On the structure of71As and 73As

The structure of the nuclei ⁷¹As and ⁷³As has been investigated by studying the decay of ⁷¹Se, ^73gSe and ^73mSe, the ⁷²Ge(p, 2nγ)⁷¹As reaction, the ⁷³Ge(p, nγ)⁷³As reaction and the ⁷²Ge(³He, d) ⁷³As reaction. Level schemes of ⁷¹As and ⁷³As are constructed on basis of the energies and intensities of the gamma transitions and their coincidence relations. Spins and parities are deduced from log ft values, l-values and the decay properties of the excited states. The measured half-life of the lowest excited state in ⁷¹As is $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 59 ± 10}\text{ns}$. The experimental level-schemes are compared with the predictions of the cluster-vibrational coupling model.     

The magnetic dipole moment of 55Co

The ground state g-factor for ⁵⁵Co has been measured as $\text{¦g¦= 1.378±0.001}$ by the technique of nuclear magnetic resonance on oriented nuclei. The temperature dependence of γ-ray anisotropy in the ⁵⁵Fe daughter decay determines both the 1408 keV level spin and the ⁵⁵Co ground state spin to be $\text{7}\text{2}$, and yields values of mixing ratios in the 1037 keV β-transition and the 477 keV γ-transition. The configuration mixing model is used to discuss 1f_{$\text{7}\text{2}$} moment systematics.     

Measurement of the parity non-conservation in nuclear forces in 75As, 171Tm,and 175Lu and of the polarized bremsstrahlung from 51Cr, 170Tm, 177Lu,and 198Au

The circular polarization P of γ-rays from unpolarized sources of ⁷⁵Se, ¹⁷¹Er, and ¹⁷⁵Yb of strengths ? 500 Ci has been measured with a Compton polarimeter of the radial transmission type. Eight NaI crystals and a four-fold current integration system were used to simultaneously record the data in four independent channels. The results are: P = ?(1.8 ± 6.0) × 10^?5 for the 401 keV transition in ⁷⁵As (the experimental error is ± 1.5 × 10^?5, the remaining part is due to the uncertainty in the decay scheme of ⁷⁵Se), P = (0.8 ± 1.5) × 10^?4 for the 296 keV and 308 keV transition in ¹⁷¹Tm, and P = (5.7 ± 0.8) × 10^?5 for the 396 keV transition in ¹⁷⁵Lu. The last value confirms the parity non-conservation in nuclear forces. The polarimeter was calibrated with bremsstrahlung from ¹⁷⁰Tm. The correction for polarized bremsstrahlung was given special attention. Correction factors are derived for ⁵¹Cr, ¹⁷⁷Lu, and ¹⁹⁸Au from a comparison of the measured and calculated bremsstrahlung yields.     

The magnetic moment of the 828 keV level in 115In

The magnetic moment of the 828 keV level in ¹¹⁵In was found to be 0.80 ± 0.14 μ_N by measuring the γ-γ integral angular correlation perturbed by an external magnetic field. Several assumptions concerning the nature of the state investigated have been discussed.     

Nuclear magnetic moment of the 9.7 h 12− isomer 196mAu

The magnetic hyperfine splitting v_M=|gμ_NB_HF/h| of ^196mAu (j^π=12^?; configuration ¦(π$\text{11}\text{2}$($\text{v}\text{13}\text{2}{}^{\mathrm{+}}\text{)〉}{}_{12}{}^{\mathrm{?}}$; $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 9.7}\text{h}\text{)}$ as dilute impurity in Ni has been determined with nuclear magnetic resonance on oriented nuclei as 96.0(2) MHz. With the known hyperfine field B_HF = ?264.4(3.9) kG corrected for hyperfine anomalies the g-factor and magnetic moment of ^196mAu are deduced to be |g| = 0.476(7) and |μ| = 5.72(8) μ_N. Taking into account the known magnetic properties of $\text{π}\text{1}\text{2}{}^{\mathrm{?}}$ and $\text{v}\text{13}\text{2}{}^{\mathrm{+}}$ isomeric states in the neighbouring odd Pt, Au and Hg nuclei the structure of the 12^? state is discussed.     

Decay studies of neutron-rich products from 76Ge induced multinucleon transfer reactions including the new isotopes 62Mn, 63Fe and 71, 72, 73Cu

By irradiating a ^natW target with 9 MeV/u ⁷⁶Ge ions, neutron-rich isotopes in the chromiumgermanium region were produced. On-line mass-separated samples were investigated. The new isotopes ⁶²Mn, ⁷¹Cu, ⁷²Cu and ⁷³Cu were identified and their half-lives measured to be 0.88(15), 19.5(16), 6.6(1) and 3.9(3) s, respectively. The half-life of ⁶³Fe, a nucleus which has previously been detected using particle-identification techniques, was measured to be 4.9(5) s. Decay schemes were derived in most cases. Additional spectroscopic information was obtained on the decays of ⁷³Zn and ⁷⁴Zn. We give evidence that the earlier reported γ-ray activity attributed to ⁶⁷Ni belongs to the decay of the ⁷⁰Cu isomers. At A = 67 we observed a new β-ray activity of 21(1) s half-life which is here assigned to the decay of ⁶⁷Ni.     

An investigation of the level scheme of 72As through the 72Ge(p,nγ)72As reaction

The level scheme of the doubly odd nucleus ⁷²As has been investigated by the (p, nγ) reaction up to an excitation energy of about 800 keV. Spin and parity assignments were made by measuring internal conversion coefficients and by an analysis of the (p, n) cross sections through the statistical model of the compound nuclear reaction. The level scheme obtained was interpreted by a simple model calculation based on the shell model.     

The nuclear structure of 225Ra

The level structure of ²²⁵Ra has been studied using the (d, t) reaction with both unpolarised and polarised deuterons and the β^? decay of ²²⁵Fr. Cross sections and excitation energies have been measured for 41 levels below 1800 keV in the (d, t) reaction, and levels up to 724 keV have been established from the β^? decay measurements. The level structure is interpreted in terms of the Nilsson model.     

The half-life of 207Bi and decays of 211At and 211Po

The half-life of ²⁰⁷Bi was obtained from the genetic relation between ²⁰⁷Po and ²⁰⁷Bi, and between ²¹¹At and ²⁰⁷Bi. The half-life was found to be 33.4 ± 0.8 y. The half-life of ²⁰⁷Po was determined to be 5.81 ± 0.04 h by following the decay of the characteristic γ-rays from ²⁰⁷Po. The half-life of ²¹¹ At was determined tobe 7.23 ± 0.02 h by following the decay of γ-rays and α-particles from ²¹¹At and ²¹¹Po. The half-lives determined in the present work for ²⁰⁷Po and ²¹¹At agree with the literature although the half-life of ²⁰⁷Bi differs considerably from the currently accepted value of 38 y. The branching ratio of ²¹¹ At decaying through EC and α-decay modes was determined together with the branching ratios of the three α-particles emitted from ²¹¹Po.     

A study on the decay of ^72As

The excited states of the ⁷²Ge nucleus were investigated in radioactive decay of ⁷²As. Three new transitions with 1996.58, 2125.59 and 2255.49keV have been found for the first time. One γ-ray with 912.09keV has been placed in the decay scheme for the first time, and the placement of 1938.88, 2116.79, 2785.59, 2833.03, 2950.69 and 3338.00keV γ-rays are confirmed again in the present work. One new level at 2027.72keV excitation energy is proposed. The level scheme was established and for a number of levels spin-parity assignments are suggested on the basis of logft values and γ-branching ratios.     

The quadrupole moments of the 5− states in 116Sn, 118Sn and 120Sn

The quadrupole interaction frequencies $\text{ω}{}_0\text{=}\text{3eQ}{}_1\text{V}{}_{\mathrm{zz}}\text{41(21-1)}\text{h}\text{?}$ in the 5^? state of ¹¹⁸Sn have been measured by time differential perturbed angular correlation technique in Sn, Sb and (95% Sn+5% Sb) environments. The ω₀ for ¹¹⁶Sn was determined in Sn environment only. With the help of the known electric field gradient ¹) of Sn in a Sn lattice the quadrupole moments have been deduced as $\text{Q(5}{}^{\mathrm{?}}\text{,}{}^{118}\text{Sn}\text{) = ±0.10(4) b}\text{and}\text{Q(5}{}^{\mathrm{?}}\text{,}{}^{116}\text{Sn}\text{) = ±0.165(60)}\text{b}$. These values together with the known²) quadrupole moment of the analogous 5^? state in ¹²⁰Sn are interpreted in terms of the pure single-particle model. The data exhibit the expected strong systematic variation of Q_I with the number of particles in the h_{$\text{11}\text{2}$}. subshell which is being filled with 1, 3 and 5 neutrons in ¹¹⁶Sn, ¹¹⁸Sn, and ¹²⁰Sn, respectively.     

The β− decay of 102Mo

The ¹⁰²Mo activity was obtained by photofission of natural U and thermal-neutron induced fission of ²³⁵U, with subsequent chemical separation of the molybdenum fraction. In addition, nuclei with mass 102 were separated from fission products of ²³⁵U(n_th, f) using the mass separator LOHENGRIN. A decay scheme and absolute γ-intensities are deduced from measured γ-ray, X-ray and γ-coincidence spectra. Logftvalues are calculated. Shell-model calculations for a $\text{(πlg}{}_{\mathrm{<mtext>9</mtext><mtext>2</mtext>}}\text{)}{}^3$$\text{(νlg}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}\text{)}{}^3$ multiplet have been carried out using effective nucleon-nucleon interactions. The γ-decay between low-lying, low-spin members of this multiplet was studied in detail and compared with the experimental data.     

Decay of 48K, 49K and 50K

The ⁴⁸K, ⁴⁹K and ⁵⁰K nuclides have been produced in high energy fragmentation and analyzed by mass spectroscopy techniques. Their half-lives have been measured as 6 ± 1 s, 1.1 ± 0.3 s and and 0.7 ± 0.3 s, respectively. The γ-rays from their radioactive decay have been observed and the corresponding γ-intensities measured. The nuclide ⁵⁰K is shown to be a delayed neutron emitter. The antianalog states in the daughter Ca nuclei with a $\text{(1d}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}\text{)}{}^{\mathrm{?}}$ neutron configuration, preferentially populated in the β-decay, have been located. The corresponding $\text{1d}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}$ neutron single-particle energy is found to remain approximately constant for these neutron-rich Ca isotopes.     

Beta decays of 25Na, 25Al and 29Al

The radioactivities ²⁵Na, ²⁵Al, and ²⁹Al were produced in the ²³Na(t, p)²⁵Na, ²⁴Mg(d, n)²⁵Al, and ²⁷Al(t, p)²⁹Al reactions using a 3.5 MV Van de Graaff. γ-radiations were measured by means of a target-transfer system and a Ge(Li) detector with or without Compton suppression. Decay schemes derived for ²⁵Na and ²⁹Al are in general agreement with earlier results, but with improved accuracy of branching ratios and much sharper limits on the intensities of certain unobserved β- and γ-ray transitions. Precision measurements of the energies of principal γ-rays gave results in keV for the listed decaying bodies as follows: ²⁵Na ? 1611.716(11); ²⁵Al ? 1611.708(11); and ²⁹Al ? 1273.361(9). The energy determinations of the ²⁵Mg 1612 keV γ-transition measured in the decays of ²⁵Na and ²⁵Al differ by 8 ± 9 eV.     

Mass excesses of 79As, 81As,and 80Ge

Accurate mass measurements for the nuclides ⁷⁹As, ⁸¹As, and ⁸⁰Ge have been measured. Good agreement has been found for ⁷⁹As and ⁸¹As with the Garvey-Kelson transverse mass relation and with several mass model predictions. The agreement for ⁸⁰Ge is not as satisfactory and presents a challenge for understanding mass values far off the line of stability.     

The level structure of 184W FROM THE β− decay of 184Ta

Levels of ¹⁸⁴W populated in the decay of 8.7 h ¹⁸⁴Ta have been studied by a variety of experimental techniques. As a result of β and γ-ray energy and intensity determinations and extensive β-γ and γ-γ coincidence measurements, a detailed ¹⁸⁴Ta decay scheme accommodating more than 99.5% of the decay intensity has been established. Intense β-ray groups of end-point energies 1165±26 and 1123±26 keV populate levels in ¹⁸⁴W at 1699 and 1746 keV, which de-excite predominantly to the 8.3 μs isomeric level at 1285 keV, recently identified as the $\text{1}\text{2}{}^{\mathrm{?}}\text{[510]ν?}\text{11}\text{2}{}^{\mathrm{+}}\text{[615]ν K}{}^{\mathrm{\pi }}\text{= 5}{}^{\mathrm{?}}$ band origin. The 1699 keV level also de-excites to members of a $\text{1}\text{2}{}^{\mathrm{?}}\text{[510]ν?}\text{7}\text{2}\text{[503]ν K}{}^{\mathrm{\pi }}\text{= 3}{}^{\mathrm{+}}$ band based at 1425 keV. New information about the properties of the γ-vibrational and K = 2 octupole bands in ¹⁸⁴W is presented and the possible configurations of the levels directly populated in the β^? decay are discussed. The configuration $\text{7}\text{2}{}^{\mathrm{+}}\text{[404]π ?}\text{3}\text{2}{}^{\mathrm{?}}\text{[512]ν K}{}^{\mathrm{\pi }}\text{= 5}{}^{\mathrm{?}}$ is indicated for the ¹⁸⁴Ta ground state.     

Sudden change of quadrupole moment between the first 52− states of 197Hg and 199Hg

Low-temperature time differential perturbed angular correlation experiments with the 164 keV-134 keV cascade of ^197mHg in a zinc matrix give evidence that the hitherto accepted value of the quadrupole moment of the first $\text{5}\text{2}{}^{\mathrm{?}}$ state of ¹⁹⁷Hg is erroneous. A new value is derived from a time differential perturbed angular correlation experiment with the 374 keV?158 keV cascade of ^199mHg implanted into a Be single crystal and comparison with an analogous experiment for ^197mHg. Taking $\text{Q(}\text{5}\text{2}{}^{\mathrm{?}}\text{,}{}^{199}\text{Hg) = +0.95(7)}\text{b}$ we derive $\text{|Q(}\text{5}\text{2}{}^{\mathrm{?}}\text{,}{}^{197}\text{Hg)¦= 0.081(6)}\text{b}$. This change of quadrupole moment is discussed in the framework of the shell model.     

Beta-decay of 32C1 and 40Sc

The β⁺ decays of ³²C1 and ⁴⁰Sc have been investigated with a rabbit system. New β-branches and γ-lines are reported. Branching ratios and log ft values are determined. The 6.66 MeV state of ³²S is shown to have J^π = 1⁺ or 2⁺.     

Nuclear magnetic moment of the 3.9 s112− isomer 193mAu

The magnetic hyperfine splitting ν_M = |gμ_NB_HF/h| of ${}^{\mathrm{<mtext>193</mtext><mtext>m</mtext>}}\text{Au}\text{(j}{}^{\mathrm{\pi }}\text{=}\text{11}\text{2}{}^{\mathrm{?}}\text{, E = 290}\text{keV}$; $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 3.9}\text{s}\text{)}$ as a dilute impurity in Ni has been measured with nuclear magnetic resonance on oriented nuclei as 226.4(2) MHz. With the known hyperfine field B_HF = ?264.4(3.9) kG corrected for hyperfine anomalies the g-factor and magnetic moment of ^193mAu are deduced to be |g| = 1.123(17) and |μ| = 6.18(9) μ_N.     

Nuclear magnetic resonance of 55Mn and 75As in MnAs

Four sets of NMR signals, two each, from ⁵⁵Mn and ⁷⁵As nuclei have been observed. The temperature dependences of ⁵⁵Mn resonances have been studied from 77 to 311 K and that of ⁷⁵As, from 77 K to about 250 K. The results show that there is a phase transition at T₁ ≈ 220 K. This transition may be due to introduction of a local spontaneous distortion in the region of the domain walls in the lattice, resulting in lowering of symmetry at low temperatures. Another possibility is the canting of spins which would lower the magnetic group symmetry. The observed resonances have been assigned to arise from the nuclei at the edge and the centre of the domain walls at temperatures T >T₁ and from two types of wall edges with inequivalent orientation of atomic spins at T < T₁. The isotropic hyperfine field at 0 K obtained by extrapolating the resonance frequencies are 227 and 285.1 kOe at ⁵⁵As nuclei, respectively. The anisotropy in the hyperfine field is nearly zero at ⁵⁵Mn nuclei and about 5.8 kOe at ⁷⁵As nuclei at 0 K.