Measurement and understanding of magnetization in AC and DC fields and the determination of intragrainH c1 in highT c RBa2Cu3O7 superconductors

We present DC and low frequency AC magnetization measurements on various RBa₂Cu₃O₇ superconductors. We identify features intrinsic to these compounds, and establish the features originating from intergranular links in sintered pellets. The isothermal magnetization curves, and the temperature dependence of magnetization in field-cooled and zero field-cooled states are shown to be consistent with the calculations done following a recent extension of Bean’s model. Low field anomalies predicted within this model are observed, and yieldH _c1 values of a few Oe. These values are shown to be consistent with the temperature variation of magnetization. A comparison is made with the other existing data and it is demonstrated that earlier quoted values ofH _c1 are gross overestimates.     

Field-cooled measurements of harmonic generation in magnetization of high-T c superconductors

We present measurements of harmonic generation in the magnetization of sintered pellets of YBa₂Cu₃O₇ and Bi_1.7Pb_0.3Sr₂Ca₂Cu₃O₁₀ as a function of DC field. The DC field is applied in the field-cooled mode. Measurements are made at 77 K for various values of the AC field amplitude. A comparison is made with calculations done within the critical state model.     

Influence of gadolinium on magnetization and DC resistivity of Ni-Zn nanoferrites

The study of gadolinium substitution in small amounts on the saturation magnetization and DC resistivity of nickel-zinc nanoferrite has led to the understanding of the degree of formation of a secondary orthoferrite GdFeO₃ phase, the generation of cationic and oxygen vacancies and the dilution of gadolinium in the lattice. The role of secondary phase in modifying the electromagnetic properties has been stressed by making further investigations on the Curie temperature and the activation energies.     

交流接触器I-U特性及直流运行

分析了交流接触器I—U特性，并设计了附属电路，使交流接触器线圈可通直流电运行。     

Effective AC and DC Responses of Nonlinear Composites at Higher Concentration

For higher concentration of inclusions, an effective medium approximation （EMA） method is used to investigate the bulk effective response of weakly nonlinear composites, which are subject to the constitutive relation of electric displacement and electric field, Dα = εαE ＋Xα｜E｜^2 E. As an example of three dimensions, under the external AC and DC electric fields Eapp = Eα（1 ＋ sinωt）, we have derived the general effective nonh＇near response of composites by the EMA method for higher concentration of spherical inclusions. Furthermore, the effective nonlinear responses at harmonics are predicted.     

Even harmonics of AC susceptibility in some sintered pellets of high temperature superconductors

The real (χ′ _n) and imaginary (χ″ _n) parts of even harmonic susceptibility (n⩽6) are measured as a function of external DC field (H _dc) in the field increasing (H↑) and decreasing (H↑) cycle. Hysteresis is observed betweenH↑ andH↓ cycles. In theH↓ cycle, at a field,H _comp=4·2G, bothχ′ andχ″ of all the even harmonics vanish indicating a true cancellation of fields in the intergrain region (H _eff≈0) caused by the balance betweenH _dc and the remanent magnetization of the grains. The position of the extrema and the zero of the various harmonics undergo a shift proportional to the remanent magnetization of the grains at that particular field.     

Magnetic phase diagram of anisotropic layered superconductors via magnetization measurements forH‖c in Bi2212

The Bi₂Sr₂CaCu₂O₈ system is viewed as an archetypal of superconductors modelled as Josephson coupled CuO₂ bilayers. The isothermal and temperature dependent DC and AC magnetization measurements forH‖c in a single crystal of Bi2212 have been performed. Qualitative changes are observed to occur over a narrow range of temperature values before reaching the superconducting-normal transition. The observed behaviour can be ascribed to the rapid variation in the strength of the coupling between the superconducting CuO₂ planes (i.e., bilayers in the case of Bi2212). Strongly coupled planes behave like a 3D superconductor, whereas weakly coupled planes have a two component response attributable to 2D planes and interplanar couplings. We believe that this paper is a plethora of new findings. Our observations imply that resistivity across the planes becomes zero earlier than that within the planes. A new line (designated asH _2D(T)) above which the change in the electromagnetic response is dominated by quasi 2D-planes has been determined for the first time. This paper also contains the first observation of Differential Diamagnetic Effect (DDE) in the In-phase AC susceptibility data which signals the onset (atT _2D(H)) of dominance of response from 2D-planes. In addition to a host of interesting thermomagnetic history effects which are a consequence of interplay between the diamagnetic responses from the two components, a comparison of irreversibility lines (of the 3D state) determined by different methods on the same specimen of a HTSC is also being presented for the first time. We have come across Paramagnetic Meissner Effect (PME), first recognized in ceramic samples of Bi2212, in the temperature region of dimensional crossover in our single crystal sample, whichinter-alia confirms our labelling of the two component behaviour. A schematic phase diagram summarizing the various transformations that can occur nearT _c in the electromagnetic response of an anisotropic layered system has been drawn.     

Effective response of nonlinear cylindrical coated composites under external AC and DC electric field

This paper uses the perturbation method to study effective response of nonlinear cylindrical coated composites. Under the external AC and DC electric field E_a(1 + sinωt), the local potentials of composites at all harmonic frequencies are induced. An effective nonlinear response to composite is given for the cylindrical coated inclusions in the dilute limit.     

非线性柱形涂层复合介质有效的直流-交流电响应

利用摄动展开方法, 研究了由圆柱形带涂层杂质随机嵌入基质所形成的非线性复合介质在外加 的带有不同频率和振幅的混合电场E₀ + E₁ sinωt+E₃ sin3ωt作用下有效的直流-交流电响应, 分别推导了复合介质在杂质核、涂层及基质区域的电势分布, 并在低杂质浓度下给出了复合介质有效的非线性响应及它们之间的关系. 关键词： 非线性柱形涂层复合介质 有效的非线性响应 外加交直流电场     

Effective response in nonlinear spherical coated composites under external AC and DC electric field

By using the perturbation method, effective nonlinear direct current (DC) and alternating current (AC) responses of nonlinear composites with spherical coated inclusions randomly embedded in a host medium are studied under the action of external electric field E_a =E₀ +E₁ sin ωt+E₃ sin 3ωt with different amplitudes and frequencies. The local potentials of composites at all harmonics are given in the inclusion particles and the host regions. All effective nonlinear responses to composites and the relationship between the effective nonlinear responses at all harmonics are also deduced for the spherical coated inclusions in a dilute limit.     

Anomalous magnetic hysteresis loops and smallH c1 values in highT c superconductors

We have studied the hysteresis loops of RBa₂Cu₃O₇ (R=Gd, Ho and Y) and detected anomalies in some of them. The observed anomalies support a recent prediction by Ravi Kumar and Chaddah based on an extension of Bean’s model. The anomalies indicate lowH _c1 values and we have confirmed this by studying the onset of low-field hysteresis in less than 10 Oe at 77 K for these highT _c superconductors.     

高温超导材料、物理、应用和实验方法研究进展

文章介绍了中国科学院物理研究所超导国家重点实验室在新超导材料探索合成、高质量样品的制备、超导机理和物理性质研究、以及仪器建设方面的研究进展.在超导材料方面,生长出具有国际一流水平的氧化物高温超导单晶;在铁基高温超导材料方面,获得最高的超导转变温度;在超导机理的研究方面,建立了一些行之有效的手段,如低温比热、隧道谱、角分辨光电子谱、红外光电导谱等等,利用这些重要手段获得了一些重要结果,如从比热角度提出欠掺杂氧化物超导体应该具有一个费米弧基态,利用高精度角分辨光电子谱测量第一次观察到115meV和150meV两个新的高能量精细结构.另外,还在介观尺度超导薄膜上面观察到一些有趣的现象,如磁通系统和人工微结构之间的匹配效应.     

无序超导体磁通运动的两次退钉扎效应和重新进入超导相

考虑平面内和不同平面磁通之间的相互作用力，计算了无序各向异性超导体中磁通运动的平均速度、微分电阻随驱动力F_l的变化规律，用层间关联函数C_z的值来判断2D塑性流动和3D关联流动的运动图像.观察到随着外驱动力的增大微分电阻出现两个尖峰，它对应着磁通运动存在两次退钉扎现象.在一定层间耦合条件下，在微分电阻双峰之间，可观察到重新进入微分电阻为零的钉扎相.这与最近实验上新发现的无序弱钉扎超导体有重新进入超导相的巨大峰值效应相吻合.同时，也可发现随着驱动电流的增大，磁通运动出现由2D塑性流动到3D弹性流动的相变，这一维度的变化对应着微分电阻dV/dI曲线中的二次峰位置. 并证明当层间耦合(即代表磁场的大小)在一定范围时，3D-2D相变对应的临界电流随磁场的增大而增大, 反映了第二磁化峰附近的磁通格子软硬度改变的微观图像. 关键词： 第Ⅱ类超导体 磁通线格子 钉扎 峰值效应     

Phase diagram and critical fields of organic quasi-1d superconductors in an applied magnetic field

No consensus has been reached about the symmetry of the Bechgaard salts superconducting phase. An RG analysis is in favor of interactions dominant in the singlet channel, but very close and sub-dominant in the triplet channel. We study the properties, in a magnetic field along the b′ direction, of a d-wave singlet phase, as well as of an f-wave triplet phase. Recent data about NMR Knight shift, as well as upper critical fields have brought strong indications about the possible symmetries. We have analyzed theoretically the consequences of these experimental data: our results are in favor of a singlet phase in low field, but of a triplet phase in large fields.     

Comparison of transport and magnetic AC losses in Bi-2223/Ag tapes — the role of superconducting core geometry

AC losses were measured by 4-probe transport method and by external magnetization method in three samples of Bi-2223/Ag tape: a multifilamentary tape with separated filaments, another multifilamentary tape with ‘bridges' between filaments, and a two-shell tape. The transport losses agreed with those calculated using I_c from DC experiment. Magnetization experiments gave indications about the various paths of induced currents. For the tape with well separated filaments the main part of screening current closes inside individual filaments. Additional screening of the whole filamentary zone involves the normal metal matrix, leading to frequency dependent losses. In the case of tape with ‘bridged' filaments, supercurrents interconnect the filaments into bundles whose screening (and loss) is frequency-independent. Matching the experimental data indicates that a typical bundle was composed of 8 filaments. Magnetic losses of the two-shell tape were explained by a model for magnetization of superconducting wire with elliptical cross-section.     

Investigation of the magnetic field angle dependence of resistance, irreversibility field, upper critical field and critical current density in DC sputtered Bi-2223 thin film

We measured resistivity and transport critical current density, J_c, as a function of DC magnetic field and the angle (?) between the surface of the film and the magnetic field on ex-situ annealed, c-axis oriented Bi-2223 thin films fabricated by DC sputtering method. Irreversibility field (μ₀H_irr) and upper critical field (μ₀H_c2) were determined from the resistivity versus the applied magnetic field graph. It is observed that critical temperature (T_c), μ₀H_irr,μ₀H_c2 and J_c of the films strongly depend on the direction and strength of the field. While T_c of the film without magnetic field is observed to be about 102 K, it is found to decrease to 90 K (85 K) for the applied field perpendicular (parallel) to c-axis of the film. Not only were μ₀H_irr(0) and μ₀H_c2(0) values determined from the μ₀H_irr and μ₀H_c2 versus temperature graphs, respectively, but also penetration depths and coherence lengths were interpreted. Anisotropy of the film was also discussed by means of the change of irreversibility as a function of angle. Moreover at 4.2 K, J_c was observed to be 3000 A/cm² at zero field; however, it was found to abruptly decrease to 1982 (1 1 2 0) A/cm² under low magnetic field at ?=0° (?=90°), which indicates that anisotropic J_c behavior of the film is intrinsic. Furthermore, we provided a theoretical analysis of the obtained results in the framework of intrinsic pinning theory of superconductors. Microstructural properties of the produced films were also reinvestigated by X-ray diffractometer (XRD) and scanning electron microscopy (SEM) measurements. XRD patterns indicate that the films are c-axis oriented based on the prominent (0 0 l) peaks. SEM images show needle-like grain structures dominate the surface morphology of the films.     

Effect of pinning and driving force on the metastability effects in weakly pinned superconductors and the determination of spinodal line pertaining to order—disorder transition

We explore the effect of varying drive on metastability features exhibited by the vortex matter in single crystals of 2H-NbSe₂ and CeRu₂ with varying degree of random pinning. The metastable nature of vortex matter is reflected in the path dependence of the critical current density, which in turn is probed in a contact-less way via AC-susceptibility measurements. The sinusoidal AC magnetic field applied during AC susceptibility measurements appears to generate a driving force on the vortex matter. In a nascent pinned single crystal of 2H-NbSe₂, where the peak effect (PE) pertaining to the order—disorder phenomenon is a sharp first-order-like transition, the supercooling feature below the peak temperature is easily wiped out by the reorganization caused by the AC driving force. In this paper, we elucidate the interplay between the drive and the pinning which can conspire to make the path-dependent AC-susceptibility response of different metastable vortex states appear identical. An optimal balance between the pinning and driving force is needed to view the metastability effects in typically weakly pinned specimen of low temperature superconductors. As one uses samples with larger pinning in order to differentiate the response of different metastable vortex states, one encounters a new phenomenon, viz., the second magnetization peak (SMP) anomaly prior to the PE. Supercooling/superheating can occur across both the PE and the SMP anomalies and both of these are known to display non-linear characteristics as well. Interplay between the path dependence in the critical current density and the non-linearity in the electromagnetic response determine the metastability effects seen in the first and the third harmonic response of the AC susceptibility across the temperature regions of the SMP and the PE. The limiting temperature above which metastability effects cease can be conveniently located in the third harmonic data, and the observed behavior can be rationalized within the Bean’s critical state model. A vortex phase diagram showing different vortex phases for a typically weakly pinned specimen has been constructed via the AC susceptibility data in a crystal of 2H-NbSe₂ which shows the SMP and the PE anomalies. The phase space of coexisting weaker and stronger pinned regions has been identified. It can be bifurcated into two parts, where the order and disorder dominate, respectively. The former part continuously connects to the reentrant disordered vortex phase pertaining to the small bundle pinning regime, where the vortices are far apart, interaction effects are weak and the polycrystalline form of flux line lattice prevails.     

Rotation of magnetization in unison and langevin equations for a large spin

A single-domain ferromagnetic particle is represented as a large spin (model of rotation in unison) whose stochastic dynamics is derived from a spin-boson Hamiltonian. It is shown in the Markovian limit that thermal equilibrium exists provided that the fluctuation-dissipation theorem is supplemented by a symmetry constraint which for bilinear anisotropic and nonlinear (magnetoelastic) spin-bath coupling can only be satisfied in the underdamped limit. Only for bilinear isotropic coupling (Gilbert's theory) is it satisfied identically for arbitrary damping strength. Uniaxial and cubic symmetries are considered. For a model uniaxial crystal the thermal decay rate of M and the thermal enhancement of the macroscopic quantum tunneling rate are calculated for Gilbert and magnetoelastic dissipative couplings and compared. The effects of memory are discussed.     

Determination of the in-plane anisotropy field in hexagonal systems via rotational magnetization: Theoretical model and Monte Carlo simulations

The magnetic anisotropy field in thin films with in-plane uniaxial anisotropy can be deduced from the VSM magnetization curves measured in magnetic fields of constant magnitudes. This offers a new possibility of applying rotational magnetization curves to determine the first- and second-order anisotropy constant in these films. In this paper we report a theoretical derivation of rotational magnetization curve in hexagonal crystal system with easy-plane anisotropy based on the principle of the minimum total energy. This model is applied to calculate and analyze the rotational magnetization process for magnetic spherical particles with hexagonal easy-plane anisotropy when rotating the external magnetic field in the basal plane. The theoretical calculations are consistent with Monte Carlo simulation results. It is found that to well reproduce experimental curves, the effect of coercive force on the magnetization reversal process should be fully considered when the intensity of the external field is much weaker than that of the anisotropy field. Our research proves that the rotational magnetization curve from VSM measurement provides an effective access to analyze the in-plane anisotropy constant K ₃ in hexagonal compounds, and the suitable experimental condition to measure K ₃ is met when the ratio of the magnitude of the external field to that of the anisotropy field is around 0.2. Supported by the National Natural Science Foundation of China (Grant Nos. 90505007 and 10774061) Recommended by LI FaShen     

Comparison of band structure and superconductivity in FeSe_(0.5)Te_(0.5) and FeS

The isovalent iron chalcogenides,FeSe_(0.5)Te_(0.5) and FeS,share similar lattice structures but behave very differently in superconducting properties.We study the underlying mechanism theoretically.By first principle calculations and tightbinding fitting,we find the spectral weight of the d_(X~2-Y~2) orbital changes remarkably in these compounds.While there are both electron and hole pockets in FeSe_(0.5)Te_(0.5) and Fe S,a small hole pocket with a mainly d_(X~2-Y~2) character is absent in FeS.We find the spectral weights of d_(X~2-Y~2) orbital change remarkably,which contribute to electron and hole pockets in FeSe_(0.5)Te_(0.5) but only to electron pockets in FeS.We then perform random-phase-approximation and unbiased singular-mode functional renormalization group calculations to investigate possible superconducting instabilities that may be triggered by electron-electron interactions on top of such bare band structures.For FeSe_(0.5)Te_(0.5) ,we find a fully gapped s~±-wave pairing that can be associated with spin fluctuations connecting electron and hole pockets.For Fe S,however,a nodal dxy(or d_(x~2-y~2) in an unfolded Broullin zone)is favorable and can be related to spin fluctuations connecting the electron pockets around the corner of the Brillouin zone.Apart from the difference in chacogenide elements,we propose the main source of the difference is from the d_(X~2-Y~2) orbital,which tunes the Fermi surface nesting vector and then influences the dominant pairing symmetry.