The TITAN mass measurement facility at TRIUMF-ISAC

The TITAN facility at TRIUMF-ISAC will use four ion traps with the primary goal of determining nuclear masses with high precision, particularly for short lived isotopes with lifetimes down to approximately 10 ms. The design value for the accuracy of the mass measurement is 1 ×10^???8. The four main components in the facility are an RF cooler/buncher (RFCT) receiving the incoming ion beam, an electron beam ion trap (EBIT) to breed the ions to higher charge states, a cooler Penning trap (CPET) to cool the highly charged ions, and finally the measurement Penning trap (MPET) for the precision mass determination. Additional goals for this system are laser spectroscopy on ions extracted from the RFCT and beta spectroscopy in the EBIT (in Penning trap mode) on ions that are purified using selective buffer gas cooling in the CPET. The physics motivation for the mass measurements are manifold, from unitarity tests of the CKM matrix to nuclear structure very far from the valley of stability, nuclear astrophysics and the study of halo-nuclei. As a first measurement the mass of ¹¹Li will be determined. With a lifetime of 8.7 ms and a demonstrated production rate of 4×10⁴ ions/sec at ISAC the goal for this measurement at TITAN is a relative uncertainty of 5×10^???8. This would check previous conflicting measurements and provide information for nuclear theory and models.     

A cooler ion trap for the TITAN on-line trapping facility at TRIUMF

We present simulations of electron and proton cooling of highly charged ions in a Penning trap, including the potentially detrimental effects of radiative, dielectronic, and three-body recombination in electron cooling. We show a preliminary design for a cooler trap accommodating both electron and proton cooling, which will be a component of the TITAN ion-trap facility under construction at TRIUMF for precision mass measurements of short-lived radioactive nuclei.      

Cooling of short-lived, radioactive, highly charged ions with the TITAN cooler Penning trap

TITAN is an on-line facility dedicated to precision experiments with short-lived radioactive isotopes, in particular mass measurements. The achievable resolution on mass measurement, which depends on the excitation time, is limited by the half life of the radioactive ion. One way to bypass this is by increasing the charge state of the ion of interest. TITAN has the unique capability of charge-breeding radioactive ions using an electron-beam ion trap (EBIT) in combination with Penning trap mass spectrometry. However, the breeding process leads to an increase in energy spread, ??E, which in turn negatively influences the mass uncertainty. We report on the development of a cooler Penning trap which aims at reducing the energy spread of the highly charged ions prior to injection into the precision mass measurement trap. Electron and proton cooling will be tested as possible routes. Mass selective cooling techniques are also envisioned.     

A high-current electron beam ion trap as an on-line charge breeder for the high precision mass measurement TITAN experiment

The precision of atomic mass measurements in a Penning trap is directly proportional to the charge state q of the ion and, hence, can be increased by using highly charged ions (HCI). For this reason, charge breeding with an electron beam ion trap (EBIT) is employed at TRIUMF’s Ion Trap for Atomic and Nuclear science (TITAN) on-line facility in Vancouver, Canada. By bombarding the injected and trapped singly charged ions with an intense beam of electrons, the charge state of the ions is rapidly increased inside the EBIT. To be compatible with the on-line requirements of short-lived isotopes, very high electron beam current densities are needed. The TITAN EBIT includes a 6 Tesla superconducting magnet and is designed to have electron beam currents and energies of up to 5 A and 60 keV, respectively. Once operational at full capacity, most species can be bred into a He-like configuration within tens of ms. Subsequently, the HCI are extracted, pass a Wien filter to reduce isobaric contamination, are cooled, and injected into a precision Penning trap for mass measurement. We will present the first results and current status of the TITAN EBIT, which has recently been moved to TRIUMF after assembly and commissioning at the Max-Planck-Institute (MPI) for Nuclear Physics in Heidelberg, Germany.     

First use of high charge states for mass measurements of short-lived nuclides in a Penning trap

Penning trap mass measurements of short-lived nuclides have been performed for the first time with highly charged ions, using the TITAN facility at TRIUMF. Compared to singly charged ions, this provides an improvement in experimental precision that scales with the charge state q. Neutron-deficient Rb isotopes have been charge bred in an electron beam ion trap to q=8-12+ prior to injection into the Penning trap. In combination with the Ramsey excitation scheme, this unique setup creating low energy, highly charged ions at a radioactive beam facility opens the door to unrivaled precision with gains of 1-2 orders of magnitude. The method is particularly suited for short-lived nuclides such as the superallowed β emitter 74Rb (T(1/2)=65 ms). The determination of its atomic mass and an improved Q(EC) value are presented.     

Testing atomic structure theories with high accuracy mass measurements on highly charged ions

The mass of a highly charged ion is the sum of the mass of the nucleus, the mass of the electrons and the electronic binding energies. High accuracy mass measurements on highly charged ions in a sequence of different charge states yield informations on atomic binding energies, i.e., the ionisation potentials. In our contribution we discuss the possibility of determining atomic binding energies of highly charged ions to better than 20 eV via cyclotron frequency measurements in a Penning trap. At this level of accuracy different contributions to the binding energies, like relativistic corrections, Breit corrections and QED corrections, can be measured. This revised version was published online in August 2006 with corrections to the Cover Date.     

Nuclear-polarization correction to the bound-electron g factor in heavy hydrogenlike ions

The influence of nuclear polarization on the bound-electron g factor in heavy hydrogenlike ions is investigated. Numerical calculations are performed for the K- and L-shell electrons taking into account the dominant virtual nuclear excitations. This determines the ultimate limit for tests of QED utilizing measurements of the bound-electron g factor in highly charged ions.     

SMILETRAP — Atomic mass measurements with ppb accuracy by using highly charged ions

In the SMILETRAP facility externally produced highly charged ions are captured in a Penning trap and utilized for high precision measurements of atomic masses. Accuracy tests on a ppb level have been performed, using highly charged carbon, oxygen and neon ions. In all cases hydrogen ions served as a reference for the calibration and monitoring of the magnetic field in the trap. Deviations smaller than 3 ppb from the expected results were found in mass measurements of the¹⁶O and²⁰Ne atomic masses. The proton atomic mass, determined from the reference measurements on hydrogen ions, is in good agreement with the accepted value [1]. A direct mass measurement on the⁸⁶Kr-isotope, using trapped⁸⁶Kr²⁹⁺-ions is reported.     

Sympathetic cooling of 4He+ ions in a radio-frequency trap

We have generated Coulomb crystals of ultracold 4He+ ions in a linear radio-frequency trap, by sympathetic cooling via laser-cooled 9Be+. Stable crystals containing up to 150 localized He+ ions at approximately 20 mK were obtained. Ensembles or single ultracold He+ ions open up interesting perspectives for performing precision tests of QED and measurements of nuclear radii. This Letter also indicates the feasibility of cooling and crystallizing highly charged atomic ions using 9Be+ as coolant.     

The trap design of PENTATRAP

A novel Penning-trap tower consisting of five compensated cylindrical Penning traps is developed for the PENTATRAP mass spectrometer at the Max-Planck-Institut für Kernphysik in Heidelberg, Germany. An analytical expression for the electrostatic potential inside the trap tower is derived to calculate standard Penning-trap properties like the compensation of anharmonicities and an orthogonal geometry of the trap electrodes. Since the PENTATRAP project described in the preceding article aims for ultra high-precision mass-ratio measurements of highly charged ions up to uranium, systematic effects for highly charged ions inside the trap tower are considered for the design process as well. Finally, a limit due to remaining anharmonic shifts at large amplitudes is estimated for the resulting geometry, which is important for phase-sensitive measurements of the reduced cyclotron frequency of the ions.     

Schottky mass spectrometry at the heavy ion storage ring ESR

Schottky mass spectrometry is a novel method of precision nuclear mass spectrometry based on the measurement of the revolution frequencies of cooled ions in storage rings performed by non-destructive frequency analysis of the beam noise, the well-established Schottky diagnosis technique. The method was applied for the first time at the Experimental Storage Ring ESR at GSI observing electron cooled highly charged ions up to bare nuclei at relativistic energies around several hundred MeV/u. To demonstrate the performance and feasibility of the method at the ESR, experimental tests have been carried out using beams of nuclear fragments produced in the ring itself by the interaction of different primary beams with the internal gas jet target. Futhermore, first Schottky mass measurements of secondary nuclear beams produced by projectile fragmentation of Au and Bi primary beams in a thick Be-target were carried out in order to determine the masses for numerous heavy neutron deficient nuclei which had not been measured before. Relative accuracies for the measured mass values in the order of 1×10^–6 and below can be achieved. The method is briefly discussed and some early results are presented.     

Simulating the stopping dynamics of highly charged ions in an ultra-cold, strongly coupled plasma

We introduce a method for stopping highly charged ions (HCIs) in a laser-cooled one-component plasma (OCP) of ²⁴Mg⁺ ions and present results on stopping times derived from realistic molecular dynamics simulations of the complete stopping process. This stopping scheme can provide ultra-cold highly charged ions for future in-trap precision mass measurements. The choice of an ultra-cold ion plasma as a stopping medium is governed by the almost negligible charge exchange of the HCI with the laser-cooled ions and the very low temperatures which can be reached. In our analysis we focus on the stability and fast recooling of the plasma – two features essential for the experimental realization of this stopping scheme.      

Ground state hyperfine structure of heavy hydrogen like ions

Laser spectroscopy of highly charged heavy ions in the storage ring provides an excellent tool for a test of QED in ultra-high electric and magnetic fields. Discrepancies between experimental and theoretical values are so far mainly explained by uncertainties of nuclear properties. New experimental possibilities can avoid these problems by additional measurements in lithium-like systems. This revised version was published online in August 2006 with corrections to the Cover Date.     

Report on recent activities at the TITAN mass spectrometer at ISAC/TRIUMF

The present report gives a short summary of current work at the TITAN mass spectrometer, including on-line mass measurements and systematic studies. A list of recent references for work published is given.     

Precision mass measurements of neutron halo nuclei using the TITAN Penning trap

Precise atomic mass determinations play a key role in various fields of physics, including nuclear physics, testing of fundamental symmetries and constants and atomic physics. Recently, the TITAN Penning trap measured the masses of several neutron halos. These exotic systems have an extended, diluted, matter distribution that can be modelled by considering a nuclear core surrounded by a halo formed by one or more of loosely bound neutrons. Combined with laser spectroscopy measurements of isotopic shifts precise masses can be used to obtain reliable charge radii and two-neutron-seperation energies for these halo nuclei. It is shown that these results can be used as stringent tests of nuclear models and potentials providing an important metric for our understanding of the interactions in all nuclei.     

PENTATRAP: a novel cryogenic multi-Penning-trap experiment for high-precision mass measurements on highly charged ions

The novel five-Penning-trap mass spectrometer Pentatrap is developed at the Max-Planck-Institut für Kernphysik (MPIK), Heidelberg. Ions of interest are long-lived highly charged nuclides up to bare uranium. Pentatrap aims for an accuracy of a few parts in 10¹² for mass ratios of mass doublets. A physics program for Pentatrap includes Q-value measurements of β-transitions relevant for neutrino physics, stringent tests of quantum electrodynamics in the regime of extreme electric fields, and a test of special relativity. Main features of Pentatrap are an access to a source of highly charged ions, a multi-trap configuration, simultaneous measurements of frequencies, a continuous precise monitoring of magnetic field fluctuations, a fast exchange between different ions, and a highly sensitive cryogenic non-destructive detection system. This article gives a motivation for the new mass spectrometer Pentatrap, presents its experimental setup, and describes the present status.     

Electron Magnetic Moment in Highly Charged Ions: The ARTEMIS Experiment

The magnetic moment (g‐factor) of the electron is a fundamental quantity in physics that can be measured with high accuracy by spectroscopy in Penning traps. Its value has been predicted by theory, both for the case of the free (unbound) electron and for the electron bound in a highly charged ion. Precision measurements of the electron magnetic moment yield a stringent test of these predictions and can in turn be used for a determination of fundamental constants such as the fine structure constant or the atomic mass of the electron. For the bound‐electron magnetic‐moment measurement, two complementary approaches exist, one via the so‐called “continuous Stern–Gerlach effect”, applied to ions with zero‐spin nuclei, and one a spectroscopic approach, applied to ions with nonzero nuclear spin. Here, the latter approach is detailed, and an overview of the experiment and its status is given.     

Mass measurements and evaluation around A = 22

Frequency ratio measurements with different combinations of the singly charged ions from ^{21, 22, 23}Na , ^{22, 24}Mg , and ^{37, 39}K were performed at the on-line Penning trap mass spectrometer ISOLTRAP, CERN, Geneva. The masses and mass differences were deduced with a relative uncertainty of about or even below one part in 10⁸ for the ions of interest using a least-squares analysis of all measured relations. The results have direct consequences for weak-interaction study as they give additional input to the test of CVC, and for nuclear astrophysics, because they help to establish the minimum observable signal for a NeNa cycle in a nova burst. We report here about the measurements and the detailed evaluation.     

TITAN: An ion trap facility for on-line mass measurement experiments

Precision determinations of ground state or even isomeric state masses reveal fingerprints of nuclear structure. In particular, at the limits of existence for very neutron-rich or -deficient isotopes, one can extract detailed information about nuclear structure from separation energies or binding energies. Mass measurements are important to uncover new phenomena, to test new theoretical predictions, or to refine model approaches. For example, the N?=?28 shell has proven more stable than previously expected; however, the predicted new “magic” number at N?=?34 in the K and Ca isotopes has yet to be confirmed experimentally. For these neutron-rich nuclei, the inclusion of three-body forces leads to significantly better predictions of the ground-state mass. Similarly, halo nuclei present an excellent application for ab-initio theory, where ground state properties, like masses and radii, test our understanding of nuclear structure. Precision mass determinations at TRIUMF are carried out with the TITAN (TRIUMF’s Ion Traps for Atomic and Nuclear science) facility. It is an ion-trap setup coupled to the on-line facility ISAC. TITAN has measured masses of isotopes as short-lived as 9 ms (almost an order of magnitude shorter-lived than any other Penning trap system), and it is the only one with charge breeding capabilities, which allow us to boost the precision by almost 2 orders of magnitude. We recently made use of this feature by measuring short-lived, proton-rich Rb-isotopes, up to ⁷⁴Rb while reaching the 12?+ charge state, which together with other improvements led to an increase in precision by a factor 36.     

HITRAP: A Facility for Experiments with Trapped Highly Charged Ions

HITRAP is a planned ion trap facility for capturing and cooling of highly charged ions produced at GSI in the heavy-ion complex of the UNILAC-SIS accelerators and the ESR storage ring. In this facility heavy highly charged ions up to uranium will be available as bare nuclei, hydrogen-like ions or few-electron systems at low temperatures. The trap for receiving and studying these ions is designed for operation at extremely high vacuum by cooling to cryogenic temperatures. The stored highly charged ions can be investigated in the trap itself or can be extracted from the trap at energies up to about 10 keV/q. The proposed physics experiments are collision studies with highly charged ions at well-defined low energies (eV/u), high-accuracy measurements to determine the g-factor of the electron bound in a hydrogen-like heavy ion and the atomic binding energies of few-electron systems, laser spectroscopy of HFS transitions and X-ray spectroscopy. This revised version was published online in July 2006 with corrections to the Cover Date.