非线性频率转换新原理新平台与新应用研究

作为最早发现的非线性光学现象之一,非线性频率转换经过几十年的发展,从原理到应用均已不断成熟。非线性频率转换过程中新的相位匹配原理被不断提出和实现。除此之外,随着集成光学、结构光子学及量子光学等领域的不断发展,非线性频率转换在各领域的研究和应用又重新焕发活力,并发挥着不可替代的作用。本篇综述围绕非线性频率转换主题,突出非线性频率转换的新原理、新平台与新应用研究,并以本团队研究成果为基础,介绍相关领域的研究进展,主要分为以下几个方面:非线性界面相位匹配新原理;结构光场非线性谐波调控;铌酸锂薄膜集成非线性光学新平台;单光子频率转换、光量子接口等新应用。     

Quantum Tomography, Wave Packets, and Solitons

The wave packets, both linear and nonlinear (like solitons) signals described by a complex time-dependent function, are mapped onto positive probability distributions (tomograms). The quasidistributions, wavelets, and tomograms are shown to have an intrinsic connection. The analysis is extended to signals obeying to the von Neumann-like equation. For solitons (nonlinear signals) obeying the nonlinear Schrödinger equation, the tomographic probability representation is introduced. It is shown that in the probability representation the soliton satisfies a nonlinear generalization of the Fokker–Planck equation. Solutions to the Gross–Pitaevskii equation corresponding to solitons in a Bose–Einstein condensate are considered.     

Periodic,quasi‐periodic,and random quadratic nonlinear photonic crystals

Quadratic nonlinear photonic crystals are materials in which the second order susceptibility χ⁽²⁾ is spatially modulated while the linear susceptibility remains constant. These structures are significantly different than the more common photonic crystals, in which the linear susceptibility is modulated. Nonlinear processes in nonlinear photonic crystals are governed by the phase matching requirements, which are determined by the reciprocal lattice of these crystals. Therefore, the modulation of the nonlinear susceptibility enables to engineer the spatial and spectral response in various three‐wave mixing processes. It enables to support the efficient generation of new optical frequencies at multiple directions. We analyze three wave mixing processes in nonlinear photonic crystals in which the modulation is either periodic, quasi‐periodic, radially symmetric or even random. We discuss both one‐dimensional and two‐dimensional modulations. In addition to harmonic generations, we outline several new possibilities for all‐optical control of the spatial and polarization properties of optical beams in specially designed nonlinear photonic crystals.     

A unified theory of nonlinear Langmuir waves, ion-acousticsolitons, and double layers

Steady-state, nonlinear potential solutions in a two-fluid plasma are formulated in terms of an integral equation that expresses the conservation of total pressure. By appropriately specifying the conservation constants and boundary conditions of the effective potential function, the integral curves yield, respectively, three types of solutions: nonlinear Langmuir waves, ion-acoustic solitons, and double layers. The similarities and differences of the existence conditions for these nonlinear potential structures are discussed     

Discretely tunable, all-solid-state laser in the green, yellow, and red

We report an all-solid-state intracavity Raman laser with intracavity nonlinear sum-frequency generation providing visible output wavelengths selected from second harmonics and sum frequencies of the fundamental and Stokes fields. The laser comprises a diode end-pumped Nd:YAG laser, an acousto-optic Q switch, a KGd(WO4)2 Raman crystal, and a lithium borate nonlinear converter in a resonator designed to accommodate dynamic thermal lensing. For 20 W of pump power, output powers up to 1.8 W are demonstrated at wavelengths of 532, 555, 579, and 606 nm, selectable by angle and temperature tuning of the nonlinear medium.     

Investigation of the nonlinear optical characteristics of composite materials based on sapphire with silver, copper, and gold nanoparticles by the reflection Z-scan method

The nonlinear optical characteristics of silver, copper, and gold nanoparticles synthesized in a sapphire matrix by ion implantation are studied. The measurements are performed by the RZ-scan method with optical reflection at the radiation wavelength of a picosecond Nd:YAG laser (λ = 1064 nm). The nonlinear refractive indices and the real parts of the third-order nonlinear susceptibility of the composites are determined. It is shown that the nonlinear refraction in the samples is caused by the Kerr effect.     

Nonlinear analysis of wiggler taper, node competition, andspace-charge effects for a 280-GHz free electron laser

The nonlinear characteristics of a 280-GHz free electron laser (FEL) are simulated by numerical computation. The three-dimensional set of coupled nonlinear differential equations is solved for a set of TE and TM modes valid for the high gain Compton regime. The use of a nonlinear taper for efficiency enhancement, the sensitivity of gain to competing mode power levels, space-charge effects, and the effect of electron beam source distributions on gain and efficiency are examined for a 10-MeV, 3-kA beam. It is found that the nonlinear taper greatly enhances the gain and efficiency and makes the saturation power levels relatively insensitive to the competing mode power levels. The efficiency is increased to 48% by means of a nonlinear taper in which the 3-D and wiggler-averaged codes are compared and the effects of space charge are found to reduce the efficiency to a level of 32%. The effect of beam quality in terms of the four volume phase space is examined and found to have an observable effect at this wavelength     

Nonlinear standing waves,resonance phenomena,and frequency characteristics of distributed systems

This review is dedicated to resonator oscillations under conditions of a strongly expressed nonlinearity under which steep shock fronts emerge in the wave profiles. Models and approximated methods for their analysis for quadratic and cubic nonlinear media are examined, as well as for nonlinearity when taking into account the mobility of boundaries. The forms of the profiles are calculated both for a steady-state oscillation regime and during the establishment of the profiles. Dissipative losses and selective losses at specially chosen frequencies are considered. An analysis of nonlinear Q-factor is given. The possibility of increasing the acoustic energy accumulated in the cavity of the resonator is discussed. Special attention is given to various physical phenomena that are exhibited only in nonlinear acoustic fields.     

Strong and weak nonlinear dynamics: Models, classification, examples

The difference between strong and weak nonlinear systems is discussed. A classification of strong nonlinearities is given. It is based on the divergence or inanity of series expansions of the equation of state commonly used in the study of weak nonlinear phenomena. Such power or functional series cannot be used in three cases: (i) if the equation of state contains a singularity; (ii) if the series diverges for strong disturbances; (iii) if the linear term is absent, and higher nonlinearity dominates. Strong nonlinearities are known in acoustics, optics, mechanics and in quantum field theory. Mathematical models, solutions and observed phenomena are presented. For example, an equation of Heisenberg type and its generalization for strongly nonlinear wave system are given. In particular, exact solutions of new “quadratically cubic” Burgers and Riemann-Hopf equations are discovered.     

Stochastic representation of nearly-Gaussian,nonlinear processes

The use of polynomial functionals of the white noise process is discussed for the treatment of nonlinear random processes. It is noted that such treatments are useful for nearly-Gaussian processes. Applications of such representations to nonlinear systems and to nonlinear fluid mechanics problems (turbulence) are reviewed.     

共振、混沌与束晕形成

研究强流束中的非线性共振、混沌与束晕形成的关系.给出强流束中非线性共振范围的表达式及其随束流空间电荷效应变化的数值结果和图表曲线,提出由非线性共振而激发的束晕形成的空间电荷效应极限,并分析束晕形成的过程.     

Multicomponent photorefractive cnoidal waves: stability, localization, and soliton asymptotics

An algorithm of building up a different class of stable self-consistent multicomponent periodical solutions of the nonlinear Schr?dinger equation--multicomponent cnoidal waves--has been formulated by the example of a nonlinear wave propagating through a photorefractive crystal with a drift nonlinear response. Exact analytical expressions, describing distribution of light field in the components, have been obtained for solutions, which include up to three mutually incoherent components. It has been shown that such cnoidal waves are stable and their spatial structure is robust to collisions with the same cnoidal waves and to stochastic perturbations of the components' intensity distributions in a sufficiently wide range of changing spatial period.     

Modeling the terahertz radiation generation process,obtained by filtration of spectral supercontinuum,formed during propagation of femtosecond laser pulse in GaAs crystal

We present the results of theoretical studies of the process of generation of terahertz radiation arising via interaction of few-cycle laser pulses propagating in an isotropic nonlinear medium. Numerical time-integration, by the finite-difference method, of the system of nonlinear Maxwell equations has been performed. We consider the interaction of mutually-orthogonal linearly polarized pulses, both having the central wavelength of 1.98 μm, durations of 30 fs, and the energies of 30 nJ, propagating along the normal to the 〈110〉 plane in a 1 mm-thickness GaAs crystal. In the nonlinear part of the medium polarization the without-inertia nonlinear second-order susceptibility is taken into account. The process of formation of a terahertz pulse arising via spectral filtration of supercontinuum formed in the spectra of pump pulses at the output of nonlinear crystal is studied. The dependences of both the current frequency of the pump pulses on time for different lengths of nonlinear crystal and of pump pulse durations on the crystal length are obtained. Also the dependences of the current frequency of the terahertz pulse on time at different crystal lengths, as well as of the efficiency of generation of terahertz radiation on the length of nonlinear crystal and on the energy of pump pulses are obtained.     

Classical analogs for Rabi-oscillations,Ramsey-fringes,and spin-echo in Josephson junctions

We investigate the results of recently published experiments on the quantum behavior of Josephson circuits in terms of the classical modeling based on the resistively and capacitively-shunted (RCSJ) junction model. Our analysis shows evidence for a close analogy between the nonlinear behavior of a pulsed microwave-driven Josephson junction at low temperature and low dissipation and the experimental observations reported for the Josephson circuits. Specifically, we demonstrate that Rabi-oscillations, Ramsey-fringes, and spin-echo observations are not phenomena with a unique quantum interpretation. In fact, they are natural consequences of transients to phase-locking in classical nonlinear dynamics and can be observed in a purely classical model of a Josephson junction when the experimental recipe for the application of microwaves is followed and the experimental detection scheme followed. We therefore conclude that classical nonlinear dynamics can contribute to the understanding of relevant experimental observations of Josephson response to various microwave perturbations at very low temperature and low dissipation.     

Fluctuation,relaxation, and extensivity of macrovariables in nonequilibrium systems

The extensive property of a macrovariable is proved for a quantal system whose Hamiltonian depends on time and for a stochastic system whose temporal evolution operator depends on time. These generalized situations are concerned with bulk-contact open systems. The extensive property, fluctuation, and nonlinear relaxation are investigated explicitly by calculating rigorously generating functions in exactly soluble models such as the linear stochastic model and linearXY model. The relation between the nonlinear critical slowing down and linear critical slowing down is also discussed.     

Nonlinear wave mechanics,information theory,and thermodynamics

A logarithmic nonlinear term is introduced in the Schrödinger wave equation, and a physical justification and interpretation are provided within the context of information theory and thermodynamics. From the resulting nonlinear Schrödinger equation for a system at absolute temperatureT>0, the energy equivalence,kT 1n 2, of a bit of information is derived.     

Rogue waves: Classification,measurement and data analysis,and hyperfast numerical modeling

The last twenty years has seen the birth and subsequent evolution of a fundamental new idea in nonlinear wave research: Rogue waves, freak waves or extreme events in the wave field dynamics can often be classified as coherent structure solutions of the requisite nonlinear partial differential wave equations (PDEs). Since a large number of generic nonlinear PDEs occur across many branches of physics, the approach is widely applicable to many fields including the dynamics of ocean surface waves, internal waves, plasma waves, acoustic waves, nonlinear optics, solid state physics, geophysical fluid dynamics and turbulence (vortex dynamics and nonlinear waves), just to name a few. The first goal of this paper is to give a classification scheme for solutions of this type using the inverse scattering transform (IST) with periodic boundary conditions. In this context the methods of algebraic geometry give the solutions of particular PDEs in terms of Riemann theta functions. In the classification scheme the Riemann spectrum fully defines the coherent structure solutions and their mutual nonlinear interactions. I discuss three methods for determining the Riemann spectrum: (1) algebraic-geometric loop integrals, (2) Schottky uniformization and (3) the Nakamura-Boyd approach. I give an overview of several nonlinear wave equations and graph some of their coherent structure solutions using theta functions. The second goal is to discuss how theta functions can be used for developing data analysis (nonlinear Fourier) algorithms; nonlinear filtering techniques allow for the extraction of coherent structures from time series. The third goal is to address hyperfast numerical models of nonlinear wave equations (which are thousands of times faster than traditional spectral methods).     

Existence and analytical predictions of periodic motions in a periodically forced,nonlinear friction oscillator

The grazing bifurcation, stick phenomena and periodic motions in a periodically forced, nonlinear friction oscillator are investigated. The nonlinear friction force is approximated by a piecewise linear, kinetic friction model with the static force. The total forces for the input and output flows to the separation boundary are introduced, and the force criteria for the onset and vanishing of stick motions are developed through such input and output flow forces. The periodic motions of such an oscillator are predicted analytically through the corresponding mapping structure. Illustrations of the periodic motions in such a piecewise friction model are given for a better understanding of the stick motion with the static friction. The force responses are presented, which agreed very well with the force criteria. If the fully nonlinear friction force is modeled by several portions of piecewise linear functions, the periodically forced, nonlinear friction oscillator can be predicted more accurately. However, for the fully nonlinear friction force model, only the numerical investigation can be carried out.     

Z-Scan studies of KYW, KYbW, KGW, and Ba(NO3)2 crystals

We present the studies of nonlinear refraction and nonlinear absorption in promising crystals which are extensively used in Raman lasers or as solid-state laser host materials: Ba(NO₃)₂, KGW, KYW, and KYbW. The single-beam z-scan technique with 1 ps laser pulses at 790 and 395 nm has been applied for the study. Nonlinear refraction-index intensity-coefficients and two-photon absorption coefficients have been determined for the crystals. The considerable enhancement of nonlinear refraction is observed in the crystals at 395 nm.     

Ultra-compact all-optical phase-controlled NAND,OR, XOR,XNOR, and NOT multi-function logic gate

Optical and Quantum Electronics - A theoretical analysis of the modulational instability (MI) in a nonlinear oppositely directional coupler with one channel fabricated from nonlinear medium having...