Nuclear structure studies of 97Ru from the decay of 97g,mRh

The energy levels of ⁹⁷Ru have been studied through the decay of 31.1 min ^97gRh and 44.3 min ^97mRh using Ge(Li), Si(Li), Nal, plastic and anthracene detectors in singles and in coincidence experiments. A total of 139 γ-rays were observed. Ninety-eight γ-rays have been placed into the decay schemes involving 38 excited levels in ⁹⁷Ru. The level energy of ^97mRh was determined to be 258.6 keV. The spin and parity of ^97gRh and ^97mRh are assigned as $\text{9}\text{2}{}^{\mathrm{+}}\text{and}\text{1}\text{2}{}^{\mathrm{?}}$, respectively. The fraction of decay of the isomer by the isomeric transition was measured with the Si(Li) detector, and α_k values were determined for strong transitions. The half-life of the 188.6 keV, $\text{3}\text{2}{}^{\mathrm{+}}$ state in ⁹⁷Ru was determined as 0.23 ± 0.02 ns by delayed e-γ coincidence measurements. The nuclear structure of low-lying levels is compared with similar levels in other odd-mass nuclei (N = 53) isotones and Ru isotopes).     

High-spin states in 40K investigated with the 26MG + 16O reaction

Yrast levels in ⁴⁰K and ⁴⁰Ar have been investigated with the ²⁶Mg(¹⁶O, pnγ)⁴⁰K and ²⁶Mg(¹⁶O, 2pγ)⁴⁰Ar reactions at a beam energy of 34 MeV. Gamma-ray angular distribution and γ-γ coincidence measurements have been performed with a high-resolution large volume Ge(Li)-NaI(Tl) Compton-suppression spectrometer. Gamma-ray linear polarizations have been measured with a three-crystal Ge(Li) Compton polarimeter. The ⁴⁰K decay scheme involves new high-spin levels at E_tx = 4365.6±0.3, 4875.6±0.4 and 6227.0±0.5 keV with lifetime limits of < 1, < 1 and < 2ps, respectively. Unambiguous spin-parity assignments of $\text{J}{}^{\mathrm{\pi }}\text{= 5}{}^{\mathrm{?}}\text{, 6}{}^{\mathrm{+}}\text{, 8}{}^{\mathrm{+}}\text{, 9}{}^{\mathrm{+}}\text{and}\text{(8, 10)}{}^{\mathrm{?}}$ to the ⁴⁰K levels at E_x = 0.89, 2.88, 4.37, 4.88 and 6.23 and of $\text{J}{}^{\mathrm{\pi }}\text{= 4}{}^{\mathrm{+}}\text{and}\text{6}{}^{\mathrm{+}}\text{to the}{}^{40}\text{Ar}$ levels at E_x = 2.89 and 3.46 MeV, respectively, have been obtained. Branching ratios and multipole mixing ratios are reported.     

A microscopic DWBA analysis of (6Li, 6He) reactions

The spin-isospin flip (⁶Li, ⁶He) reaction has been studied. The experiment was performed with a 34 MeV ⁶Li beam incident upon ^{25, 26}Mg and ²⁷Al targets. Angular distributions associated with the lowest $\text{5}\text{2}{}^{\mathrm{+}}\text{,}\text{1}\text{2}{}^{\mathrm{+}}\text{,}\text{7}\text{2}{}^{\mathrm{+}}{}^{25}\text{Al}\text{, 5}{}^{\mathrm{+}}\text{, 3}{}^{\mathrm{+}}\text{, 1}{}^{\mathrm{+}}{}^{26}\text{Al and}\text{5}\text{2}{}^{\mathrm{+}}{}^{27}\text{Si}$ states were measured. Microscopic DWBA calculations were performed using Yukawa central and r². Yukawa (r² · Y) tensor (μ = 1.0 fm^?1) potentials averaged over the ⁶Li(⁶He) cluster model wave functions. Knock-on (KO) exchange corrections corresponding to the central interaction are included using the local-energy approximation (LEA) method. The conclusion is that the quasi-elastic process is of major importance in the (⁶Li, ⁶He) transition studied in this work.     

Nuclear orientation of negative parity states of 131Xe

The anisotropies of the 177, 326, and 503 keV γ-transitions between negative parity states of ¹³¹Xe have been remeasured in the decay of oriented ¹³¹I nuclei. In addition the linear polarization of the 503 keV radiation has been determined with a Compton polarimeter consisting of two Ge(Li) detectors. A combined analysis of the reported experiment and earlier internal conversion and angular distribution data yields the unique assignments $\text{9}\text{2}{}^{\mathrm{?}}\text{and}\text{7}\text{2}{}^{\mathrm{?}}$ for the levels at 341 and 667 keV. The $\text{E2}\text{M1}$ mixing ratios of the 177 and 326 keV transitions are δ(177) = ?4.5 ± 1.5 and δ(326) = ?4.4 ± 1.6. The intensity of the L = 2 component in the first forbidden β-decay to the 667 keV level is at most 60 %.     

Lifetimes and g-factors of the 6− and 7− isomers in 66Ga and 68Ga

The 6^? and 7^? isomeric states in ⁶⁶Ga and ⁶⁸Ga at 1440.9 and 1229.6 keV, respectively, have been populated with the (¹³C, 2np) and (¹⁵N, n2p) reactions on natural Fe. The half-lives of these states have been measured to be $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{(6}{}^{\mathrm{?}}\text{,}{}^{66}\text{Ga}\text{) = 57.3 ± 1.2}\text{ns}$ and $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{(7}{}^{\mathrm{?}}\text{,}{}^{68}\text{Ga}\text{) = 64 ± 2}\text{ns}$. Using previous data on the hyperfine field of Ga in Fe, the g-factors of these states have been determined by means of the TDPAD method. The results are $\text{g(6}{}^{\mathrm{?}}\text{,}{}^{66}\text{Ga}\text{) = 0.129 ± 0.003}$ and $\text{g(7}{}^{\mathrm{?}}\text{,}{}^{68}\text{Ga}\text{) = 0.105 ± 0.003}$. These values are in very good agreement with the independent particle model if one assumes the and configurations and uses the empirical proton and neutron g-factors from odd-A neighboring nuclei instead of the Schmidt values. The large disagreements with experiment when Schmidt values are used show that core polarization effects are important in these nuclei.     

Author index

High-spin states in ^167,168Hf and ^{170, 171}W have been excited by the reactions ${}^{159}\text{Tb}\text{(}{}^{14}\text{N}\text{, x}\text{n}\text{)}{}^{\mathrm{173\; ?\; x}}\text{Hf and}{}^{155}\text{Gd}\text{(}{}^{20}\text{Ne}\text{, x}\text{n}\text{)}{}^{\mathrm{175\; ?\; x}}\text{W}$. The yrast bands have been observed up to $\text{J}{}^{\mathrm{\pi }}\text{=}\text{49}\text{2}{}^{\mathrm{+}}$ in ¹⁶⁷Hf, J^π = 28⁺ in ¹⁶⁸Hf, $\text{J}{}^{\mathrm{\pi }}\text{=}\text{45}\text{2}{}^{\mathrm{+}}$ in ¹⁷¹W and J^π = 22⁺ in ¹⁷⁰W. Both even-even nuclei display a strong backbend around J^π = 14⁺, whereas ¹⁶⁷Hf shows an upbend at ω ～- 0.33 MeV and ¹⁷¹W exhibits a progressive gain in aligned angular momentum above ω ～- 0.26 MeV. At even higher rotational frequencies, bridges have been found in the central valleys of the γ-γ correlation matrices at ω ～- 0.42 and 0.52 MeV for the Hf isotopes and ω ～- 0.45 and 0.47 MeV for the W isotopes. Deduced moments of inertia for the Hf isotopes using the correlation data show a smooth increase up to about the rigid-sphere value at ω ～- 0.5 MeV. The data are satisfactorily accounted for by cranked shell-model calculations. In particular, a qualitative interpretation is given for the experimentally observed systematic difference in the strength of the interaction potential for the N = 95 and N = 97 isotopes of Hf and W.     

β-delayed charged particles from 9Li and 11Li

β-delayed emission of α-particles from ⁹Li and of both α and ⁶He particles from ¹¹Li is observed. Singles energy spectra and two-dimensional energy spectra of coincident particles are measured. A time-of-flight versus energy measurement is used to identify the mass of the particle. New β-branches are observed which populate high-energy levels in the daughter nuclei. The branching ratios are measured and the β-delayed neutron emission probabilities $\text{P}{}_{\mathrm{<mtext>n</mtext>}}\text{for}{}^9\text{Li and}\text{P}{}_{\mathrm{3n}}\text{for}{}^{11}\text{Li}$ are deduced.     

High-spin yrast levels of 38Ar

High-spin states of ³⁸Ar have been studied with the ³⁵Cl(α, pγ)³⁸Ar reaction at E_α = 18 MeV and with the ²⁴Mg(¹⁶O, 2pγ)³⁸Ar reaction at $\text{E(}{}^{16}\text{O}\text{) = 38}\text{and}\text{45}\text{MeV}$. The ³⁸Ar level scheme is obtained with the former reaction from a proton-γ coincidence measurement. Gamma-gamma coincidence, γ-ray angular distribution and linear polarization experiments have been performed with a Ge(Li)-Na(Tl) Compton suppression spectrometer and a three-crystal Ge(Li) Compton polarimeter. Unambiguous spin-parity assignments of $\text{J}{}^{\mathrm{\pi }}\text{= 7}{}^{\mathrm{?}}\text{, 7}{}^{\mathrm{+}}\text{, 8}{}^{\mathrm{+}}\text{, 7}{}^{\mathrm{?}}\text{, 9}{}^{\mathrm{?}}\text{and}\text{11}{}^{\mathrm{?}}$to the ³⁸Ar levels at E_x = 7.51, 8.08, 8.57, 8.97, 10.17 and 11.61 MeV, respectively, are obtained. The 8.57 MeV, 8⁺ level has a mean life below 0.8 ps. Excitation energies, branching ratios, multipole mixing ratios and transition strengths are reported. The experimental results are compared with shell-model calculations.     

The 6Li-induced three-nucleon transfer reaction on 40Ca

Analog (fp)³ states preferentially excited in the ${}^{40}\text{Ca}\text{(}{}^6\text{Li,t}\text{)}{}^{43}\text{Ti}$ and the ${}^{40}\text{Ca}\text{(}{}^6\text{Li}\text{, τ)}{}^{43}\text{Sc}$ reactions have been identified in the mass 43 mirror nuclei. A simple zero-range DWBA calculation made with a cluster form factor gives good agreement with the measured angular distributions, but spectroscopic strengths deduced for mirror levels do not agree. The 3p-0h states are excited with a rather uniform cross section not strongly correlated with spins.     

g-factors of 2.7 h 93Tc, 4.9 h 94Tc and 20 h 95Tc

The hyperfine splitting frequencies gμ_NB_H.F./h of 2.7 h ⁹³Tc $\text{(J}{}^{\mathrm{\pi }}\text{=}\text{9}\text{2}{}^{\mathrm{+}}\text{)}$, 4.9 h ⁹⁴Tc (J^π = 7⁺) and 20 h ⁹⁵Tc $\text{(J}{}^{\mathrm{\pi }}\text{=}\text{9}\text{2}{}^{\mathrm{+}}\text{)}$ as dilute impurities in Fe have been measured with NMR on oriented nuclei as 336.36(5) MHz, 175.11(1) MHz and 315.97(2) MHz, respectively. From the resonance shifts with an external magnetic field B₀ the hyperfine field of Tc$\text{Fe}$ has been determined as -317(5) kG. Taking this into account the nuclear g-factors are deduced as $\text{g(}{}^{93}\text{Tc}\text{) = 1.392(22), g(}{}^{94}\text{Tc}\text{) = 0.725(11)}\text{and}\text{g(}{}^{95}\text{Tc}\text{) = 1.308(21)}$.     

Spin-parity assignments to high-spin states of 41K and 41Ca

Yrast states of ⁴¹K and ⁴¹Ca have been investigated with the ²⁶Mg(¹⁸O, p2nγ)⁴¹K and ²⁶Mg(¹⁸O, 3nγ)⁴¹Ca reactions at a beam energy of 34 MeV. Gamma-gamma coincidence, γ-ray angular distribution and linear polarization measurements were performed with a Ge(Li)-NaI(Tl) Compton suppression spectrometer and a three-crystal Ge(Li) Compton polarimeter. Unambiguous spin-parity assignments of $\text{J}{}^{\mathrm{\pi }}\text{=}\text{7}\text{2}{}^{\mathrm{+}}$, $\text{11}\text{2}{}^{\mathrm{+}}$, $\text{11}\text{2}{}^{\mathrm{?}}$, $\text{13}\text{2}{}^{\mathrm{+}}$, $\text{15}\text{2}{}^{\mathrm{?}}$ and $\text{19}\text{2}{}^{\mathrm{?}}$ to the ⁴¹K levels at E_x = 1.68, 2.53, 2.76, 2.77, 4.27 and 4.98 MeV and of $\text{9}\text{2}{}^{\mathrm{+}}\text{,}\text{11}\text{2}{}^{\mathrm{+}}\text{and}\text{15}\text{2}{}^{\mathrm{+}}$to the ⁴¹Ca levels at E_x = 3.20, 3.37 and 3.83 MeV, respectively, have been obtained. Excitation energies, branching ratios, multipole mixing ratios and transition strengths are reported. The main features of the ⁴¹K and ⁴¹Ca level and decay schemes are reproduced in a 2p-1h and 3p-2h shell-model calculation.     

The nuclear magnetic moment of 71As and 72As

Nuclear magnetic resonance of oriented ⁷¹As and ⁷²As nuclei has been observed in an iron host lattice at low temperatures. The resonance frequencies are v_l = 174.96(10) MHz and 282.00(11) MHz respectively for zero external field. Using B_h.f.(FeAs) = 342.9(3) kG the g-factors of the two isotopes are derived as $\text{g(}{}^{71}\text{As}\text{) = (+)0.6694(7)}\text{and}\text{g(}{}^{72}\text{As) = (?)1.0789(11)}$. Combining nuclear orientation data with these results the spin of ⁷¹As has been confirmed as $\text{I =}\text{5}\text{2}$. The magnetic moments of the $\text{5}\text{2}{}^{\mathrm{?}}$ and 2^? states in the As isotopes are discussed in the framework of the shell model with configuration mixing.     

Coherent production of multimeson final states on A ∼ 20 nuclei by K− of 5.5, 10.0, 12.7 GeV

Coherent production of $\text{K}\text{π,}\text{K}\text{2π}\text{and}\text{K}\text{3π}$ final states from A ～ 20 nuclei by K^? beams of 5.5, 10.0 and 12.7 GeV is analyzed. Final states with ? 2π^O are included. Coherent $\text{K}\text{π}$ production occurs (although forbidden via 0⁺ exchange) and is dominated by the $\text{K}$¹ (890). The shape of the t distribution, the alignment of the produced meson and the ratio of the cross section on nuclei to that on hydrogen are consistent with optical model predictions assuming that $\text{K}$¹ (890) are produced on single nucleons by exchange of isoscalar trajectories of natural parity (J^P = 1^?, 2⁺, etc.) and that the $\text{K}$¹ (890) absorption in nuclear matter equals that of the K^?. Coherent $\text{K}\text{ππ}$ production (allowed via 0⁺, 1^?, 2⁺, etc. exchange) is dominated by the Q phenomenon. A Dalitz plot and angular correlation analysis yields values for $\text{K}\text{?/}\text{K}{}^1\text{π}$ fractions, and shows that $\text{J}{}^{\mathrm{P}}\text{= 1}{}^{\mathrm{+}}\text{S-wave}\text{K}{}^1\text{π}$ dominates the coherently produced Q. The helicity of the Q is found to be compatible with 0. The Q^? -nucleaon total cross section is estimated to be 0.98_?0.37⁺⁰²⁴ times the $\text{K}$^? -nucleon total cross section from a comparison of the coherent Q-production cross section with corresponding hydrogen cross sections at 10 and 12.7 GeV. We observe coherent production of $\text{K}$ω. The ration $\text{K}\text{ω/}\text{K}\text{ππ}$ coherently produced in the Q mass region is (4 ± 1)%. Coherent production of $\text{K}{}^{\mathrm{?}}\text{π}{}^{\mathrm{+}}\text{π}{}^{\mathrm{?}}\text{and}\text{K}{}^{\mathrm{<mtext>O</mtext>}}\text{π}{}^{\mathrm{+}}\text{π}{}^{\mathrm{?}}\text{π}{}^{\mathrm{<mtext>O</mtext>}}$ is observed in the L region. Coherent production is not observed in the K4π channels.     

Methyl barrier to internal rotation and quadrupole coupling constants in S-methylchlorothioformate

Internal rotation A-E splittings have been observed in the ground state for both ³⁵Cl and ³⁷Cl isotopic species of S-methylchlorothioformate. The values $\text{V}{}_3\text{(}{}^{35}\text{Cl}\text{) = 893 ± 20}$ and $\text{V}{}_3\text{(}{}^{37}\text{Cl) = 890 ± 20 cal/mole}$ have been obtained. The anaalysis of the hyperfine structure gave $\text{χ}{}_{\mathrm{aa}}\text{(}{}^{35}\text{Cl}\text{) = ?49.2}$, $\text{χ}{}_{\mathrm{bb}}\text{(}{}^{35}\text{Cl}\text{) = 22.4}$ and $\text{χ}{}_{\mathrm{aa}}\text{(}{}^{37}\text{Cl}\text{) = ?39.0}$, $\text{χ}{}_{\mathrm{bb}}\text{(}{}^{37}\text{Cl) = 18.3 MHz}$. Only the syn-conformation of the methyl group with respect to the carbonyl group has been observed. A partial r₀ structure is given.     

Nuclear magnetic moment of the 9.7 h 12− isomer 196mAu

The magnetic hyperfine splitting v_M=|gμ_NB_HF/h| of ^196mAu (j^π=12^?; configuration ¦(π$\text{11}\text{2}$($\text{v}\text{13}\text{2}{}^{\mathrm{+}}\text{)〉}{}_{12}{}^{\mathrm{?}}$; $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 9.7}\text{h}\text{)}$ as dilute impurity in Ni has been determined with nuclear magnetic resonance on oriented nuclei as 96.0(2) MHz. With the known hyperfine field B_HF = ?264.4(3.9) kG corrected for hyperfine anomalies the g-factor and magnetic moment of ^196mAu are deduced to be |g| = 0.476(7) and |μ| = 5.72(8) μ_N. Taking into account the known magnetic properties of $\text{π}\text{1}\text{2}{}^{\mathrm{?}}$ and $\text{v}\text{13}\text{2}{}^{\mathrm{+}}$ isomeric states in the neighbouring odd Pt, Au and Hg nuclei the structure of the 12^? state is discussed.     

α-Vibrations

The existence of states which change the number of particles in four and wich are specifically excited in α-transfer reactions like (¹⁶O, ¹²C), (⁶Li, d), etc. is predicted, as a consequence of the existence of proton and neutron pairing vibrations which are strongly excited in two-particle transfer reactions. In particular a J^π = 0⁺ two-phonon σ-vibration (4p?4h) state is expected at ≈ 7 MeV of excitation in ²⁰⁸Pb and with a relative cross section $\text{σ(}{}^{204}\text{Hg}\text{→ 7}\text{MeV}\text{(}{}^{208}\text{Pb}\text{))/σ(}{}^{208}\text{Pb}\text{→}\text{gs}\text{(}{}^{212}\text{Po}\text{)) ≈ 1}$. Similar states are expected in neighbouring nuclei.     

A test of iso-scalar quadrupole renormalization in the 32− → 12−(Ex = 0.478 MeV) transition in 7Li

Electromagnetic studies have established that the $\text{3}\text{2}{}^{\mathrm{?}}\text{,}\text{1}\text{2}{}^{\mathrm{?}}$ ground state doublet in ⁷Li is well described by the LS coupling shell model, provided quadrupole effective charge is introduced. The results of microscopic calculations for the excitation of the $\text{1}\text{2}{}^{\mathrm{?}}$ level in inelastic proton scattering shown within indicate that an equivalent renormalization of the ⁷Li quadrupole neutron transition densities is also necessary. This verifies the assumption which was made in a previous calculation of the cross section for the excitation of the $\text{3}\text{2}{}^{\mathrm{?}}$ level in the ⁷Li+²⁴Mg reaction.     

An unambiguous Jπ assignment from γ-rays produced in heavy-ion reactions; The lowest Jπ=6+, 38Ar level

Angular correlation measurements with a Compton-suppression spectrometer in combination with polarization measurements with a three-crystal Ge(Li) Compton polarimeter of γ-rays produced in the ${}^{24}\text{Mg(}{}^{16}\text{O, 2pγ)}{}^{38}\text{Ar}$ reaction result in an unambiguous J^π = 6⁺ assignment to the 6408.3 ± level. It is exclusive decay to the 5^?, 4.59 MeV level is discussed.