磁场方向调制的InAs量子点分子量子比特

在有效质量近似条件下研究了由两个垂直耦合自组织InAs量子点组成的双电子量子点分子的电子结构，在此基础上利用系统的总自旋提出了一种磁场方向调制的量子比特方案.电子的相关效应可以导致系统的总自旋在0和1之间转换，值得注意的是，通过调节外部磁场的方向来实现这种转换，而不是像以往那样通过改变外部磁场的大小.结果支持利用系统的总自旋作为磁场方向调制的量子比特的可能性，而且因为高质量的垂直耦合量子点分子的制作工艺已经成熟，所以这是一个非常现实的量子比特设计方案. 关键词： 量子点分子 磁场方向调制 量子比特     

Quantum phase interference and spin-parity in Mn12 single-molecule magnets

Magnetization measurements of Mn12 molecular nanomagnets with spin ground states of S=10 and S=19/2 show resonance tunneling at avoided energy level crossings. The observed oscillations of the tunnel probability as a function of the magnetic field applied along the hard anisotropy axis are due to topological quantum phase interference of two tunnel paths of opposite windings. Spin-parity dependent tunneling is established by comparing the quantum phase interference of integer and half-integer spin systems.     

Probing the spin state of a single magnetic ion in an individual quantum dot

The magnetic state of a single magnetic ion (Mn2+) embedded in an individual quantum dot is optically probed using microspectroscopy. The fine structure of a confined exciton in the exchange field of a single Mn2+ ion (S=5/2) is analyzed in detail. The exciton-Mn2+ exchange interaction shifts the energy of the exciton depending on the Mn2+ spin component and six emission lines are observed at zero magnetic field. Magneto-optic measurements reveal that the emission intensities in both circular polarizations are controlled by the Mn2+ spin distribution imposed by the exchange interaction with the exciton, the magnetic field, and an effective manganese temperature which depends on both the lattice temperature and the density of photocreated carriers. Under magnetic field, the electron-Mn interaction induces a mixing of the bright and dark exciton states.     

Entanglement in a three spin system controlled by electric and magnetic fields

We study the effect of electric field and magnetic flux on spin entanglement in an artificial triangular molecule built of coherently coupled quantum dots. In a subspace of doublet states an explicit relation of concurrence with spin correlation functions and chirality is presented. The electric field modifies superexchange correlations and shifts many-electron levels (the Stark effect), as well as changing spin correlations. For some specific orientation of the electric field one can observe monogamy, for which one of the spins is separated from two others. Moreover, the Stark effect manifests itself in a different spin entanglement for small and strong electric fields. The role of magnetic flux is opposite: it leads to circulation of spin supercurrents and spin delocalization.     

Pairing of spin excitations in lateral quantum dots

We demonstrate the existence of correlated electronic states as paired spin excitations of lateral quantum dots in the integer quantum Hall regime. Starting from the spin-singlet filling-factor nu=2 droplet, by increasing the magnetic field we force the electrons to flip spins and increase the spin polarization. We identify the second spin-flip process as one accompanied by correlated, spin depolarized phases, interpreted as pairs of spin excitons. The correlated states are identified experimentally in few-electron lateral quantum dots using high source-drain voltage spectroscopy.     

Reading entanglement in terms of spin configurations in quantum magnets

We consider a quantum many-body system made of N interacting S=1/2 spins on a lattice, and develop a formalism which allows to extract, out of conventional magnetic observables, the quantum probabilities for any selected spin pair to be in maximally entangled or factorized two-spin states. This result is used in order to capture the meaning of entanglement properties in terms of magnetic behavior. In particular, we consider the concurrence between two spins and show how its expression extracts information on the presence of bipartite entanglement out of the probability distributions relative to specific sets of two-spin quantum states. We apply the above findings to the antiferromagnetic Heisenberg model in a uniform magnetic field, both on a chain and on a two-leg ladder. Using Quantum Monte Carlo simulations, we obtain the above probability distributions and the associated entanglement, discussing their evolution under application of the field.     

Spin manipulation in semiconductor quantum dots qubit

Thirty years of effort in semiconductor quantum dots has resulted in significant developments in the control of spin quantum bits(qubits). The natural two-energy level of spin states provides a path toward quantum information processing. In particular, the experimental implementation of spin control with high fidelity provides the possibility of realizing quantum computing. In this review, we will discuss the basic elements of spin qubits in semiconductor quantum dots and summarize some important experiments that have demonstrated the direct manipulation of spin states with an applied electric field and/or magnetic field. The results of recent experiments on spin qubits reveal a bright future for quantum information processing.     

Quantum Hall states near the charge-neutral Dirac point in graphene

We investigate the quantum Hall (QH) states near the charge-neutral Dirac point of a high mobility graphene sample in high magnetic fields. We find that the QH states at filling factors nu=+/-1 depend only on the perpendicular component of the field with respect to the graphene plane, indicating that they are not spin related. A nonlinear magnetic field dependence of the activation energy gap at filling factor nu=1 suggests a many-body origin. We therefore propose that the nu=0 and +/-1 states arise from the lifting of the spin and sublattice degeneracy of the n=0 Landau level, respectively.     

Implementation of Full Spin-State Interferometer

Matter-wave interferometers with spin quantum states are attractive in quantum manipulation and precision measurements. Here, five spatial interference patterns corresponding to the full spin states are observed in each run of the experiment, by the combination of the Majorana transition according to the exponential modulation of the magnetic field pulse decline curve and radio frequency coupling among multiple magnetic sub-states.Compared to the realization of two Majorana transitions, the interference fringe for the magnetic field insensitive state also has a higher contrast. After spatially overlapping the full magnetic sub-state interference patterns dozens of times in consecutive experimental measurements, clear fringes are still observed, indicating the great stability of the relative phases of different components. This indicates the potential to achieve an interferometer with multiple spin clocks.     

Few-electron molecular states and their transitions in a single InAs quantum dot molecule

We study electronic configurations in a single pair of vertically coupled self-assembled InAs quantum dots, holding just a few electrons. By comparing the experimental data of nonlinear single-electron transport spectra in a magnetic field with many-body calculations, we identify the spin and orbital configurations to confirm the formation of molecular states by filling both the quantum mechanically coupled symmetric and antisymmetric states. Filling of the antisymmetric states is less favored with increasing magnetic field, and this leads to various magnetic field induced transitions in the molecular states.     

用于指导仲氢诱导核极化状态保存的己烯分子中五自旋的单重态制备和寿命研究

仲氢诱导核极化（PHIP）技术能极大地增强核磁共振（NMR）信号的灵敏度,已被应用于磁共振成像、原位化学反应监测等领域．除了不断提高不同分子极化后的灵敏度外,延长和保存高极化度状态对PHIP技术的应用也至关重要,其中将极化后的状态制备成核自旋单重态是目前被研究较多的一种方法．本文以能被PHIP技术极化的己烯分子为研究对象,通过设计优化控制脉冲,对分子中的一个五自旋体系进行操控,制备了多种核自旋单重态,结果表明：己烯分子的碳-碳双键上存在三种不同的核自旋单重态,它们的寿命均长于仲氢极化后产生的初始态的寿命,可以作为延缓极化度衰减的一种中间态;通过对比单重态的寿命与相应自旋的纵向弛豫时间发现,将极化后己烯的状态转化为纵向磁化可能也是一种保存极化度的有效方法．     

Kondo-transport spectroscopy of single molecule magnets

We demonstrate that in a single molecule magnet strongly coupled to electrodes the Kondo effect involves all magnetic excitations. This Kondo effect is induced by the quantum tunneling of the magnetic moment. Importantly, the Kondo temperature TK can be much larger than the magnetic splittings. We find a strong modulation of the Kondo effect as a function of the transverse anisotropy parameter or a longitudinal magnetic field. Both for integer and half-integer spin this can be used for an accurate transport spectroscopy of the magnetic states in low magnetic fields on the order of the easy-axis anisotropy parameter. We set up a relationship between the Kondo effects for successive integer and half-integer spins.     

Dynamic model of ortho-para conversion of water molecules

A quantum model of mutual conversion of spin isomers of the water molecule, involving a proton of a neighboring water molecule, is proposed. Molecules interact due to magnetic dipole-dipole forces which give rise to flip-flop processes. An additional adsorption energy different in magnitude and sign for singlets and triplets arises from a fast exchange of spin states within an acceptor molecule. A slower flip-flop process controls the simultaneous evolution of all three protons, which results in the transition between singlet and triplet states. Based on the developed model, experimental data on ortho-para-water are discussed.     

Spin supersolid in an anisotropic spin-one Heisenberg chain

We consider an S=1 Heisenberg chain with strong exchange (Delta=J(z)/J(perpendicular)) and single-ion uniaxial anisotropy (D) in a magnetic field (B) along the symmetry axis. The low-energy spectrum is described by an effective S=1/2 XXZ model that acts on two different low-energy sectors for a finite range of fields. The vacuum of each sector exhibits Ising-like antiferromagnetic ordering coexisting with the finite spin stiffness obtained from the exact solution of the XXZ model. In this way, we demonstrate the existence of a spin supersolid phase. We also compute the full Delta-B quantum phase diagram using a quantum Monte Carlo method.     

Spin edge states in two-dimensional electron systems in the presence of Zeeman effect

We study the spin edge states, induced by the combined effect of Bychkov-Rashba spinorbit and Zeeman interactions or of Dresselhaus spin-orbit and Zeeman interactions in a twodimensional electron system, exposed to a perpendicular quantizing magnetic field and restricted by a hard-wall confining potential. We derive an exact analytical formula for the dispersion relations of spin edge states and analyze their energy spectrum versus the momentum and the magnetic field. We calculate the average spin components and the average transverse position of electron. It is shown that by removing the spin degeneracy, spin-orbit interaction splits the spin edge states not only in the energy but also induces their spatial separation. Depending on the type of spin-orbit coupling and the principal quantum number, the Zeeman term in the combination with spin-orbit interaction increases or decreases essentially the splitting of bulk Landau levels while it has a weak influence on the spin edge states.     

Proton exchange within water molecule

The exchange by quantum states between nuclear spins of two water molecule protons is considered. It is shown that such an intramolecular exchange does not break spin isomers of the molecule and does not cause quantum transitions between singlet and triplet states of the molecule spin system.     

Spin-orbit coupling and anisotropy of spin splitting in quantum dots

In lateral quantum dots, the combined effect of both Dresselhaus and Bychkov-Rashba spin-orbit coupling is equivalent to an effective magnetic field +/- B(SO) which has the opposite sign for s(z)= +/- 1/2 spin electrons. When the external magnetic field is perpendicular to the planar structure, the field B(SO) generates an additional splitting for electron states as compared to the spin splitting in the in-plane field orientation. The anisotropy of spin splitting has been measured and then analyzed in terms of spin-orbit coupling in several AlGaAs/GaAs quantum dots by means of resonant tunneling spectroscopy. From the measured values and sign of the anisotropy we are able to determine the dominating spin-orbit coupling mechanism.     

Voltage-selective bidirectional polarization and coherent rotation of nuclear spins in quantum dots

We propose and demonstrate that the nuclear spins of the host lattice in GaAs double quantum dots can be polarized in either of two opposite directions, parallel or antiparallel to an external magnetic field. The direction is selected by adjusting the dc voltage. This nuclear polarization manifests itself by repeated controlled electron-nuclear spin scattering in the Pauli spin-blockade state. Polarized nuclei are also controlled by means of nuclear magnetic resonance. This Letter confirms that the nuclear spins in quantum dots are long-lived quantum states with a coherence time of up to 1 ms, and may be a promising resource for quantum-information processing such as quantum memories for electron spin qubits.     

High-Spin Paramagnetic Ions as Qubits and Qutrits for Quantum Computations

Russian Physics Journal - Paramagnetic ions having two electrons and spin S = 1 in zero magnetic field are proposed for new physical performance of elementary quantum computing operations by pulsed...     

Magnetic bloch electron states and spin polarization in 2D superlattices without an inversion center with Rashba spin-orbit interaction in an electron gas

The quantum states of carriers in 2D doubly periodic n-type semiconducting superlattices without spatial inversion symmetry in an external magnetic field are calculated in the one-electron approximation. It is shown that the spin-orbit interaction and spin splitting in the magnetic field may lead to the occurrence of the photovoltaic effect in a 2D electron gas without an inversion center and to a nonzero spin magnetization of the electron gas in the plane perpendicular to the magnetic field.