barindra Sana Sierin Lim Dong‐Hwan Kim Kok‐Hwa Lim Jun Li Peng Chen 《Advanced functional materials》2014,24(20):3021-3026
Owing to their small size, biocompatibility, unique and tunable photoluminescence, and physicochemical properties, graphene quantum dots (GQDs) are an emerging class of zero‐dimensional materials promising a wide spectrum of novel applications in bio‐imaging, optical, and electrochemical sensors, energy devices, and so forth. Their widespread use, however, is largely limited by the current lack of high yield synthesis methods of high‐quality GQDs. In this contribution, a facile method to electrochemically exfoliate GQDs from three‐dimensional graphene grown by chemical vapor deposition (CVD) is reported. Furthermore, the use of such GQDs for sensitive and specific detection of ferric ions is demonstrated. 相似文献
6.
Qian Chen Junting Shen Diana Estevez Yanlin Chen Zihao Zhu Jun Yin Faxiang Qin 《Advanced functional materials》2023,33(33):2302545
3D printed graphene aerogels hold promise for flexible sensing fields due to their flexibility, low density, conductivity, and piezo-resistivity. However, low printing accuracy/fidelity and stochastic porous networks have hindered both sensing performance and device miniaturization. Here, printable graphene oxide (GO) inks are formulated through modulating oxygen functional groups, which allows printing of self-standing 3D graphene oxide aerogel microlattice (GOAL) with an ultra-high printing resolution of 70 µm. The reduced GOAL (RGOAL) is then stuck onto the adhesive tape as a facile and large-scale strategy to adapt their functionalities into target applications. Benefiting from the printing resolution of 70 µm, RGOAL tape shows better performance and data readability when used as micro sensors and robot e-skin. By adjusting the molecular structure of GO, the research realizes regulation of rheological properties of GO hydrogel and the 3D printing of lightweight and ultra-precision RGOAL, improves the sensing accuracy of graphene aerogel electronic devices and realizes the device miniaturization, expanding the application of graphene aerogel devices to a broader field such as micro robots, which is beyond the reach of previous reports. 相似文献
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Highly Sensitive,Wearable, Durable Strain Sensors and Stretchable Conductors Using Graphene/Silicon Rubber Composites 下载免费PDF全文
Ge Shi Zhiheng Zhao Jing‐Hong Pai Ivan Lee Liqun Zhang Craig Stevenson Kalana Ishara Rujing Zhang Hongwei Zhu Jun Ma 《Advanced functional materials》2016,26(42):7614-7625
Highly sensitive, wearable and durable strain sensors are vital to the development of health monitoring systems, smart robots and human machine interfaces. The recent sensor fabrication progress is respectable, but it is limited by complexity, low sensitivity and unideal service life. Herein a facile, cost‐effective and scalable method is presented for the development of high‐performance strain sensors and stretchable conductors based on a composite film consisting of graphene platelets (GnPs) and silicon rubber. Through calculation by the tunneling theory using experimental data, the composite film has demonstrated ideal linear and reproducible sensitivity to tensile strains, which is contributed by the superior piezoresistivity of GnPs having tunable gauge factors 27.7–164.5. The composite sensors fabricated in different days demonstrate pretty similar performance, enabling applications as a health‐monitoring device to detect various human motions from finger bending to pulse. They can be used as electronic skin, a vibration sensor and a human‐machine interface controller. Stretchable conductors are made by coating and encapsulating GnPs with polydimethyl siloxane to create another composite; this structure allows the conductor to be readily bent and stretched with sufficient mechanical robustness and cyclability. 相似文献
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Large‐Area Ultrathin Graphene Films by Single‐Step Marangoni Self‐Assembly for Highly Sensitive Strain Sensing Application 下载免费PDF全文
Xinming Li Tingting Yang Yao Yang Jia Zhu Li Li Fakhr E. Alam Xiao Li Kunlin Wang Huanyu Cheng Cheng‐Te Lin Ying Fang Hongwei Zhu 《Advanced functional materials》2016,26(9):1322-1329
Promoted by the demand for wearable devices, graphene has been proved to be a promising material for potential applications in flexible and highly sensitive strain sensors. However, low sensitivity and complex processing of graphene retard the development toward the practical applications. Here, an environment‐friendly and cost‐effective method to fabricate large‐area ultrathin graphene films is proposed for highly sensitive flexible strain sensor. The assembled graphene films are derived rapidly at the liquid/air interface by Marangoni effect and the area can be scaled up. These graphene‐based strain sensors exhibit extremely high sensitivity with gauge factor of 1037 at 2% strain, which represents the highest value for graphene platelets at this small deformation so far. This simple fabrication for strain sensors with highly sensitive performance of strain sensor makes it a novel approach to applications in electronic skin, wearable sensors, and health monitoring platforms. 相似文献
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Lizhi Sheng Yuan Liang Lili Jiang Qian Wang Tong Wei Liangti Qu Zhuangjun Fan 《Advanced functional materials》2015,25(41):6545-6551
Recently, macroporous graphene monoliths (MGMs), with ultralow density and good electrical conductivity, have been considered as excellent pressure sensors due to their excellent elasticity with a rapid rate of recovery. However, MGMs can only exhibit good sensitivity when the strain is higher than 20%, which is undesirable for touch‐type pressure sensors, such as artificial skin. Here, an innovative method for the fabrication of freestanding flexible graphene film with bubbles decorated on honeycomb‐like network is demonstrated. Due to the switching effect depended on “point‐to‐point” and “point‐to‐face” contact modes, the graphene pressure sensor has an ultrahigh sensitivity of 161.6 kPa?1 at a strain less than 4%, several hundred times higher than most previously reported pressure sensors. Moreover, the graphene pressure sensor can monitor human motions such as finger bending and pulse with a very low operating voltage of 10 mV, which is sufficiently low to allow for powering by energy‐harvesting devices, such as triboelectric generators. Therefore, the high sensitivity, low operating voltage, long cycling life, and large‐scale fabrication of the pressure sensors make it a promising candidate for manufacturing low‐cost artificial skin. 相似文献
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Yu Ra Jeong Heun Park Sang Woo Jin Soo Yeong Hong Sang‐Soo Lee Jeong Sook Ha 《Advanced functional materials》2015,25(27):4228-4236
Stretchable electronics have recently been extensively investigated for the development of highly advanced human‐interactive devices. Here, a highly stretchable and sensitive strain sensor is fabricated based on the composite of fragmentized graphene foam (FGF) and polydimethylsiloxane (PDMS). A graphene foam (GF) is disintegrated into 200–300 μm sized fragments while maintaining its 3D structure by using a vortex mixer, forming a percolation network of the FGFs. The strain sensor shows high sensitivity with a gauge factor of 15 to 29, which is much higher compared to the GF/PDMS strain sensor with a gauge factor of 2.2. It is attributed to the great change in the contact resistance between FGFs over the large contact area, when stretched. In addition to the high sensitivity, the FGF/PDMS strain sensor exhibits high stretchability over 70% and high durability over 10 000 stretching‐releasing cycles. When the sensor is attached to the human body, it functions as a health‐monitoring device by detecting various human motions such as the bending of elbows and fingers in addition to the pulse of radial artery. Finally, by using the FGF, PDMS, and μ‐LEDs, a stretchable touch sensor array is fabricated, thus demonstrating its potential application as an artificial skin. 相似文献
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Yuqiang Zeng Tian Li Yonggang Yao Tangyuan Li Liangbing Hu Amy Marconnet 《Advanced functional materials》2019,29(27)
Reduced graphene oxide (RGO) films are promising in applications ranging from electronics to flexible sensors. Though high electrical and thermal conductivities have been reported for RGO films, existing thermal conductivity data for RGO films show large variations from 30 to 2600 W m?1 K?1. Further, there is a lack of data at low temperatures (<300 K), which is critical for the understanding of thermal transport mechanisms. In this work, a temperature‐dependent study of thermal (10–300 K) and electrical (10–3000 K) transport in annealed RGO films indicates the potential application of RGO films for sensing temperatures across an extremely wide range. The room‐temperature thermal conductivity increases significantly from 46.1 to 118.7 W m?1 K?1 with increasing annealing temperature from 1000 to 3000 K with a corresponding increase in the electrical conductivity from 5.2 to 1481.0 S cm?1. In addition, films reduced at 3000 K are promising for sensing extreme temperatures as demonstrated through the measured electrical resistivity from 10 to 3000 K. Sensors based on RGO films are advantageous over conventional temperature sensors due to the wide temperature range and flexibility. Thus, this material is useful in many applications including flexible electronics and thermal management systems. 相似文献
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Jidong Shi Xinming Li Huanyu Cheng Zhuangjian Liu Lingyu Zhao Tingting Yang Zhaohe Dai Zengguang Cheng Enzheng Shi Long Yang Zhong Zhang Anyuan Cao Hongwei Zhu Ying Fang 《Advanced functional materials》2016,26(13):2078-2084
Transparent, stretchable films of carbon nanotubes (CNTs) have attracted significant attention for applications in flexible electronics, while the lack of structural strength in CNT networks leads to deformation and failure under high mechanical load. In this work, enhancement of the strength and load transfer capabilities of CNT networks by chemical vapor deposition of graphene in the nanotube voids is proposed. The graphene hybridization significantly strengthens the CNT networks, especially at nanotube joints, and enhances their resistance to buckling and bundling under large cyclic strain up to 20%. The hybridized films show linear and reproducible responses to tensile strains, which have been applied in strain sensors to detect human motions with fast response, high sensitivity, and durability. 相似文献
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Facile Synthesis of 3D Graphene Flowers for Ultrasensitive and Highly Reversible Gas Sensing 下载免费PDF全文
Jin Wu Shuanglong Feng Xingzhan Wei Jun Shen Wenqiang Lu Haofei Shi Kai Tao Shirong Lu Tai Sun Leyong Yu Chunlei Du Jianmin Miao Leslie K. Norford 《Advanced functional materials》2016,26(41):7462-7469
Fabrication of nanostructured graphene (Gr) for gas sensing applications has become increasingly attractive. For the first time, 3D graphene flowers (GF) cluster patterns are grown directly on an Ni foam substrate by inexpensive homebuilt microwave plasma‐enhanced chemical vapor deposition (MPCVD) using the gas mixture H2/C2H4O2@Ar as a precursor. The interim morphologies of the synthesized GF are investigated and the growth mechanism of the GF film is proposed. The GF are decomposed to few‐layer Gr sheets by ultrasonication in ethanol. For the first time, MPCVD‐synthesized Gr is exploited to fabricate a gas sensor that exhibits an ultrahigh sensitivity of 133.2 ppm?1 to NO2. Outstanding sensor responses of 1411% and 101% to 10 ppm and 200 ppb NO2, respectively, are achieved. Furthermore, a low theoretical detection limit of 785 ppt NO2 is achieved. An ultrafast (within 2 s) recovery is observed at room temperature, and an imbedded microheater is employed to improve the selectivity of NO2 detection relative to humidity. This work represents a simple, clean, and efficient route to synthesize large‐area cauliflower Gr for gas detection with high performance, including ultrahigh sensitivity, good selectivity, fast recovery, and reversibility. 相似文献
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Caihao Deng Peixiong Gao Linfeng Lan Penghui He Xin Zhao Wei Zheng Wangshou Chen Xizhou Zhong Yunhui Wu Lan Liu Junbiao Peng Yong Cao 《Advanced functional materials》2019,29(51)
Stretchable/wearable strain sensors are attracting growing interest due to their broad applications in physical and physiological measurements. However, the development of a multifunctional highly stretchable sensor satisfying the requirements of ultrahigh sensitivity (able to distinguish sound frequency) remains a challenge. An ultrasensitive and highly stretchable multifunctional strain sensor with timbre‐recognition ability based on high‐crack‐density vertical graphene (VGr) is fabricated using an ultrasonic peeling (UP) method. It can distinguish frequencies of sounds higher than 2500 Hz. Detailed microscopic examinations reveal that their ultrahigh sensitivity stems from the formation of high‐density nanocracks in the graphitic base layer, which is bridged by the top branched VGr nanowalls. These nanocracks cut the VGr film into a large number of nanopieces, which increase the natural frequency of the sensors, enabling the sensors to distinguish the sound frequency. Demonstrations are presented to highlight the sensors' potential as wearable devices for human physiological signal and timbre detections. This is the first multifunctional highly stretchable strain sensor with timbre‐recognition ability. 相似文献
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Folke Johannes Tölle Martin Fabritius Rolf Mülhaupt 《Advanced functional materials》2012,22(6):1136-1144
A novel and highly versatile synthetic route for the production of functionalized graphene dispersions in water, acetone, and isopropanol (IPA), which exhibit long‐term stability and are easy to scale up, is reported. Both graphene functionalization (wherein the oxygen content can be varied from 4 to 16 wt%) and dispersion are achieved by the thermal reduction of graphite oxide, followed by a high‐pressure homogenization (HPH) process. For the first time, binders, dispersing agents, and reducing agents are not required to produce either dilute or highly concentrated dispersions of single graphene sheets with a graphene content of up to 15 g L?1. High graphene content is essential for the successful printing of graphene dispersions by 3D microextrusion. Free‐standing graphene films and micropatterned graphene materials are successfully prepared using this method. Due to the absence of toxic reducing agents, the graphene exhibits no cytotoxicity and is biocompatible. Furthermore, the electrical conductivity of graphene is significantly improved by the absence of binders. Flexible microarrays can be printed on different substrates, producing microarrays that are mechanically stable and can be bent several times without affecting electrical conductivity. 相似文献
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Shayan Seyedin Simge Uzun Ariana Levitt Babak Anasori Genevieve Dion Yury Gogotsi Joselito M. Razal 《Advanced functional materials》2020,30(12)
The integration of nanomaterials with high conductivity into stretchable polymer fibers can achieve novel functionalities such as sensing physical deformations. With a metallic conductivity that exceeds other solution‐processed nanomaterials, 2D titanium carbide MXene is an attractive material to produce conducting and stretchable fibers. Here, a scalable wet‐spinning technique is used to produce Ti3C2Tx MXene/polyurethane (PU) composite fibers that show both conductivity and high stretchability. The conductivity at a very low percolation threshold of ≈1 wt% is demonstrated, which is lower than the previously reported values for MXene‐based polymer composites. When used as a strain sensor, the MXene/PU composite fibers show a high gauge factor of ≈12900 (≈238 at 50% strain) and a large sensing strain of ≈152%. The cyclic strain sensing performance is further improved by producing fibers with MXene/PU sheath and pure PU core using a coaxial wet‐spinning process. Using a commercial‐scale knitting machine, MXene/PU fibers are knitted into a one‐piece elbow sleeve, which can track various movements of the wearer's elbow. This study establishes fundamental insights into the behavior of MXene in elastomeric composites and presents strategies to achieve MXene‐based fibers and textiles with strain sensing properties suitable for applications in health, sports, and entertainment. 相似文献
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Yuchao Wu Yong Zeng Yizhen Chen Chao Li Renhui Qiu Wendi Liu 《Advanced functional materials》2021,31(52):2107202
Currently, most customized hydrogels can only be processed via extrusion-based 3D printing techniques, which is limited by printing efficiency and resolution. Here, a simple strategy for the rapid fabrication of customized hydrogels using a photocurable 3D printing technique is presented. This technique has been rarely used because the presence of water increases the molecular distance between the polymer chains and reduces the monomer polymerization rate, resulting in the failure of rapid solid-liquid separation during printing. Although adding cross-linkers to printing inks can effectively accelerate 3D cross-linked network formation, chemical cross-linking may result in reduced toughness and self-healing ability of the hydrogel. Therefore, an interpenetrated-network hydrogel based on non-covalent interactions is designed to form physical cross-links, affording fast solid-liquid separation. Poly(acrylic acid (AA)-N-vinyl-2-pyrrolidone (NVP)) and carboxymethyl cellulose (CMC) are cross-linked via Zn2+-ligand coordination and hydrogen bonding; the resulting mixed AA-NVP/CMC solution is used as the printing ink. The printed poly(AA-NVP/CMC) hydrogel exhibited high tensile toughness (3.38 MJ m−3) and superior self-healing ability (healed stress: 81%; healed strain: 91%). Some objects like manipulator are successfully customized by photocurable 3D printing using hydrogels with high toughness and complex structures. This high-performance hydrogel has great potential for application in flexible wearable sensors. 相似文献
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Hyosang Yoon Kyoungryul Lee Hanho Shin Seongeun Jeong Yi Jae Lee Sungwook Yang Soo Hyun Lee 《Advanced functional materials》2023,33(38):2300322
On-body strain information provides various indicators such as heart rate, physiological pulse, voice waveform, respiratory rate, and body motion status. Recent advances in wearable strain sensors using nanomaterials have significantly enhanced sensor performance with regard to sensitivity, detectable range, and response time. However, it is still challenging to obtain all types of body strain information, from small vibrations to joint movements, using one type of sensor. Herein, a full-range on-body strain (FROS) sensor covering ultrasmall-to-large strains such as vocal vibration and joint movement is reported. To achieve an ultrawide detectable range, reduced graphene oxide (rGO)-embedded laser-induced graphene (LIG) is synthesized by laser engraving on a graphene oxide (GO)-embedded polyimide (PI) complex film. An rGO-LIG homostructure based on sp2-carbons is photothermally reconstructed from the GO-PI heterostructure in a complex film by in situ co-transformation and then transferred to an elastomer substrate. The fabricated FROS sensor successfully performs on-body strain monitoring of various indicators, such as physiological pulse, vocal sound waveform, and body movement, as well as American sign language translation. Furthermore, it is believed that this rGO-LIG homostructure-based material synthesized by in situ co-transformation can potentially provide novel functionalities in fields such as wearable electronics, humanoid, soft robotics, and intelligent prosthetics. 相似文献