激光诱导的四能级系统电子布居转移H

受激拉曼绝热通道(STIRAP)为我们提供了一种有效转移原子与分子中电子布居的方法.采用数值方法系统地分析了不同的四能级系统在受激拉曼迁移过程中电子布居的转移情况,计算了各种系统处于双光子共振和共振失谐时的转移率,并且讨论了在不同情况下第四能级对转移率的影响.计算结果表明,对于许多原子或分子系统,获得高的转移率所必须满足的条件是非常严格的,而有些四能级系统根本就不能获得高的转移率.(     

级联三能级介质中非线性光学信号的增强

揭示非最大相干可能比最大相干产生更有效的非线性频率转换. 为此以三能级级联系统(没有最大相干)为例计算其非线性光学信号的强度, 并与三能级Λ型系统(具有最大相干)进行比较. 利用非微扰方法计算表明, 在双光子共振和相同参数的条件下, 级联系统产生的非线性光学信号的最大强度约是Λ系统的两倍. 利用缀饰态表象分析表明, 两个系统中耦合跃迁的自发辐射及其介入的不可逆三光子过程具有相反的作用. 它们在级联系统中加强非线性转换, 而在Λ系统中削弱非线性转换. 关键词： 电磁感应透明 非线性光学过程 双光子共振     

串接型三能级原子的感应极化

从求在双频场作用下的三能级原子系统的哈密顿量的本征函数和本征值出发,导出系统随时间的演化规律.从而得出宏观极化的表示式.计算了极化的频谱分布和它们的相对强度.     

耗散对受激拉曼绝热转移过程的影响

应用最近发展的量子耗散理论 ,研究了耗散对简单三能级体系的受激拉曼绝热转移过程的影响 ,并与pump dump过程比较 .计算结果表明 ,受激拉曼绝热转移的机制能很好地抑制中间态的弛豫与涨落的影响 .数值结果也表明了新的量子耗散理论可以正确地描述场与耗散相互耦合的动力学问题     

运动三能级原子与驻波激光场斜交相互作用的理论分析

分析了一个运动的三能级原子与一个驻波激光场地斜交相互作用时的动量传递行为。结果表明，当原子和光场由于多普勒效应满足一定条件时，将产生受激拉曼跃迁。如果作用光相对于原子而言为一个“π／２脉冲”光时，那么经过作用后，原子将处于一个相干迭加态，其中一个态与加始相同。     

由宽波段多光子作用产生的锂分子高位态受激辐射

本文报道了以６２０．６￣６６５．０ｎｍ范围内任意波长激光作用下产生的锂分子高位态紫外扩散带受激辐射的实验结果,在锂分子－原子系统中,由激光双光子激发、并通过碰撞能量转移过程以及多光子电离复合过程使锂分子高位态获得布居,从而得到紫外区扩散受激辐射,该辐射来自较高的某个三重态向低排斥态ａ＾３Σｕ＾＋的跃迁的结果。文中对有关的辐射特性及激发机制进行了详细的分析和讨论。     

窄线宽纳秒脉冲光纤拉曼放大器的理论模型和数值分析

窄线宽纳秒脉冲光纤拉曼放大器在非线性频率变换、遥感探测和量子信息等领域有广泛的应用前景.综合考虑受激拉曼散射(stimulated Raman scattering,SRS)、受激布里渊散射(stimulated Brillouin scattering,SBS)、自相位调制(self-phase modulation)和交叉相位调制(cross-phase modulation)等非线性效应,建立了窄线宽纳秒脉冲光纤拉曼放大器的非线性动力学模型.仿真分析了放大器中脉冲激光的时频演化特性,对比研究了抽运脉冲宽度、光纤长度和信号光功率等因素对放大器性能的影响.研究发现,上述因素会影响放大器的SRS阈值、SBS阈值、输出激光线宽、激光转换效率等.例如,当脉冲宽度为800 ns时,SBS随着抽运功率的增加而发生,限制了激光功率的提升;减短抽运脉宽可以抑制SBS,但是输出激光的线宽易于展宽到数百MHz以上;增加光纤长度可以获得更低的SRS阈值和更高的转换效率,但是SBS效应和光谱展宽程度也随之增强.系统搭建中需要平衡各非线性效应,选择合适的系统参数.研究内容可以为窄线宽纳秒脉冲光纤拉曼放大器的设计搭建提供参考.     

一维动理学数值模拟激光与等离子体的相互作用

利用一维(1D3V)、显式、全电磁、相对论粒子模拟代码研究动理学范畴内激光与等离子体相互作用中的受激拉曼散射,给出了粒子代码的控制方程及其数值离散的详细方案,研究表明:动理学效应在受激拉曼散射不稳定性中十分重要;时问平均的反射率在阈值强度处跃升,在更高的激光强度处达到饱和;受激拉曼背向散射周期性地在次皮秒内爆发,离子效应延迟背向拉曼散射的发生;电子俘获导致了背向拉曼散射出现爆发;Langmuir波的非线性频移使得背向散射达到饱和。     

斯托克斯束的时空分布

基于在自由空间光束的分丰是已知的条件下，推导出适用于任意束分布的广义化的耦合波方程并得到一种计算受激拉曼散射过程中泵浦束与斯托克斯束的时、空分布的简单方法。所得结果清楚地示明受激拉曼散射过程既能使斯托克斯信号得到放大，又能使脉宽受到压缩。     

硅波导受激喇曼散射放大信号光的数值模拟

提出了用连续泵浦光在硅波导中的受激喇曼散射对信号光进行放大的方法.建立了信号光和泵浦光在硅波导中传输的耦合方程,得到了计算信号光增益的理论模型.利用数值模拟结果,对泵浦功率沿波导的分布,信号光在不同波导长度以及输入功率情况下的增益等进行了分析和讨论.结果表明,适当增加波导长度和泵浦光功率可以得到较高喇曼增益的结论.     

Adiabatic population transfer in the three-level Λ-system: two-photon lineshape

We discuss the dependence of the population transfer probability in the three-level Λ-scheme using stimulated Raman adiabatic passage on detuning from the two-photon resonance. For a large decay rate of the intermediate level we found that the two-photon lineshape is close to Gaussian with linewidth inversely proportional to the square root of the decay rate. The shift of the maximum of the two-photon line from exact two-photon resonance has been investigated.     

Coherence generation and population transfer in a three-level ladder system

This work explores the effect of spontaneous emission on coherence generation and population transfer in a threelevel ladder atomic system driven by two pulses in counterintuitive order.With adiabatic evolution and the weakdephasing approximation,we find that a large coherence and population transfer can be achieved even with spontaneous decay rate.The maximum coherence and population transfer decrease with the increase of spontaneous decay rate from the highest state to intermediate state.But this effect can be compensated by shortening the pulse width and enlarging the delay time.Results show that the coherence generation and population transfer never depend on the spontaneous decay rate from the intermediate state to ground state.The validity of the analytic solution is examined by numerical calculation.     

Theory of coherent,degenerate two-photon absorption and emission

The theory of the coherent, two-photon resonant interaction of a monochromatic field with N atoms is given. It is seen that the dynamics of the atom-field system can be completely determined when the field is “strong”. Two specific examples are given: (i) two-photon absorption by atoms in ground state, and (ii) stimulated two-photon emission by fully excited atoms, assuming a coherent field in both cases. In case (ii), the field shows photon-antibunching after the decay of half of the atoms. The merits of our approach are shown by comparing with other treatments. Our results can also be applied to certain degenerate four-wave mixing processes which are described by a similar Hamiltonian.     

两色超短脉冲激光与级联三能级分子体系相互作用的动力学研究

在不采用旋波近似和慢变幅近似的条件下,采用时域有限差分法和预估矫正法求解Maxwell-Bloch方程,对两色2π超短脉冲激光在级联三能级有机分子体系(4,4′-二甲氨基二苯乙烯分子)中传播的动力学过程进行了数值模拟.该有机分子属于一维对称体系,其电子结构和电学参量在密度泛函水平上给出.在低能量范围内,该分子可以简化为三能级体系.我们研究了在不同共振条件下,两色超短脉冲的时空演化特性和三能级体系各个能级粒子数占有率的分布情况.     

Lithium atom population transfer by population trapping in a chirped microwave pulse

Using a time-dependent multilevel approach, we demonstrate that lithium atoms can be transferred to states of lower principle quantum number by exposing them to a frequency chirped microwave pulse. The population transfer from n = 79 to n = 70 states of lithium atoms with more than 80% efficiency is achieved by means of the sequential two-photon Δ n = - 1 transitions. It is shown that the coherent control of the population transfer can be accomplished by the optimization of the chirping parameters and microwave field strength. The calculation results agree well with the experimental ones and novel explanations have been given to understand the experimental results.