Thermally-boosted pumping of Nd:LiYF<Subscript>4</Subscript> using Ti:Sapphire laser

We report for the first time (to our knowledge) a 1053 nm Nd:LiYF₄ (Nd:YLF) laser by directly pumping into the upper lasing level with a tunable Ti:sapphire laser. The results obtained for direct upper laser level pumping at 872 and 880 nm of Nd:YLF were compared with traditional 806 nm pump band excitation. Highly efficient 1053 nm continuous-wave (CW) laser emission under direct pumping at 880 nm in an 8 mm thick, 1.0 at % Nd:YLF crystal is obtained. The slope efficiency is improved from 39.1% for traditional pumping at 806 nm to 63.9% for direct pumping at 880 nm.     

Lasing from a solid-state Ca<Subscript>3</Subscript>Ga<Subscript>2</Subscript>Ge<Subscript>3</Subscript>O<Subscript>12</Subscript>:Nd<Superscript>3+</Superscript> laser at a high power of diode pumping

Experimental data for cw lasing from a compact solid-state laser based on a neodymium-doped calcium-gallium-germanium-garnet crystal (Ca₃Ga₂Ge₃O₁₂:Nd³⁺) at a wavelength of 1.06 μm in the case of intense diode pumping are reported. The laser output reaches 0.7 W for a cavity 15 mm long and an active element 1 mm thick. It is shown that the output power is limited by a thermal lens placed in the active element.     

Efficiency of the generation and self-addition of laser line frequencies upon the diode pumping of Er:BaY<Subscript>2</Subscript>F<Subscript>8</Subscript> crystals

Features of the generation of laser lines upon the diode pumping of Er:BaY₂F₈ crystals are studied. Blue, violet, and UV laser lines are most efficiently generated via the nonlinear frequency self-addition of 541 and 553 nm lines of Er³⁺ radiation with the corresponding IR line of Er³⁺ for Er:BaY₂F₈ crystals pumped by a laser diode with a wavelength of 972 nm.     

Laser performance of <Emphasis Type="Italic">N</Emphasis><Subscript><Emphasis Type="Bold">g</Emphasis></Subscript>-cut flash-lamp pumped Nd:KGW at high repetition rates

A comparative study of the flash-lamp pumped laser performance of standard b-grown Nd:KGW and Nd:KGW grown for propagation along the optical axis N_g is presented. The results show that, in comparison with b-grown crystal, the N_g-grown Nd:KGW is very promising for use at high repetition flash-lamp pumping rates. With the same laser cavity configuration, the N_g-grown Nd:KGW can operate at an average flash-lamp input power of at least 1.4 kW, while the b-cut one ceases lasing at average flash-lamp input power of ∼0.5 kW. The reason for this is that the thermal lens induced in the N_g-oriented Nd:KGW rod under pump radiation is relatively weak, nearly spherical and positive, whereas the b-grown Nd:KGW rod acts as a quite weak positive lens for radiation with radial polarization, and as a much stronger negative lens for tangentially polarized radiation. PACS 42.60.Jf; 42.70.Hj     

Spectral characteristics of a Yb-doped Y<Subscript>2</Subscript>O<Subscript>3</Subscript> ceramic laser

We report the experimental observation of random wavelength emission and intensity-dependent central-wavelength shift in a diode-pumped Yb³⁺-doped Y₂O₃ ceramic laser. We show experimentally that, like conventional lasers, the emission of the laser has fixed well-defined transverse modes; however, its instantaneous emission wavelengths change randomly with time. The central wavelength of the laser emission also shifts with the intracavity light intensity. A model was developed to describe the spectral behavior of Yb³⁺-doped lasers. We show that the observed random wavelength emission and central lasing wavelength shift of the laser could be well explained based on the strong reabsorption of light in the gain medium. PACS 42.55.Rz; 42.60.Mi; 42.55.Xi     

Crystal growth,spectroscopic and CW laser properties of Nd<Subscript>0.03</Subscript>Lu<Subscript>2.871</Subscript>Gd<Subscript>0.099</Subscript>Al<Subscript>5</Subscript>O<Subscript>12</Subscript> crystal

Nd_0.03Lu_2.871Gd_0.099Al₅O₁₂ (Nd:LuGdAG) crystal was grown by the Czochralski method. The absorption, fluorescence spectra and fluorescence lifetime of Nd:LuGdAG crystal at room temperature were investigated for the first time. We reported the continuous-wave (CW) Nd:LuGdAG laser operation under diode pumping. Output power of 1.43 W at 1064 nm was achieved with a slope efficiency of 34.1%. All the results show that Nd:LuGdAG crystal is a promising laser material.     

Orthorhombic lutetium germanate NaLuGeO<Subscript>4</Subscript>: A new SRS-active crystal

The discovery of the effect of simulated Raman scattering in the NaLuGeO₄ rhombic crystal and the first results of studying the spectra of two-phonon steady χ⁽³⁾ nonlinear picosecond lasing are reported.     

Detection of stimulated Raman scattering in the LiYbF<Subscript>4</Subscript> crystal

Stimulated Raman scattering (SRS) has been observed for the first time in a tetragonal LiYbF₄ crystal. The recorded Stokes and anti-Stokes components of χ⁽³⁾ nonlinear lasing are attributed to the two SRS-active phonon modes with ω_SRS1 ~ 325 cm^–1 and ω_SRS2 ~ 432 cm^–1 of this crystal.     

Numerical analysis of conversion efficiency in second-harmonic generation in new crystal CsLiB<Subscript>6</Subscript>O<Subscript>10</Subscript>

In this paper, a detailed theoretical analysis of the second-harmonic generation (SHG) efficiency as a function of polarization ratio and crystal length of CsLiB6O₁₀ (CLBO) in the phase matching using a computer simulation is presented. The SHG efficiency was as high as 80% when the pumping radiation was a plane wave. The efficiency is 65% and 80% for the pumping waves of type I and type II Gaussian beams, respectively. An important result is that the phase matching of type II is perfectly adopted in the SHG experiment with CLBO.     

Laser performance of holmium-doped Lu<Subscript>3</Subscript>Al<Subscript>5</Subscript>O<Subscript>12</Subscript> and (Lu,Y)<Subscript>3</Subscript>Al<Subscript>5</Subscript>O<Subscript>12</Subscript> crystals pumped by Tm:fiber laser

Optical properties of Ho³⁺-doped Lu₃Al₅O₁₂ and (Lu,Y)₃Al₅O₁₂ crystals were investigated and compared. Substitution of Y for Lu in the host garnet Lu₃Al₅O₁₂ results in broad absorption and emission spectra, and improvements in the laser behavior of Ho³⁺. Pumped by Tm:fiber laser, a maximum output power of 5.02 and 5.73 W of Ho-doped Lu₃Al₅O₁₂ and (Lu,Y)₃Al₅O₁₂ have been obtained, respectively. The center lasing wavelength are 2124.5 and 2123.0 nm for Lu₃Al₅O₁₂ and (Lu,Y)₃Al₅O₁₂, respectively.     

Diode-pumped Yb:Y<Subscript>2</Subscript>SiO<Subscript>5</Subscript>-LiB<Subscript>3</Subscript>O<Subscript>5</Subscript> cyan laser at 501.7 nm

We describe the output performances of the 928 nm ⁴ F _3/2 → ⁴ I _9/2 transition in Nd:CLNGG under diode-laser pumping. An end-pumped Nd:CLNGG crystal yielded 1.3 W of continuous-wave output power for 17.8 W of absorbed pump power. The slope efficiency with respect to the absorbed pump power was 11.2%. Furthermore, with 17.8 W of diode pump power and the frequency-doubling crystal LiB₃O₅ (LBO), a maximum output power of 260 mW in the blue spectral range at 464 nm has been achieved. The blue output power stability over 4 h is better than 3.2%.     

Monoclinic niobate LaNbO<Subscript>4</Subscript> as a new SRS-active crystal

The effect of the generation of stimulated Raman scattering in monoclinic niobate LaNbO₄, which is known as a base crystal for lasant ions Ln³⁺, has been discovered. The χ⁽³⁾ nonlinear Stokes and anti-Stokes biphonon lasing of this niobate has been studied under picosecond excitation.     

Erbium excitation in a SiO<Subscript>2</Subscript>: Si-nc matrix under pulsed pumping

The photoluminescence of Er³⁺ ions in a SiO₂ matrix containing silicon nanocrystals 3.5 nm in diameter is studied under resonant and nonresonant pulsed pumping with pulses 5 ns in duration. The effective erbium excitation cross section under pulsed pumping, σ_eff = 8.7 × 10^?17 cm₂, is close to that for nanocrystals. Comparison of the erbium photoluminescence intensity obtained for a SiO₂ matrix with and without nanocrystals made it possible to determine the absolute concentration of optically active nanocrystals capable of exciting erbium ions, the concentration of optically active erbium, and the average number of erbium ions excited by one nanocrystal. The study revealed that excitation transfer from one erbium ion to another is a relatively slow process, which accounts for the low efficiency of erbium ion excitation under pulsed pumping in a SiO₂ matrix containing silicon nanocrystals.     

Yield of singlet oxygen from optically pumped CCl<Subscript>4</Subscript> solution of fullerenes

Boiling occurs in a solution of oxygen and fullerenes in CCl₄ upon optical pumping of C₆₀ upon the fast appearance of incandescent fullerenes in cold solvent. Upon single-photon absorption, a spherical zone of the critical state of CCl₄ is formed within 5 ns (with a diameter of 22–25 nm, P _cr ∼ 45 atm, and T _cr ∼ 556 K). This spherical zone (gas-bubble nucleus) expands to a diameter of ∼100–400 nm for 2–5 ns. If the external pressure (natural or artificial) is rapidly released, the bubble accelerates and emerges into a vacuum chamber within 0.7–25 μs (the length of the passage is 0.1–5 cm depending on the construction of the singlet oxygen generator). We note that singlet oxygen appears 50 ns after the absorption of a photon by fullerene (i.e., inside of the almost formed gas bubble that only begins to emerge from the liquid to a low-pressure gas region).     

Diode-pumped passively mode-locked Nd:CaNb<Subscript>2</Subscript>O<Subscript>6</Subscript> laser

We have experimentally demonstrated a diode-pumped passively mode-locked Nd:CaNb₂O₆ laser for the first time to our best knowledge. With a semiconductor saturable absorber mirror (SESAM) as a passive mode locker, the laser generated stable mode-locked pulses with pulse duration of 17.3 ps and repetition rate of 88.4 MHz. With a singe-emitter laser diode pumping, the maximum average output power of the mode-locked laser was 0.843 W, with a slope efficiency of 23%. The experimental results show the Nd:CaNb₂O₆ crystal is a promising laser gain medium for picosecond pulse generation.     

Absorption by CS<Subscript>2</Subscript> molecules on “hot” band emission lines from a TEA CO<Subscript>2</Subscript> laser

We have measured absorption of emission from a TEA CO₂ laser, lasing on hot band lines, in pure CS₂ and a mixture of CS₂ with air, and we have determined the optimal lines for optical excitation. Numerical modeling has shown that as the peak intensity of the pump radiation is increased, we observe absorption saturation, the extent of which decreases as the pressure increases. The major factor responsible for absorption saturation is the “rotational bottleneck” effect. Depending on the peak intensity of the radiation, addition of a buffer gas can lead to an increase or decrease in the absorption. __________ Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 74, No. 1, pp. 61–66, January–February, 2007.     

Multiphoton satellites in the saturated-absorption Spectrum of SiF<Subscript>4</Subscript> gas

A saturated-absorption spectrum of SiF₄ gas, free of Doppler broadening, has been recorded in the lasing range of a low-pressure CO₂ laser. Multiplets of superfine structure are observed, which are due to the tunnel transitions between the states of molecular rotation around equivalent symmetry axes. Multiplet satellites are revealed, whose origin is explained by two-photon processes. Splitting of the energy levels of the superfine structure multiplet is derived from satellite interpretation. A satellite is found, which can be caused by fourphoton processes.     

Efficient Nd:Y<Subscript>0.36</Subscript>Gd<Subscript>0.64</Subscript>VO<Subscript>4</Subscript>-GdCa<Subscript>4</Subscript>O(BO<Subscript>3</Subscript>)<Subscript>3</Subscript> red laser under diode pumping into the emitting level

We report a red laser at 671 nm generation by intracavity frequency doubling of a continuous wave (cw) laser operation of a 1342 nm Nd:Y_0.36Gd_0.64VO₄ laser under diode pumping into the emitting level ⁴ F _3/2. An GdCa₄O(BO₃)₃ (GdCOB) crystal, cut for critical type I phase matching at room temperature is used for second harmonic generation of the laser. At an incident pump power of 17.8 W, as high as 1.12 W of cw output power at 671 nm is achieved. The optical-to-optical conversion efficiency is up to 6.3%, and the fluctuation of the red output power was better than 3.5% in the given 30 min.     

All-solid-state intracavity frequency-doubled Nd:Y<Subscript>0.36</Subscript>Gd<Subscript>0.64</Subscript>VO<Subscript>4</Subscript>-GdCa<Subscript>4</Subscript>O(BO<Subscript>3</Subscript>)<Subscript>3</Subscript> green laser under direct 880 nm pumping

We report a green laser at 532 nm generation by intracavity frequency doubling of a continuous wave (CW) laser operation of a 1064 nm Nd:Y_0.36Gd_0.64VO₄ laser under in-band diode pumping at 880 nm. An GdCa₄O(BO₃)₃ (GdCOB) crystal, cut for critical type I phase matching at room temperature is used for second harmonic generation of the laser. At an incident pump power of 17.8 W, as high as 2.92 W of CW output power at 532 nm is achieved. The optical-to-optical conversion efficiency is up to 16.4%, and the fluctuation of the green output power was better than 2.5% in the given 30 min.     

Room temperature diode-pumped 1875.1 nm Tm:GdVO<Subscript>4</Subscript> laser

A diode end-pumped single-frequency Tm:GdVO₄ laser at room temperature was reported. The maximal output power of single-frequency is as high as 66 mW by using two uncoated fused etalons, which are respectively 0.05 mm thick YAG and 1 mm thick quartz. We obtained the single frequency Tm:GdVO₄ laser at 1875.1 nm. The slope efficiency is 1.5%. The change of the lasing wavelength on temperature was also measured. The single-longitudinal-mode (SLM) laser can be used as a seed laser for coherent wind measurements and differential absorption LIDAR systems.