Laser dye mixtures

Properties necessary to obtain efficient laser action from laser dyes are reviewed. It is concluded that the dye added (booster dye) to a laser dye (active dye) solution to increase its efficiency need not necessarily be a laser dye. This is illustrated by considering different spectral locations of a triplet-triplet absorption band present in the booster dye relative to the location of the laser action region (part of the fluorescence spectrum) of the active laser dye. Conditions required for booster dyes to form efficient dye mixtures are given. These observations are used to explain why specific well known laser dye mixtures show efficient, little, or no laser action at all.     

Temporal dynamics of high repetition rate pulsed single longitudinal mode dye laser

Theoretical and experimental studies of temporal dynamics of grazing incidence grating (GIG) cavity, single-mode dye laser pumped by high repetition rate copper vapour laser (CVL) are presented. Spectral chirp of the dye laser as they evolve in the cavity due to transient phase dynamics of the amplifier gain medium is studied. Effect of grating efficiency, focal spot size, pump power and other cavity parameters on the temporal behaviour of narrow band dye laser such as build-up time, pulse shape and pulse width is studied using the four level dye laser rate equation and photon evolution equation. These results are compared with experimental observations of GIG single-mode dye laser cavity. The effect of pulse stretching of CVL pump pulse on the temporal dynamics of the dye laser is studied.     

Undamped relaxation oscillations due to self-gain-switching of laser dye mixtures

Undamped relaxation oscillations were observed from a short, simple dye laser using a laser dye mixture which was pumped at 337 nm using ns pulses. The dye solution contained Rh101 as first laser dye, together with DTDCI in double function as saturable absorber and second laser dye. Two trains of intense laser pulses were generated near 619 and 685 nm, with pulse durations of ca. 4 and 2 times the resonator transit time, respectively. This method of short-pulse generation is related to double mode-locking of dye lasers. Model calculations are used to describe the pulse generation by self-gain-switching, and to estimate radiative and nonradiative contributions towards saturation of the absorber dye.     

10 ps High Power Laser System at 248 nm

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10 ps High Power Laser System at 248 nm

A simple 10 ps KrF laser system consisting of quenched dye laser oscillator pumped by a XeCl laser, a distributed feedback dye laser (DFDL), a three-stage dye amplifier and a two-stage KrF amplifier are described. The output of the laser system is 140 mJ with 10 ps pulse width by using polarization-multiplexing amplification. A focused output laser intensity of about 4×1015 W/cm2 is obtained. The saturation fluence for KrF laser is obtained with this laser.     

Study of synchronously mode-locked and internally frequency-doubledcw dye laser

The analysis of the characteristics of a synchronously mode-locked and internally frequency-doubled dye laser is presented. Dependence of dye laser pulse characteristics on the cavity length mismatch of the pump laser and dye laser is studied. Variation of the minimum pulsewidth with intracavity bandwidth and the harmonic conversion efficiency is presented in the form of graphs.     

YAG激光器往返损耗和泵浦效率的测量

依据染料调 Q 激光理论,通过实验测量计算染料调 Q YAG 激光器的往返损耗和泵浦效率。讨论染料调 Q YAG 激光器效率的有关问题。     

Generation of nearly transform-limited pulses in subnanosecond region with TEA nitrogen-laser-pumped dye laser

A dye laser is transversely pumped by a TEA nitrogen laser with 700 ps duration. The dye laser pulse has a spectral linewidth of 0.007 nm and a pulse width of ≈ 140 ps, giving a time-bandwidth product of 1.5. It is pointed out that the fluorescence lifetime of the laser dye plays an important role in generation of laser emission using a long laser cavity under subnanosecond pulse pumping.     

“波长等效激光”作用下铀原子的单色三光子共振电离谱测量

用Nd:YAG532nm激光泵浦的混合染料激光得到了在相当于铜蒸气激光器泵浦染料激光的某个波段上增强的激光输出，测得了铀原子在562-586nm波段内的单色三光子共振电离谱中140个能级，其中575.814和575.836nm两个峰很好地分开了，它们的相对强度也能测定，若用单一染料的激光是难以做到，因为目前尚无合适的染料在上述波段内能有强的激光输出。     

New efficient laser dye for pulsed and CW operation in the UV

A new laser dye for pulsed and cw operation has been synthesized which can be tuned from 362 nm up to 412 nm. For pulsed excitation with a XeCl excimer laser an energy conversion of 18.5% has been measured at the tuning maximum of the dye; this is the highest efficiency for any known dye in the UV. For cw operation a low laser threshold and a goof efficiency have been observed. The range of tuned cw dye lasers is extended by 30 nm to shorter wavelengths. The dye shows high photochemical stability even at high pump laser power.     

染料激光放大器最佳增益长度研究

在横向泵浦脉冲染料激光器中,虑及染料激发态在激光波长处的吸收,根据稳态运转转条件,应用极值原理,给出其最佳增益与染料长度的关系式。     

染料激光放大器最佳增益长度研究

在横向泵浦脉冲染料激光器中,虑及染料激发态在激光波长处的吸收,根据稳态运转转条件,应用极值原理,给出其最佳增益与染料长度的关系式。     

Power output coupling in a dye laser pumped by a nitrogen laser

A simple model for the operation of a pulsed dye laser, transversely pumped by a nitrogen laser, is presented. We consider the combined effect of the transmission of the laser output coupler, its distance from the dye cell and the saturated gain characteristics of the dye laser medium, on the operation of the laser. Experimental results are interpreted in terms of this model.     

高功率脉冲染料激光放大器物理设计

从理论研究出发,用激光增益理论得到了在平衡状态下忽略染料分子激发态吸收时,高功率脉冲梁料激光放大器物理设计的简单方法,同时以铜蒸气激光器双侧抽运的平均输出功率52.5W的脉冲染料激光放大器为例,对其物理尺寸进行了模拟设计。     

Polarization and power characteristics of pulsed dye lasers with transverse pumping

Starting from the classical theory on molecular luminescence in liquids, rate equation for two-polarization-mode laser oscillation under transverse pumping with intense excitation have been set forth neglecting the influence of orientational relaxation of the dye molecules. Hence, the laser output power and polarization under different configurations have been obtained. The results show that the dye laser is partially polarized even when the pump beam is unpolarized and no polarizing elements exist in the cavity. If we define a reference plane consisting of the axes of the pump beam and the dye laser, the laser system has to adopt the plane perpendicular to the reference plane as the polarization direction in order to yield a highly efficient, linearly polarized laser output. Experiments on a copper-vapor laser pumped dye laser verified these analytical results.     

An experimental study and theoretical analysis of the mode characteristics of a narrow line-width,pulsed dye laser oscillator at different pump powers

This paper presents an experimental study and theoretical analysis on the effect of pump power on the divergence, pointing, line-width and wavelength stability of a narrow line-width, high repetition rate dye laser oscillator. The dye laser oscillator, based on the hybrid multiple-prism grazing-incidence grating cavity, was pumped by copper vapor laser (CVL). The dye laser mode characteristics were studied at CVL average pump powers of 2, 4 and 8 W. The single pulse dye laser divergence/pointing stability was studied by far-field intensity distributions. The line-width and wavelength stability were studied using a high resolution wave-meter. The experimental results were theoretically analyzed in terms of dye laser mode structure drift induced by beam pointing instability, beam divergence and thermally induced optical path length fluctuation. A comprehensive theoretical treatment on pointing stability of dye laser beam and its influence in the dye laser wavelength stability is presented. The theoretical and experimental trends were found to be in good agreement.     

多波长染料激光系统

本文报道由四台染料激光器组成的四波长染料激光系统、测量了四个波长激光合束后的激光参量和时间特性,简要地讨论了影响有效染料激光功率的诸因素.本系统输出总功率8.9W.     

多孔硅／激光染料复合体的发光

将激光染料分子有效地嵌入多孔硅中，获得多孔硅／染料分子复合体，嵌入微量梁料分子时，复合体的发光兼有多孔硅和激光染料两者的发光特征，增加染料分子的嵌入量，复合体的发光增强，荧光的时间响应快、脉宽窄，主要表面为激光染料的发光特性。     

Angularly resolved coherent Raman spectroscopy (ARCS)

This new crossed beam configuration produces an angularly separated Coherent Anti-Stokes Raman spectrum, eliminating the need for a spectrometer. Since one of the driving laser beams is always linearly opposed to the dye laser, it may also be used as a dye pump and the experiment performed within the dye cavity for efficient laser energy utilization. With this arrangement, a broad bandwidth dye laser produces a several wavenumber resolution spectrum from a small volume with relatively simple alignment. The spectrum is scanned by varying the incidence angle of the probe beam or taken is a single pulse using a fan shaped probe beam.     

Stilbene 420激光染料的光谱特性分析

配制了Stilbene 420染料溶液。测量了其吸收光谱。以调Q倍频Nd∶YAG激光为抽运源,实现了对Stilbene 420染料的激光光谱和荧光光谱的分析。激光光谱在425 nm处获得最强峰值,半峰高宽(FWHM)为1 nm,光谱范围为420～440 nm。荧光光谱峰值在428.5 nm,与激光最强峰值相差3.5 nm。最高染料转换效率为9.26%。