Polarization dependence of photoexcitation in photofield emission

The mechanisms of one-photon photoexcitation in photofield emission have been studied experimentally by measuring the photocurrent from selected crystallographic planes of a tungsten field emitter as a function of the polarization of the incident light. Two distinct components of the photocurrent were identified. The corresponding excitation mechanisms were deduced from the results of the polarization measurements supplemented by band structure considerations. Surface effect emission dominates at large angles of light incidence, and is observed even from within the geometric shadow of the tip. It depends on the light polarization inside the metal in a characteristic way. Indirect bulk photoemission is prominent at small angles of light incidence and is independent of the polarization inside the metal. It is concluded that bulk and surface excitations in photofield emission can be distinguished by appropriately selecting the direction of polarization and the angle of incidence of the incident light.     

Investigations of aluminum films with synchrotron radiation of wavelengths 500 to 1000 Å

Measurements of the photocurrent from thin Al cathodes in a windowless electron multiplier as a function of wavelength, polarization, angle of incidence, and film thickness have been carried out in the extreme vacuum ultraviolet. A normal incidence monochromator utilizing synchrotron radiation provided highly polarized light. A marked difference is found between the photocurrent measured during irradiation of thin films with “s” and “p” polarized light at wavelengths near the Al plasma wavelength (835 Å). For films thicker than about 500 Å pronounced interference effects are found in both “p” and “s” light at wavelengths less than the plasma wavelength. The observations can be explained by assuming the photocurrent is related to the photon density (electromagnetic energy density) in the photocathode. Calculations of the energy density in films irradiated with light give the structure found in the measured photocurrent. The measurements indicate our monochromator yields light with a degree of polarization consistent with the calculated polarization of the synchrotron radiation incident upon our grating (about 85%).     

Circular photocurrent in Ag/Pd resistive films upon excitation by femtosecond laser pulses

This paper presents the results of the experimental investigation of the generation of nanosecond photocurrent pulses in silver–palladium (Ag/Pd) resistive films under excitation by laser pulses with a duration of 120 fs at a wavelength of 795 nm. The photocurrent was detected in the direction perpendicular to the plane of incidence of the laser beam on the film. The 20-μm-thick films under investigation were a porous polycrystalline material consisting predominantly of nanocrystallites of the palladium oxide PdO and the Ag–Pd solid solution. The direction of the photocurrent observed in the films depends on the sign of the circular polarization of the incident radiation. It was found that the observed photocurrent depends on the angle of incidence in accordance with the odd law and consists of the circular and linear contributions, which are dependent on and independent of the sign of the circular polarization, respectively. It was shown that the circular photocurrent is significantly higher than the linear photocurrent. It was established that, for both the circular and linear polarizations, the photocurrent is directly proportional to the power of the excitation radiation. For the linearly polarized laser radiation, the photocurrent depends on the polarization angle in accordance with the odd law. The regularities revealed are consistent with the mechanism of the generation of transverse photocurrent with the photon drag effect.     

Anomalous polarization effects during light scattering in random media

The dependence of the intensity of light backscattered from a layer of a randomly inhomogeneous medium on the polarization of incident light and the size of scatterers has been investigated. The results of numerical simulation have demonstrated that the direction of rotation of the plane of polarization is different in systems with small- and large-scale inhomogeneities. It is shown for the first time that the dependence of the sign of the residual circular polarization on the size of scatterers can be observed in systems described by the Henyey-Greenstein phase function used in simulating biological tissues. A similar anomalous polarization effect, which consists in changing the direction of rotation of the plane of polarization of backscattered light with an increase in the scattering angle, is revealed in studying the coherent backscattering component. These polarization effects are observed in light backscattering from optically active media.     

Polarization characteristics and magneto-optic diffraction efficiency at oblique light incidence

In a great number of papers that deal with the study of the magneto-optic diffraction (MOD), theoretical analysis and interpretation of experimental data are performed without regard for reflection effects of the incident and diffracted light beams on the entrance and exit surfaces of the transparent film. In consequence the MOD parameters are not connected with the angle of light incidence and the orientation of the incident light polarization plane. In the present work the reflection effects are taken into account. For the Raman-Nat diffraction region the general expressions involving the relationships of diffracted light polarization and intensity with the symmetry of the grating, angle of incidence and polarization of the incident light are obtained. In particular it is shown that even for a symmetrical grating the polarization of the zeroth-order diffracted beam differs from that of the incident light, and the polarization of higher-order beams differs from the orthogonal one providing that the incident light is not s- or p-polarized. A maximum in the angular dependence of diffraction efficiency is predicted being observed experimentally.     

Linear intensity dependence of photo-induced field emission from tungsten

As a first step in an investigation of the polarization dependence of photo-induced field emission from tungsten, the dependence of the photocurrent on the intensity of illumination has been studied. The beam from a CW krypton ion laser operating at selected wavelengths in the visible region of the spectrum was focussed onto the field emitter, and the emission current in a narrow energy range (chosen to minimize tip heating effects) was measured as a function of intensity. The apparatus was designed to ensure that the position of the focal spot and the intensity of illumination could be adjusted without mutual influence. The photocurrent from each crystal plane was found to be linearly proportional to the luminous intensity over the range of intensity investigated (0–35 MW m^?2). It is concluded that in tungsten there exists a low intensity regime where the external current in photo-induced field emission is caused predominantly by one-photon excitations.     

半导体中相干控制光电流对光场的偏振依赖性

采用黄金定则方法和Kane六能带模型，分析了半导体中的量子干涉控制光生电流效应.计算了不同偏振光场下载流子在动量空间的初始布居分布，从微观上阐明了相干电流对光场的偏振依赖特性.在平行线偏振情况下，相干电流方向沿光场的偏振方向；而在正交线偏振情况下，电流方向与倍频光的偏振方向相同.还证明了只有当单光子跃迁和双光子跃迁相平衡时才能获得最大的电流注入效率. 关键词： 量子干涉 光电流 线偏振光     

Thin-film capacitor M/Pb(ZrTi)O3/M as a polarization-sensitive photocell

A steady-state short-circuit photocurrent of preliminarily polarized submicron capacitors with a polycrystalline Pb(ZrTi)O₃ (PZT) film is investigated under irradiation by light with a wavelength λ > 0.4 μm. The structures with different M/PZT interfaces that differ in the leakage current by more than an order of magnitude are found to demonstrate virtually the same value of the photocurrent, which is always directed opposite to the ferroelectric polarization of the PZT film. Although the magnitude of photocurrent is determined by the degree of polarization of the film, the observed photocurrent is not a depolarization current of the ferroelectric film. Therefore, the M/PZT/M capacitor behaves like a polarization-sensitive photocell. Within the proposed theory of a heterophase medium, the dependence of the photocurrent on the magnitude of the preliminary polarization is calculated and proves to be in reasonable agreement with the experimental results.

     

纳米ZnO薄膜的反射及偏振特性研究

用电子束蒸发镀膜法制备了纳米ZnO薄膜．通过测量其X射线衍射谱,计算出纳米ZnO颗粒的平均粒径大小为30nm．实验研究了纳米ZnO薄膜的反射和偏振性质,结果表明：当振动方向平行于入射面的线偏振光（简称P光）入射纳米ZnO薄膜时,不存在严格意义上的布儒斯特角,但对于入射角却存在一个临界角β．当入射角小于β时,反射光的振动面随着入射角的增大向左旋转;当入射角大于β时,振动面转而向右旋转;当振动方向垂直于入射面的线偏振光（简称S光）入射纳米ZnO薄膜时,反射光的振动面始终向左旋转．     

Rotation of the light polarization plane by an ensemble of oriented linear associates: Model representations

In an “oriented gas” model expressions are obtained for the angle of nongyrotropic rotation of the polarization plane (NRPP) of transmitted light by an ensemble of oriented associates consisting of nongyrotropic molecules. The cluster character of the nongyrotropic rotation of the polarization plane and the dependence of its angle on the incident light polarization vector azimuth are noted, which distinguish linear and circular polarization effects. Measurement of linear dichroism by the angle of nongyrotropic rotation of the polarization plane with the use of commercial spectropolarimeters is theoretically justified. Institute of Molecular and Atomic Physics, National Academy of Sciences of Belarus, 70, F. Skorina Ave., Minsk, 220072 Belarus. Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 65, No. 1, pp. 95–101, January–February, 1998.     

Capture of polarized electrons into excited atomic states in grazing scattering from a magnetized Ni(110) surface

The spin polarization of electrons captured into excited atomic levels of atoms during the scattering of fast ions from a magnetized Ni(110) surface under a grazing angle of incidence is deduced from the polarization of the fluorescence light. In our studies we have investigated the dependence of the spin polarization on projectile velocity and angle of incidence and observed generally small polarizations for captured electrons.     

Excitation of eigenmodes at gyroelectromagnetic gratings in conical mounting

We study the diffraction of electromagnetic waves at periodically corrugated isotropic–gyroelectromagnetic surfaces, in the index-matching situation, when the plane of incidence forms an arbitrary angle with the main section of the grating (“conical mounting”). It is shown that, under these conditions, eigenmodes can be excited at certain angles of incidence, which can be calculated. We analyze the variation of the position of the anomalies when the orientations of the plane of incidence and of the optic axis are varied. We also show the dependence of the maximum reflected power as a function of the groove height-to-period ratio.     

A study on polarization dependence of quadratic photocurrent in light emitting diodes using real time cross-polarized autocorrelation signals

An experimental study on the polarization dependence of the quadratic photocurrent in commercial light emitting diodes (LEDs) has been carried out using 200 fs laser pulses from a cw mode-locked Nd:glass oscillator. The variation of induced quadratic current with respect to orientation of polarization of the laser beam is measured using single and double beams. Cross-polarized autocorrelation measurements have been performed in real time at different orientations of the LEDs to differentiate the contributions to the quadratic photocurrent of two-photon absorption and second harmonic generation. The theoretical analysis of cross-polarized signals under different orientations is presented. PACS 42.65.Re; 42.65.ky; 42.50.Hz; 85.60.Jb     

The interference enhancement of light polarization conversion from structures with a quantum well

The optical activity of crystals leads to the occurrence of ellipticity at the reflection of light which is linearly polarized in the interface plane or normally to it. The effect experimentally discovered in the investigated structures with quantum wells is due to a spin-orbit interaction and birefringence. The qualitative dependence of the effect on the change in the orientation of the linear polarization of the incident light has been revealed. A sharp increase in the degree of the polarization conversion in a narrow range of incidence angles for light polarized in the incidence plane has been detected. The latter is due to the influence of the interference of the reflected wave on the structure thickness.     

The vectorial photoelectric effect on cesiated GaAs (110) and Si (111) surfaces

Polarization dependence of photoelectric emission at 45° incidence was investigated on cesiated Si (111) and GaAs (110) surfaces. Yield and energy distributions from surfaces covered with submonolayers of cesium did not depend on polarization of the light. Energy distributions and emitted current depend on the plane of polarization when more than a monolayer of cesium was deposited onto cooled samples. These phenomena can be explained in terms of radiation density calculated from Fresnel's equation and bulk optical properties of the semiconductor; no polarization dependence of the optical excitation need be invoked.     

Influence of polarization direction, incidence angle, and geometry on near-field enhancement in two-layered gold nanowires

The influences of polarization direction, incidence angle, and geometry on near-field enhancements in two-layered gold nanowires (TGNWs) have been investigated by using the vector wave function method. When the polarization direction is perpendicular to the incidence plane, the local field factor (LFF) in TGNW decreases first and then increases with the increase in the incidence angle. The minimum LFF is observed at an incidence angle of 41°. It is found that the increase in the dielectric constant of the inner core leads to a decrease in the LFF. With the increase in the inner core radius, the LFF in TGNW increases first and then decreases, and the maximum LFF is observed at an inner core radius of 27 nm. On the other hand, when the polarization direction is parallel to the incidence plane, the collective motions of the induced electrons are enhanced gradually with the decrease in the incidence angle, and hence the near-field enhancement is increased.     

One-dimensional photonic crystals with a planar oriented nematic layer: Temperature and angular dependence of the spectra of defect modes

Transmission spectra of a one-dimensional photonic crystal (PC) formed by two multilayer dielectric mirrors and a planar oriented layer of 5CB nematic liquid crystal (LC) that is sandwiched between these mirrors and serves as a structure defect are investigated experimentally. Specific features of the behavior of the spectrum of defect modes as a function of the angle of incidence of light on the crystal are studied for two polarizations: parallel and perpendicular to the director of the LC; the director either lies in the plane of incidence or is perpendicular to it. It is shown that, for the configurations considered, the maxima of the defect modes shift toward the short-wavelength region as the tilt angle of incidence radiation increases; this tendency is more manifest for the parallel-polarized component, when the director lies in the plane of incidence. In the latter case, the width of the photonic band gap (PBG) appreciably decreases. The temperature dependence of the polarization components of the transmission spectra of a PC is investigated in the case of normal incidence of light. The spectral shift of defect modes due to the variation of the refractive index of the LC at the nematic-isotropic liquid phase transition point is measured. It is shown that, in real PCs, the amplitude of defect modes decreases when approaching the center of the band gap, as well as when the number of layers in the dielectric mirrors increases. Theoretical transmission spectra of the PCs calculated by the method of recurrence relations with regard to the decay of defect modes are in good agreement with experimental data.     

The temporal Mueller matrix solution for polarimetric scattering from a layer of random non-spherical scatterers

The Mueller matrix solution of the vector radiative transfer equation with time dependence is derived in this paper. It is applied to simulation of polarimetric bistatic scattering from a layer of non-uniformly oriented, random non-spherical scatterers when a Gaussian plane pulse is incident upon. Co-polarized and cross-polarized bistatic scattering are numerically calculated. The pulse echoes are compared with the incidence, and demonstrate its functional dependence on the physical parameters of random medium, such as spatial orientation and fractional volume of scatterers, incidence angle and polarization, the layer depth and others.     

Magneto-optical effects upon reflection of light from a ferrodielectric with an arbitrary orientation of magnetization

The boundary problem for a semi-infinite magnetic medium with arbitrary orientation of the magnetization vector is solved and polarization-and intensity-related characteristics of the reflected light wave are analyzed. It is shown that variations of the angle of incidence and of the orientation of the magnetization and polarization plane substantially affect the polarization characteristics of the reflected wave and give rise to specific features of the dependences under study.     

偏振干涉成像光谱仪中格兰-泰勒棱镜全视场角透过率的分析与计算

论述了自行设计研制的偏振干涉成像光谱仪的工作原理,分析了其核心部件格兰-泰勒棱镜的分光机理;运用光线追迹方法,推导出了格兰-泰勒棱镜全视场角透过率计算公式;通过计算机模拟分析了入射面、入射角和空气隙厚度对该棱镜透过率的影响,并利用方解石Sellmeier色散方程,给出了该棱镜在仪器系统要求的光谱范围内透过率与波长的关系曲线;实验测试结果与理论计算公式相符,验证了理论公式的正确性.